arXiv subjects

S. Vasiliev

Publications and source records attributed to S. Vasiliev.

At least 19 recordsLinked to original sources

arXiv2025

Zero-energy resonances in ultracold hydrogen sticking to liquid helium films of finite thickness

We investigated quantum states of ultracold hydrogen atoms in a combined potential comprising the H-He film interaction in the presence of a substrate and the Earth gravitational field. We show that the shift and width of the gravitational quantum states are determined by the complex scattering length for the H-He film-substrate potential. We demonstrate that for specific helium film thicknesses above a substrate, zero-energy resonances occur if the combined potential supports a bound state exactly at the threshold. This effect leads to a complete restructuring of the bound states spectrum. The dynamics of gravitational levels as a function of the van der Waals interaction depth controlled by the helium film thickness is analyzed. It reveals the critical thicknesses at about 6.1 and 1.8 nm, at which resonances appear in the case of the conductive substrate. With imaginary integral operators, we incorporate non-perturbatively the inelastic effects originating from the ripplon coupling. The inelastic effects show dramatic changes in the sticking-coefficient behavior near the critical points. The enhanced sticking coefficients provide a probe for studying critical phenomena and measuring atom-surface interaction parameters with unprecedented sensitivity.

cond-mat.quant-gas↗

arXiv2025

Cold source of atomic hydrogen for loading large magnetic traps

We present a design and performance tests of an intense source of cold hydrogen atoms for loading large magnetic traps. Our source is based on a cryogenic dissociator of molecular hydrogen at 0.6 K followed by a series of thermal accommodators at 0.5, 0.2 and 0.13 K with inner surfaces covered by a superfluid helium film. All components are thermally anchored to corresponding stages of a dilution refrigerator. The source provides a continuous flux of 7$\cdot$$10^{13}$ H atoms/s in a temperature range of 130-200 mK. We have successfully used the source for loading a large Ioffe-Pritchard magnetic trap recently built in our laboratory [arXiv:2108.09123 or Rev. Sci. Instr. 93 (2), 023201 (2022)]. Calorimetric measurements of the atomic recombination heat allow reliable determination of the atomic flux and H gas density in the trap. We have tested the performance of the source and loading of H atoms into the trap at various configurations of the trapping field, reducing the magnetic barrier height to 75% and 50% of the nominal value of 0.8 T (0.54 K) as well as at the open configuration of the trap at its lower end, when the atoms are in contact with the trapping cell walls covered by a superfluid helium film. In the latter case, raising the trapping cell temperature to 200-250 mK, the low-field seeking atoms at densities exceeding 10$^{11}$ cm$^{-3}$ can be stored for the time over 1000 s, sufficiently long for experiments on precision spectroscopy of cold H gas.

physics.atom-ph↗

arXiv2021

A large octupole magnetic trap for research with atomic hydrogen

We describe the design and performance of a large magnetic trap for storing and cooling of atomic hydrogen (H). The trap operates in the vacuum space of a dilution refrigerator at a temperature of 1.5 K. Aiming at a large volume of the trap we implemented the octupole configuration of linear currents (Ioffe bars) for the radial confinement, combined with two axial pinch coils and a 3 T solenoid for the cryogenic H dissociator. The octupole magnet consists of eight race-track segments which are compressed towards each other with magnetic forces. This provides a mechanically stable and robust construction with a possibility of replacement or repair of each segment. A maximum trap depth of 0.54 K (0.8 T) was reached, corresponding to an effective volume of 0.5 liters for hydrogen gas at 50 mK. This is an order of magnitude larger than ever used for trapping atoms.

physics.atom-ph↗

arXiv2019

Dynamic nuclear polarization and ESR hole burning in As doped silicon

We present an experimental study of the Dynamic Nuclear Polarization (DNP) of \si{} nuclei in silicon crystals of natural abundance doped with As in the temperature range 0.1-1 K and in strong magnetic field of 4.6 T. This ensures very high degree of electron spin polarization, extremely slow nuclear relaxation and optimal conditions for realization of Overhauser and resolved solid effects. We found that the solid effect DNP leads to an appearance of a pattern of holes and peaks in the ESR line, separated by the super-hyperfine interaction between the donor electron and \si{} nuclei closest to the donor. On the contrary, the Overhauser effect DNP mainly affects the remote \si{} nuclei having the weakest interaction with the donor electron. This leads to an appearance of a very narrow ($\approx$ 3 mG wide) hole in the ESR line. We studied relaxation of the holes after burning, which is caused by the nuclear spin diffusion. Analyzing the spin diffusion data with a simple one-dimensional spectral diffusion model leads to a value of the spectral diffusion coefficient $D=8(3)\times 10^{-3}$ mG$^2$/s. Our data indicate that the spin diffusion is not completely prevented even in the frozen core near the donors. The emergence of the narrow hole after the Overhauser DNP may be explained by a partial "softening" of the frozen core caused by Rabi oscillations of the electron spin.

