arXiv subjects

S. Seidelin

Publications and source records attributed to S. Seidelin.

At least 19 recordsLinked to original sources

arXiv2024

Anomalous sub-kelvin thermal frequency shifts of ultra narrow-linewidth solid state emitters

We investigate the frequency response of narrow spectral holes in a doped crystal structure as a function of temperature below 1 K. We identify a particular regime in which this response significantly deviates from the expected two-phonon Raman scattering theory. Namely, near 290 mK, we observed a behaviour exhibiting a temperature-dependent frequency shift of zero, to first-order. This is of particular interest for applications which require high frequency-stability, such as laser frequency stabilization, as by operating the scheme at this specific point would result in the spectral hole frequency being highly immune to temperature fluctuations, providing the potential for a laser fractional frequency instability as low as $\mathrm{\sim6\times10^{-22}}$ at 1 s.

physics.optics↗

arXiv2024

First-order thermal insensitivity of the frequency of a narrow spectral hole in a crystal

The possibility of generating an narrow spectral hole in a rare-earth doped crystal opens the gateway to a variety of applications, one of which is the realization of an ultrastable laser. As this is achieved by locking in a pre-stabilized laser to the narrow hole, a prerequisite is the elimination of frequency fluctuations of the spectral hole. One potential source of such fluctuations can arise from temperature instabilities. However, when the crystal is surrounded by a buffer gas subject to the same temperature as the crystal, the effect of temperature-induced pressure changes may be used to counterbalance the direct effect of temperature fluctuations. For a particular pressure, it is indeed possible to identify a temperature for which the spectral hole resonant frequency is independent of the first-order thermal fluctuations. Here, we measure frequency shifts as a function of temperature for different values of the pressure of the surrounding buffer gas, and identify the ``magic'' environment within which the spectral hole is largely insensitive to temperature.

physics.optics↗

arXiv2023

Multi-mode Heterodyne Laser Interferometry Realized via Software Defined Radio

The agile generation and control of multiple optical frequency modes combined with the realtime processing of multi-mode data provides access to experimentation in domains such as optomechanical systems, optical information processing, and multi-mode spectroscopy. The latter, specifically spectroscopy of spectral-hole burning (SHB), has motivated our development of a multi-mode heterodyne laser interferometric scheme centered around a software-defined radio platform for signal generation and processing, with development in an entirely open-source environment. A challenge to SHB is the high level of shot noise due to the laser power constraint imposed by the spectroscopic sample. Here, we have demonstrated the production, detection, and separation of multiple optical frequency modes to the benefit of optical environment sensing for realtime phase noise subtraction as well as shot noise reduction through multi-mode averaging. This has allowed us to achieve improved noise performance in low-optical-power interferometry. Although our target application is laser stabilization via SHB in cryogenic temperature rare-earth doped crystals, these techniques may be employed in a variety of different contexts.

physics.optics↗

arXiv2021

Precision measurements of electric-field-induced frequency displacements of an ultranarrow optical transition in ions in a solid

We report a series of measurements of the effect of an electric field on the frequency of the ultranarrow linewidth $^7F_0 \rightarrow$ $^5D_0$ optical transition of $\rm Eu^{3+}$ ions in an $\rm Y_2SiO_5$ matrix at cryogenic temperatures. We provide linear Stark coefficients along two dielectric axes and for the two different substitution sites of the $\rm Eu^{3+}$ ions, with an unprecedented accuracy, and an upper limit for the quadratic Stark shift. The measurements, which indicate that the electric field sensitivity is a factor of seven larger for site 1 relative to site 2 for a particular direction of the electric field are of direct interest both in the context of quantum information processing and laser frequency stabilization with rare-earth doped crystals, in which electric fields can be used to engineer experimental protocols by tuning transition frequencies.

physics.atom-ph↗

arXiv2020

Inhomogeneous response of an ion ensemble from mechanical stress

Material strain has recently received growing attention as a complementary resource to control the energy levels of quantum emitters embedded inside a solid-state environment. Some rare-earth ion dopants provide an optical transition which simultaneously has a narrow linewidth and is highly sensitive to strain. In such systems, the technique of spectral hole burning, in which a transparent window is burnt within the large inhomogeneous profile, allows to benefit from the narrow features, which are also sensitive to strain, while working with large ensembles of ions. However, working with ensembles may give rise to inhomogeneous responses among different ions. We investigate experimentally how the shape of a narrow spectral hole is modified due to external mechanical strain, in particular, the hole broadening as a function of the geometry of the crystal sites and the crystalline axis along which the stress is applied. Studying these effects are essential in order to optimize the existing applications of rare-earth doped crystals in fields which already profit from the more well-established coherence properties of these dopants such as frequency metrology and quantum information processing, or even suggest novel applications of these materials, for example as robust devices for force-sensing or highly sensitive accelerometers.

