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S. Stobbe

Publications and source records attributed to S. Stobbe.

At least 19 recordsLinked to original sources

Engineering nanoscale hypersonic phonon transport

Controlling the vibrations in solids is crucial to tailor their mechanical properties and their interaction with light. Thermal vibrations represent a source of noise and dephasing for many physical processes at the quantum level. One strategy to avoid these vibrations is to structure a solid such that it possesses a phononic stop band, i.e., a frequency range over which there are no available mechanical modes. Here, we demonstrate the complete absence of mechanical vibrations at room temperature over a broad spectral window, with a 5.3 GHz wide band gap centered at 8.4 GHz in a patterned silicon nanostructure membrane measured using Brillouin light scattering spectroscopy. By constructing a line-defect waveguide, we directly measure GHz localized modes at room temperature. Our experimental results of thermally excited guided mechanical modes at GHz frequencies provides an eficient platform for photon-phonon integration with applications in optomechanics and signal processing transduction.

physics.optics

Single-photon superradiance from a quantum dot

We report on the observation of single-photon superradiance from an exciton in a semiconductor quantum dot. The confinement by the quantum dot is strong enough for it to mimic a two-level atom, yet sufficiently weak to ensure superradiance. The electrostatic interaction between the electron and the hole comprising the exciton gives rise to an anharmonic spectrum, which we exploit to prepare the superradiant quantum state deterministically with a laser pulse. We observe a five-fold enhancement of the oscillator strength compared to conventional quantum dots. The enhancement is limited by the base temperature of our cryostat and may lead to oscillator strengths above 1000 from a single quantum emitter at optical frequencies.

cond-mat.mes-hall

Optical refrigeration with coupled quantum wells

Refrigeration of a solid-state system with light has potential applications for cooling small-scale electronics and photonics. We show theoretically that two coupled semiconductor quantum wells are efficient cooling media for optical refrigeration because they support long-lived indirect electron-hole pairs. Thermal excitation of these pairs to distinct higher-energy states with faster radiative recombination allows an efficient escape channel to remove thermal energy from the system. This allows reaching much higher cooling efficiencies than with single quantum wells. From band-diagram calculations along with an experimentally realistic level scheme we calculate the cooling efficiency and cooling yield of different devices with coupled quantum wells embedded in a suspended nanomembrane. The dimension and composition of the quantum wells allow optimizing either of these quantities, which cannot, however, be maximized simultaneously. Quantum-well structures with electrical control allow tunability of carrier lifetimes and energy levels so that the cooling efficiency can be optimized over time as the thermal population decreases due to the cooling.

cond-mat.mes-hall

Single-photon nonlinear optics with a quantum dot in a waveguide

Strong nonlinear interactions between photons enable logic operations for both classical and quantum-information technology. Unfortunately, nonlinear interactions are usually feeble and therefore all-optical logic gates tend to be inefficient. A quantum emitter deterministically coupled to a propagating mode fundamentally changes the situation, since each photon inevitably interacts with the emitter, and highly correlated many-photon states may be created . Here we show that a single quantum dot in a photonic-crystal waveguide can be utilized as a giant nonlinearity sensitive at the single-photon level. The nonlinear response is revealed from the intensity and quantum statistics of the scattered photons, and contains contributions from an entangled photon-photon bound state. The quantum nonlinearity will find immediate applications for deterministic Bell-state measurements and single-photon transistors and paves the way to scalable waveguide-based photonic quantum-computing architectures.

quant-ph

Efficient out-coupling of high-purity single photons from a coherent quantum dot in a photonic-crystal cavity

We demonstrate a single-photon collection efficiency of $(44.3\pm2.1)\%$ from a quantum dot in a low-Q mode of a photonic-crystal cavity with a single-photon purity of $g^{(2)}(0)=(4\pm5)\%$ recorded above the saturation power. The high efficiency is directly confirmed by detecting up to $962\pm46$ kilocounts per second on a single-photon detector on another quantum dot coupled to the cavity mode. The high collection efficiency is found to be broadband, as is explained by detailed numerical simulations. Cavity-enhanced efficient excitation of quantum dots is obtained through phonon-mediated excitation and under these conditions, single-photon indistinguishability measurements reveal long coherence times reaching $0.77\pm0.19$ ns in a weak-excitation regime. Our work demonstrates that photonic crystals provide a very promising platform for highly integrated generation of coherent single photons including the efficient out-coupling of the photons from the photonic chip.

quant-ph

Near-unity coupling efficiency of a quantum emitter to a photonic-crystal waveguide

