arXiv subjects

S. S. Bhattacharjee

Publications and source records attributed to S. S. Bhattacharjee.

At least 19 recordsLinked to original sources

arXiv2026

First observation of the fine structure of the Pygmy Dipole Resonance in a nucleus away from stability via the $β^-$ decay of $^{92}$Rb to $^{92}$Sr

A comprehensive $γ$-ray spectroscopy study of excited states in $^{92}$Sr populated via $β^-$ decay of $^{92}$Rb ($J^π=0^-$, $Q_β=8095(6)$~keV) was performed with the GRIFFIN spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high $γ$-ray efficiency of the GRIFFIN spectrometer combined with the intense rubidium beams produced allowed for 864 $γ$-ray transitions to be placed in the level scheme with 190 excited levels populated, most of them identified for the first time. The excitation energies of low-spin states in $^{92}$Sr are well reproduced by large-scale Shell Model calculations up to 5~MeV. The $β$-feeding intensities are in very good agreement with results from a recent study employing Modular Total Absorption Spectroscopy, indicating a significant suppression of the Pandemonium effect. The experimental picture reveals the energy level dependence of log~$ft$ values in unprecedented detail. These log~$ft$ values are well reproduced by Multiple-Commutator Model calculations that identify the features in the excited levels' wavefunctions that enable the population of high-lying levels with a low effective Q-value that belong to the Pygmy Dipole Resonance.

nucl-ex↗

arXiv2026

Core Breaking at Low Spin in $^{68}$Zn from Nuclear Resonance Fluorescence

Low-spin excited states in $^{68}$Zn have been studied at the High Intensity Gamma-Ray Source (HI$γ$S) from the ground state up to the particle emission threshold using the nuclear resonance fluorescence technique (NRF) and the newly developed Clover Array. Low-spin levels were excited by linearly-polarized, $2.90 - 9.79$ MeV photon beams. Spin-parity quantum numbers as well as associated $M1$ and $E1$ decay strengths were determined for a large fraction of the 158 states observed. In addition, long-duration coincidence measurements at 9.46 and 9.79 MeV enabled the investigation of the level scheme near the ground state. The results have been interpreted with shell-model calculations using two different model spaces and several effective interactions often used to describe nuclei in this mass region. While the structure near the ground state can be understood in terms of excitations involving solely valence nucleons, core breaking is required to account for the evolution of the total $M1$ strength at excitation energies above $\sim5$ MeV.

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arXiv2025

Direct measurement of $^{59}$Cu($p$,$α$)$^{56}$Ni precludes a strong NiCu cycle in Type-I X-ray bursts

Model-observation comparisons of type-I X-ray bursts (XRBs) can reveal the properties of accreting neutron star systems, including the neutron star compactness. XRBs are powered by nuclear burning and a handful of reactions have been shown to impact the model results. Reactions in the NiCu cycles, featuring a competition between $^{59}$Cu($p$,$γ$)$^{60}$Zn and $^{59}$Cu($p$,$α$)$^{56}$Ni, have been shown to be among the most important reactions as they are a critical checkpoint in $rp$-process flow and significantly impact the light curves and burst ashes. We report a direct measurement of $^{59}$Cu($p$,$α$)$^{56}$Ni bringing stringent constraints on this reaction rate. New results rule out a strong NiCu cycle in XRBs, with a negligible degree of recycling, $\leq$5\% up to 1.5 GK. The new reaction rate, when varied within new uncertainty limits, shows no impact on one-zone XRB model light-curves tailored for clocked-burster $\tt{GS 1826-24}$, hence removing an important nuclear physics uncertainty in the model-observation comparison.

astro-ph.HE↗

arXiv2024

Cross-shell excited configurations in the structure of 34Si

The cross-shell excited states of $^{34}$Si have been investigated via $β$-decays of the $4^-$ ground state and the $1^+$ isomeric state of $^{34}$Al. Since the valence protons and valence neutrons occupy different major shells in the ground state as well as the intruder $1^+$ isomeric state of $^{34}$Al, intruder levels of $^{34}$Si are populated via allowed $β$ decays. Spin assignments to such intruder levels of $^{34}$Si were established through $γ$-$γ$ angular correlation analysis for the negative parity states with dominant configurations $(νd_{3/2})^{-1} \otimes (νf_{7/2})^{1}$ as well as the positive parity states with dominant configurations $(νsd)^{-2} \otimes (νf_{7/2}p_{3/2})^2$. The configurations of such intruder states play crucial roles in our understanding of the $N=20$ shell gap evolution. A configuration interaction model derived from the FSU Hamiltonian was utilized in order to interpret the intruder states in $^{34}$Si. Shell model interaction derived from a more fundamental theory with the Valence Space In Medium Similarity Renormalization Group (VS-IMSRG) method was also employed to interpret the structure of $^{34}$Si.

