arXiv subjects

S. Shin

Publications and source records attributed to S. Shin.

At least 73 records · Page 4Linked to original sources

arXiv2016

High repetition pump-and-probe photoemission spectroscopy based on a compact fiber laser system

The paper describes a time-resolved photoemission (TRPES) apparatus equipped with a Yb-doped fiber laser system delivering 1.2-eV pump and 5.9-eV probe pulses at the repetition rate of 95 MHz. Time and energy resolutions are 11.3 meV and ~310 fs, respectively; the latter is estimated by performing TRPES on a highly oriented pyrolytic graphite (HOPG). The high repetition rate is suited for achieving high signal-to-noise ratio in TRPES spectra, thereby facilitating investigations of ultrafast electronic dynamics in the low pump fluence (p) region. TRPES of polycrystalline bismuth (Bi) at p as low as 30 nJ/mm2 is demonstrated. The laser source is compact and is docked to an existing TRPES apparatus based on a 250-kHz Ti:sapphire laser system. The 95-MHz system is less prone to space-charge broadening effects compared to the 250-kHz system, which we explicitly show in a systematic probe-power dependency of the Fermi cutoff of polycrystalline gold. We also describe that the TRPES response of an oriented Bi(111)/HOPG sample is useful for fine-tuning the spatial overlap of the pump and probe beams even when p is as low as 30 nJ/mm2.

physics.ins-det↗

arXiv2016

Unusual nodal behaviors of the superconducting gap in the iron-based superconductor Ba(Fe$_{0.65}$Ru$_{0.35}$)$_2$As$_2$: Effects of spin-orbit coupling

We have investigated the superconducting gap of optimally doped Ba(Fe$_{0.65}$Ru$_{0.35}$)$_2$As$_2$ by angle-resolved photoemission spectroscopy (APRES) using bulk-sensitive 7 eV laser and synchrotron radiation. It was found that the gap is isotropic in the $k_x$-$k_y$ plane both on the electron and hole Fermi surfaces (FSs). The gap magnitudes of two resolved hole FSs show similar $k_z$ dependences and decrease as $k_z$ approaches $\sim$ 2$π$/$c$ (i.e., around the Z point) unlike the other Fe-based superconductors reported so far, where the superconducting gap of only one hole FS shows a strong $k_z$ dependence. This unique gap structure can be understood in the scenario that the $d_{z^2}$ orbital character is mixed into both hole FSs due to the finite spin-orbit coupling between almost degenerate FSs and is reproduced by calculations within the random phase approximation including the spin-orbit coupling.

cond-mat.supr-con↗

arXiv2016

Ultrafast Melting of Spin Density Wave Order in BaFe$_{2}$As$_{2}$ Observed by Time- and Angle-Resolved Photoemission Spectroscopy with Extreme-Ultraviolet Higher Harmonic Generation

Transient single-particle spectral function of BaFe$_{2}$As$_{2}$, a parent compound of iron-based superconductors, has been studied by time- and angle-resolved photoemission spectroscopy with an extreme-ultraviolet laser generated by higher harmonics from Ar gas, which enables us to investigate the dynamics in the entire Brillouin zone. We observed electronic modifications from the spin-density-wave (SDW) ordered state within $\sim$ 1 ps after the arrival of a 1.5 eV pump pulse. We observed optically excited electrons at the zone center above $E_{F}$ at 0.12 ps, and their rapid decay. After the fast decay of the optically excited electrons, a thermalized state appears and survives for a relatively long time. From the comparison with the density-functional theory band structure for the paramagnetic and SDW states, we interpret the experimental observations as the melting of the SDW. Exponential decay constants for the thermalized state to recover back to the SDW ground state are $\sim$ 0.60 ps both around the zone center and the zone corner.

cond-mat.supr-con↗

arXiv2016

Suppression of Vertical Oscillation and Observation of Flux Improvement during Top-up Injection at PLS-II

This paper reports a start-to-end study of suppression of stored beam oscillation at PLS-II. We report that the fast counter-kicker implemented in PLS-II suppressed vertical oscillation of the stored beam. During top-up injection in the magnetic spectroscopy beamline of PLS-II, the stored beam oscillation was suppressed by a factor of nine, and flux was improved by a factor of three.

physics.acc-ph↗

arXiv2016

Coherent control over three-dimensional spin polarization for the spin-orbit coupled surface state of Bi$_2$Se$_3$

