arXiv subjects

S. V. Bhat

Publications and source records attributed to S. V. Bhat.

34 records · Page 2Linked to original sources

arXiv2005

Magnetic field dependence of kinetic inductance in Bi2Sr2Ca2Cu3O10 superconducting strip and its feasible applications

The kinetic inductance properties of a thin superconducting sample of BSCCO-2223 compound is studied. A strong dependence of kinetic inductance with the variation of applied magnetic field is found at low temperature in the superconducting state. The kinetic inductance of a thin superconductor increases linearly with increasing magnetic field. This behavior is used for designing a superconducting modulator circuit. This behavior can be useful for device applications and designing of superconducting electronic circuits like superconducting power amplifier, superconducting transmitter and superconducting ac current controller.

cond-mat.supr-con↗

arXiv2005

Anomalous spin dynamics in charge ordered, 'two-electron' doped manganite Ca_0.9Ce_0.1MnO_3 : consequence of a spin-liquid phase?

The 'two-electron' doped rare earth mangnites Ca_1-x Ce_x MnO_3 (x = 0.1,0.2) are probed using resistivity, ac susceptibility and electron paramagnetic resonance (EPR) measurements across their respective charge ordering (CO) temperatures T_CO = 173 K and 250 K. The EPR 'g' factor and intensity as well as the transport and magnetic behaviours of the two compositions are qualitatively similar and are as expected for CO systems. However, the EPR linewidth, reflective of the spin dynamics, for x = 0.1, shows a strongly anomalous temperature dependence, decreasing with decreasing temperature below T_CO in contrast with the sample with x = 0.2 and other CO systems. Keeping in view the evidence for magnetic frustration in the system, we propose that the anomalous temperature dependence of the linewidth is the signature of the occurrence of a disorder driven spin liquid phase, present along with charge ordering.

cond-mat.str-el↗

arXiv2005

Electron magnetic resonance studies of nanomanganite Nd0.67Sr0.33MnO3

Nd_0.67Sr_0.33MnO_3 nanoparticles with the grain size of about 30 nm are prepared by sol-gel method.These nanopowders are annealed at four different temperatures viz. 800 oC, 900 oC, 1000 oC and 1100 oC to study the effect of particle size on magnetic, transport and electron magnetic resonance (EMR) spectral parameters. The samples are characterized by XRD, SEM, EDAX and TEM. The ac susceptibility experiments show that as the particle size increases the ferromagnetic to paramagnetic transition temperature (Tc) decreases. The metal-insulator transition temperature also changes with the particle size as revealed by resistivity measurements. EMR spectra of the nanopowders are recorded from room temperature down to 4K using an X-band EPR spectrometer. the spectra could be fitted using two broad-Gaussian lineshapes below Tc and suggested the ferromagnetic nature of the samples. Above Tc a single Lorenzian fits the signals as expetced for paramagnetic samples. The EMR spectral parameters are found to be different from the bulk (polycrystalline)sample data. The spectral parameters show variation with the particle size. The presence of the two signals in the ferromagnetic phase is attributed to core and shell regions in the nanoparticles. We could estimate the shell thickness from the EMR intensity data as 0.7 - 1 nm which agrees with other measurements.

cond-mat.str-el↗

arXiv2005

Angular dependence of direct rf power absorption studies in Bi2Sr2CaCu2O8 single crystals

We have studied rf power dissipation in Bi2Sr2CaCu2O8 single crystals as a function of angle between the applied field and c-axis of the crystal by using a novel technique of measuring direct rf power absorption. We observed two peaks in power absorption as a function of temperature. The amplitude and position of the first peak (peak A) change with orientation and attributed to Josephson junctions decoupling. The second peak (peak B) appears just below Tc has been attributed to the vortex motion and its amplitude depends on the angle of orientation.

cond-mat.supr-con↗

arXiv2005

Experimental Evidence for Zero DC Resistance of Superconductors

Even after nearly a century of discovery of superconductivity, there has been no direct experimental proof of the expected zero resistance of superconductors. Indeed, it has been believed that it is impossible to experimentally show that the resistance has fallen exactly to zero. In this work we demonstrate that the dc resistivity of a superconducting material below the transition temperature has to be exactly zero.

cond-mat.supr-con↗

arXiv2005

Charge order suppression and antiferromagnetic to ferromagnetic switch over in Pr_0.5Ca_0.5MnO_3 nanowires

We have prepared crystalline nanowires (diameter ~ 50 nm, length ~ a few microns) of the charge ordering manganite Pr_0.5Ca_0.5Mn_O3 using a low reaction temperature hydrothermal method and characterized them using X-ray diffraction, transmission electron microscopy, SQUID magnetometry and electron magnetic resonance measurements. While the bulk sample shows a charge ordering transition at 245 K and an antiferromagnetic transition at 175 K, SQUID magnetometry and electron magnetic resonance experiments reveal that in the nanowires phase, a ferromagnetic transition occurs at ~ 105 K. Further, the antiferromagnetic transition disappears and the charge ordering transition is suppressed. This result is particularly significant since the charge order in Pr_0.5Ca_0.5MnO_3 is known to be very robust, magnetic fields as high as 27 T being needed to melt it.

