arXiv subjects

S. V. Nekrasov

Publications and source records attributed to S. V. Nekrasov.

7 recordsLinked to original sources

arXiv2026

Cascade spin dynamics of excitons localized in indirect-band-gap (In,Al)As/AlAs quantum dots with type-I band alignment

We investigate the spin dynamics of excitons localized in type I (In,Al)As/AlAs quantum dots with an indirect in momentum space band structure. Polarized selective photoluminescence spectroscopy, i.e. fluorescence line narrowing, under magnetic fields up to 5 T applied in the Faraday geometry is employed. The experiment reveals a cascade spin evolution process of excitons in the indirect band-gap quantum dots: an initial short term spin dynamics associated with excited direct exciton states possessing a large oscillator strength is followed by electron relaxation into the X valley of the Brillouin zone and subsequent long term spin dynamics of indirect excitons. The two step mechanism manifests itself in the distinct features of the magnetic field dependences of photoluminescence: two component recovery of optical orientation, two component linear to circular polarization conversion and the presence of the linear polarization plane rotation. At the same time, suppression of the optical alignment shows one-component behavior governed by the spin dynamics of the indirect exciton states. Within the pseudospin formalism, we derive analytical expressions that quantitatively describe the observed dependences and yield estimates for the anisotropic exchange splitting: 210 μeV for direct excitons and 1.3 μeV for indirect excitons. Further analysis using the density matrix formalism agrees well with the pseudospin model calculations and shows that the finite optical orientation at zero magnetic field is due to comparable magnitudes of the anisotropic splitting of the indirect exciton states and the splitting of the X-valley electron states caused by the hyperfine interaction with nuclei.

cond-mat.mes-hall↗

arXiv2023

Influence of Gamma-X mixing on optical orientation and alignment of excitons in (In,Al)As/AlAs quantum dots

The effect of Gamma-X mixing on the energy levels fine structure of indirect in k-space excitons in an ensemble of (In,Al)As/AlAs quantum dots with type I band alignment was experimentally studied. Using the methods of optical spin orientation and optical alignment in a magnetic field, an increase in the anisotropic exchange splitting of excitonic levels (from approximately 0.6 to 5 ueV) due to the Gamma-X mixing was revealed. The extent of direct electronic states admixing to indirect ones depends on the size of the quantum dot. On the other hand, the optical and spin properties of excitons change radically with increasing of the Gamma states admixture to the X states: in the absence of a magnetic field, the optical orientation of excitons decreases from 18 to 3%, while the alignment of excitons is restored from 6 to 53%.

cond-mat.mes-hall↗

arXiv2023

Electrical resistance associated with the scattering of optically oriented electrons in n-GaAs

In a bulk GaAs crystal, an unusual magnetoresistance effect, which takes place when a spin-polarized current flows through the sample, was detected. Under conditions of optical pumping of electron spins, an external magnetic field directed along the electric current and perpendicular to the oriented spins decreases the resistance of the material. The phenomenon is due to the spin-dependent scattering of electrons by neutral donors. It was found that the sign of the magnetoresistance does not depend on the sign of the exciting light circular polarization, the effect is even with respect to the sign of the spin polarization of the carriers, which indicates a correlation between the spins of optically oriented free electrons and electrons localized on donors.

cond-mat.mes-hall↗

arXiv2023

Optical orientation of excitons in a longitudinal magnetic field in indirect band gap (In,Al)As/AlAs quantum dots with type-I band alignment

The exciton recombination and spin dynamics in (In,Al)As/AlAs quantum dots (QDs) with indirect band gap and type-I band alignment are studied. The negligible (less than $0.2~μ$eV) value of the anisotropic exchange interaction in these QDs prevents a mixing of the excitonic basis states with pure spin and allows for the formation of spin polarized bright excitons for quasi-resonant circularly polarized excitation. In a longitudinal magnetic field, the recombination and spin dynamics of the excitons are controlled by the hyperfine interaction between the electron and nuclear spins. A QD blockade by dark excitons is observed in magnetic field eliminating the impact of the nuclear spin fluctuations. A kinetic equation model, which accounts for the population dynamics of the bright and dark exciton states as well as for the spin dynamics, has been developed, which allows for a quantitative description of the experimental data.

cond-mat.mes-hall↗

arXiv2022

Optical alignment and orientation of excitons in ensemble of core/shell CdSe/CdS colloidal nanoplatelets

We report on the experimental and theoretical studies of optical alignment and optical orientation effects in an ensemble of core/shell CdSe/CdS colloidal nanoplatelets. The dependences of three Stokes parameters on the magnetic field applied in the Faraday geometry are measured under continuous wave resonant excitation of the exciton photoluminescence. Theoretical model is developed to take into account both bright and dark exciton states in the case of strong electron and hole exchange interaction and random in-plane orientation of the nanoplatelets in ensemble. The data analysis allows us to estimate the time and energy parameters of the bright and dark excitons. The optical alignment effect enables identification of the exciton and trion contributions to the photoluminescence spectrum even in the absence of a clear spectral line resolution.

cond-mat.mes-hall↗

arXiv2019

Spin beats in the photoluminescence polarization dynamics of charged excitons in InP/(In,Ga)P quantum dots in presence of nuclear quadrupole interaction

The spin dynamics of positively (X$^{+}$) and negatively (X$^{-}$) charged excitons in InP/In$_{0.48}$Ga$_{0.52}$P quantum dots subject to a magnetic field is studied. We find that a characteristic feature of the system under study is the presence of nuclear quadrupole interaction, which leads to stabilization of the nuclear and electron spins in a quantum dot in zero external magnetic field. In detail, the nuclear quadrupole interaction leads to pinning of the Overhauser field along the quadrupole axis, which is close to the growth axis of the heterostructure. The nuclear effects are observed only when resident electrons are confined in the quantum dots, i.e. for X$^{-}$ trion photoexcitation. The presence of X$^{-}$ and X$^{+}$ trion contributions to the photoluminescence together with the quadrupole interaction significantly affects the dynamics of optical orientation in Voigt magnetic field. In absence of dynamic nuclear spin polarization the time evolution of the photoluminescence polarization was fitted by a form which describes the electron spin relaxation in "frozen" nuclear field fluctuations. In relatively large external magnetic fields exceeding 60 mT good agreement between theory and experiment is achieved.

cond-mat.mes-hall↗

arXiv2019

Optical orientation and alignment of excitons in direct and indirect band gap (In,Al)As/AlAs quantum dots with type-I band alignment

The spin structure and spin dynamics of excitons in an ensemble of (In,Al)As/AlAs quantum dots (QDs) with type-I band alignment, containing both direct and indirect band gap dots, are studied. Time-resolved and spectral selective techniques are used to distinguish between the direct and indirect QDs. The exciton fine structure is studied by means of optical alignment and optical orientation techniques in magnetic fields applied in the Faraday or Voigt geometries. A drastic difference in emission polarization is found for the excitons in the direct QDs involving a $Γ$-valley electron and the excitons in the indirect QDs contributed by an $X$-valley electron. We show that in the direct QDs the exciton spin dynamics is controlled by the anisotropic exchange splitting, while in the indirect QDs it is determined by the hyperfine interaction with nuclear field fluctuations. The anisotropic exchange splitting is determined for the direct QD excitons and compared with model calculations.

cond-mat.mes-hall↗