nucl-ex↗

arXiv2023

Structure Studies of $^{13}\text{Be}$ from the $^{12}$Be(d,p) reaction in inverse kinematics on a solid deuteron target

The low-lying structure of $^{13}$Be has remained an enigma for decades. Despite numerous experimental and theoretical studies, large inconsistencies remain. Being both unbound, and one neutron away from $^{14}$Be, the heaviest bound beryllium nucleus, $^{13}$Be is difficult to study through simple reactions with weak radioactive ion beams or more complex reactions with stable-ion beams. Here, we present the results of a study using the $^{12}$Be(d,p)$^{13}$Be reaction in inverse kinematics using a 9.5~MeV per nucleon $^{12}$Be beam from the ISAC-II facility. The solid deuteron target of IRIS was used to achieve an increased areal thickness compared to conventional deuterated polyethylene targets. The Q-value spectrum below -4.4~MeV was analyzed using a Bayesian method with GEANT4 simulations. A three-point angular distribution with the same Q-value gate was fit with a mixture of $s$- and $p$-wave, $s$- and $d$-wave, or pure $p$-wave transfer. The Q-value spectrum was also compared with GEANT simulations obtained using the energies and widths of states reported in four previous works. It was found that our results are incompatible with works that revealed a wide $5/2^+$ resonance but shows better agreement with ones that reported a narrower width.

nucl-ex↗

arXiv2023

Decay Spectroscopy of $^{160}$Eu: Quasiparticle Configurations of Excited States and Structure of $K^π$=$4^+$ Band-heads in $^{160}$Gd

\noindent \textbf{Background:} Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. \noindent \textbf{Purpose:} To improve the understanding of the nuclear structure of $^{160}$Gd, specifically the $K^π$=$4^+$ bands, as well as study the $β$-decay of $^{160}$Eu into $^{160}$Gd. \noindent \textbf{Methods:} High-statistics decay spectroscopy of $^{160}$Gd resulting from the $β$-decay of $^{160}$Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. \noindent \textbf{Results:} Two new excited states and ten new transitions were observed in $^{160}$Gd. The $β$-decaying half-lives of the low- and high-spin isomer in $^{160}$Eu were determined, and the low-spin state's half-life was measured to be $t_{1/2}=26.0(8)$~s, $\sim$16\% shorter than previous measurements. Lifetimes of the two $K^π$=$4^+$ band-heads in $^{160}$Gd were measured for the first time, as well as $γ$-$γ$ angular correlations and mixing ratios of intense transitions out of those band-heads. \noindent \textbf{Conclusions:} Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the $K^π$=$4^+$ band-heads in $^{160}$Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0 keV state in $^{160}$Gd heavily populated in $β$-decay is shown to have positive parity, which raises questions regarding the structure of the high-spin $β$-decaying state in $^{160}$Eu.

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arXiv2023

Cross Sections of the $^{83}$Rb(p,$γ)^{84}$Sr and $^{84}$Kr(p,$γ)^{85}$Rb Reactions at Energies Characteristic of the Astrophysical $γ$ Process

We have measured the cross section of the $^{83}$Rb(p,$γ)^{84}$Sr radiative capture reaction in inverse kinematics using a radioactive beam of $^{83}$Rb at incident energies of 2.4 and $2.7 A$ MeV. Prior to the radioactive beam measurement, the $^{84}$Kr(p,$γ)^{85}$Rb radiative capture reaction was measured in inverse kinematics using a stable beam of $^{84}$Kr at an incident energy of $2.7 A$ MeV. The effective relative kinetic energies of these measurements lie within the relevant energy window for the $γ$ process in supernovae. The central values of the measured partial cross sections of both reactions were found to be $0.17-0.42$ times the predictions of statistical model calculations. Assuming the predicted cross section at other energies is reduced by the same factor leads to a slightly higher calculated abundance of the $p$ nucleus $^{84}$Sr, caused by the reduced rate of the $^{84}$Sr($γ$,p)$^{83}$Rb reaction derived from the present measurement.