cond-mat.str-el↗

arXiv2005

Magnetic field dependent direct rf power absorption studies in Bi_2 Sr_2 CaCu_2 O_8 single crystals

Using a novel technique of measuring direct rf power dissipation, the temperature and magnetic field dependence of rf absorption in superconducting single crystals of Bi_2Sr_2CaCu_2O_8 is studied. An unexpected, larger than normal state, dissipation is observed below Tc, which exhibits peaks at magnetic field dependent temperatures. An explanation is provided for this observation in terms of the energy required to decouple the intrinsic Josephson junctions in the crystals.

cond-mat.supr-con↗

arXiv2005

A new method for direct rf power absorption studies in CMR materials and high T_c superconductors

The design, fabrication and performance of an apparatus for the measurement of direct rf power absorption in colossal magnetoresistive (CMR) and superconducting samples are described. The system consists of a self-resonant LC tank circuit of an oscillator driven by a NOT logic gate. The samples under investigation are placed in the core of the coil forming the inductance L and the absorbed power is determined from the measured change in the current supplied to the oscillator circuit. A customized low temperature insert is used to integrate the experiment with a commercial Oxford Instruments cryostat and temperature controller. The oscillator working in the rf range between 1 MHz to 25 MHz is built around an IC 74LS04. The temperature can be varied from 4.2 to 400 K and the magnetic field from 0 to 1.4 T. The apparatus is capable of measuring direct power absorption in CMR and superconducting samples of volume as small as 1/1000 cm^3 with a signal to noise ratio of 10:1. Further increase in the sensitivity can be obtained by summing the results of repeated measurements obtained at a given temperature. The system performance is evaluated by measuring the absorbed power in La_0.7 Sr_0.3 MnO_3 (LSMO) CMR manganite samples and superconducting Y Ba_2 Cu_3 O_7 (YBCO) samples at different rf frequencies. All operations during the measurements are automated using a computer with a menu-driven software system, user input being required only for the initiation of the measurement sequence.

cond-mat.supr-con↗

arXiv2005

Josephson junction decoupling is the main origin of AC resistivity in the superconducting state

The origin of AC resistivity in the high Tc superconductors is not addressed adequately in literature. We found out, Josephson Junction (JJ) decoupling is the main origin of the AC resistivity in high Tc superconductors. We have measured the AC resistivity in the superconductors in the low frequency range by measuring the complex AC impedance of superconducting YBa2Cu3O7 (YBCO) polycrystalline samples. Our data shows that under certain conditions when the number density of Josephson Junctions (JJ) present in the sample and the JJ critical current crosses a threshold value, AC resistivity in the superconducting state keeps on increasing with lowering temperature. The underlying mechanism is an interesting interplay of JJ coupling energy, amplitude of the supply AC voltage and the current applied to the superconducting sample. The effect of the applied AC current of different frequencies and the variation of temperature were studied in detail. To find out the exact relation between the JJ coupling energy, JJ number density, applied AC frequency, the amplitude of AC current and the AC resistivity in the superconductors, we have studied samples of different grain sizes, pressurized with different pressure and sintered at different physical situations. These results have important implications for the understanding of the origin of AC resistivity and characterization of superconducting samples. In this paper we also extend the capability of the AC impedance studies in superconductors for the characterization of materials for device applications.

cond-mat.supr-con↗

arXiv2003

Electron Paramagnetic Resonance Study of Phase Segregation in Nd$_{0.5}$Sr$_{0.5}$MnO$_3$

We present results of an electron paramagnetic resonance (EPR) study of Nd$_{1-x}$Sr$_x$MnO$_3$ with x = 0.5 across the paramagnetic to ferromagnetic, insulator to metal transition at 260 K (T$_c$) and the antiferromagnetic, charge ordering transition (T$_N$ = T$_{co}$) at 150 K. The results are compared with those on Nd$_{0.45}$Sr$_{0.55}$MnO$_3$ which undergoes a transition to a homogeneous A-type antiferromagnetic phase at T$_N$ = 230 K and on La$_{0.77}$Ca$_{0.23}$MnO$_3$ which undergoes a transition to coexisting ferromagnetic metallic and ferromagnetic insulating phases. For x = 0.5, the EPR signals below T$_c$ consist of two Lorentzian components attributable to the coexistence of two phases. From the analysis of the temperature dependence of the resonant fields and intensities, we conclude that in the mixed phase ferromagnetic and A-type antiferromagnetic (AFM) phases coexist. The x = 0.55 compound shows a single Lorentzian throughout the temperature range. The signal persists for a few degrees below T_N. The behaviour of the A-type AFM phase is contrasted with that of the two ferromagnetic phases present in La$_{0.77}$Ca$_{0.23}$MnO$_3$. The comparison of behaviour of A-type AFM signal observed in both Nd$_{0.5}$Sr$_{0.5}$MnO$_3$and Nd$_{0.45}$Sr$_{0.55}$MnO$_3with the two FM phases of La$_{0.77}$Ca$_{0.23}$MnO$_3$, vis-a-vis the shift of resonances with respect to the paramagnetic phases and the behaviour of EPR intensity as a function of temperature conclusively prove that the Nd$_{0.5}$Sr$_{0.5}$MnO$_3$undergoes phase separation into A-type AFM and FM phases.

