arXiv subjects

S. T. Cundiff

Publications and source records attributed to S. T. Cundiff.

16 recordsLinked to original sources

arXiv2019

Quantum Interference Control of Carriers and Currents in Zincblende Semiconductors based on Nonlinear Absorption Processes

Quantum interference between optical absorption processes can excite carriers with a polarized distribution in the Brillouin zone depending on properties of the incident optical fields. The polarized distribution of carriers introduces a current that can be controlled by the phases and polarizations of the incident optical fields. Here we study the quantum interference of 2- and 3-photon absorption processes in AlGaAs. We present theoretical predictions for carrier and current injection rates considering different frequencies, phases, and polarizations of the incident fields. We also discuss the important features that result from only nonlinear optical processes being involved, which leads for instance to a sharper distribution of carriers in the Brillouin zone.

cond-mat.mtrl-sci↗

arXiv2019

Quantum Interference Control of Photocurrents in Semiconductors by Nonlinear Optical Absorption Processes

We report experiments demonstrating Quantum Interference Control (QuIC) based on two nonlinear optical absorption processes in semiconductors. We use two optical beams of frequencies $ω$ and $3ω/2$ incident on AlGaAs and measure the injection current due to the interference between 2- and 3-photon absorption processes. We analyze the dependence of the injection current on the intensities and phases of the incident fields.

cond-mat.mes-hall↗

arXiv2018

Vibrational Coupling Modifies Spectral Diffusion in Core-Shell Colloidal Quantum Dots

We perform two-dimensional coherent spectroscopy on CdSe/CdZnS core/shell colloidal quantum dots at cryogenic temperatures. In the two-dimensonal spectra, sidebands due to electronic coupling with CdSe lattice LO-phonon modes are observed that have evolutions deviating from the exponential dephasing expected from Markovian spectral diffusion. Comparison to simulations provides further evidence that the LO-phonon mode coupling itself significantly modifies the exciton lineshapes and results in the underlying spectral diffusion on ultrafast timescales.

cond-mat.mtrl-sci↗

arXiv2015

Comment on "Nonlinear fluctuations and dissipation in matter revealed by quantum light"

In a recent paper [Phys.~Rev.~A {\bf 91}, 053844 (2015)], Mukamel and Dorfman compare spectroscopies performed with classical vs.~quantum light, and conclude that \textit{nonlinear} quantum-spectroscopy signals cannot be obtained from averaging their classical-spectroscopy counterparts over the Glauber--Sudarshan quasiprobability distribution of the quantum field. In this Comment, we show that this interpretation is correct only if one assumes that a classical signal is given by a classical approximation for the field. While such an assumption can be useful for comparing theoretical results, it is never realized in laser spectroscopy experiments that typically use coherent states. Thus, instead of using classical signals, the connection between coherent states and quantum states of light must be considered. We rigorously show that quantum spectroscopy can always be projected from the experimentally realized coherent-state spectroscopy regardless how nonlinear the system response is.

cond-mat.mes-hall↗

arXiv2013

Exciton-Trion Coherent Interactions in a CdTe/CdMgTe Quantum Well

We present a collection of zero-, one- and two-quantum two-dimensional coherent spectra of excitons and trions in a CdTe/(Cd,Mg)Te quantum well. The set of spectra provides a unique and comprehensive picture of the exciton and trion nonlinear optical response. Exciton-exciton and exciton-trion coherent coupling is manifest as distinct peaks in the spectra, whereas signatures of trion-trion interactions are absent. Excellent agreement using density matrix calculations is obtained, which highlights the essential role of many-body effects on coherent interactions in the quantum well.

cond-mat.mes-hall↗

arXiv2012

Fifth-order nonlinear optical response of excitonic states in an InAs quantum dot ensemble measured with 2D spectroscopy

Exciton, trion and biexciton dephasing rates are measured within the inhomogeneous distribution of an InAs quantum dot (QD) ensemble using two-dimensional Fourier-transform spectroscopy. The dephasing rate of each excitonic state is similar for all QDs in the ensemble and the rates are independent of excitation density. An additional spectral feature -- too weak to be observed in the time-integrated four-wave mixing signal -- appears at high excitation density and is attributed to the $χ^{\textrm{(5)}}$ biexcitonic nonlinear response.

cond-mat.mes-hall↗

arXiv2011

A Versatile Ultra-Stable Platform for Optical Multidimensional Fourier-Transform Spectroscopy

The JILA Multidimensional Optical Nonlinear SpecTRometer (JILA-MONSTR) is a robust, ultra-stable platform consisting nested and folded Michelson interferometers that can be actively phase stabilized. This platform generates a square of identical laser pulses that can be adjusted to have arbitrary time delay between them, while maintaining phase stability. The JILA-MONSTR provides output pulses for nonlinear excitation of materials and phase-stabilized reference pulses for heterodyne detection of the induced signal. This arrangement is ideal for performing coherent optical experiments, such as multidimensional Fourier-transform spectroscopy, which records the phase of the nonlinear signal as a function of the time delay between several of the excitation pulses. The resulting multidimensional spectrum is obtained from a Fourier transform. This spectrum can resolve, separate and isolate coherent contributions to the light-matter interactions associated with electronic excitation at optical frequencies. To show the versatility of the JILA-MONSTR, several demonstrations of two-dimensional Fourier-transform spectroscopy are presented, including an example of a phase-cycling scheme that reduces noise.

physics.optics↗

arXiv2011

Electric field-induced quantum interference control in a semiconductor: A new manifestation of the Franz-Keldysh effect

