Intensity nonlinearity of the error-signal frequency shift in the modulation spectroscopy of dark resonances and approaches to its reduction
We have found that the error-signal frequency corresponding to the coherent population trapping resonance can be displaced from that of "$0-0$" transition unperturbed by the optical field, although the frequency is not sensitive to changes in its intensity. We consider the double $Λ$-system of levels interacting with the asymmetric polychromatic optical field to demonstrate that this effect arises due to intensity nonlinearity of the error-signal frequency shift. The experiment with $^{87}$Rb atoms in Ar-N$_2$ buffer gas atomic cell shows how the displacement value depends on different parameters. The possible influence of the effect on the clocks' frequency stability and reproducibility are discussed.
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