cond-mat.mtrl-sci↗

arXiv2020

Microscale crystalline rare-earth doped resonators for strain-coupled optomechanics

Rare-earth ion doped crystals for hybrid quantum technologies is an area of growing interest in the solid-state physics community. We have earlier theoretically proposed a hybrid scheme of a mechanical resonator which is fabricated out of a rare-earth doped mono-crystalline structure. The rare-earth ion dopants have absorption energies which are sensitive to crystal strain, and it is thus possible to couple the ions to the bending motion of the crystal cantilever. Here, we present the design and fabrication method based on focused-ion-beam etching techniques which we have successfully employed in order to create such microscale resonators, as well as the design of the environment which will allow to study the quantum behavior of the resonators.

physics.app-ph↗

arXiv2020

Position- and momentum-squeezed quantum states in micro-scale mechanical resonators

A challenge of modern physics is to investigate the quantum behavior of a bulk material object, for instance a mechanical oscillator. We have earlier demonstrated that by coupling a mechanical oscillator to the energy levels of embedded rare-earth ion dopants, it is possible to prepare such a resonator in a low phonon number state. Here, we describe how to extend this protocol in order to prepare momentum- and position squeezed states, and we analyze how the obtainable degree of squeezing depends on the initial conditions and on the coupling of the oscillator to its thermal environment.

quant-ph↗

arXiv2020

Double-heterodyne probing for ultra-stable laser based on spectral hole burning in a rare-earth doped crystal

We present an experimental technique for realizing a specific absorption spectral pattern in a rare-earth-doped crystal at cryogenic temperatures. This pattern is subsequently probed on two spectral channels simultaneously, thereby producing an error signal allowing frequency locking of a laser on the said spectral pattern. Appropriate combination of the two channels leads to a substantial reduction of the detection noise, paving the way to realizing an ultra-stable laser for which the detection noise can be made arbitrarily low when using multiple channels. We use such technique to realize a laser with a frequency instability of $1.7\times 10^{-15}$ at 1 second, not limited by the detection noise but by environmental perturbation of the crystal. This is comparable with the lowest instability demonstrated at 1 second to date for rare-earth doped crystal stabilized lasers.

physics.optics↗

arXiv2019

Mechanical tunability of an ultra-narrow spectral feature with uniaxial stress

Rare-earth doped crystals have numerous applications ranging from frequency metrology to quantum information processing. To fully benefit from their exceptional coherence properties, the effect of mechanical strain on the energy levels of the dopants - whether it is a resource or perturbation - needs to be considered. We demonstrate that by applying uniaxial stress to a rare-earth doped crystal containing a spectral hole, we can shift the hole by a controlled amount that is larger than the width of the hole. We deduce the sensitivity of $\rm Eu^{3+}$ ions in an $\rm Y_2SiO_5$ matrix as a function of crystal site and the crystalline axis along which the stress is applied.

cond-mat.mtrl-sci↗

arXiv2011

Amplitude to phase conversion of InGaAs pin photo-diodes for femtosecond lasers microwave signal generation

When a photo-diode is illuminated by a pulse train from a femtosecond laser, it generates microwaves components at the harmonics of the repetition rate within its bandwidth. The phase of these components (relative to the optical pulse train) is known to be dependent on the optical energy per pulse. We present an experimental study of this dependence in InGaAs pin photo-diodes illuminated with ultra-short pulses generated by an Erbium-doped fiber based femtosecond laser. The energy to phase dependence is measured over a large range of impinging pulse energies near and above saturation for two typical detectors, commonly used in optical frequency metrology with femtosecond laser based optical frequency combs. When scanning the optical pulse energy, the coefficient which relates phase variations to energy variations is found to alternate between positive and negative values, with many (for high harmonics of the repetition rate) vanishing points. By operating the system near one of these vanishing points, the typical amplitude noise level of commercial-core fiber-based femtosecond lasers is sufficiently low to generate state-of-the-art ultra-low phase noise microwave signals, virtually immune to amplitude to phase conversion related noise.

physics.optics↗

arXiv2009

Scalable ion traps for quantum information processing

We report on the design, fabrication, and preliminary testing of a 150 zone array built in a `surface-electrode' geometry microfabricated on a single substrate. We demonstrate transport of atomic ions between legs of a `Y'-type junction and measure the in-situ heating rates for the ions. The trap design demonstrates use of a basic component design library that can be quickly assembled to form structures optimized for a particular experiment.

quant-ph↗

arXiv2007

Simplified motional heating rate measurements of trapped ions

We have measured motional heating rates of trapped atomic ions, a factor that can influence multi-ion quantum logic gate fidelities. Two simplified techniques were developed for this purpose: one relies on Raman sideband detection implemented with a single laser source, while the second is even simpler and is based on time-resolved fluorescence detection during Doppler recooling. We applied these methods to determine heating rates in a microfrabricated surface-electrode trap made of gold on fused quartz, which traps ions 40 microns above its surface. Heating rates obtained from the two techniques were found to be in reasonable agreement. In addition, the trap gives rise to a heating rate of 300 plus or minus 30 per second for a motional frequency of 5.25 MHz, substantially below the trend observed in other traps.

