arXiv subjects

S. Wakimoto

Publications and source records attributed to S. Wakimoto.

65 records · Page 4Linked to original sources

arXiv2001

Neutron Diffuse Scattering from Polar Nanoregions in the Relaxor Pb(Mg1/3Nb2/3)O3

We have studied the neutron diffuse scattering in the relaxor PMN. The diffuse scattering appears around the Burns temperature (~620K), indicating its origin from the polar nanoregions (PNR). While the relative diffuse intensities are consistent with previous reports, they are entirely different from those of the lowest-energy TO phonon. Because of that, it has been considered that this TO mode could not be the ferroelectric soft mode. Recently, a neutron scattering study has unambiguously shown that the TO mode does soften on cooling. If the diffuse scattering in PMN originates from the soft mode condensation, then the atomic displacements must satisfy the center of mass condition. But, the atomic displacements determined from diffuse scattering intensities do not fulfill this condition. To resolve this contradiction, we propose a simple model in which the total atomic displacement consists of two components: $δ_{CM}$ is created by the soft mode condensation, satisfying the center of mass condition, and, $δ_{shift}$ represents a uniform displacement of the PNR along their polar direction relative to the surrounding (unpolarized) cubic matrix. Within this framework, we can successfully describe the neutron diffuse scattering intensities observed in PMN.

cond-mat.mtrl-sci↗

arXiv2001

Soft Mode Dynamics Above and Below the Burns Temperature in the Relaxor Pb(Mg_1/3Nb_2/3)O_3

We report neutron inelastic scattering measurements of the lowest-energy transverse optic (TO) phonon branch in the relaxor Pb(Mg_1/3Nb_2/3)O_3 from 400 to 1100 K. Far above the Burns temperature T_d ~ 620 K we observe well-defined propagating TO modes at all wave vectors q, and a zone center TO mode that softens in a manner consistent with that of a ferroelectric soft mode. Below T_d the zone center TO mode is overdamped. This damping extends up to, but not above, the waterfall wave vector q_wf, which is a measure of the average size of the PNR.

cond-mat.mtrl-sci↗

arXiv2001

Diagonal static spin correlation in the low temperature orthorhombic Pccn phase of La1.55Nd0.4Sr0.05CuO4

Elastic neutron scattering measurements have been performed on Nd, Sr co-doped La1.55Nd0.4Sr0.05CuO4, which exhibits a structural phase transition at Ts ~ 60K from the low temperature orthorhombic Bmab phase (labelled LTO1) to the low temperature orthorhombic Pccn phase (labelled LTO2). At low temperatures, well below Ts, elastic magnetic peaks are observed at the ``diagonal'' incommensurate (IC) positions (0, 1+/-0.055, 0), with modulation direction only along the orthorhombic b-axis just as in Nd-free La1.95Sr0.05CuO4. In the present study, the one-dimensionality of the IC modulation, which is naturally explained by a stripe model, is clearly demonstrated with our "single-domain" crystal. The temperature dependence of the IC peak intensity suggests a substantial contribution from the Nd3+ spins below ~3K. Consistent with this, the L dependence of the magnetic scattering is accurately accounted for by a model in which the contribution of the Nd3+ spins is explicitly included.

cond-mat.supr-con↗

arXiv2001

Hole concentration dependence of the magnetic moment in superconducting and insulating La2-xSrxCuO4

Recent neutron scattering measurements on the La2-xSrxCuO4 system have revealed a drastic change of the incommensurate static spin correlations from diagonal in the insulating region to parallel in the superconducting region. We report the doping dependence of the ordered magnetic moment for the hole concentration region 0.03 <= x <= 0.12, focusing on the relationship between the static magnetism and the superconductivity. The elastic magnetic crosssection decreases monotonically with increasing x for 0.03 <= x <= 0.07. We find that the ordered magnetic moment μvaries from ~0.18 (x=0.03) to \~0.06 μ_B/Cu (x=0.07). No significant anomaly is observed at the insulator-superconductor boundary (x ~ 0.055). The elastic magnetic crosssection is enhanced in the vicinity of x=0.12 whose resolution limited width peaks are observed in neutron scattering measurements and where the apparent magntic and superconducting transitions coincide.

