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S. Reitzenstein

Publications and source records attributed to S. Reitzenstein.

At least 19 recordsLinked to original sources

Self-aligned photonic defect microcavities with site-controlled quantum dots

Despite the superiority in quantum properties, self-assembled semiconductor quantum dots face challenges in terms of scalable device integration because of their random growth positions, originating from the Stranski-Krastanov growth mode. Even with existing site-controlled growth techniques, for example, nanohole or buried stressor concepts, a further lithography and etching step with high spatial alignment requirements isnecessary to accurately integrate QDs into the nanophotonic devices. Here, we report on the fabrication and characterization of strain-induced site-controlled microcavities where site-controlled quantum dots are positioned at the antinode of the optical mode field in a self-aligned manner without the need of any further nano-processing. We show that the Q-factor, mode volume, height, and the ellipticity of site-controlled microcavities can be tailored by the size of an integrated AlAs/Al2O3 buried stressor, with an opening ranging from 1 to 4 $\mu$m. Lasing signatures, including super-linear input-output response, linewidth narrowing near threshold, and gain competition above threshold, are observed for a 3.6-$\mu$m self-aligned cavity with a Q-factor of 18000. Furthermore, by waiving the rather complex lateral nano-structuring usually performed during the fabrication process of micropillar lasers and vertical-cavity surface emitting lasers, quasi-planar site-controlled cavities exhibit no detrimental effects of excitation power induced heating and thermal rollover. Our straightforward deterministic nanofabrication concept of high-quality quantum dot microcavities integrates seamlessly with the industrial-matured manufacturing process and the buried-stressor techniques, paving the way for exceptional scalability and straightforward manufacturing of high-\b{eta} microlasers and bright quantum light sources.

cond-mat.mes-hall

Energy-time entanglement from a resonantly driven quantum dot three-level system

Entanglement is a major resource in advanced quantum technology, where it can enable secure exchange of information over large distances. Energy-time entanglement is particularly attractive for its beneficial robustness in fiber-based quantum communication and can be demonstrated in the Franson interferometer. We report on Franson-type interference from a resonantly driven biexciton cascade under continuous wave excitation. Our measurements yield a maximum visibility of (73 $\pm$ 2)% surpassing the limit of violation of Bell's inequality (70.7%) by more than one standard deviation. Despite being unable to satisfy a loophole free violation, our work demonstrates promising results concerning future works on such a system. Furthermore, our systematical studies on the impact of driving strength indicate that dephasing mechanisms and deviations from the cascaded emission have major impact on the degree of the measured energy-time entanglement.

quant-ph

Quantum fluctuations and lineshape anomaly in a high-$\beta$ silver-coated InP-based metallic nanolaser

Metallic nanocavity lasers provide important technological advancement towards even smaller integrable light sources. They give access to widely unexplored lasing physics in which the distinction between different operational regimes, like those of thermal or a coherent light emission, becomes increasingly challenging upon approaching a device with a near-perfect spontaneous-emission coupling factor $\beta$. In fact, quantum-optical studies have to be employed to reveal a transition to coherent emission in the intensity fluctuation behavior of nanolasers when the input-output characteristic appears thresholdless for $\beta = 1$ nanolasers. Here, we identify a new indicator for lasing operation in high-$\beta$ lasers by showing that stimulated emission can give rise to a lineshape anomaly manifesting as a transition from a Lorentzian to a Gaussian component in the emission linewidth that dominates the spectrum above the lasing threshold.

physics.optics

Measuring higher-order photon correlations of faint quantum light: a short review

Normalized correlation functions provide expedient means for determining the photon-number properties of light. These higher-order moments, also called the normalized factorial moments of photon number, can be utilized both in the fast state classification and in-depth state characterization. Further, non-classicality criteria have been derived based on their properties. Luckily, the measurement of the normalized higher-order moments is often loss-independent making their observation with lossy optical setups and imperfect detectors experimentally appealing. The normalized higher-order moments can for example be extracted from the photon-number distribution measured with a true photon-number-resolving detector or accessed directly via manifold coincidence counting in the spirit of the Hanbury Brown and Twiss experiment. Alternatively, they can be inferred via homodyne detection. Here, we provide an overview of different kind of state classification and characterization tasks that take use of normalized higher-order moments and consider different aspects in measuring them with free-traveling light.

quant-ph

Intrinsic circularly-polarized exciton emission in a twisted van-der-Waals heterostructure