cond-mat.mes-hall↗

arXiv2018

Spin Waves in Quantum Gases --- The Quality Factor of the Identical Spin Rotation Effect

Our recent experimental work on electron spin waves in atomic hydrogen gas has prompted a revisit of the theory of the Identical Spin Rotation Effect (ISRE). A key characteristic determining the properties of the spin waves is the quality factor of ISRE. Unfortunately, calculating this quality factor takes some toil. In this paper we summarize some results of the ISRE theory in dilute gases. We also derive asymptotic formulae for the quality factor and examine their accuracy for hydrogen and $^3$He.

cond-mat.quant-gas↗

arXiv2018

Identical Spin Rotation Effect and Electron Spin Waves in Quantum Gas of Atomic Hydrogen

We present an experimental study of electron spin waves in atomic hydrogen gas compressed to high densities of $\sim 5 \times 10^{18}$ cm$^{-3}$ at temperatures ranging from 0.26 to 0.6 K in strong magnetic field of 4.6 T. Hydrogen gas is in a quantum regime when the thermal de Broglie wavelength is much larger than the s-wave scattering length. In this regime the identical particle effects play major role in atomic collisions and lead to the Identical Spin Rotation effect (ISR). We observed a variety of spin wave modes caused by this effect with strong dependence on the magnetic potential caused by variations of the polarizing magnetic field. We demonstrate confinement of the ISR modes in the magnetic potential and manipulate their properties by changing the spatial profile of magnetic field. We have found that at a high enough density of H gas the magnons accumulate in their ground state in the magnetic trap and exhibit long coherence, which has a profound effect on the electron spin resonance spectra. Such macroscopic accumulation of the ground state occurs at a certain critical density of hydrogen gas, where the chemical potential of the magnons becomes equal to the energy of their ground state in the trapping potential.

cond-mat.quant-gas↗

arXiv2017

Quantum reflection of antihydrogen from a liquid helium film

We study the quantum reflection of ultracold antihydrogen atoms bouncing on the surface of a liquid helium film. The Casimir-Polder potential and quantum reflection are calculated for different thicknesses of the film supported by different substrates. Antihydrogen can be protected from anni- hilation for as long as 1.3s on a bulk of liquid 4He, and 1.7s for liquid 3He. These large lifetimes open interesting perspectives for spectroscopic measurements of the free fall acceleration of antihydrogen. Variation of the scattering length with the thickness of a film of helium shows interferences which we interpret through a Liouville transformation of the quantum reflection problem.

physics.atom-ph↗

arXiv2016

Dynamic Polarization and Relaxation of 75As Nuclei in Silicon at High Magnetic Field and Low Temperature

We present the results of experiments on dynamic nuclear polarization and relaxation of 75As in silicon crystals. Experiments are performed in strong magnetic fields of 4.6 T and temperatures below 1 K. At these conditions donor electron spins are fully polarized, and the allowed and forbidden ESR transitions are well resolved. We demonstrate effective nuclear polarization of 75As nuclei via the Overhauser effect on the time scale of several hundred seconds. Excitation of the forbidden transitions leads to a polarization through the solid effect. The relaxation rate of donor nuclei has strong temperature dependence characteristic of Orbach process.

cond-mat.mtrl-sci↗

arXiv2016

Dynamic nuclear polarization and relaxation of H and D atoms in solid mixtures of hydrogen isotopes

We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times ($T_{1e}$ and $T_{1N}$) were measured within the temperature range 0.15-2.5$\,$K in a magnetic field of 4.6 T, conditions which ensure a high polarization of electron spins. We found that $T_{1e}$ is nearly temperature independent in this temperature range, while $T_{1N}$ decreased by 2 orders of magnitude. Such strong temperature dependence is typical for the nuclear Orbach mechanism of relaxation via the electron spins. We found that the nuclear spins of H atoms in solid D$_{2}$ and D$_{2}:$HD can be efficiently polarized by the Overhauser effect. Pumping the forbidden transitions of H atoms also leads to DNP, with the efficiency strongly dependent on the concentration of D atoms. This behaviour indicates the Cross effect mechanism of the DNP and nuclear relaxation, which turns out to be well resolved in the conditions of our experiments. Efficient DNP of H atoms was also observed when pumping the middle D line located in center of the ESR spectrum. This phenomenon can be explained in terms of clusters or pairs of H atoms with strong exchange interaction. These clusters have partially allowed transitions in the center of the ESR spectrum and DNP may be created via the resolved Cross effect.

