arXiv subjects

S. Sukiasyan

Publications and source records attributed to S. Sukiasyan.

3 recordsLinked to original sources

arXiv2023

Intense high-order harmonic generation in giant fullerene molecule C$_{240}$

In this work the extreme nonlinear optical response of a giant fullerene molecule C$_{240}$ in strong laser field is studied. The investigation of high-order harmonic generation in such quantum nanostructure is presented modeling the C$_{240}$ molecule and its interaction with the laser field in the scope of the tight-binding mean-field approach. Electron-electron interaction is modeled by the parametrized Ohno potentail, which takes into account long-range Coulomb interaction. The essential role of many body Coulomb interaction in determining of harmonics intensities is demonstrated. We also consider vacancy-deffected molecule C$_{240}$. The presence of a single vacancy breaks the icosahedral symmetry leading to the emergence of intense even-order harmonics. We examine the dependence of moderate harmonics on laser frequency that shows the multiphoton resonant nature of high harmonics generation. The dependence of cutoff harmonics on both laser intensity and frequency are examined too.

physics.optics↗

arXiv2023

Disorder-induced effects in high-harmonic generation process in fullerene molecules

The objective of this article is to investigate the profound nonlinear optical response exhibited by inversion symmetric fullerene molecules under the influence of different types of disorders described by the Anderson model. Our aim is to elucidate the localization effects on the spectra of high harmonic generation in such molecules. We show that the disorder-induced effects are imprinted onto molecules' high-harmonic spectrum. Specifically, we observe a presence of strong even-order harmonic signals already for relatively small disorders. The odd-order harmonics intrinsic for disorder-free systems are generally robust to minor disorders. Both diagonal and off-diagonal disorders lift the degeneracy of states, opening up new channels for interband transitions, leading to the enhancement of the high-harmonic emission. The second harmonic signal has a special behavior depending on the disorder strength. Specifically in the case of diagonal disorder, the second harmonic intensity exhibits a quadratic scaling with the disorder strength, which enables the usage of the harmonic spectrum as a tool in measuring the type and the strength of a disorder.

physics.optics↗

arXiv2022

Reconciling conflicting approaches for the tunneling time delay in strong field ionization

Several recent attoclock experiments have investigated the fundamental question of a quantum mechanically induced time delay in tunneling ionization via extremely precise photoelectron momentum spectroscopy. The interpretations of those attoclock experimental results were controversially discussed, because the entanglement of the laser and Coulomb field did not allow for theoretical treatments without undisputed approximations. The method of semiclassical propagation matched with the tunneled wavefunction, the quasistatic Wigner theory, the analytical R-matrix theory, the backpropagation method, and the under-the-barrier recollision theory are the leading conceptual approaches put forward to treat this problem, however, with seemingly conflicting conclusions on the existence of a tunneling time delay. To resolve the contradicting conclusions of the different approaches, we consider a very simple tunneling scenario which is not plagued with complications stemming from the Coulomb potential of the atomic core, avoids consequent controversial approximations and, therefore, allows us to unequivocally identify the origin of the tunneling time delay.

quant-ph↗