The investigation of excitons in van-der-Waals heterostructures has led to profound insights into the interplay of crystal symmetries and fundamental effects of light-matter coupling. In particular, the polarization selection rules in undistorted, slightly twisted heterostructures of MoSe$_2$/WSe$_2$ were found to be connected with the Moir\'e superlattice. Here, we report the emergence of a significant degree of circular polarization of excitons in such a hetero-structure upon non-resonant driving with a linearly polarized laser. The effect is present at zero magnetic field, and sensibly reacts on perpendicularly applied magnetic field. The giant magnitude of polarization, which cannot be explained by conventional birefringence or optical activity of the twisted lattice, suggests a kinematic origin arising from an emergent pyromagnetic symmetry in our structure, which we exploit to gain insight into the microscopic processes of our device.

cond-mat.mes-hall

Optical pumping of quantum dot micropillar lasers

Arrays of quantum dot micropillar lasers are an attractive technology platform for various applications in the wider field of nanophotonics. Of particular interest is the potential efficiency enhancement as consequence of cavity quantum electrodynamics effects which makes them prime candidates for next generation photonic neurons in neural network hardware. However, in particular for optical pumping their power-conversion efficiency can be very low. Here we perform an in-depth experimental analysis of quantum dot microlasers and investigate their input-output relationship over a wide range of optical pumping conditions. We find that the current energy efficiency limitation is caused by disadvantageous optical pumping concepts and by a low exciton conversion efficiency. Our results indicate that for non-resonant pumping into the GaAs matrix (wetting layer), 3.4% (0.6%) of the optical pump is converted into lasing-relevant excitons, and of those only 2% (0.75%) provide gain to the lasing transition. Based on our findings we propose to improve the pumping efficiency by orders of magnitude by increasing the aluminium content of the AlGaAs/GaAs mirror pairs in the upper Bragg reflector.

physics.optics

Developing of a photonic hardware platform for brain-inspired computing based on $5\times5$ VCSEL arrays

Brain-inspired computing concepts like artificial neural networks have become promising alternatives to classical von Neumann computer architectures. Photonic neural networks target the realizations of neurons, network connections and potentially learning in photonic substrates. Here, we report the development of a nanophotonic hardware platform of fast and energy-efficient photonic neurons via arrays of high-quality vertical cavity surface emitting lasers (VCSELs). The developed $5\times5$ VCSEL arrays provide high optical injection locking efficiency through homogeneous fabrication combined with individual control over the laser wavelengths. Injection locking is crucial for the reliable processing of information in VCSEL-based photonic neurons, and we demonstrate the suitability of the VCSEL arrays by injection locking measurements and current-induced spectral fine-tuning. We find that our investigated array can readily be tuned to the required spectral homogeneity, and as such show that VCSEL arrays based on our technology can act as highly energy efficient and ultra-fast photonic neurons for next generation photonic neural networks. Combined with fully parallel photonic networks our substrates are promising for ultra-fast operation reaching 10s of GHz bandwidths, and we show that a nonlinear transformation based on our lasers will consume only about 100 fJ per VCSEL, which is highly competitive, compared to other platforms.

cs.ET

Deterministically fabricated quantum dot single-photon source emitting indistinguishable photons in the telecom O-band

In this work we develop and study single-photon sources based on InGaAs quantum dots (QDs) emitting in the telecom O-band. The quantum devices are fabricated using in-situ electron beam lithography in combination with the thermocompression bonding to realize a backside gold mirror. Our structures are based on InGaAs/GaAs heterostructures, where the QD emission is redshifted towards the telecom O-band at 1.3 {\mu}m via a strain reducing layer. QDs pre-selected by cathodoluminescence mapping are embedded into mesa structures with a back-side gold mirror for enhanced photon-extraction efficiency. Photon-autocorrelation measurements under pulsed non-resonant wetting-layer excitation are performed at temperatures up to 40 K showing pure single-photon emission which makes the devices compatible with stand-alone operation using Stirling cryocoolers. Using pulsed p-shell excitation we realize single-photon emission with high multi-photon suppression of g(2)(0) = 0.027 +- 0.005, post-selected two-photon interference of about (96 +- 10) % and an associated coherence time of (212 +- 25) ps. Moreover, the structures show an extraction efficiency of ~5 %, which compares well with values expected from numeric simulations of this photonic structure. Further improvements on our devices will enable implementations of quantum communication via optical fibers.

physics.app-ph

Photon-number parity of heralded single photons from a Bragg-reflection waveguide reconstructed loss-tolerantly via moment generating function