Interference of spin-up and spin-down eigenstates depicts spin rotation of electrons, which is a fundamental concept of quantum mechanics and accepts technological challenges for the electrical spin manipulation. Here, we visualize this coherent spin physics through laser spin- and angle-resolved photoemission spectroscopy on a spin-orbital entangled surface-state of a topological insulator. It is unambiguously revealed that the linearly polarized laser can simultaneously excite spin-up and spin-down states and these quantum spin-basis are coherently superposed in photoelectron states. The superposition and the resulting spin rotation is arbitrary manipulated by the direction of the laser field. Moreover, the full observation of the spin rotation displays the phase of the quantum states. This presents a new facet of laser-photoemission technique for investigation of quantum spin physics opening new possibilities in the field of quantum spintronic applications.

cond-mat.mtrl-sci↗

arXiv2016

Effects of Elliptically Polarizing Undulator on Beam Dynamics in PLS-II

The non-linear effects caused by the intrinsic field transverse roll-off in an Elliptically Polarizing Undulator with 72-mm period and maximum peak field of 0.72 T (EPU72) on the dynamics aperture of the Pohang Light Source II (PLS-II) were investigated. A kick map and Frequency map analysis both demonstrated that EPU72 will not reduce the lifetime or cause injection problems in PLS-II.

physics.acc-ph↗

arXiv2016

A New PLS-II In-Vacuum Undulator and Characterization of Undulator Radiation

This paper describes the result of overall studies from development to characterization of undulator radiation. After three years of upgrading, PLS-II [1, 2] has been operating successfully since 21st March 2012. During the upgrade, we developed and installed an in-vacuum undulator (IVU) that generates brilliant X-ray beam. The IVU with 3 GeV electron beam generates undulator radiation up to ~ 21 keV using 11th higher harmonic. The characterizations of the undulator radiation at an X-ray beam line in PLS-II agreed well with the simulation. Based on this performance demonstration, the in-vacuum undulator is successfully operating at PLS-II.

physics.acc-ph↗

arXiv2016

Multiple-pseudogap phases in hydrogen-doped LaFeAsO system

The low energy electronic structure of LaFeAsO1-xHx (0.0 < x < 0.60), the system which exhibits two superconducting domes in its phase diagram, is investigated by utilizing the laser photoemission spectroscopy. From the precise temperature-dependent measurement of the spectra near the Fermi level, we find the suppression of the density of states with cooling, namely the pseudogap formation, for all doping range. The pseudogap in the low x range (i.e. the first superconducting dome regime) gets suppressed with increasing x, more or less similarly to the previous results in F-doped LaFeAsO system. On the other hand, the pseudogap behavior in the second superconducting dome regime at high-x becomes stronger with increasing the H-doping level. The systematic doping dependence shows that the pseudogap is enhanced toward the both ends of the phase diagram where the different types of antiferromagnetic order exist.

cond-mat.supr-con↗

arXiv2016

Slater to Mott crossover in the metal to insulator transition of Nd2Ir2O7

We present an angle-resolved photoemission study of the electronic structure of the three-dimensional pyrochlore iridate Nd2Ir2O7 through its magnetic metal-insulator transition. Our data reveal that metallic Nd2Ir2O7 has a quadratic band, touching the Fermi level at the Gamma point, similarly to that of Pr2Ir2O7. The Fermi node state is, therefore, a common feature of the metallic phase of the pyrochlore iridates. Upon cooling below the transition temperature, this compound exhibits a gap opening with an energy shift of quasiparticle peaks like a band gap insulator. The quasiparticle peaks are strongly suppressed, however, with further decrease of temperature, and eventually vanish at the lowest temperature, leaving a non-dispersive flat band lacking long-lived electrons. We thereby identify a remarkable crossover from Slater to Mott insulators with decreasing temperature. These observations explain the puzzling absence of Weyl points in this material, despite its proximity to the zero temperature metal-insulator transition.

cond-mat.str-el↗

arXiv2016

Revealing the ultrafast light-to-matter energy conversion before heat diffusion in a layered Dirac semimetal

There is still no general consensus on how one can describe the out-of-equilibrium phenomena in matter induced by an ultrashort light pulse. We investigate the pulse-induced dynamics in a layered Dirac semimetal SrMnBi2 by pump-and-probe photoemission spectroscopy. At ~<1 ps, the electronic recovery slowed upon increasing the pump power. Such a bottleneck-type slowing is expected in a two-temperature model (TTM) scheme, although opposite trends have been observed to date in graphite and in cuprates. Subsequently, an unconventional power-law cooling took place at ~100 ps, indicating that spatial heat diffusion is still ill defined at ~100 ps. We identify that the successive dynamics before the emergence of heat diffusion is a canonical realization of a TTM scheme. Criteria for the applicability of the scheme is also provided.