A quantum emitter efficiently coupled to a nanophotonic waveguide constitutes a promising system for the realization of single-photon transistors, quantum-logic gates based on giant single-photon nonlinearities, and high bit-rate deterministic single-photon sources. The key figure of merit for such devices is the $β$-factor, which is the probability for an emitted single photon to be channeled into a desired waveguide mode. We report on the experimental achievement of $β= 98.43 \pm 0.04\%$ for a quantum dot coupled to a photonic-crystal waveguide, corresponding to a single-emitter cooperativity of $η= 62.7 \pm 1.5$. This constitutes a nearly ideal photon-matter interface where the quantum dot acts effectively as a 1D "artificial" atom, since it interacts almost exclusively with just a single propagating optical mode. The $β$-factor is found to be remarkably robust to variations in position and emission wavelength of the quantum dots. Our work demonstrates the extraordinary potential of photonic-crystal waveguides for highly efficient single-photon generation and on-chip photon-photon interaction.

quant-ph

Influence of multi-electronic states on few-quantum-dot nanolasers

We present an experimental and theoretical study on the gain mechanism in a photonic-crystal-cavity nanolaser with embedded quantum dots. From time-resolved measurements at low excitation power we find that four excitons are coupled to the cavity. At high excitation power we observe a smooth low-threshold transition from spontaneous emission to lasing. Before lasing emission sets in, however, the excitons are observed to saturate, and the gain required for lasing originates rather from multi-electronic transitions, which give rise to a broad emission background. We compare the experiment to a model of quantum-dot microcavity lasers and find that the number of emitters feeding the cavity must greatly exceed four, which confirms that the gain is provided by multi-electronic states. Our results are consistent with theoretical predictions.

cond-mat.mes-hall

Measuring the effective phonon density of states of a quantum dot

We employ detuning-dependent decay-rate measurements of a quantum dot in a photonic-crystal cavity to study the influence of phonon dephasing in a solid-state quantum-electrodynamics experiment. The experimental data agree with a microscopic non-Markovian model accounting for dephasing from longitudinal acoustic phonons, and identifies the reason for the hitherto unexplained difference between non-resonant cavity feeding in different nanocavities. From the comparison between experiment and theory we extract the effective phonon density of states experienced by the quantum dot. This quantity determines all phonon dephasing properties of the system and is found to be described well by a theory of bulk phonons.

cond-mat.mes-hall

Extraction of optical Bloch modes in a photonic-crystal waveguide

We perform phase-sensitive near-field scanning optical microscopy on photonic-crystal waveguides. The observed intricate field patterns are analyzed by spatial Fourier transformations, revealing several guided TE- and TM-like modes. Using the reconstruction algorithm proposed by Ha, et al. (Opt. Lett. 34 (2009)), we decompose the measured two-dimensional field pattern in a superposition of propagating Bloch modes. This opens new possibilities to study specific modes in near-field measurements. We apply the method to study the transverse behavior of a guided TE-like mode, where the mode extends deeper in the surrounding photonic crystal when the band edge is approached.

physics.optics

Photonic-Crystal Waveguides with Disorder: Measurement of a Band-Edge Tail in the Density of States

We measure localized and extended mode profiles at the band edge of slow-light photonic-crystal waveguides using phase-sensitive near-field microscopy. High-resolution band structures are obtained and interpreted, allowing the retrieval of the optical density of states (DOS). This constitutes a first observation of the DOS of a periodic system with weak disorder. The Van Hove singularity in the DOS expected at the band edge of an ideal 1D periodic structure is removed by the disorder. The Anderson-localized states form a "tail" in the density of states, as predicted by Lifshitz for solid-state systems.

physics.optics

On the interpretation of wave function overlaps in quantum dots

The spontaneous emission rate of excitons strongly confined in quantum dots is proportional to the overlap integral of electron and hole envelope wave functions. A common and intuitive interpretation of this result is that the spontaneous emission rate is proportional to the probability that the electron and the hole are located at the same point or region in space, i.e. they must coincide spatially to recombine. Here we show that this interpretation is not correct even loosely speaking. By general mathematical considerations we compare the envelope wave function overlap, the exchange overlap integral, and the probability of electrons and holes coinciding and find that the frequency dependence of the envelope wave function overlap integral is very different from that expected from the common interpretation. We show that these theoretical considerations lead to predictions for measurements. We compare our qualitative predictions with recent measurements of the wave function overlap and find good agreement.

cond-mat.mes-hall

Optoelectronic cooling of mechanical modes in a semiconductor nanomembrane

Optical cavity cooling of mechanical resonators has recently become a research frontier. The cooling has been realized with a metal-coated silicon microlever via photo-thermal force and subsequently with dielectric objects via radiation pressure. Here we report cavity cooling with a crystalline semiconductor membrane via a new mechanism, in which the cooling force arises from the interaction between the photo-induced electron-hole pairs and the mechanical modes through the deformation potential coupling. The optoelectronic mechanism is so efficient as to cool a mode down to 4 K from room temperature with just 50 uW of light and a cavity with a finesse of 10 consisting of a standard mirror and the sub-wavelength-thick semiconductor membrane itself. The laser-cooled narrow-band phonon bath realized with semiconductor mechanical resonators may open up a new avenue for photonics and spintronics devices.