cond-mat.str-el↗

arXiv2003

Magnetic study of an amorphous conducting polyaniline

We show that newly found BF3-doped polyaniline, though highly conducting, remains amorphous. Magnetic studies reveal many unusual properties, while suggesting that the intrinsic conductivity of this system is significantly larger than all other known forms of conducting polyaniline, establishing it as an interesting class of highly conducting amorphous polymer.

cond-mat.mtrl-sci↗

arXiv2002

An Electron Paramagnetic Resonance Study of Electron-Hole Asymmetry in Charge Ordered Pr_1-x Ca_xMnO_3 (x=0.64, 0.36)

We present and compare the results of temperature-dependent electron paramagnetic resonance (EPR) studies on Pr_1-x Ca_xMnO_3 for x = 0.64 which is electron-doped with those on the hole doped x = 0.36 composition. The temperature dependence of the various parameters obtained from the powder and single crystal spectra show significant differences between the two manganites. At room temperature the `g' parameter for the electron doped system is less than the free electron `g' value `g_e', whereas for the hole-doped system it is more than `g_e'. Further, the `g' value and the linewidth obtained from the powder spectra as well as the single crystal spectra show different functional dependences on temperature in the two systems. Quite strikingly, the peak observed at T_{co} in the temperature dependence of the asymmetry parameter, alpha, of the single crystal spectra in the hole-doped system is absent in the electron-doped system. We understand this contrasting behaviour of the EPR parameters in the two systems in terms of very different nature of microscopic interactions in them.

cond-mat.str-el↗

arXiv2002

Electron paramagnetic resonance studies of the insulating ferromagnetic manganite Nd_0.8Pb_0.2MnO_3 above the transition temperature

Single crystals of Nd_{1-x}Pb_{x}MnO_{3} with x=0.2 are grown by high temperature solution growth technique using PbO-PbF_{2} flux. Magnetization studies on the samples show a transition to a ferromagnetic state below T_c ~ 125 K and the resistivity measurements show it to be an insulator throughout the temperature range 50 - 300 K. Electron Paramagnetic Resonance studies have been performed for T > T_{C} with a view to comparing the results with those on metallic ferromagnetic manganites. The temperature dependence of various parameters like g-value, linewidth and intensity has been studied in the temperature range 150 - 300 K. It is found that they behave in a manner similar to that exhibited by metallic ferromagnetic manganites.

cond-mat.str-el↗

arXiv2001

Temperature-dependent electron paramagnetic resonance studies of charge ordered Nd_0.5Ca_0.5MnO_3

We report Electron Paramagnetic Resonance measurements on single crystalline and powder samples of Nd_0.5Ca_0.5MnO_3 across the charge-ordering transition at T_co=240 K down to the antiferromagnetic ordering transition at T_N = 140 K. The changes in the linewidth, g-factor and intensity as functions of temperature are studied to understand the nature of spin-dynamics in the system. We explain the observed large decrease in the linewidth from T_N to T_co in terms of motional narrowing caused by the hopping of the Jahn-Teller polarons yielding an activation energy of E_a = 0.13 eV. Similar analysis of data on Pr_0.6Ca_0.4MnO_3 published earlier gives E_a=0.2 eV. Below T_co, the g-value increases continuously suggesting a gradual strengthening of the orbital ordering. We give a qualitative explanation of the temperature dependence and of the maximum in the asymmetry ratio A/B observed at T_co in single crystal spectra which also supports the themodel of motional narrowing.

cond-mat.str-el↗

arXiv2001

Non-resonant microwave absorption studies of superconducting MgB_2

Non-resonant microwave absorption(NRMA) studies of superconducting MgB_2 at a frequency of 9.43 GHz in the field range -50 Gauss to 5000 Gauss are reported. The NRMA results indicate near absence of intergranular weak links. A linear temperature dependence of the lower critical field H_c1 is observed indicating a non s-wave superconductivity. However, the phase reversal of the NRMA signal which could suggest d-wave symmetry is also not observed.

cond-mat.supr-con↗

arXiv2000

An electron paramagnetic resonance study of Pr_{0.6}Ca_{0.4}MnO_{3} across the charge ordering transition

We report the first electron paramagnetic resonance studies of single crystals and powders of Pr_{0.6}Ca_{0.4}MnO_{3} in the 300-4.2 K range, covering the charge ordering transition at ~ 240 K and antiferromagnetic transition (T_N) at ~ 170 K. The asymmetry parameter for the Dysonian single crystal spectra shows anomalous increase at T_{co}. Below T_{co} the g-value increases continuously, suggesting a gradual strengthening of orbital ordering. The linewidth undergoes a sudden increase at T_{co} and continues to increase down to T_N. The intensity increases as the temperature is decreased till T_{co} due to the renormalization of magnetic susceptibility arising from the build up of ferromagnetic correlations. The value of the exchange constant, J, is estimated to be 154 K.

cond-mat.str-el↗