arXiv subjects

S. Patankar

Publications and source records attributed to S. Patankar.

5 recordsLinked to original sources

arXiv2017

Antiferromagnetic resonance and terahertz continuum in $α-$RuCl$_3$

We report measurements of optical absorption in the zig-zag antiferromagnet $α$-RuCl$_3$ as a function of temperature, $T$, magnetic field, $B$, and photon energy, $\hbarω$ in the range $\sim$ 0.3 to 8.3 meV, using time-domain terahertz spectroscopy. Polarized measurements show that 3-fold rotational symmetry is broken in the honeycomb plane from 2 K to 300 K. We find a sharp absorption peak at 2.56 meV upon cooling below the Néel temperature of 7 K at $B=0$ that we identify as magnetic-dipole excitation of a zero-wavevector magnon, or antiferromagnetic resonance (AFMR). With application of $B$, the AFMR broadens and shifts to lower frequency as long-range magnetic order is lost in a manner consistent with transitioning to a spin-disordered phase. From direct, internally calibrated measurement of the AFMR spectral weight, we place an upper bound on the contribution to the $dc$ susceptibility from a magnetic excitation continuum.

cond-mat.str-el↗

arXiv2017

Counter-propagating radiative shock experiments on the Orion laser

We present new experiments to study the formation of radiative shocks and the interaction between two counter-propagating radiative shocks. The experiments were performed at the Orion laser facility which was used to drive shocks in xenon inside large aspect ratio gas-cells. The collision between the two shocks and their respective radiative precursors, combined with the formation of inherently 3-dimensional shocks, provides a novel platform particularly suited for benchmarking of numerical codes. The dynamics of the shocks before and after the collision were investigated using point-projection X-ray backlighting while, simultaneously, the electron density in the radiative precursor was measured via optical laser interferometry. Modelling of the experiments using the 2-D radiation hydrodynamic codes NYM/PETRA show a very good agreement with the experimental results.

physics.plasm-ph↗

arXiv2017

Giant anisotropic nonlinear optical response in transition metal monopnictide Weyl semimetals

Although Weyl fermions have proven elusive in high-energy physics, their existence as emergent quasiparticles has been predicted in certain crystalline solids in which either inversion or time-reversal symmetry is broken\cite{WanPRB2011,BurkovPRL2011, WengPRX2015,HuangNatComm2015}. Recently they have been observed in transition metal monopnictides (TMMPs) such as TaAs, a class of noncentrosymmetric materials that heretofore received only limited attention \cite{XuScience2015, LvPRX2015, YangNatPhys2015}. The question that arises now is whether these materials will exhibit novel, enhanced, or technologically applicable electronic properties. The TMMPs are polar metals, a rare subset of inversion-breaking crystals that would allow spontaneous polarization, were it not screened by conduction electrons \cite{anderson1965symmetry,shi2013ferroelectric,kim2016polar}. Despite the absence of spontaneous polarization, polar metals can exhibit other signatures of inversion-symmetry breaking, most notably second-order nonlinear optical polarizability, $χ^{(2)}$, leading to phenomena such as optical rectification and second-harmonic generation (SHG). Here we report measurements of SHG that reveal a giant, anisotropic $χ^{(2)}$ in the TMMPs TaAs, TaP, and NbAs. With the fundamental and second harmonic fields oriented parallel to the polar axis, the value of $χ^{(2)}$ is larger by almost one order of magnitude than its value in the archetypal electro-optic materials GaAs \cite{bergfeld2003second} and ZnTe \cite{wagner1998dispersion}, and in fact larger than reported in any crystal to date.

cond-mat.mtrl-sci↗

arXiv2017

Counter-propagating radiative shock experiments on the Orion laser and the formation of radiative precursors

We present results from new experiments to study the dynamics of radiative shocks, reverse shocks and radiative precursors. Laser ablation of a solid piston by the Orion high-power laser at AWE Aldermaston UK was used to drive radiative shocks into a gas cell initially pressurised between $0.1$ and $1.0 \ bar$ with different noble gases. Shocks propagated at {$80 \pm 10 \ km/s$} and experienced strong radiative cooling resulting in post-shock compressions of { $\times 25 \pm 2$}. A combination of X-ray backlighting, optical self-emission streak imaging and interferometry (multi-frame and streak imaging) were used to simultaneously study both the shock front and the radiative precursor. These experiments present a new configuration to produce counter-propagating radiative shocks, allowing for the study of reverse shocks and providing a unique platform for numerical validation. In addition, the radiative shocks were able to expand freely into a large gas volume without being confined by the walls of the gas cell. This allows for 3-D effects of the shocks to be studied which, in principle, could lead to a more direct comparison to astrophysical phenomena. By maintaining a constant mass density between different gas fills the shocks evolved with similar hydrodynamics but the radiative precursor was found to extend significantly further in higher atomic number gases ($\sim$$4$ times further in xenon than neon). Finally, 1-D and 2-D radiative-hydrodynamic simulations are presented showing good agreement with the experimental data.

physics.plasm-ph↗

arXiv2015

Photoexcited states of the harmonic honeycomb iridate γ-Li$_2$IrO$_3$

We report equilibrium and nonequilibrium optical measurements on the recently synthesized "harmonic" honeycomb iridate γ-Li$_2$IrO$_3$ (LIO), as well as the layered honeycomb iridate Na$_2$IrO$_3$ (NIO). Using Fourier transform infrared microscopy we performed reflectance measurements on LIO, from which we obtained the optical conductivity below 2 eV. In addition we measured the photoinduced changed in reflectance, ΔR, as a function of time, t, temperature, T, and probe field polarization in both LIO and NIO. In LIO, ΔR(t,T) is anisotropic and comprised of three T dependent components. Two of these components are related to the onset of magnetic order and the third is related to a photoinduced population of metastable electronic excited states. In NIO, ΔR(t,T) has a single T dependent component that is strikingly similar to the electronic excitation component of ΔR in LIO. Through analysis and comparison of ΔR(t,T) for two compounds, we extract information on the onset of magnetic correlations at and above the transition temperature in LIO, the bare spin-flip scattering rate in equilibrium, the lifetime of low-lying quasiparticle excitations, and the polarization dependence of optical transitions that are sensitive to magnetic order.

cond-mat.str-el↗