arXiv subjects

S. Quan

Publications and source records attributed to S. Quan.

6 recordsLinked to original sources

arXiv2025

New insights into hydrogen-assisted intergranular cracking in nickel

We characterize the grain boundary (GB) susceptibility to hydrogen-assisted intergranular cracking in pure nickel as a function of coincident site lattice value ($\Sigma$-n), over a wide range of hydrogen concentrations (4 to 14 wppm). Cracks on the surface and within the bulk material were identified across the entire gauge region of the specimens. The susceptibility of GBs to crack initiation and propagation was evaluated by separating cracks containing single GB or multiple GBs. A larger loss in fracture strain, a smaller reduction in area, and an increase in the percentage of intergranular fracture indicated a higher degree of embrittlement at elevated hydrogen concentrations. The number of cracks was significantly higher on the surface than in the bulk for the most severe hydrogen charging conditions ($\geq$ 8 wppm), while a similar number was observed for lower concentrations. The propensity for hydrogen-assisted intergranular cracking at different types of GBs on the surface and in the bulk material was consistent, indicating that while cathodic charging can promote surface cracks, it does not significantly impact the GBs relative susceptibility. The $\Sigma$-3 boundaries were the most resistant to cracking, as evidenced by the considerably lower fraction of these GBs exhibiting intergranular cracking at all hydrogen concentrations considered. This contrasts literature findings for Ni alloys and can be explained by the segregation energies and reductions in the cohesive strength with hydrogen, with less favorable trapping at the $\Sigma$-3 boundaries. No evidence of plasticity-mediated cracking initiation was observed.

cond-mat.mtrl-sci↗

arXiv2024

High Performance Operation of a Direct-Current and Superconducting Radio-Frequency Combined Photocathode Gun

Superconducting radio-frequency (SRF) guns are promising candidates to deliver high brightness continuous-wave (CW) electron beams for new generations of coherent linac light sources, ultrafast electron diffractions, MeV pulsed beam applications, etc. To solve the compatibility problem of semiconductor photocathodes, a hybrid gun combining a direct-current gap and an SRF cavity has been developed. The gun, employing K2CsSb photocathodes driven by a green laser, has been brought into stable CW operation with a dark current below 100 pA, delivering electron beams at an energy gain of 2.4 MeV, an electron bunch charge of 100 pC, and a repetition rate of 1 MHz. A normalized beam emittance of 0.54 mm-mrad has been achieved at the bunch charge of 100 pC and peak current of about 6 A. CW operation at 81.25 MHz repetition rate has also been tested with the maximum average beam current reaching 3 mA.

physics.acc-ph↗

arXiv2019

Microscopic core-quasiparticle coupling model for spectroscopy of odd-mass nuclei with octupole correlations

[Background] Predictions of spectroscopic properties of low-lying states are critical for nuclear structure studies. Theoretical methods can be particularly involved for odd-mass nuclei because of the interplay between the unpaired nucleon and collective degrees of freedom. Only a few models have been developed for systems in which octupole collective degrees of freedom play a role. [Purpose] We aim to predict spectroscopic properties of odd-mass nuclei characterized by octupole shape deformation, employing a model that describes single-particle and collective degrees of freedom within the same microscopic framework. [Method] A microscopic core-quasiparticle coupling (CQC) model based on the covariant density functional theory is developed, which includes collective excitations of even-mass core nuclei and single-particle states of the odd nucleon, calculated using a quadrupole-octupole collective Hamiltonian combined with a constrained reflection-asymmetric relativistic Hartree-Bogoliubov model. [Results] Model predictions for low-energy excitation spectra and transition rates of odd-mass radium isotopes $^{223, 225, 227}$Ra are shown to be in good agreement with available data. [Conclusions] A microscopic CQC model based on covariant density functional theory has been developed for odd-mass nuclei characterized by both quadrupole and octupole shape deformations. Theoretical results reproduce data in odd-mass Ra isotopes and provide useful predictions for future studies of octupole correlations in nuclei and related phenomena.

nucl-th↗

arXiv2018

Nuclear quantum shape-phase transitions in odd-mass systems

Microscopic signatures of nuclear ground-state shape phase transitions in odd-mass Eu isotopes are explored starting from excitation spectra and collective wave functions obtained by diagonalization of a core-quasiparticle coupling Hamiltonian based on energy density functionals. As functions of the physical control parameter -- the number of nucleons -- theoretical low-energy spectra, two-neutron separation energies, charge isotope shifts, spectroscopic quadrupole moments, and $E2$ reduced transition matrix elements accurately reproduce available data, and exhibit more pronounced discontinuities at neutron number $N=90$, compared to the adjacent even-even Sm and Gd isotopes. The enhancement of the first-order quantum phase transition in odd-mass systems can be attributed to a shape polarization effect of the unpaired proton which, at the critical neutron number, starts predominantly coupling to Gd core nuclei that are characterized by larger quadrupole deformation and weaker proton pairing correlations compared to the corresponding Sm isotopes.

nucl-th↗

arXiv2017

Microscopic core-quasiparticle coupling model for spectroscopy of odd-mass nuclei

Predictions of the spectroscopic properties of low-lying states are critical for nuclear structure studies, but are problematic for nuclei with an odd nucleon due to the interplay of the unpaired single particle with nuclear collective degrees of freedom. In this work, a microscopic core-quasiparticle coupling (CQC) model based on the covariant density functional theory is developed that contains the collective excitations of even-mass cores and spherical single-particle states of the odd nucleon as calculated from a quadrupole collective Hamiltonian combined with a constrained triaxial relativistic Hartree-Bogoliubov model. Predictions of the new model for excitation energies, kinematic and dynamic moments of inertia, and transition rates are shown to be in good agreement with results of low-lying spectroscopy measurements of the axially deformed odd-proton nucleus $^{159}$Tb and the odd-neutron nucleus $^{157}$Gd. Future studies with additional nuclei are planned.

nucl-th↗

arXiv2017

Global analysis of quadrupole shape invariants based on covariant energy density functionals

Coexistence of different geometric shapes at low energies presents a universal structure phenomenon that occurs over the entire chart of nuclides. Studies of the shape coexistence are important for understanding the microscopic origin of collectivity and modifications of shell structure in exotic nuclei far from stability. The aim of this work is to provide a systematic analysis of characteristic signatures of coexisting nuclear shapes in different mass regions, using a global self-consistent theoretical method based on universal energy density functionals and the quadrupole collective model. The low-energy excitation spectrum and quadrupole shape invariants of the two lowest $0^{+}$ states of even-even nuclei are obtained as solutions of a five-dimensional collective Hamiltonian (5DCH) model, with parameters determined by constrained self-consistent mean-field calculations based on the relativistic energy density functional PC-PK1, and a finite-range pairing interaction. The theoretical excitation energies of the states: $2^+_1$, $4^+_1$, $0^+_2$, $2^+_2$, $2^+_3$, as well as the $B(E2; 0^+_1\to 2^+_1)$ values, are in very good agreement with the corresponding experimental values for 621 even-even nuclei. Quadrupole shape invariants have been implemented to investigate shape coexistence, and the distribution of possible shape-coexisting nuclei is consistent with results obtained in recent theoretical studies and available data. The present analysis has shown that, when based on a universal and consistent microscopic framework of nuclear density functionals, shape invariants provide distinct indicators and reliable predictions for the occurrence of low-energy coexisting shapes. This method is particularly useful for studies of shape coexistence in regions far from stability where few data are available.

nucl-th↗