cond-mat.supr-con↗

arXiv2000

Static and dynamic spin correlations in the spin-glass phase of slightly-doped La_{2-x}Sr_xCuO_4

Neutron scattering experiments reveal that a diagonal spin modulation, which is a one-dimensional modulation rotated away by 45$^\circ$ from that in the superconducting phase, occurs universally across the insulating spin-glass phase in La$_{2-x}$Sr$_x$CuO$_4$ (0.02$\le x\le$0.055). This establishes an intimate relation between the magnetism and the transport properties in the high-temperature copper oxide superconductors. Furthermore, it is found that the charge density per unit length estimated using a charge stripe model is almost constant throughout the phase diagram, even when the modulation rotates away by 45$^\circ$ at the superconducting boundary. However, at the lowest values for $x$ the density changes approaching 1 hole/Cu as in La$_{2-x}$Sr$_x$NiO$_4$. Magnetic excitation spectra suggest that magnetic correlations change from incommensurate to commensurate at $ω\sim$7 meV and $T\sim$70 K, indicating a characteristic energy for the incommensurate structure of 6-7 meV.

cond-mat.supr-con↗

arXiv2000

Systematic Study of Short Range Antiferromagnetic Order and The Spin-Glass State in Lightly Doped La2-xSrxCuO4

Systematic measurements of the magnetic susceptibility were performed on single crystals of lightly doped La2-xSrxCuO4 (x=0.03, 0.04 and 0.05). For all samples the temperature dependence of the in-plane magnetic susceptibility shows typical spin-glass features with spin-glass transition temperatures Tg of 6.3K, 5.5K and 5.0K for x=0.03, 0.04 and 0.05, respectively. The canonical spin-glass order parameter extracted from the in-plane susceptibility of all the samples follows a universal scaling curve. On the other hand, the out-of-plane magnetic susceptibility deviates from Curie law below a temperature Tdv, higher than Tg. Comparing with previous neutron scattering results with an instrumental energy resolution of 0.25 meV from Wakimoto et al., the x-dependence of Tdv is qualitatively the same as that of Tel, the temperature below which the elastic magnetic scattering develops around (pi, pi). Thus, a revised magnetic phase diagram in the lightly doped region of La2-xSrxCuO4 is proposed. The Curie constants calculated from the in-plane susceptibility are independent of the Sr concentration. On the basis of the cluster spin-glass model, this fact might reflect an inhomogeneous distribution of doped holes in the CuO2 plane, such as in a stripe structure.

cond-mat.supr-con↗

arXiv1999

Direct Observation of a One Dimensional Static Spin Modulation in Insulating La1.95Sr0.05CuO4

We report the results of an extensive elastic neutron scattering study of the incommensurate (IC) static spin correlations in La1.95Sr0.05CuO4 which is an insulating spin glass at low temperatures. The present neutron scattering experiments on the same x=0.05 crystal employ a narrower instrumental Q-resolution and thereby have revealed that the crystal has only two orthorhombic twins at low temperatures with relative populations of 2:1. We find that, in a single twin, only two satellites are observed at (1, +/-0.064, L)(ortho) and (0, 1+/-0.064, L)(ortho), that is, the modulation vector is only along the orthorhombic b*-axis. This demonstrates unambiguously that La1.95Sr0.05CuO4 has a one-dimensional static diagonal spin modulation at low temperatures, consistent with certain stripe models. We have also reexamined the x=0.04 crystal that previously was reported to show a single commensurate peak. By mounting the sample in the (H, K, 0) zone, we have discovered that the x=0.04 sample in fact has the same IC structure as the $x=0.05$ sample. The incommensurability parameter d for x=0.04 and 0.05, where d is the distance from (1/2, 1/2) in tetragonal reciprocal lattice units, follows the linear relation d=x. These results demonstrate that the insulator to superconductor transition in the under doped regime (0.05 </= x </= 0.06) in La2-xSrxCuO4 is coincident with a transition from diagonal to collinear static stripes at low temperatures thereby evincing the intimate coupling between the one dimensional spin density modulation and the superconductivity.

