arXiv subjects

S. Thakur

Publications and source records attributed to S. Thakur.

13 recordsLinked to original sources

arXiv2023

Epitaxial monolayers of magnetic 2D semiconductor FeBr$_{2}$ grown on Au(111)

Magnetic two-dimensional (2D) semiconductors have attracted a lot of attention because modern preparation techniques are capable of providing single crystal films of these materials with precise control of thickness down to the single-layer limit. It opens up a way to study rich variety of electronic and magnetic phenomena with promising routes towards potential applications. We have investigated the initial stages of epitaxial growth of the magnetic van der Waals semiconductor FeBr\textsubscript{2} on a single-crystal Au(111) substrate by means of low-temperature scanning tunneling microscopy, low-energy electron diffraction, x-ray photoemission spectroscopy, low-energy electron emission microscopy and x-ray photoemission electron microscopy. Magnetic properties of the one- and two-layer thick films were measured via x-ray absorption spectroscopy/x-ray magnetic circular dichroism. Our findings show a striking difference in the magnetic behaviour of the single layer of FeBr\textsubscript{2} and its bulk counterpart, which can be attributed to the modifications in the crystal structure due to the interaction with the substrate.

cond-mat.mtrl-sci↗

arXiv2021

Rabi-like splitting and refractive index sensing with hybrid Tamm plasmon-cavity modes

Rabi-like splitting and self-referenced refractive index sensing in hybrid plasmonic-1D photonic crystal structures have been theoretically demonstrated. The coupling between Tamm plasmon and cavity photon modes are tuned by incorporating a low refractive index spacer layer adjacent to the metallic layer to form their hybrid modes. Anticrossing of the modes observed at different values of spacer layer thickness validates the strong coupling between the two modes and causes Rabi-like splitting with different splitting energy. Rabi-like splitting energy decreases with increasing number of periods (N) and refractive index contrast (η) of two dielectric materials used to make the 1D photonic crystals, and the observed variation is explained by an analytical model. Angular and polarization dependency of the hybrid modes shows that the polarization splitting of the lower hybrid mode is much stronger than that of the upper hybrid mode. On further investigation, it is seen that one of the hybrid modes remains unchanged while other mode undergoes significant change with varying the cavity medium. This nature of the hybrid modes has been utilized for designing self-referenced refractive index sensors for sensing different analytes. For η=1.333 and N=10 in a hybrid structure, the sensitivity increases from 51 nm/RIU to 201 nm/RIU with increasing cavity thickness from 170 nm to 892 nm. For the fixed cavity thickness of 892 nm, the sensitivity increases from 201 nm/RIU to 259 nm/RIU by increasing η from 1.333 to 1.605. The sensing parameters such as detection accuracy, quality factor, and figure of merit for two different hybrid structures ([η=1.333, N=10] and [η=1.605, N=6]) have been evaluated and compared. The value of resonant reflectivity of one of the hybrid modes changes considerably with varying analyte medium which can be used for refractive index sensing.

physics.optics↗

arXiv2021

Simulation studies for source optimization in $^{96}$Zr $β$ decay

The single $β$ decay of $^{96}$Zr to the ground state of $^{96}$Nb is spin forbidden and poses a great experimental challenge. The $β$ decay of $^{96}$Zr can be studied via coincident detection of de-exciting gamma rays in $^{96}$Mo, which is the end product of $^{96}$Nb $β$ decay. Simulations are done with four HPGe detector setup (~33% relative efficiency each) to optimize the source configuration. The results suggest that ~70g of 50% enriched $^{96}$Zr will yield sensitivity comparable to the reported results.

physics.ins-det↗

arXiv2021

Ultrafast optically induced ferromagnetic state in an elemental antiferromagnet

We present evidence for an ultrafast optically induced ferromagnetic alignment of antiferromagnetic Mn in Co/Mn multilayers. We observe the transient ferromagnetic signal at the arrival of the pump pulse at the Mn L$_3$ resonance using x-ray magnetic circular dichroism in reflectivity. The timescale of the effect is comparable to the duration of the excitation and occurs before the magnetization in Co is quenched. Theoretical calculations point to the imbalanced population of Mn unoccupied states caused by the Co interface for the emergence of this transient ferromagnetic state.