cond-mat.mes-hall

Mutual Coupling of two Semiconductor Quantum Dots via an Optical Nanocavity Mode

We present an experimental and theoretical study of a system consisting of two spatially separated self-assembled InGaAs quantum dots strongly coupled to a single optical nanocavity mode. Due to their different size and compositional profiles, the two quantum dots exhibit markedly different DC Stark shifts. This allows us to tune them into mutual resonance with each other and a photonic crystal nanocavity mode as a bias voltage is varied. Photoluminescence measurements show a characteristic triple peak during the double anticrossing, which is a clear signature of a coherently coupled system of three quantum states. We fit the entire set of emission spectra of the coupled system to theory and are able to investigate the coupling between the two quantum dots via the cavity mode, and the coupling between the two quantum dots when they are detuned from the cavity mode. We suggest that the resulting quantum V-system may be advantageous since dephasing due to incoherent losses from the cavity mode can be avoided.

cond-mat.mes-hall

Large quantum dots with small oscillator strength

We have measured the oscillator strength and quantum efficiency of excitons confined in large InGaAs quantum dots by recording the spontaneous emission decay rate while systematically varying the distance between the quantum dots and a semiconductor-air interface. The size of the quantum dots is measured by in-plane transmission electron microscopy and we find average in-plane diameters of 40 nm. We have calculated the oscillator strength of excitons of that size and predict a very large oscillator strength due to Coulomb effects. This is in stark contrast to the measured oscillator strength, which turns out to be much below the upper limit imposed by the strong confinement model. We attribute these findings to exciton localization in local potential minima arising from alloy intermixing inside the quantum dots.

cond-mat.mes-hall

Controlling Anderson localization in disordered photonic crystal waveguides

We prove Anderson localization in a disordered photonic crystal waveguide by measuring the ensemble-averaged localization length which is controlled by the dispersion of the photonic crystal waveguide. In such structures, the localization length shows a 10-fold variation between the fast- and the slow-light regime and, in the latter case, it becomes shorter than the sample length thus giving rise to strongly confined modes. The dispersive behavior of the localization length demonstrates the close relation between Anderson localization and the photon density of states in disordered photonic crystals, which opens a promising route to controlling and exploiting Anderson localization for efficient light confinement.

physics.optics

Polarization dependent spontaneous-emission rate of single quantum dots in photonic crystal membranes

We have measured the variation of the spontaneous emission rate with polarization for self-assembled single quantum dots in two-dimensional photonic crystal membranes. We observe a maximum anisotropy factor of 6 between the decay rates of the two bright exciton states. This large anisotropy is attributed to the substantially different projected local density of optical states for differently oriented dipoles in the photonic crystal.

quant-ph

Electrical control of spontaneous emission and strong coupling for a single quantum dot

We report the design, fabrication and optical investigation of electrically tunable single quantum dot - photonic crystal defect nanocavities operating in both the weak and strong coupling regimes of the light matter interaction. Unlike previous studies where the dot-cavity spectral detuning was varied by changing the lattice temperature, or by the adsorption of inert-gases at low temperatures, we demonstrate that the quantum confined Stark effect can be employed to quickly and reversibly switch the dot-cavity coupling simply by varying a gate voltage. Our results show that exciton transitions from individual dots can be tuned by ~4 meV relative to the nanocavity mode before the emission quenches due to carrier tunneling escape. This range is much larger than the typical linewidth of the high-Q cavity modes (~0.10 meV) allowing us to explore and contrast regimes where the dots couple to the cavity or decay by spontaneous emission into the 2D photonic bandgap. In the weak coupling regime, we show that the dot spontaneous emission rate can be tuned using a gate voltage, with Purcell factors >=7. New information is obtained on the nature of the dot-cavity coupling in the weak coupling regime and electrical control of zero dimensional polaritons is demonstrated for the highest-Q cavities (Q>=12000). Vacuum Rabi splittings up to ~0.13 meV are observed, much larger than the linewidths of either the decoupled exciton or cavity mode. These observations represent a voltage switchable optical non-linearity at the single photon level, paving the way towards on-chip dot based nano-photonic devices that can be integrated with passive optical components.

cond-mat.mtrl-sci

Decay dynamics of quantum dots influenced by the local density of optical states of two-dimensional photonic crystal membranes

We have performed time-resolved spectroscopy on InAs quantum dot ensembles in photonic crystal membranes. The influence of the photonic crystal is investigated by varying the lattice constant systematically. We observe a strong slow down of the quantum dots' spontaneous emission rates as the two-dimensional bandgap is tuned through their emission frequencies. The measured band edges are in full agreement with theoretical predictions. We characterize the multi-exponential decay curves by their mean decay time and find enhancement of the spontaneous emission at the bandgap edges and strong inhibition inside the bandgap in good agreement with local density of states calculations.

cond-mat.mes-hall