cond-mat.supr-con↗

arXiv1999

Freezing of anisotropic spin clusters in La1.98Sr0.02CuO4

A spin-glass compound, La$_{1.98}$Sr$_{0.02}$CuO$_4$, shows quasi-three-dimensional magnetic ordering below $\sim$40 K. A remarkable feature is that the magnetic correlation length along the orthorhombic $a\rm_{ortho}$ axis is much longer than that along the $b\rm_{ortho}$ axis, suggesting that the spin structure is closely related to the diagonal stripe structure. The spin-glass state can be expressed as a random freezing of quasi-three-dimensional spin clusters with anisotropic spin correlations ($ξ'_a\sim160$ Å, $ξ'_b\sim25$ Å, and $ξ'_c\sim4.7$ Åat 1.6 K). The new magnetic state is important as an intermediate phase between the three-dimensional antiferromagnetic ordered phase in La$_2$CuO$_4$ and the incommensurate phase in La$_{1.95}$Sr$_{0.05}$CuO$_4$ in which the positions of the incommensurate peaks are rotated by 45$^\circ$ in reciprocal space about ($π$,$π$) from those observed in the superconducting La$_2$CuO$_4$ compounds.

cond-mat.str-el↗

arXiv1999

Neutron Scattering Study of Spin Density Wave Order in the Superconducting State of Excess-Oxygen-Doped La2CuO4+y

We report neutron scattering measurements of spin density wave order within the superconducting state of a single crystal of predominately stage-4 La2CuO4+y with a Tc(onset) of 42 K. The low temperature elastic magnetic scattering is incommensurate with the lattice and is characterized by long-range order in the copper-oxide plane with the spin direction identical to that in the insulator. Between neighboring planes, the spins exhibit short-range correlations with a stacking arrangement reminiscent of that in the undoped antiferromagnetic insulator. The elastic magnetic peak intensity appears at the same temperature within the errors as the superconductivity, suggesting that the two phenomena are strongly correlated. These observations directly reveal the persistent influence of the antiferromagnetic order as the doping level increases from the insulator to the superconductor. In addition, our results confirm that spin density wave order for incommensurabilities near 1/8 is a robust feature of the La2CuO4-based superconductors.

cond-mat.supr-con↗

arXiv1999

Observation of New Incommensurate Magnetic Correlations at the Lower Critical Concentration for Superconductivity (x=0.05) in La(2-x)Sr(x)CuO4

Neutron-scattering experiments have been performed on lightly-doped La(2-x)Sr(x)CuO4 single crystals in both the insulating (x=0.03,0.04,0.05) and superconducting (x=0.06) regions. Elastic magnetic peaks are observed at low temperatures in all samples with the maximum peak linewidth occuring at the critical concentration x_c=0.05. New incommensurate peaks are observed only at x=0.05, the positions of which are rotated by 45 degrees in reciprocal space about (pi,pi) from those observed for x>=0.06 in the superconducting phase.

cond-mat.supr-con↗

arXiv1999

Neutron Scattering Study of Elastic Magnetic Signals in Superconducting La1.94Sr0.06Cu4

Recent neutron-scattering experiments on La(2-x)Sr(x)CuO4 single crystals by Wakimoto et al. have revealed that elastic magnetic peaks appear at low temperatures in both insulating (x=0.02-0.05) and superconducting (x=0.06) samples. We have carried out further investigations particularly on the elastic incommensurate peaks for x=0.06, and found that the integrated intensity drastically changes across the low temperature insulator- superconductor boundary; the intensity of x=0.06 is 4 times smaller than that of x=0.05, while the intensity in the insulating region stays constant.

cond-mat.supr-con↗