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arXiv2023

First Evidence of Axial Shape Asymmetry and Configuration Coexistence in $^{74}$Zn: Suggestion for a Northern Extension of the $N=40$ Island of Inversion

The excited states of $N=44$ $^{74}$Zn were investigated via $γ$-ray spectroscopy following $^{74}$Cu $β$ decay. By exploiting $γ$-$γ$ angular correlation analysis, the $2_2^+$, $3_1^+$, $0_2^+$ and $2_3^+$ states in $^{74}$Zn were firmly established. The $γ$-ray branching and $E2/M1$ mixing ratios for transitions de-exciting the $2_2^+$, $3_1^+$ and $2_3^+$ states were measured, allowing for the extraction of relative $B(E2)$ values. In particular, the $2_3^+ \to 0_2^+$ and $2_3^+ \to 4_1^+$ transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are discussed in terms of underlying shapes, as well as the role of neutron excitations across the $N=40$ gap. Enhanced axial shape asymmetry (triaxiality) is suggested to characterize $^{74}$Zn in its ground state. Furthermore, an excited $K=0$ band with a significantly larger softness in its shape is identified. A shore of the $N=40$ ``island of inversion'' appears to manifest above $Z=26$, previously thought as its northern limit in the chart of the nuclides.

nucl-ex↗

arXiv2022

High spin states of $^{204}$At: isomeric states and shears band structure

High-spin states of neutron deficient Trans-Lead nucleus $^{204}$At were populated up to $\sim 8\,{\rm MeV}$ excitation through the $^{12}$C + $^{197}$Au fusion evaporation reaction. Decay of the associated levels through prompt and delayed $γ$-ray emissions were studied to evaluate the underlying nuclear structure. The level scheme, which was partly known, was extended further. An isomeric $16^+$ level with observed lifetime $τ=52 \pm 5\, {\rm ns}$, was established from our measurements. Attempts were made to interpret the excited states based on multi quasiparticle and hole structures involving $2f_{5/2}$, $1h_{9/2}$, and $1i_{13/2}$ shell model states, along with moderate core excitation. Magnetic dipole band structure over the spin parity range:~$16^+ - 23^+$ was confirmed and evaluated in more detail, including the missing cross-over $E2$ transitions. Band-crossing along the shears band was observed and compared with the evidence of similar phenomena in the neighbouring neutron deficient $^{202}$Bi, $^{205}$Rn isotones and the $^{203}$At isotope. Based on comparison of the measured $B(M1)/B(E2)$ values for transitions along the band with the semiclassical model based estimates, the shears band of $^{204}$At was established along with the level scheme.

nucl-ex↗

arXiv2022

Single neutron transfer on 23Ne and its relevance forthepathway ofnucleosynthesis in astrophysical X-ray bursts

We present new experimental measurements of resonance strengths in the astrophysical 23Al(p, γ)24Si reaction, constraining the pathway of nucleosynthesis beyond 22Mg in X-ray burster scenarios. Specifically, we have performed the first measurement of the (d, p) reaction using a radioactive beam of 23Ne to explore levels in 24Ne, the mirror analog of 24Si. Four strong single-particle states were observed and corresponding neutron spectroscopic factors were extracted with a precision of {\sim}20{\%}. Using these spectroscopic factors, together with mirror state identifications, we have reduced uncertainties in the strength of the key {\ell} = 0 resonance at Er= 157 keV, in the astrophysical 23Al(p, γ) reaction, by a factor of 4. Our results show that the 22Mg(p, γ)23Al(p, γ) pathway dominates over the competing 22Mg(α, p) reaction in all but the most energetic X-ray burster events (T>0.85GK), significantly affecting energy production and the preservation of hydrogen fuel.

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arXiv2022

Improved measurement of the $0_2^+\rightarrow0_1^+$ E0 transition strength for $^{72}$Se using the SPICE spectrometer

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $^{72}$Se by internal conversion electron and $γ$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $0_2^+$ state were performed yielding a determination of $ρ^2(E0;0_2^+{\rightarrow}0_1^+)=29(3)$ milliunits. two state mixing calculations were performed that highlighted the importance of interpretation of such $E0$ strength values in the context of shape-coexistence.

nucl-ex↗

arXiv2022

Single Particle Configurations of the Excited States of $^{203}$Po

Excited states of the $^{203}$Po ($Z = 84, N = 119$) have been investigated after populating them through $^{194}$Pt($^{13}$C,4n) fusion-evaporation reaction at E$_{beam}$ = 74 MeV and using a large array of Compton suppressed HPGe clover detectors as the detection setup for the emitted $γ$-rays. Standard techniques of $γ$-ray spectroscopy have been applied towards establishing the level structure of the nucleus. Twenty new $γ$-ray transitions have been identified therein, through $γ-γ$ coincidence measurements, and spin-parity assignments of several states have been determined or confirmed, following the angular correlation and linear polarization measurements on the observed $γ$-rays. The excited states have been interpreted in the framework of large basis shell model calculations, while comparing their calculated and experimental energies. They have been principally ascribed to proton population in the $h_{9/2}$ and $i_{13/2}$ orbitals outside the $Z = 82$ closure and neutron occupation of the $f_{5/2}$, $p_{3/2}$ and $i_{13/2}$ orbitals in the $N = 126$ shell.