quant-ph↗

arXiv2007

Fluorescence during Doppler cooling of a single trapped atom

We investigate the temporal dynamics of Doppler cooling of an initially hot single trapped atom in the weak binding regime using a semiclassical approach. We develop an analytical model for the simplest case of a single vibrational mode for a harmonic trap, and show how this model allows us to estimate the initial energy of the trapped particle by observing the fluorescence rate during the cooling process. The experimental implementation of this temperature measurement provides a way to measure atom heating rates by observing the temperature rise in the absence of cooling. This method is technically relatively simple compared to conventional sideband detection methods, and the two methods are in reasonable agreement. We also discuss the effects of RF micromotion, relevant for a trapped atomic ion, and the effect of coupling between the vibrational modes on the cooling dynamics.

quant-ph↗

arXiv2007

Randomized Benchmarking of Quantum Gates

A key requirement for scalable quantum computing is that elementary quantum gates can be implemented with sufficiently low error. One method for determining the error behavior of a gate implementation is to perform process tomography. However, standard process tomography is limited by errors in state preparation, measurement and one-qubit gates. It suffers from inefficient scaling with number of qubits and does not detect adverse error-compounding when gates are composed in long sequences. An additional problem is due to the fact that desirable error probabilities for scalable quantum computing are of the order of 0.0001 or lower. Experimentally proving such low errors is challenging. We describe a randomized benchmarking method that yields estimates of the computationally relevant errors without relying on accurate state preparation and measurement. Since it involves long sequences of randomly chosen gates, it also verifies that error behavior is stable when used in long computations. We implemented randomized benchmarking on trapped atomic ion qubits, establishing a one-qubit error probability per randomized pi/2 pulse of 0.00482(17) in a particular experiment. We expect this error probability to be readily improved with straightforward technical modifications.

quant-ph↗

arXiv2007

Errors in trapped-ion quantum gates due to spontaneous photon scattering

We analyze the error in trapped-ion, hyperfine qubit, quantum gates due to spontaneous scattering of photons from the gate laser beams. We investigate single-qubit rotations that are based on stimulated Raman transitions and two-qubit entangling phase-gates that are based on spin-dependent optical dipole forces. This error is compared between different ion species currently being investigated as possible quantum information carriers. For both gate types we show that with realistic laser powers the scattering error can be reduced to below current estimates of the fault-tolerance error threshold.

quant-ph↗

arXiv2006

Transport dynamics of single ions in segmented microstructured Paul trap arrays

It was recently proposed to use small groups of trapped ions as qubit carriers in miniaturized electrode arrays that comprise a large number of individual trapping zones, between which ions could be moved. This approach might be scalable for quantum information processing with a large numbers of qubits. Processing of quantum information is achieved by transporting ions to and from separate memory and qubit manipulation zones in between quantum logic operations. The transport of ion groups in this scheme plays a major role and requires precise experimental control and fast transport. In this paper we introduce a theoretical framework to study ion transport in external potentials that might be created by typical miniaturized Paul trap electrode arrays. In particular we discuss the relationship between classical and quantum descriptions of the transport and study the energy transfer to the oscillatory motion during near-adiabatic transport. Based on our findings we suggest a numerical method to find electrode potentials as a function of time to optimize the local potential an ion experiences during transport. We demonstrate this method for one specific electrode geometry that should closely represent the situation encountered in realistic trap arrays.

quant-ph↗

arXiv2006

Cantilever cooling with radio frequency circuits

We consider a method to reduce the kinetic energy in a low-order mode of a miniature cantilever. If the cantilever contributes to the capacitance of a driven RF circuit, a force on the cantilever exists due to the electric field energy stored in the capacitance. If this force acts with an appropriate phase shift relative to the motion of the cantilever, it can oppose the velocity of the cantilever, leading to cooling. Such cooling may enable reaching the quantum regime of cantilever motion.

quant-ph↗

arXiv2006

A microfabricated surface-electrode ion trap in silicon

The prospect of building a quantum information processor underlies many recent advances ion trap fabrication techniques. Potentially, a quantum computer could be constructed from a large array of interconnected ion traps. We report on a micrometer-scale ion trap, fabricated from bulk silicon using micro-electromechanical systems (MEMS) techniques. The trap geometry is relatively simple in that the electrodes lie in a single plane beneath the ions. In such a trap we confine laser-cooled 24Mg+ ions approximately 40 microns above the surface. The fabrication technique and planar electrode geometry together make this approach amenable to scaling up to large trap arrays. In addition we observe that little laser cooling light is scattered by the electrodes.

quant-ph↗