cond-mat.mes-hall↗

arXiv2020

PRISA: a simple software for determining refractive index, extinction co-efficient, dispersion energy, band gap, and thickness of semiconductor and dielectric thin films

A simple user-friendly software named PRISA has been developed to determine optical constants (refractive index and extinction co-efficient), dispersion parameters (oscillator energy and dispersion energy), absorption co-efficient, band gap and thickness of semiconductor and dielectric thin films from their measured transmission spectrum, only. The thickness, refractive index, and extinction co-efficient of the films have been derived using Envelope method proposed by Swanepoel. The absorption co-efficient in the strong absorption region is calculated using the method proposed by Connel and Lewis. Subsequently, both direct and indirect bandgap of the films is estimated from the absorption co-efficient spectrum using Tauc plot. The codes for the software are written in Python and the graphical user interface is programmed with tkinter package of Python. It provides convenient input and output of the measured and derived data. The software has a feature to retrieve transmission spectrum using the derived parameters in order to check their reliability. The performance of the software is verified by analyzing numerically generated transmission spectra of a-Si:H amorphous semiconductor thin films, and experimentally measured transmission spectra of electron beam evaporated HfO2 dielectric thin films as examples. PRISA is found to be much simpler and accurate as compared to the other freely available softwares. To help other researchers working on thin films, the software is made freely available at https://www.shuvendujena.tk/download.

cond-mat.mtrl-sci↗

arXiv2018

Multiplicity spectra in $e^{+}e^{-}$ and $\overline{p}p$ collisions in terms of Tsallis and Weibull distributions

Charged hadron production in the $e^{+}e^{-}$ annihilations at 91 to 206 GeV in full phase space and in $\overline{p}p$ collisions at 200 to 900~GeV collision energies are studied using non-extensive Tsallis and stochastic Weibull probability distributions.~The Tsallis distribution shows better description of the data than the Weibull distribution. The 2-jet modification of the statistical distribution is applied to describe $e^{+}e^{-}$ data.~The main features of these distributions can be described by a two-component model with soft, collective interactions at low transverse energy and hard, constituent interactions dominating at high transverse energy.~This modification is found to give much better description than a full-sample fit, and again Tsallis function is found to better describe the data than the Weibull one pointing at the non-extensive character of the multiparticle production process.

hep-ph↗

arXiv2018

Direct observation of strain-induced orbital valence band splitting in HfSe$_2$ by sodium intercalation

By using angle-resolved photoemission spectroscopy (ARPES), the variation of the electronic structure of HfSe$_2$ has been studied as a function of sodium intercalation. We observe how this drives a band splitting of the p-orbital valence bands and a simultaneous reduction of the indirect band gap by values of up to 400 and 280 meV respectively. Our calculations indicate that such behaviour is driven by the band deformation potential, which is a result of our observed anisotropic strain induced by sodium intercalation. The applied uniaxial strain calculations based on density functional theory (DFT) agree strongly with the experimental ARPES data. These findings should assist in studying the physical relationship between doping and strain, as well as for large-scale two-dimensional straintronics.

cond-mat.mtrl-sci↗

arXiv2017

Modified Weibull and Tsallis Distributions for multiplicities in $e^{+}e^{-}$ collisions at LEP2 energies

Multiplicity distributions of charged particles produced in the $e^{+}e^{-}$ collisions at LEP2 energies ranging from 91 to 206 GeV in full phase space, are compared with predictions from Tsallis $q$-statistics and the recently proposed Weibull distribution functions.~The analysis uses data from two LEP experiments, L3 and OPAL.~It is shown that Tsallis $q$-statistics explains the data in a statistically acceptable manner in full phase space at all energies, while the Weibull distribution fails to explain the underlying properties of the data.~Modifications to the distributions proposed earlier, are applied to uncover manifold improvements in explaining the data characteristics.

hep-ph↗

arXiv2017

Modified Tsallis and Weibull distributions for multiplicities in e+e- collisions

Multiplicity distributions of charged particles produced in the e^{+}e^{-} collisions at energies ranging from 14 to 91 GeV are studied using Tsallis q-statistics and the recently proposed Weibull distribution functions, in both restricted rapidity windows as well as in full phase space. It is shown that Tsallis $q$-statistics explains the data excellently in all rapidity ranges while the Weibull distribution fails to reproduce the data in full phase space. Modifications to the distributions are proposed to establish manifold improvements in the fitting of the data.