physics.atm-clus↗

arXiv2016

ESR study of atomic hydrogen and tritium in solid T$_{2}$ and T$_{2}$:H$_{2}$ matrices below 1K

We report on the first ESR study of atomic hydrogen and tritium stabilized in a solid T$_{2}$ and T$_{2}$:H$_{2}$ matrices down to 70$\,$mK. The concentrations of T atoms in pure T$_{2}$ approached $2\times10^{20}$cm$^{-3}$ and record-high concentrations of H atoms $\sim1\times10^{20}$cm$^{-3}$ were reached in T$_{2}$:H$_{2}$ solid mixtures where a fraction of T atoms became converted into H due to the isotopic exchange reaction T+H$_2\rightarrow$TH+H. The maximum concentrations of unpaired T and H atoms was limited by their recombination which becomes enforced by efficient atomic diffusion due to a presence of a large number of vacancies and phonons generated in the matrices by $β$-particles. Recombination also appeared in an explosive manner both being stimulated and spontaneously in thick films where sample cooling was insufficient. We suggest that the main mechanism for H and T migration is physical diffusion related to tunneling or hopping to vacant sites in contrast to isotopic chemical reactions which govern diffusion of H and D atoms created in H$_{2}$ and D$_{2}$ matrices by other methods.

cond-mat.other↗

arXiv2016

Tunneling chemical exchange reaction $\textrm{D}+\textrm{HD}\rightarrow\textrm{D}_{2}+\textrm{H}$ in solid HD and D$_2$ at temperatures below 1$\,$K

We report on a study of the exchange tunneling reaction D+HD$\rightarrow$D$_{2}$+H in a pure solid HD matrix and in a D$_{2}$ matrix with 0.23$\%$ HD admixture at temperatures between 130$\,$mK and 1.5$\,$K. We found that the exchange reaction rates, $k_{exHD}\sim3\times10^{-27}$cm$^{3}$s$^{-1}$ in the pure HD matrix, and $k_{exD_{2}}=9(4)\times10^{-28}$cm$^{-3}$ in the D$_{2}$ matrix are nearly independent of temperature within this range. This confirms quantum tunnelling nature of these reactions, and their ability to proceed at temperatures down to absolute zero. Based on these observations we concluded that exchange tunneling reaction H+H$_{2}\rightarrow$H$_{2}$+H should also proceed in a H$_{2}$ matrix at the lowest temperatures. On contrary, the recombination of H atoms in solid H$_{2}$ and D atoms in solid D$_{2}$ is substantially suppressed at the lowest temperatures as a result of increasing of violation for resonance tunneling of atoms when they approach each other.

physics.chem-ph↗

arXiv2015

Bose-Einstein condensation of magnons in atomic hydrogen gas

We report on experimental observation of BEC-like behaviour of quantized electron spin waves (magnons) in a dense gas of spin polarized atomic hydrogen. The magnons are trapped and controlled with inhomogeneous magnetic fields, and described by a Schrödinger-like wave equation, in analogy to the BEC experiments with neutral atoms. We have observed the appearance of a sharp feature in the ESR spectrum displaced from the normal spin wave spectrum. We believe that this observation corresponds to a sudden growth of the ground state population of the magnons and emergence of their spontaneous coherence for hydrogen gas densities exceeding a critical value, dependent on the trapping potential. We interpret the results as a BEC of non-equilibrium magnons which were formed by applying the rf power.

cond-mat.quant-gas↗

arXiv2015

Microscopic control of $^{29}$Si nuclear spins near phosphorus donors in silicon

We demonstrate an efficient control of $^{29}$Si nuclear spin orientation for specific lattice sites near $^{31}$P donors in silicon crystals at temperatures below 1 K and in high magnetic field of 4.6 T. Excitation of the forbidden electron-nuclear transitions leads to a pattern of narrow holes and peaks in the ESR lines of $^{31}$P. The pattern originates from dynamic polarization the $^{29}$Si nuclear spins near the donors via the solid effect. This method can be used for initialization of qubits based on $^{29}$Si nuclear spins in the all-silicon quantum computer. In comparison, polarization of $^{29}$Si performed by pumping the allowed ESR transitions, did not create any patterns. Instead, a single narrow spectral hole was burnt in the ESR line. The difference is explained by a rapid spin diffusion during the microwave pumping of the allowed transitions.

physics.atm-clus↗

arXiv2014

Efficient Dynamic Polarization of Phosphorus Nuclei in Silicon in Strong Magnetic Fields and Low Temperatures

