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S. Ruiz-Gómez

Publications and source records attributed to S. Ruiz-Gómez.

9 recordsLinked to original sources

Domain-wall circulation gating and pinning via compositional engineering of cylindrical nanowires

Spintronic devices based on cylindrical magnetic nanowires have been proposed as a route toward three-dimensional information storage and processing by harnessing the controlled motion of domain walls (DWs). In this geometry, the Bloch-point wall (BPW) is the characteristic DW type. It features a curling of magnetization around a Bloch Point singularity, a topology that has been predicted to enable propagation at high speed without undergoing a Walker breakdown. We demonstrate that compositional modulations of larger magnetization, which host spontaneous curling states while the rest of the wire remains axial, fulfil a dual role: they act as deterministic pinning sites and as active gates for BPW circulation. Combining magnetic transmission X-ray microscopy and micromagnetic simulations, we reveal that DW-modulation interactions are the result of a superposition of long-range magnetostatic repulsion and short-range, circulation-dependent exchange contributions: parallel circulation produces an attractive well, while opposite circulation generates a repulsive barrier. This results in DW pinning at or near a compositional modulation. A DW's internal circulation can be inverted upon traversing a modulation, enabling on-demand switching of its circulation state. This dual mechanism demonstrates that both DW position and circulation can be tuned in a controlled manner, with potential implications for multistate spintronic devices.

cond-mat.mes-hall↗

Topological analysis and experimental control of transformations of domain walls in magnetic cylindrical nanowires

Topology is a powerful tool for categorizing magnetization textures by defining a topological index in both two-dimensional (2D) systems, such as thin films or curved surfaces, and in 3D bulk systems. In the emerging field of 3D nanomagnetism, both volume and surface topological numbers must be considered, requiring the identification of a proper global topological invariant to support categorization. Here we consider domain walls in cylindrical nanowires as an excellent playground for 3D nanomagnetic systems, excited by a charge current, that generates an OErsted field. We first provide experimental evidence of previously unreported domain-wall transformations of topology occurring at the nanosecond timescale. We investigate these transformations with micromagnetic simulations, tracking both bulk and surface topological signatures.We demonstrate a topological invariant combining both signatures, while the topological charge varies from bulk to surface during the dynamics. The experimental change of topology is reproduced when the pulse duration matches the timescale of the internal transformations of the wall, and the current is switched off before the transformation is complete. We expect that the topological categorization and dynamical exploitation apply to any 3D nanomagnetic system.

cond-mat.mes-hall↗

Preservation of scalar spin chirality across a metallic spacer in synthetic antiferromagnets with chiral interlayer interactions

Chiral magnetic textures are key for the development of modern spintronic devices. In multilayered thin films, these are typically stabilized via the interfacial intralayer Dzyaloshinskii-Moriya interaction (DMI). Additionally, it has been recently observed that DMI may also promote vector spin chirality along the third dimension, coupling spins in different magnetic layers via non-magnetic spacer layers, an effect referred to as interlayer DMI (IL-DMI). This interaction holds promise for 3D nanomagnetism, from the creation of 3D spin structures such as hopfions to new forms of magnetic functionality in the vertical direction via remote control of chiral spin states. Here, we investigate via magnetic X-ray scattering and imaging techniques the chiral nature of orthogonal magnetic states that form in a synthetic antiferromagnet with IL-DMI. We find that the vector spin chirality of the textures formed in an in-plane layer is determined by the net out-of-plane spin configuration of a neighboring layer, leading as a result to complex spin states across a metallic interface where the overall scalar spin chirality is preserved. This work thus uncovers a new flavor of chiral interlayer interactions, demonstrating new ways to control magnetic chirality in three dimensions.

cond-mat.mes-hall↗

Determination of optimal experimental conditions for accurate 3D reconstruction of the magnetization vector via XMCD-PEEM

In this work we present a detailed analysis on the performance of X-ray magnetic circular dichroism photo-emission electron microscopy (XMCD-PEEM) as a tool for vector reconstruction of the magnetization. For this, we choose 360$^{\circ}$ domain wall ring structures which form in a synthetic antiferromagnet as our model to conduct the quantitative analysis. We assess how the quality of the results is affected depending on the number of projections that are involved in the reconstruction process, as well as their angular distribution. For this we develop a self-consistent error metric, which indicates that the main factor of improvement comes from selecting the projections evenly spread out in space, over having a larger number of these spanning a smaller angular range. This work thus poses XMCD-PEEM as a powerful tool for vector imaging of complex 3D magnetic structures.

cond-mat.mes-hall↗

FeCo Nanowire-Strontium Ferrite Powder Composites for Permanent Magnets with High-Energy Products

