arXiv subjects

S. Rohart

Publications and source records attributed to S. Rohart.

17 recordsLinked to original sources

arXiv2024

Spin-Wave-Assisted Thermal Reversal of Epitaxial Perpendicular Magnetic Nanodots

The magnetic susceptibility of self-organized two-dimensional Co nanodots on Au(111) has been measured as a function of their size in the 2-7~nm diameter range. We show that the activation energy for the thermal reversal displays a power law behavior with the dot volume. Atomic scale simulations based on the Heisenberg hamiltonian show that this behavior is due to a deviation from the macrospin model for dot size as small as 3~nm in diameter. This discrepancy is attributed to finite temperature effects through the thermal excitation of spin-wave modes inside the particles

cond-mat.mes-hall↗

arXiv2021

Staggered spin-orbit interaction in a nanoscale device

The coupling of the spin and the motion of charge carriers stems directly from the atomic structure of a conductor. It has become an important ingredient for the emergence of topological matter, and, in particular, topological superconductivity which could host non-abelian excitations such as Majorana modes or parafermions. These modes are sought after mostly in semiconducting platforms which are made of heavy atoms and therefore exhibit naturally a large spin-orbit interaction. Creating domain walls in the spin orbit interaction at the nanoscale may turn out to be a crucial resource for engineering topological excitations suitable for universal topological quantum computing. For example, it has been proposed for exploring exotic electronic states or for creating hinge states. Realizing this in natural platforms remains a challenge. In this work, we show how this can be alternatively implemented by using a synthetic spin orbit interaction induced by two lithographically patterned magnetically textured gates. By using a double quantum dot in a light material -- a carbon nanotube -- embedded in a microwave cavity, we trigger hopping between two adjacent orbitals with the microwave photons and directly compare the wave functions separated by the domain wall via the light-matter coupling. We show that we can achieve an engineered staggered spin-orbit interaction with a change of strength larger than the hopping energy between the two sites.

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arXiv2020

Strength and length-scale of the interaction between domain walls and pinning disorder in thin ferromagnetic films

We explore the magnetic-field-driven motion of domain walls with different chiralities in thin ferromagnetic films made of Pt/Co/Pt, Au/Co/Pt, and Pt/Co/Au. From the analysis of domain wall dynamics, we extract parameters characterizing the interaction between domain walls and weak pinning disorder of the films. The variations of domain wall structure, controlled by an in-plane field, are found to modify the characteristic length-scale of pinning in strong correlation with the domain wall width, whatever its chirality and the interaction strength between domain walls and pinning defects. These findings should be also relevant for a wide variety of elastic interfaces moving in weak pinning disordered media.

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arXiv2019

Synthetic spin orbit interaction for Majorana devices

The interplay of superconductivity with a non-trivial spin texture holds promises for the engineering of non-abelian Majorana quasi-particles. A wide class of systems expected to exhibit exotic correlations are based on nanoscale conductors with strong spin-orbit interaction, subject to a strong external magnetic field. The strength of the spin-orbit coupling is a crucial parameter for the topological protection of Majorana modes as it forbids other trivial excitations at low energy. The spin-orbit interaction is in principle intrinsic to a material. As a consequence, experimental efforts have been recently focused on semiconducting nano-conductors or spin-active atomic chains contacted to a superconductor. Alternatively, we show how both a spin-orbit and a Zeeman effect can be autonomously induced by using a magnetic texture coupled to any low dimensional conductor, here a carbon nanotube. Transport spectroscopy through superconducting contacts reveals oscillations of Andreev like states under a change of the magnetic texture. These oscillations are well accounted for by a scattering theory and are absent in a control device with no magnetic texture. A large synthetic spin-orbit energy of about 1.1 meV, larger than the intrinsic spin orbit energy in many other platforms, is directly derived from the number of oscillations. Furthermore, a robust zero energy state, the hallmark of devices hosting localized Majorana modes, emerges at zero magnetic field. Our findings synthetize all the features for the emergence of Majorana modes at zero magnetic field in a controlled, local and autonomous fashion. It could be used for advanced experiments, including microwave spectroscopy and braiding operations, which are at the heart of new schemes of topological quantum computation.

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arXiv2018

Current-induced nucleation and dynamics of skyrmions in a Co-based Heusler alloy

We demonstrate room-temperature stabilization of dipolar magnetic skyrmions with diameters in the range of $100$ nm in a single ultrathin layer of the Heusler alloy Co$_2$FeAl (CFA) under moderate magnetic fields. Current-induced skyrmion dynamics in microwires is studied with a scanning Nitrogen-Vacancy magnetometer operating in the photoluminescence quenching mode. We first demonstrate skyrmion nucleation by spin-orbit torque and show that its efficiency can be significantly improved using tilted magnetic fields, an effect which is not specific to Heusler alloys and could be advantageous for future skyrmion-based devices. We then show that current-induced skyrmion motion remains limited by strong pinning effects, even though CFA is a magnetic material with a low magnetic damping parameter.

cond-mat.mtrl-sci↗

arXiv2017

Skyrmion morphology in ultrathin magnetic films

Nitrogen-vacancy magnetic microscopy is employed in quenching mode as a non-invasive, high resolution tool to investigate the morphology of isolated skyrmions in ultrathin magnetic films. The skyrmion size and shape are found to be strongly affected by local pinning effects and magnetic field history. Micromagnetic simulations including static disorder, based on a physical model of grain-to-grain thickness variations, reproduce all experimental observations and reveal the key role of disorder and magnetic history in the stabilization of skyrmions in ultrathin magnetic films. This work opens the way to an in-depth understanding of skyrmion dynamics in real, disordered media.