cond-mat.mtrl-sci↗

arXiv2016

Quasi-particles ultrafastly releasing kink bosons to form Fermi arcs in a cuprate superconductor

In a conventional framework, superconductivity is lost at a critical temperature (T_c) because, at higher temperatures, gluing bosons can no longer bind two electrons into a Cooper pair. In high-T_c cuprates, it is still unknown how superconductivity vanishes at T_c. We provide evidence that the so-called <~70-meV kink bosons that dress the quasi-particle excitations are playing a key role in the loss of superconductivity in a cuprate. We irradiated a 170-fs laser pulse on Bi2Sr2CaCu2O8+δand monitored the responses of the superconducting gap and dressed quasi-particles by time- and angle-resolved photoemission spectroscopy. We observe an ultrafast loss of superconducting gap near the d-wave node, or light-induced Fermi arcs, which is accompanied by spectral broadenings and weight redistributions occurring within the kink binding energy. We discuss that the underlying mechanism of the spectral broadening that induce the Fermi arc is the undressing of quasi-particles from the kink bosons. The loss mechanism is beyond the conventional framework, and can accept the unconventional phenomena such as the signatures of Cooper pairs remaining at temperatures above T_c.

cond-mat.supr-con↗

arXiv2015

Quadratic Fermi Node in a 3D Strongly Correlated Semimetal

Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central to this emerging area are the 5d transition metal iridium oxides. Here, in the pyrochlore iridate Pr2Ir2O7, we identify a nontrivial state with a single point Fermi node protected by cubic and time-reversal symmetries, using a combination of angle-resolved photoemission spectroscopy and first principles calculations. Owing to its quadratic dispersion, the unique coincidence of four degenerate states at the Fermi energy, and strong Coulomb interactions, non-Fermi liquid behavior is predicted, for which we observe some evidence. Our discovery implies that Pr2Ir2O7 is a parent state that can be manipulated to produce other strongly correlated topological phases, such as topological Mott insulator, Weyl semi-metal, and quantum spin and anomalous Hall states.

cond-mat.str-el↗

arXiv2015

Temperature-Dependence of Magnetically-Active Charge Excitations in Magnetite across the Verwey Transition

We have studied the electronic structure of bulk single crystals and epitaxial films of magnetite Fe$_3$O$_4$. Fe $2p$ core-level spectra show clear differences between hard x-ray (HAX-) and soft x-ray (SX-) photoemission spectroscopy (PES), indicative of surface effects. The bulk-sensitive spectra exhibit temperature ($T$)-dependent charge excitations across the Verwey transition at $T_V$=122 K, which is missing in the surface-sensitive spectra. An extended impurity Anderson model full-multiplet analysis reveals roles of the three distinct Fe-species (A-Fe$^{3+}$, B-Fe$^{2+}$, B-Fe$^{3+}$) below $T_V$ for the Fe $2p$ spectra, and its $T-$dependent evolution. The Fe $2p$ HAXPES spectra show a clear magnetic circular dichroism (MCD) in the metallic phase of magnetized 100-nm-thick films. The model calculations also reproduce the MCD and identify the magnetically distinct sites associated with the charge excitations. Valence band HAXPES shows finite density of states at $E_F$ for the polaronic metal with remnant order above $T_V$, and a clear gap formation below $T_V$. The results indicate that the Verwey transition is driven by changes in the strongly correlated and magnetically active B-Fe$^{2+}$ and B-Fe$^{3+}$ electronic states, consistent with resistivity and bulk-sensitive optical spectra.

cond-mat.str-el↗

arXiv2015

Hybridization gap formation in the Kondo insulator YbB$_{12}$ observed using time-resolved photoemission spectroscopy

A detailed low-energy electronic structure of a Kondo insulator YbB$_{12}$ was revealed by a synergetic combination of ultrahigh-resolution laser photoemission spectroscopy (PES) and time-resolved PES. The former confirmed a 25-meV pseudogap corresponding to the Kondo temperature of this material, and more importantly, it revealed that a 15-meV gap and a Kondo-peak feature developed below a crossover temperature $T^\ast \sim 110$ K. In harmony with this, the latter discovered a very long recombination time exceeding 100 ps below $\sim$$T^\ast$. This is a clear manifestation of photoexcited carriers due to the bottleneck in the recovery dynamics, which is interpreted as a developing hybridization gap of a hard gap.