Due to their strict photon-number correlation, the twin beams produced in parametric down-conversion (PDC) work well for heralded state generation. Often, however, this state manipulation is distorted by the optical losses in the herald and by the higher photon-number contributions inevitable in the PDC process. In order to find feasible figures of merit for characterizing the heralded states, we investigate their normalized factorial moments of the photon number that can be accessed regardless of the optical losses in the detection. We then perform a measurement of the joint photon statistics of twin beams from a semiconductor Bragg-reflection waveguide with transition-edge sensors acting as photon-number-resolving detectors. We extract the photon-number parity of heralded single photons in a loss-tolerant fashion by utilizing the moment generating function. The photon-number parity is highly practicable in quantum state characterization, since it takes into account the complete photon-number content of the target state.

quant-ph

A deterministically fabricated spectrally-tunable quantum dot based single-photon source

Spectrally-tunable quantum-light sources are key elements for the realization of long-distance quantum communication. A deterministically fabricated single-photon source with a photon-extraction efficiency of {\eta}=(20 +- 2) % and a tuning range of {\Delta}E=2.5 meV is presented here. The device consists of a single pre-selected quantum dot monolithically integrated into a microlens which is bonded onto a piezoelectric actuator via thermocompression goldbonding. The thin gold layer simultaneously acts as a backside mirror for the quantum dot emission, which is efficiently extracted from the device by an optimized lens structure patterned via 3D in-situ electron-beam lithography. The single-photon nature of the emission is proven by photon-autocorrelation measurements with $g^{(2)}$ ({\tau}=0)=0.04 +- 0.02. The combination of deterministic fabrication, spectral-tunability and high broadband photon-extraction efficiency makes the microlens single-photon source an interesting building block towards the realization of quantum repeaters networks.

cond-mat.mes-hall

Photon number-resolved measurement of an exciton-polariton condensate

We measure the full photon-number distribution emitted from a Bose condensate of microcavity exciton-polaritons confined in a micropillar cavity. The statistics are acquired by means of a photonnumber resolving transition edge sensor. We directly observe that the photon-number distribution evolves with the non-resonant optical excitation power from geometric to quasi-Poissonian statistics, which is canonical for a transition from a thermal to a coherent state. Moreover, the photon-number distribution allows evaluating the higher-order photon correlations, shedding further light on the coherence formation and phase transition of the polariton condensate. The experimental data is analyzed in terms of thermal coherent states which allows one to directly extract the thermal and coherent fraction from the measured distributions. These results pave the way for a full understanding of the contribution of interactions in light-matter condensates in the coherence buildup at threshold.

cond-mat.mes-hall

Controlling the gain contribution of background emitters in few-quantum-dot microlasers

We provide experimental and theoretical insight into single-emitter lasing effects in a quantum dot (QD)-microlaser under controlled variation of background gain provided by off-resonant discrete gain centers. For that purpose, we apply an advanced two-color excitation concept where the background gain contribution of off-resonant QDs can be continuously tuned by precisely balancing the relative excitation power of two lasers emitting at different wavelengths. In this way, by selectively exciting a single resonant QD and off-resonant QDs, we identify distinct single-QD signatures in the lasing characteristics and distinguish between gain contributions of a single resonant emitter and a countable number of off-resonant background emitters to the optical output of the microlaser. We address the important question whether single-QD lasing is feasible in experimentally accessible systems and show that, for the investigated microlaser, the single-QD gain needs to be supported by the background gain contribution of off-resonant QDs to reach the transition to lasing. Interestingly, while a single QD cannot drive the investigated micropillar into lasing, its relative contribution to the emission can be as high as 70% and it dominates the statistics of emitted photons in the intermediate excitation regime below threshold.

cond-mat.mes-hall

Pump-power-driven mode switching in a microcavity device and its relation to Bose-Einstein condensation

We investigate the switching of the coherent emission mode of a bimodal microcavity device, occurring when the pump power is varied. We compare experimental data to theoretical results and identify the underlying mechanism to be based on the competition between the effective gain on the one hand and the intermode kinetics on the other. When the pumping is ramped up, above a threshold the mode with the largest effective gain starts to emit coherent light, corresponding to lasing. In contrast, in the limit of strong pumping it is the intermode kinetics that determines which mode acquires a large occupation and shows coherent emission. We point out that this latter mechanism is akin to the equilibrium Bose-Einstein condensation of massive bosons. Thus, the mode switching in our microcavity device can be viewed as a minimal instance of Bose-Einstein condensation of photons. We, moreover, show that the switching from one cavity mode to the other occurs always via an intermediate phase where both modes are emitting coherent light and that it is associated with both superthermal intensity fluctuations and strong anticorrelations between both modes.

physics.optics

Impact of phonons on dephasing of individual excitons in deterministic quantum dot microlenses