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arXiv2017

Making the Dzyaloshinskii-Moriya interaction visible

Brillouin light spectroscopy is a powerful and robust technique for measuring the interfacial Dzyaloshinskii-Moriya interaction in thin films with broken inversion symmetry. Here we show that the magnon visibility, i.e. the intensity of the inelastically scattered light, strongly depends on the thickness of the dielectric seed material - SiO$_2$. By using both, analytical thin-film optics and numerical calculations, we reproduce the experimental data. We therefore provide a guideline for the maximization of the signal by adapting the substrate properties to the geometry of the measurement. Such a boost-up of the signal eases the magnon visualization in ultrathin magnetic films, speeds-up the measurement and increases the reliability of the data.

cond-mat.mtrl-sci↗

arXiv2016

Path to collapse for an isolated Néel skyrmion

A path method is implemented in order to precisely and generally describe the collapse of isolated skyrmions in a Co/Pt(111) monolayer, on the basis of atomic scale simulations. Two collapse mechanisms with different energy barriers are found. The most obvious path, featuring a homogeneous shrinking gives the largest energy, whereas the lowest energy barrier is shown to comply with the outcome of Langevin dynamics under a destabilizing field of 0.25 T, with a lifetime of 20~ns at around 80~K. For this lowest energy barrier path, skyrmion destabilization occurs much before any topology change, suggesting that topology plays a minor role in the skyrmion stability. On the contrary, an important role appears devoted to the Dzyaloshinskii-Moriya interaction, establishing a route towards improved skyrmion stability.

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arXiv2016

Direct measurement of interfacial Dzyaloshinskii-Moriya interaction in X/CoFeB/MgO heterostructures with a scanning-NV magnetometer

The Dzyaloshinskii-Moriya Interaction (DMI) has recently attracted considerable interest owing to its fundamental role in the stabilization of chiral spin textures in ultrathin ferromagnets, which are interesting candidates for future spintronic technologies. Here we employ a scanning nano-magnetometer based on a single nitrogen-vacancy (NV) defect in diamond to locally probe the strength of the interfacial DMI in CoFeB/MgO ultrathin films grown on different heavy metal underlayers X=Ta,TaN, and W. By measuring the stray field emanating from DWs in micron-long wires of such materials, we observe deviations from the Bloch profile for TaN and W underlayers that are consistent with a positive DMI value favoring right-handed chiral spin structures. Moreover, our measurements suggest that the DMI constant might vary locally within a single sample, illustrating the importance of local probes for the study of magnetic order at the nanoscale.

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arXiv2014

The nature of domain walls in ultrathin ferromagnets revealed by scanning nanomagnetometry

The recent observation of current-induced domain wall (DW) motion with large velocity in ultrathin magnetic wires has opened new opportunities for spintronic devices. However, there is still no consensus on the underlying mechanisms of DW motion. Key to this debate is the DW structure, which can be of Bloch or Néel type, and dramatically affects the efficiency of the different proposed mechanisms. To date, most experiments aiming to address this question have relied on deducing the DW structure and chirality from its motion under additional in-plane applied fields, which is indirect and involves strong assumptions on its dynamics. Here we introduce a general method enabling direct, in situ, determination of the DW structure in ultrathin ferromagnets. It relies on local measurements of the stray field distribution above the DW using a scanning nanomagnetometer based on the Nitrogen-Vacancy defect in diamond. We first apply the method to a Ta/Co40Fe40B20(1 nm)/MgO magnetic wire and find clear signature of pure Bloch DWs. In contrast, we observe left-handed Néel DWs in a Pt/Co(0.6 nm)/AlOx wire, providing direct evidence for the presence of a sizable Dzyaloshinskii-Moriya interaction (DMI) at the Pt/Co interface. This method offers a new path for exploring interfacial DMI in ultrathin ferromagnets and elucidating the physics of DW motion under current.

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arXiv2014

NV-center imaging of bubble domains in a 6 Å film of cobalt with perpendicular magnetization

We employ a scanning NV-center microscope to perform stray field imaging of bubble magnetic domains in a perpendicularly magnetized Pt/Co/AlOx trilayer with 6 Å of Co. The stray field created by the domain walls is quantitatively mapped with few-nanometer spatial resolution, with a probe-sample distance of about 100 nm. As an example of application, we show that it should be possible to determine the Bloch or Néel nature of the domain walls, which is of crucial importance to the understanding of current-controlled domain wall motion.