Due to the issues associated with rare-earth elements, there arises a strong need for magnets with properties between those of ferrites and rare-earth magnets that could substitute the latter in selected applications. Here, we produce a high remanent magnetization composite bonded magnet by mixing FeCo nanowire powders with hexaferrite particles. In the first step, metallic nanowires with diameters between 30 and 100 nm and length of at least 2 μm are fabricated by electrodeposition. The oriented as-synthesized nanowires show remanence ratios above 0.76 and coercivities above 199 kA/m and resist core oxidation up to 300 °C due to the existence of a > 8 nm thin oxide passivating shell. In the second step, a composite powder is fabricated by mixing the nanowires with hexaferrite particles. After the optimal nanowire diameter and composite composition are selected, a bonded magnet is produced. The resulting magnet presents a 20% increase in remanence and an enhancement of the energy product of 48% with respect to a pure hexaferrite (strontium ferrite) magnet. These results put nanowire-ferrite composites at the forefront as candidate materials for alternative magnets for substitution of rare earths in applications that operate with moderate magnet performance.

cond-mat.mtrl-sci↗

Epitaxial monolayers of magnetic 2D semiconductor FeBr$_{2}$ grown on Au(111)

Magnetic two-dimensional (2D) semiconductors have attracted a lot of attention because modern preparation techniques are capable of providing single crystal films of these materials with precise control of thickness down to the single-layer limit. It opens up a way to study rich variety of electronic and magnetic phenomena with promising routes towards potential applications. We have investigated the initial stages of epitaxial growth of the magnetic van der Waals semiconductor FeBr\textsubscript{2} on a single-crystal Au(111) substrate by means of low-temperature scanning tunneling microscopy, low-energy electron diffraction, x-ray photoemission spectroscopy, low-energy electron emission microscopy and x-ray photoemission electron microscopy. Magnetic properties of the one- and two-layer thick films were measured via x-ray absorption spectroscopy/x-ray magnetic circular dichroism. Our findings show a striking difference in the magnetic behaviour of the single layer of FeBr\textsubscript{2} and its bulk counterpart, which can be attributed to the modifications in the crystal structure due to the interaction with the substrate.

cond-mat.mtrl-sci↗

Observation and formation mechanism of 360° domain wall rings in Synthetic Anti-Ferromagnets with interlayer chiral interactions

The Interlayer Dzyaloshinskii-Moriya interaction (IL-DMI) chirally couples spins in different ferromagnetic layers of multilayer heterostructures. So far, samples with IL-DMI have been investigated utilizing magnetometry and magnetotransport techniques, where the interaction manifests as a tunable chiral exchange bias field. Here, we investigate the nanoscale configuration of the magnetization vector in a synthetic anti-ferromagnet (SAF) with IL-DMI, after applying demagnetizing field sequences. We add different global magnetic field offsets to the demagnetizing sequence in order to investigate the states that form when the IL-DMI exchange bias field is fully or partially compensated. For magnetic imaging and vector reconstruction of the remanent magnetic states we utilize X-ray magnetic circular dichroism photoemission electron microscopy, evidencing the formation of 360$^{\circ}$ domain wall rings of typically 0.5-3.0 $μm$ in diameter. These spin textures are only observed when the exchange bias field due to the IL-DMI is not perfectly compensated by the magnetic field offset. From a combination of micromagnetic simulations, magnetic charge distribution and topology arguments, we conclude that a non-zero remanent effective field with components both parallel and perpendicular to the anisotropy axis of the SAF is necessary to observe the rings. This work shows how the exchange bias field due to IL-DMI can lead to complex metastable spin states during reversal, important for the development of novel spintronic devices.

cond-mat.mes-hall↗

Micromagnetics of magnetic chemical modulations in soft-magnetic cylindrical nanowires

We analyze the micromagnetics of short longitudinal modulations of a high-magnetization material in cylindrical nanowires made of a soft-magnetic material of lower magnetization such as permalloy, combining magnetic microscopy, analytical modeling, and micromagnetic simulations. The mismatch of magnetization induces curling of magnetization around the axis in the modulations, in an attempt to screen the interfacial magnetic charges. The curling angle increases with modulation length, until a plateau is reached with nearly full charge screening for a specific length scale~$Δ_\mathrm{mod}$, larger than the dipolar exchange length of any of the two materials. The curling circulation can be switched by the Oersted field arising from a charge current with typical magnitude $10^{12} A/m^{2}$ for a diameter of $\sim$100 nm, and reaching a maximum for $Δ_\mathrm{mod}$.

cond-mat.mes-hall↗

Domain wall automotion in three-dimensional magnetic helical interconnectors

The fundamental limits currently faced by traditional computing devices necessitate the exploration of new ways to store, compute and transmit information. Here, we propose a three-dimensional (3D) magnetic interconnector that exploits geometry-driven automotion of domain walls (DWs), for the transfer of magnetic information between functional magnetic planes. By combining state-of-the-art 3D nanoprinting and standard physical vapor deposition, we prototype 3D helical DW conduits. We observe the automotion of DWs by imaging their magnetic state under different field sequences using X-ray microscopy, observing a robust unidirectional motion of DWs from the bottom to the top of the spirals. From experiments and micromagnetic simulations, we determine that the large thickness gradients present in the structure are the main mechanism for 3D DW automotion. We obtain direct evidence of how this tailorable magnetic energy gradient is imprinted in the devices, and how it competes with pinning effects due to local changes in the energy landscape. Our work also predicts how this effect could lead to high DW velocities, reaching the Walker limit during automotion. This work provides new possibilities for efficient transfer of magnetic information in three dimensions.

cond-mat.mes-hall↗