nucl-ex↗

arXiv2022

High-precision half-life determination of $^{14}$O via direct $β$ counting

The half-life of the superallowed Fermi $β^+$ emitter $^{14}$O was determined to high precision via a direct $β$ counting experiment performed at the Isotope Separator and Accelerator (ISAC) facility at TRIUMF. The result, $T_{1/2}$($^{14}$O) = 70619.2(76) ms, is consistent with, but is more precise than, the world average obtained from 11 previous measurements. Combining the $^{14}$O half-life deduced in the present work with the previous most precise measurements of this quantity leads to a reduction in the overall uncertainty, by nearly a factor of 2. The new world average is $T_{1/2}$($^{14}$O) = 70619.6(63) ms with a reduced $χ^2$ value of 0.87 obtained from 8 degrees of freedom.

nucl-ex↗

arXiv2021

Use of Bayesian Optimization to Understand the Structure of Nuclei

Monte Carlo simulations are widely used in nuclear physics to model experimental systems. In cases where there are significant unknown quantities, such as energies of states, an iterative process of simulating and fitting is often required to describe experimental data. We describe a Bayesian approach to fitting experimental data, designed for data from a $^{12}$Be(d,p) reaction measurement, using simulations made with GEANT4. Q-values from the $^{12}$C(d,p) reaction to well-known states in $^{13}$C are compared with simulations using BayesOpt. The energies of the states were not included in the simulation to reproduce the situation for $^{13}$Be where the states are poorly known. Both cases had low statistics and significant resolution broadening owing to large proton energy losses in the solid deuterium target. Excitation energies of the lowest three excited states in $^{13}$C were extracted to better than 90 keV, paving a way for extracting information on $^{13}$Be.

physics.comp-ph↗

arXiv2021

First Direct Measurement of an Astrophysical p-Process Reaction Cross Section Using a Radioactive Ion Beam

We have performed the first direct measurement of the 83Rb(p,g) radiative capture reaction cross section in inverse kinematics using a radioactive beam of 83Rb at incident energies of 2.4 and 2.7 A MeV. The measured cross section at an effective relative kinetic energy of Ecm = 2.393 MeV, which lies within the relevant energy window for core collapse supernovae, is smaller than the prediction of statistical model calculations. This leads to the abundance of 84Sr produced in the astrophysical p process being higher than previously calculated. Moreover, the discrepancy of the present data with theoretical predictions indicates that further experimental investigation of p-process reactions involving unstable projectiles is clearly warranted.

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arXiv2021

First direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni: A step towards constraining the Ni-Cu cycle in the Cosmos

Reactions on the proton-rich nuclides drive the nucleosynthesis in Core-Collapse Supernovae (CCSNe) and in X-ray bursts (XRBs). CCSNe eject the nucleosynthesis products to the interstellar medium and hence are a potential inventory of p-nuclei, whereas in XRBs nucleosynthesis powers the light curves. In both astrophysical sites the Ni-Cu cycle, which features a competition between $^{59}$Cu(p,$α$)$^{56}$Ni and $^{59}$Cu(p,$γ$)$^{60}$Zn, could potentially halt the production of heavier elements. Here, we report the first direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni using a re-accelerated $^{59}$Cu beam and cryogenic solid hydrogen target. Our results show that the reaction proceeds predominantly to the ground state of $^{56}$Ni and the experimental rate has been found to be lower than Hauser-Feshbach-based statistical predictions. New results hint that the $νp$-process could operate at higher temperatures than previously inferred and therefore remains a viable site for synthesizing the heavier elements.

nucl-ex↗

arXiv2020

High-Precision Branching Ratio Measurement and Spin Assignment Implications for $^{62}$Ga Superallowed $β$ Decay

A high-precision branching ratio measurement for the superallowed Fermi $β^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $γ$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $β^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $β$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $γ-γ$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $δ_{C1}$, in $^{62}$Ga superallowed Fermi $β$ decay.

nucl-ex↗

arXiv2020

Absence of Low-Energy Shape Coexistence in $^{80}$Ge: The Nonobservation of a Proposed Excited 0$_2^+$ Level at 639 keV

The $^{80}$Ge structure was investigated in a high-statistics $β$-decay experiment of $^{80}$Ga using the GRIFFIN spectrometer at TRIUMF-ISAC through $γ$, $β$-$e$, $e$-$γ$ and $γ$-$γ$ spectroscopy. No evidence was found for the recently reported 0$_2^{+}$ 639-keV level suggested as evidence for low-energy shape coexistence in $^{80}$Ge. Large-scale shell model calculations performed in $^{78,80,82}$Ge place the $0^{+}_{2}$ level in $^{80}$Ge at 2\,MeV. The new experimental evidence combined with shell model predictions indicate that low-energy shape coexistence is not present in $^{80}$Ge.

nucl-ex↗