hep-ph↗

arXiv2016

Study of ZrO2 Thin Films Deposited at Glancing Angle by Magnetron Sputtering under Varying Substrate Rotation

In the present work, a set of ZrO2 thin films have been deposited at 82 degree angle of deposition at several substrate rotation speeds and at 0 degree. The effect of substrate rotation on optical, structural, morphological properties and residual stress has been studies thoroughly. Refractive index estimated from ellipsometric measurement and suitable modeling depicts an interesting decreasing behavior with substrate rotation and has been explained in the light of varying columnar structure with substrate rotation. Refractive index of GLAD ZrO2 films varies between and 1.901 to 2.011. Normally deposited film exhibits refractive index value of 2.178 which is substantially greater than that of GLAD films. Lowering in refractive index of glancing angle deposited films is the attribute of dominant atomic shadowing at glancing angles. Further, correlation length which is the representative of surface grain size was obtained from suitable modeling of atomic force microscopy data and it exhibits a decreasing trend with substrate rotation. The trend has also been attributed to the varying columnar microstructure with substrate rotation. All the glancing angle deposited ZrO2 films possess root mean square roughness between 4.6 and 5.1 nm whereas normally deposited film depicts 1.0 nm rms roughness. Dominant atomic shadowing is responsible for high roughness of GLAD films. Both glancing angle and normally deposited films exhibit preferential growth of monoclinic phase oriented in different directions. GLAD films also depict a tetragonal peak which has been attributed to the fine nano-crystallite size (~13 nm). Residual stress depicts a great switching from large compressive to small tensile as the deposition angle switches from normal to glancing angle

cond-mat.mtrl-sci↗

arXiv2014

Structure related optical properties of electron beam evaporated ZrO2:10%SiO2 thin films

ZrO2:10%SiO2 thinfilms have been deposited on fused silica substrate by reactive electron beam co-evaporation technique at different oxygen partial pressure. The structural analysis shows tetragonal phase with residual tensile stress in the films. The intensity of the tetragonal t(110) phase are found increasing with increasing oxygen pressure. The optical band gap is found increasing from 5.06 eV to 5.28 eV because of increasing crystalinity of monoclinic phase, while the film grain size remains almost constant with increase of oxygen pressure, concludes that the crystallite or grain size has no effect on the optical properties of the films. The dispersion of the refractive index is discussed in terms of single oscillator Wimple-DiDomenico model. The dispersion energy parameter better known as structural order parameter are found increasing with the intensity of t(110) phase. It is observed that films having higher value of order parameter show lower surface roughness which concludes that the local microstructure ordering can predominantly influence the grain morphology which in turn can lead to better surface for higher value of order parameter.

cond-mat.mtrl-sci↗

arXiv2013

Anomaly in the electronic structure of a BCS superconductor, ZrB(12)

We investigate the electronic structure of a complex conventional superconductor, ZrB12 employing high resolution photoemission spectroscopy and ab initio band structure calculations. The experimental valence band spectra could be described reasonably well within the local density approximation. Energy bands close to the Fermi level possess t_(2g) symmetry and the Fermi level is found to be in the proximity of quantum fluctuation regime. The spectral lineshape in the high resolution spectra is complex exhibiting signature of a deviation from Fermi liquid behavior. A dip at the Fermi level emerges above the superconducting transition temperature that gradually grows with the decrease in temperature. The spectral simulation of the dip and spectral lineshape based on a phenomenological self energy suggests a finite electron pair lifetime and a pseudogap above the superconducting transition temperature.

cond-mat.supr-con↗

arXiv2013

Surface bulk differences in a conventional superconductor, ZrB(12)

We studied the electronic structure of a conventional superconductor, ZrB(12) using high resolution x-photoemission spectroscopy and single crystalline samples. Experimental results with different bulk sensitivity reveals boron deficiency and different valence states of Zr at the surface relative to the bulk. Signature of a satellite features is observed in the Zr core level spectra corresponding to the bulk of the material suggesting importance of electron correlation among the conduction electrons in the bulk while the surface appears to be uncorrelated. These results provide an insight in fabricating devices based on such superconductors.

cond-mat.supr-con↗