S. Sergeenkov — Page 3

arXiv1999

Negative magnetoresistance in La(0.6)Y(0.1)Ca(0.3)MnO(3): Evidence for charge localization governed by the Curie-Weiss law

Colossal negative magnetoresistance Δρ(T,B) observed in La(0.6)Y(0.1)Ca(0.3)MnO(3) at B=1T shows a nearly perfect symmetry around T_0=160K suggesting a universal field-induced transport mechanism in this material. Attributing this symmetry to strong magnetic fluctuations (triggered by the Y substitution and further enhanced by magnetic field, both above and below the field-dependent Curie temperature T_C(B)=T_0), the data are interpreted in terms of the nonthermal spin hopping and magnetization M dependent charge carrier localization scenario leading to Δρ(T,B)= -ρ_s(1-exp(-γM^2)) with M(T,B)=CB/|T-T_C|^n. The separate fits through all the data points above and below T_C yield C^{+}\simeq C^{-} and n^{+}\simeq n^{-}\simeq 1. The obtained results corroborate the importance of fluctuation effects in this material recently found (cond-mat/9812219) to dominate its magneto-thermopower behavior far beyond T_C.

cond-mat.str-el↗

arXiv1998

Estimation of the charge carrier localization length from Gaussian fluctuations in the magneto-thermopower of La_{0.6}Y_{0.1}Ca_{0.3}MnO_3

The magneto-thermoelectric power (TEP) $ΔS(T,H)$ of perovskite type manganise oxide $La_{0.6}Y_{0.1}Ca_{0.3}MnO_3$ is found to exhibit a sharp peak at some temperature $T^{*}=170K$. By approximating the true shape of the measured magneto-TEP in the vicinity of $T^{*}$ by a linear triangle of the form $ΔS(T,H)\simeq S_p(H)\pm B^{\pm}(H)(T^{*}-T)$, we observe that $B ^{-}(H)\simeq 2B ^{+}(H)$. We adopt the electron localization scenario and introduce a Ginzburg-Landau (GL) type theory which incorporates the two concurrent phase transitions, viz., the paramagnetic-ferromagnetic transition at the Curie point $T_C$ and the "metal-insulator" (M-I) transition at $T_{MI}$. The latter is characterized by the divergence of the field-dependent charge carrier localization length $ξ(T,H)$ at some characteristic field $H_0$. Calculating the average and fluctuation contributions to the total magnetization and the transport entropy related magneto-TEP $ΔS(T,H)$ within the GL theory, we obtain a simple relationship between $T^{*}$ and the above two critical temperatures ($T_{C}$ and $T_{MI}$). The observed slope ratio $B ^{-}(H)/B ^{+}(H)$ is found to be governed by the competition between the electron-spin exchange $JS$ and the induced magnetic energy $M_sH_0$. The comparison of our data with the model predictions produce $T_{C}=195K$, $JS=40meV$, $M_0=0.4M_s$, $ξ_0=10Å$, and $n_e/n_i=2/3$ for the estimates of the Curie temperature, the exchange coupling constant, the critical magnetization, the localization length, and the free-to-localized carrier number density ratio, respectively.

cond-mat.str-el↗