In (100)-oriented GaAs illuminated at normal incidence by a laser and its second harmonic, interference between one- and two-photon absorption results in ballistic current injection, but not modulation of the overall carrier injection rate. Results from a pump-probe experiment on a transversely biased sample show that a constant electric field enables coherent control of the carrier injection rate. We ascribe this to the nonlinear optical Franz-Keldysh effect and calculate it for a two-band parabolic model. The mechanism is relevant to centrosymmetric semiconductors as well.

cond-mat.other↗

arXiv2010

Polarization dependence of the two-photon Franz-Keldysh effect

The effect of a constant electric field on two-photon absorption in a direct band gap semiconductor is calculated using an independent-particle theory. Two band structure models for GaAs are used: a two-band parabolic model and an eight-band "k dot p" model. Both predict a strong dependence of the two-photon electroabsorption spectrum on the polarization of the light with respect to the constant field. We attribute the polarization dependence to the strong effect of a constant field on intraband dynamics.

cond-mat.mes-hall↗

arXiv2010

Two-dimensional Fourier-transform Spectroscopy of Potassium Vapor

Optical two-dimensional Fourier-transformed (2DFT) spectroscopy is used to study the coherent optical response of potassium vapor in a thin transmission cell. Rephasing and non-rephasing spectra of the D1 and D2 transitions are obtained and compared to numerical simulations. Calculations using the optical Bloch equations gives very good agreement with the experimental peak strengths and line shapes. Non-radiative Raman-like coherences are isolated using a different 2DFT projection. Density-dependent measurements show distortion of 2DFT spectra due to pulse propagation effects.

physics.atom-ph↗

arXiv2009

Extraction of many-body configurations from nonlinear absorption in semiconductor quantum wells

Detailed electronic many-body configurations are extracted from quantitatively measured timeresolved nonlinear absorption spectra of resonantly excited GaAs quantum wells. The microscopic theory assigns the observed spectral changes to a unique mixture of electron-hole plasma, exciton, and polarization effects. Strong transient gain is observed only under co-circular pump-probe conditions and is attributed to the transfer of pump-induced coherences to the probe.

cond-mat.mes-hall↗

arXiv2009

Ultrafast Spin Dynamics in Optically Excited Bulk GaAs at Low Temperatures

This paper presents a study of electron spin dynamics in bulk GaAs at low temperatures for elevated optical excitation conditions. Our time-resolved Faraday rotation measurements yield sub-nanosecond electron spin dephasing-times over a wide range of n-doping concentrations in quantitative agreement with a microscopic treatment of electron spin dynamics. The calculation shows the occurrence and breakdown of motional narrowing for spin dephasing under elevated excitation conditions. We also find a peak of the spin dephasing time around a doping density for which, under lower excitation conditions, a metal-insulator transition occurs. However, the experimental results for high excitation can be explained without a metal-insulator transition. We therefore attribute the peak in spin-dephasing times to the influence of screening and scattering on the spin-dynamics of the excited electrons.

cond-mat.mtrl-sci↗

arXiv2008

Temperature dependence of the electron spin g factor in GaAs

The temperature dependence of the electron spin $g$ factor in GaAs is investigated experimentally and theoretically. Experimentally, the $g$ factor was measured using time-resolved Faraday rotation due to Larmor precession of electron spins in the temperature range between 4.5 K and 190 K. The experiment shows an almost linear increase of the $g$ value with the temperature. This result is in good agreement with other measurements based on photoluminescence quantum beats and time-resolved Kerr rotation up to room temperature. The experimental data are described theoretically taking into account a diminishing fundamental energy gap in GaAs due to lattice thermal dilatation and nonparabolicity of the conduction band calculated using a five-level kp model. At higher temperatures electrons populate higher Landau levels and the average $g$ factor is obtained from a summation over many levels. A very good description of the experimental data is obtained indicating that the observed increase of the spin $g$ factor with the temperature is predominantly due to band's nonparabolicity.

cond-mat.mtrl-sci↗

arXiv2008

The quantum-limited comb lineshape of a mode-locked laser: Fundamental limits on frequency uncertainty

We calculate the quantum-limited shape of the comb lines from a mode-locked Ti:sapphire laser using experimentally-derived parameters for the linear response of the laser to perturbations. The free-running width of the comb lines is found across the laser spectrum. By modeling the effect of a simple feedback loop, we calculate the spectrum of the residual phase noise in terms of the quantum noise and the feedback parameters. Finally, we calculate the frequency uncertainty in an optical frequency measurement if the limiting factor is quantum noise in the detection of the optical heterodyne beat.

physics.optics↗

arXiv2007

Experimental setup for low-energy laser-based angle resolved photoemission spectroscopy

A laser-based angle resolved photoemission (APRES) system utilizing 6 eV photons from the fourth harmonic of a mode-locked Ti:sapphire oscillator is described. This light source greatly increases the momentum resolution and photoelectron count rate, while reducing extrinsic background and surface sensitivity relative to higher energy light sources. In this review, the optical system is described, and special experimental considerations for low-energy ARPES are discussed. The calibration of the hemispherical electron analyzer for good low-energy angle-mode performance is also described. Finally, data from the heavily studied high T_c superconductor Bi2Sr2CaCu2O8+δ(Bi2212) is compared to the results from higher photon energies.

cond-mat.other↗

arXiv2007

Signatures of Many-Particle Correlations in Two-Dimensional Fourier-Transform Spectra of Semiconductor Nanostructures

On the basis of a microscopic theory, the signatures of many-particle correlations in Two-Dimensional Fourier-Transform Spectra (2D-FTS) of semiconductor nanostructures are identified and compared to experimental data. Spectra in the photon energy range of the heavy-hole and light-hole excitonic resonances show characteristic features due to correlations, which depend on the relative polarization directions of the excitation pulses.

cond-mat.other↗