cond-mat.str-el↗

arXiv2015

Emergent photovoltage on SmB6 surface upon bulk-gap evolution revealed by pump-and-probe photoemission spectroscopy

Recent studies suggest that an exemplary Kondo insulator SmB6 belongs to a new class of topological insulators (TIs), in which non-trivial spin-polarized metallic states emerge on surface upon the formation of Kondo hybridization gap in the bulk. Remarkably, the bulk resistivity reaches more than 20 Ohm cm at 4 K, making SmB6 a candidate for a so-called bulk-insulating TI. We here investigate optical-pulse responses of SmB6 by pump-and-probe photoemission spectroscopy. Surface photovoltage effect is observed below ~90 K. This indicates that an optically-active band bending region develops beneath the novel metallic surface upon the bulk-gap evolution. The photovoltaic effect persists for >200 microsec, which is long enough to be detected by electronics devices, and could be utilized for optical gating of the novel metallic surface.

cond-mat.str-el↗

arXiv2015

Point nodes persisting far beyond Tc in Bi2212

In contrast to a complex feature of antinodal state, suffering from competing order(s), the "pure" pairing gap of cuprates is obtained in the nodal region, which therefore holds the key to the superconducting mechanism. One of the biggest question is whether the point nodal state as a hallmark of d-wave pairing collapses at Tc like the BCS-type superconductors, or it instead survives above Tc turning into the preformed pair state. A difficulty in this issue comes from the small magnitude of the nodal gap, which has been preventing experimentalists from solving it. Here we use a laser ARPES capable of ultrahigh energy resolution, and detect the point nodes surviving far beyond Tc in Bi2212. By tracking the temperature evolution of spectra, we reveal that the superconductivity occurs when the pair breaking rate is suppressed smaller than the single particle scattering rate on cooling, which governs the value of Tc in cuprates.

cond-mat.supr-con↗

arXiv2015

Numerical simulation of super-square patterns in Faraday waves

We report the first simulations of the Faraday instability using the full three-dimensional Navier-Stokes equations in domains much larger than the characteristic wavelength of the pattern. We use a massively parallel code based on a hybrid Front-Tracking/Level-set algorithm for Lagrangian tracking of arbitrarily deformable phase interfaces. Simulations performed in rectangular and cylindrical domains yield complex patterns. In particular, a superlattice-like pattern similar to those of [Douady & Fauve, Europhys. Lett. 6, 221-226 (1988); Douady, J. Fluid Mech. 221, 383-409 (1990)] is observed. The pattern consists of the superposition of two square superlattices. We conjecture that such patterns are widespread if the square container is large compared to the critical wavelength. In the cylinder, pentagonal cells near the outer wall allow a square-wave pattern to be accommodated in the center.

physics.flu-dyn↗

arXiv2014

A Solver for Massively Parallel Direct Numerical Simulation of Three-Dimensional Multiphase Flows

We present a new solver for massively parallel simulations of fully three-dimensional multiphase flows. The solver runs on a variety of computer architectures from laptops to supercomputers and on 65536 threads or more (limited only by the availability to us of more threads). The code is wholly written by the authors in Fortran 2003 and uses a domain decomposition strategy for parallelization with MPI. The fluid interface solver is based on a parallel implementation of the LCRM hybrid Front Tracking/Level Set method designed to handle highly deforming interfaces with complex topology changes. We discuss the implementation of this interface method and its particular suitability to distributed processing where all operations are carried out locally on distributed subdomains. We have developed parallel GMRES and Multigrid iterative solvers suited to the linear systems arising from the implicit solution of the fluid velocities and pressure in the presence of strong density and viscosity discontinuities across fluid phases. Particular attention is drawn to the details and performance of the parallel Multigrid solver. The code includes modules for flow interaction with immersed solid objects, contact line dynamics, species and thermal transport with phase change. Here, however, we focus on the simulation of the canonical problem of drop splash onto a liquid film and report on the parallel performance of the code on varying numbers of threads. The 3D simulations were run on mesh resolutions up to $1024^3$ with results at the higher resolutions showing the fine details and features of droplet ejection, crown formation and rim instability observed under similar experimental conditions. Keywords:

physics.flu-dyn↗