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross relaxation via the forbidden flip-flop or flip-flip transitions. Nuclear polarization values $P>0.98$ were reached after 20 min of pumping with 0.4 $μ$W of microwave power. We evaluated that the ratio of hyperfine state populations increased by three orders of magnitude after 2 hours of pumping, and an extremely pure nuclear spin system containing $<10^{-11}$ of the other spin state can be created. An inverted DNP has been obtained by pumping the low field ESR line of P followed by the flip-flip cross relaxation. This transition has much smaller relaxation rate and required substantially longer pumping times. We found that the nuclear polarization dynamics deviates substantially from a simple exponential function. The evolution of the polarization is characterized by two time constants $T^{'}_{ac}\approx$15 s in the beginning, and $T^{"}_{ac}\approx$1100 s for long pumping time. Temperature dependence of the nuclear relaxation rate of $^{31}$P was studied down to 0.75 K, below which the relaxation time became too long to be measured. The nuclear polarization followed a bi-exponential time dependence during relaxation. We suggest that the non-exponential behavior of DNP dynamics and the subsequent relaxation is mediated by the nuclei of $^{29}$Si surrounding $^{31}$P donors, which affect the transition probabilities of the forbidden cross-relaxation processes.

cond-mat.mes-hall↗

arXiv2012

Guiding and Trapping Electron Spin Waves in Atomic Hydrogen Gas

We present a high magnetic field study of electron spin waves in atomic hydrogen gas compressed to high densities of 10^18 cm^-3 at temperatures ranging from 0.26 to 0.6 K. We observed a variety of spin wave modes caused by the identical spin rotation effect with strong dependence on the spatial profile of the polarizing magnetic field. We demonstrate confinement of these modes in regions of strong magnetic field and manipulate their spatial distribution by changing the position of the field maximum.

cond-mat.quant-gas↗

arXiv2009

Three terminal capacitance technique for magnetostriction and thermal expansion measurements

An instrument has been constructed to measure a large range of magnetostriction and thermal expansion between room temperature and 4 K in a superconductive split-coil magnet, that allows investigation in magnetic fields up to 12 T. The very small bulk samples (up to 1 mm in size) as well as big ones (up to 13 mm) of the irregular form can be measured. The possibility of magnetostriction investigation in thin films is shown. A general account is given of both electrical and the mechanical aspects of the design of capacitance cell and their associated electronic circuitry. A simple lever device is proposed to increase the sensitivity twice. The resulting obtained sensitivity can be 0.5 Angstrom. The performance of the technique is illustrated by some preliminary measurements of the magnetostriction of superconducting MgB2, thermal expansion of (La0.8Ba0.2)0.93MnO3 single crystal and magnetoelastic behavior of the Ni/Si(111) and La0.7Sr0.3CoO3/SAT0.7CAT0.1LA0.2(001) cantilevers.

cond-mat.mtrl-sci↗

arXiv2008

Operation of a GERDA Phase I prototype detector in liquid argon and nitrogen

The GERDA (GERmanium Detector Array) experiment aiming to search for the neutrinoless double beta decay of 76Ge at the Laboratori Nazionali Del Gran Sasso (LNGS), Italy, will operate bare enriched high-purity germanium (HPGe) detectors in liquid argon. GERDA Phase I will use the enriched diodes from the previous Heidelberg-Moscow (HdM) and IGEX experiments. With the HPGe detectors mounted in a low-mass holder, GERDA aims at an excellent energy resolution and extremely low background. The goal is to check the claim for the neutrinoless double beta decay evidence in the HdM 76Ge experiment within one year of data taking. Before dismounting the enriched diodes from their cryostat, the performance parameters of the HdM and the IGEX detectors have been measured. The diodes have been removed from their cryostats, their dimensions measured and they have been put under va-cuum in a transportation container. They are now being refurbished for GERDA Phase I at Canberra Semiconductor NV. Before operating the enriched diodes, a non-enriched HPGe p-type detector mounted in a low-mass holder is operated in the liquid argon test facility of the GERDA Detector Laboratory (GDL) at LNGS. Since January 2006, the testing of the prototype detector is being carried out in the GDL as well as at the site of the detector manufacturer.

nucl-ex↗

arXiv2008

Highly sensitive gamma-spectrometers of GERDA for material screening: Part I

The GERDA experiment aims to search for the neutrinoless double beta-decay of 76Ge and possibly for other rare processes. The sensitivity of the first phase is envisioned to be more than one order of magnitude better than in previous neutrinoless double beta-decay experiments. This implies that materials with ultra-low radioactive contamination need to be used for the construction of the detector and its shielding. Therefore the requirements on material screening include high-sensitivity low-background detection techniques and long measurement times. In this article, an overview of material-screening laboratories available to the GERDA collaboration is given, with emphasis on the gamma-spectrometry. Additionally, results of an intercomparison of the evaluation accuracy in these laboratories are presented.

physics.ins-det↗