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arXiv2014

Quantitative stray field imaging of a magnetic vortex core

Thin-film ferromagnetic disks present a vortex spin structure whose dynamics, added to the small size (~10 nm) of their core, earned them intensive study. Here we use a scanning nitrogen-vacancy (NV) center microscope to quantitatively map the stray magnetic field above a 1 micron-diameter disk of permalloy, unambiguously revealing the vortex core. Analysis of both probe-to-sample distance and tip motion effects through stroboscopic measurements, allows us to compare directly our quantitative images to micromagnetic simulations of an ideal structure. Slight perturbations with respect to the perfect vortex structure are clearly detected either due to an applied in-plane magnetic field or imperfections of the magnetic structures. This work demonstrates the potential of scanning NV microscopy to map tiny stray field variations from nanostructures, providing a nanoscale, non-perturbative detection of their magnetic texture.

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arXiv2013

Skyrmion confinement in ultrathin film nanostructures in the presence of Dzyaloshinskii-Moriya interaction

We study the modification of micromagnetic configurations in nanostructures, due to the Dzyaloshinskii-Moriya interaction (DMI) that appear at the interface of an ultrathin film. We show that this interaction leads to new micromagnetic boundary conditions that bend the magnetization at the edges. We explore several cases of ultrathin film nanostructures that allow analytical calculations (1D systems, domain walls, cycloids and skyrmions), compare with fully numerical calculations, and show that a good physical understanding of this new type of micromagnetics can be reached. We particularly focus on skyrmions confined in circular nanodots and show that edges allow for the isolation of single skyrmions for a large range of the DMI parameter.

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arXiv2013

Stray-field imaging of magnetic vortices with a single diamond spin

Despite decades of advances in magnetic imaging, obtaining direct, quantitative information with nanometer scale spatial resolution remains an outstanding challenge. Recently, a new technique has emerged that employs a single nitrogen-vacancy (NV) defect in diamond as an atomic-size magnetometer. Although NV magnetometry promises significant advances in magnetic imaging, the effectiveness of the technique, when applied to realistic magnetic nanostructures, remains to be demonstrated. Here we use a scanning NV magnetometer to image a magnetic vortex, which is one of the most iconic object of nanomagnetism, owing to the small size (~10 nm) of the vortex core. We report three-dimensional, vectorial, and quantitative measurements of the stray magnetic field emitted by a vortex in a ferromagnetic square dot, including the detection of the vortex core. We find excellent agreement with micromagnetic simulations, both for regular vortex structures and for higher-order magnetization states. These experiments establish scanning NV magnetometry as a practical and unique tool for fundamental studies in nanomagnetism.

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arXiv2013

Domain wall tilting in the presence of the Dzyaloshinskii-Moriya interaction in out-of-plane magnetized magnetic nanotracks

We show that the Dzyaloshinskii-Moriya interaction (DMI) can lead to a tilting of the domain wall (DW) surface in perpendicularly magnetized magnetic nanotracks when DW dynamics is driven by an easy axis magnetic field or a spin polarized current. The DW tilting affects the DW dynamics for large DMI and the tilting relaxation time can be very large as it scales with the square of the track width. The results are well explained by an analytical model based on a Lagrangian approach where the DMI and the DW tilting are included. We propose a simple way to estimate the DMI in a magnetic multilayers by measuring the dependence of the DW tilt angle on a transverse static magnetic field. Our results shed light on the current induced DW tilting observed recently in Co/Ni multilayers with inversion asymmetry, and further support the presence of DMI in these systems.

cond-mat.mtrl-sci↗

arXiv2013

Spatially periodic domain wall pinning potentials: Asymmetric pinning and dipolar biasing

Domain wall propagation has been measured in continuous, weakly disordered, quasi-two-dimensional, Ising-like magnetic layers that are subject to spatially periodic domain wall pinning potentials. The potentials are generated non-destructively using the stray magnetic field of ordered arrays of magnetically hard [Co/Pt]$_m$ nanoplatelets which are patterned above and are physically separated from the continuous magnetic layer. The effect of the periodic pinning potentials on thermally activated domain wall creep dynamics is shown to be equivalent, at first approximation, to that of a uniform, effective retardation field, $H_{ret}$, which acts against the applied field, $H$. We show that $H_{ret}$ depends not only on the array geometry but also on the relative orientation of $H$ and the magnetization of the nanoplatelets. A result of the latter dependence is that wall-mediated hysteresis loops obtained for a set nanoplatelet magnetization exhibit many properties that are normally associated with ferromagnet/antiferromagnet exchange bias systems. These include a switchable bias, coercivity enhancement and domain wall roughness that is dependent on the applied field polarity.

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arXiv2012

Nanoscale magnetic field mapping with a single spin scanning probe magnetometer

We demonstrate quantitative magnetic field mapping with nanoscale resolution, by applying a lock-in technique on the electron spin resonance frequency of a single nitrogen-vacancy defect placed at the apex of an atomic force microscope tip. In addition, we report an all-optical magnetic imaging technique which is sensitive to large off-axis magnetic fields, thus extending the operation range of diamond-based magnetometry. Both techniques are illustrated by using a magnetic hard disk as a test sample. Owing to the non-perturbing and quantitative nature of the magnetic probe, this work should open up numerous perspectives in nanomagnetism and spintronics.

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