Optimized light-matter coupling in semiconductor nanostructures is a key to understand their optical properties and can be enabled by advanced fabrication techniques. Using in-situ electron beam lithography combined with a low-temperature cathodoluminescence imaging, we deterministically fabricate microlenses above selected InAs quantum dots (QDs) achieving their efficient coupling to the external light field. This enables to perform four-wave mixing micro-spectroscopy of single QD excitons, revealing the exciton population and coherence dynamics. We infer the temperature dependence of the dephasing in order to address the impact of phonons on the decoherence of confined excitons. The loss of the coherence over the first picoseconds is associated with the emission of a phonon wave packet, also governing the phonon background in photoluminescence (PL) spectra. Using theory based on the independent boson model, we consistently explain the initial coherence decay, the zero-phonon line fraction, and the lineshape of the phonon-assisted PL using realistic quantum dot geometries.

cond-mat.mes-hall

Emission from quantum-dot high- microcavities: transition from spontaneous emission to lasing and the effects of superradiant emitter coupling

Measured and calculated results are presented on the emission properties of a new class of emitters operating in the cavity quantum electrodynamics regime. The structures are based on high-finesse GaAs/AlAs micropillar cavities, each with an active medium consisting of a layer of InGaAs quantum dots and distinguishing feature of having substantial fraction of spontaneous emission channeled into one cavity mode (high-beta factor). This paper shows that the usual criterion for lasing with a conventional (low-beta factor) cavity, a sharp nonlinearity in an input-output curve accompanied by noticeable linewidth narrowing, has to be reinforced by the equal-time second-order photon autocorrelation function for confirming lasing. It will also show that the equal-time second-order photon autocorrelation function is useful for recognizing superradiance, a manifestation of the correlations possible in high- microcavities operating with quantum dots. In terms of consolidating the collected data and identifying the physics underlying laser action, both theory and experiment suggest a sole dependence on intracavity photon number. Evidence for this comes from all our measured and calculated data on emission coherence and fluctuation, for devices ranging from LEDs and cavity-enhanced LEDs to lasers, lying on the same two curves: one for linewidth narrowing versus intracavity photon number and the other for g(2)(0) versus intracavity photon number.

cond-mat.mes-hall

Photon-Statistics Excitation Spectroscopy of a Single Two Level System

We investigate the influence of the photon statistics on the excitation dynamics of a single two level system. A single semiconductor quantum dot represents the two level system and is resonantly excited either with coherent laser light, or excited with chaotic light, with photon statistics corresponding to that of thermal radiation. Experimentally, we observe a reduced absorption cross-section under chaotic excitation in the steady-state. In the transient regime, the Rabi oscillations observable under coherent excitation disappear under chaotic excitation. Likewise, in the emission spectrum the well-known Mollow triplet, which we observe under coherent drive, disappears under chaotic excitation. Our observations are fully consistent with theoretical predictions based on the semi-classical Bloch equation approach.

quant-ph

Generating single photons at GHz modulation-speed using electrically controlled quantum dot microlenses

We report on the generation of single-photon pulse trains at a repetition rate of up to 1 GHz. We achieve this high speed by modulating the external voltage applied on an electrically contacted quantum dot microlens, which is optically excited by a continuous-wave laser. By modulating the photoluminescence of the quantum dot microlens using a square-wave voltage, single-photon emission is triggered with a response time as short as 270 ps being 6.5 times faster than the radiative lifetime of 1.75 ns. This large reduction in the characteristic emission time is enabled by a rapid capacitive gating of emission from the quantum dot placed in the intrinsic region of a p-i-n-junction biased below the onset of electroluminescence. Here, the rising edge of the applied voltage pulses triggers the emission of single photons from the optically excited quantum dot. The non-classical nature of the photon pulse train generated at GHz-speed is proven by intensity autocorrelation measurements. Our results combine optical excitation with fast electrical gating and thus show promise for the generation of indistinguishable single photons at high rates, exceeding the limitations set by the intrinsic radiative lifetime.

cond-mat.mes-hall

Exploring Dephasing of a Solid-State Quantum Emitter via Time- and Temperature- Dependent Hong-Ou-Mandel Experiments

We probe the indistinguishability of photons emitted by a semiconductor quantum dot (QD) via time- and temperature- dependent two-photon interference (TPI) experiments. An increase in temporal-separation between consecutive photon emission events, reveals a decrease in TPI visibility on a nanosecond timescale, theoretically described by a non-Markovian noise process in agreement with fluctuating charge-traps in the QD's vicinity. Phonon-induced pure dephasing results in a decrease in TPI visibility from $(96\pm4)\,$\% at 10\,K to a vanishing visibility at 40\,K. In contrast to Michelson-type measurements, our experiments provide direct access to the time-dependent coherence of a quantum emitter at a nanosecond timescale.

quant-ph