arXiv subjects

S. Williams

Publications and source records attributed to S. Williams.

28 records · Page 2Linked to original sources

arXiv2015

Spectra of radiation emitted by single-walled and multi-walled carbon nanotubes during multiple microwave irradiation and cooling cycles

Carbon nanotubes have been observed to emit ultraviolet, visible, and infrared radiation when exposed to microwave fields. We have performed experiments in which both single-walled (~1 nm diameters) and multi-walled carbon nanotubes (>50 nm diameters) were exposed to 2.45 GHz microwaves during several irradiation and cooling cycles at a pressure of ~10-6 torr. A comparison of the spectra of the radiation emitted by the nanotubes indicates that the intensity of radiation with wavelengths ranging from 700 to 1000 nm increased substantially during the course of five irradiation and cooling cycles. The data suggests that the mechanism responsible for the emissions is field emission-induced luminescence and that the intensity of the radiation emitted increased due to the opening of nanotube ends. Furthermore, the intensity of the radiation emitted by the multi-walled carbon nanotubes was much greater than the radiation emitted by the single-walled nanotubes. Scanning electron microscopy images indicate that most of the single-walled nanotubes were bundled together, while the multi-walled nanotubes were not. This bundling may have resulted in a lower field enhancement factor and/or screening effects which might help to explain the difference in the intensities of the radiation emitted by the samples.

cond-mat.mtrl-sci↗

arXiv2015

Spectra of Radiation Emitted from Open-Ended and Closed Carbon Nanotubes Exposed to Microwave Fields

We performed experiments in which both open-ended and closed carbon nanotubes were exposed to 2.46 GHz microwaves over the course of several irradiation and cooling cycles at a pressure of ~10-6 torr. The spectra of the radiation emitted from the nanotubes indicate that the intensity of the emitted radiation with wavelengths of 650-1000 nm increased during the irradiation cycles. However, the intensity of the radiation emitted from untreated nanotubes increased substantially more than the intensity of the radiation emitted from nanotubes that had been chemically treated in order to open nanotube ends. As open-ended nanotubes have a lower work function than closed nanotubes, and as nanotube ends are known to open as they are heated, our results suggest that the mechanism responsible for the emission of infrared, visible, and ultra-violet radiation from carbon nanotubes exposed to microwaves is field emission-induced luminescence.

cond-mat.mtrl-sci↗

arXiv2015

Neutron single-particle strength in silicon isotopes: Constraining the driving forces of shell evolution

Shell evolution is studied in the neutron-rich silicon isotopes 36,38,40 Si using neutron single-particle strengths deduced from one-neutron knockout reactions. Configurations involving neutron excita- tions across the N = 20 and N = 28 shell gaps are quantified experimentally in these rare isotopes. Comparisons with shell model calculations show that the tensor force, understood to drive the col- lective behavior in 42 Si with N = 28, is already important in determining the structure of 40 Si with N = 26. New data relating to cross-shell excitations provide the first quantitative support for repulsive contributions to the cross-shell T = 1 interaction arising from three-nucleon forces.

nucl-ex↗

arXiv2015

Analysis of ZDDP content and thermal decomposition in motor oils using NAA and NMR

Zinc dialkyldithiophosphates (ZDDPs) are one of the most common anti-wear additives present in commercially-available motor oils. The ZDDP concentrations of motor oils are most commonly determined using inductively coupled plasma atomic emission spectroscopy (ICP-AES). As part of an undergraduate research project, we have determined the Zn concentrations of eight commercially-available motor oils and one oil additive using neutron activation analysis (NAA), which has potential for greater accuracy and less sensitivity to matrix effects as compared to ICP-AES. The 31P nuclear magnetic resonance (31P-NMR) spectra were also obtained for several oil additive samples which have been heated to various temperatures in order to study the thermal decomposition of ZDDPs.

cond-mat.mtrl-sci↗

arXiv2013

Angular Distribution of Bremsstrahlung Produced by 10-keV and 20-keV Electrons Incident on a Thick Au Target

The relative intensities of the thick-target bremsstrahlung produced by 10-keV and 20-keV electrons incident on Au at forward angles ranging from 0 degrees to 25 degrees are compared. Following corrections for photon absorption within the target, the detected radiation appears to be distributed anisotropically only for photon energies, k, that are approximately equal to the initial energy of the incident electrons, E. The results are compared to the theoretical angular distributions of Kissel et al. [At. Data Nucl. Data Tables 28, 381 (1983)]. The comparison suggests that when k/E is approximately equal to 1, the angular distribution of bremsstrahlung emitted by electrons incident on thick targets is similar to the theoretical angular distribution of bremsstrahlung emitted by electrons incident on free-atom targets.

physics.atom-ph↗

arXiv2013

Angular distribution of thick-target bremsstrahlung produced by electrons with initial energies ranging from 10 to 20-keV incident on Ag

Experimental results are presented comparing the intensity of the bremsstrahlung produced by electrons with initial energies ranging from 10 to 20-keV incident on a thick Ag target, measured at forward angles in the range 0 degrees to 55 degrees. When the data are corrected for attenuation due to photon absorption within the target, the results indicate that the detected radiation is distributed anisotropically only at photon energies, k, that are approximately equal to the initial energy of the incident electrons, Eo. The results of our experiments suggest that as k /Eo goes to 0, the detected radiation becomes essentially isotropic due primarily to the scattering of electrons within the target. A comparison to the theoretical work of Kissel et al. [At. Data Nucl. Data Tables 28, 381 (1983)] suggests that the angular distribution of bremsstrahlung emitted by electrons incident on thick targets is similar to the angular distribution of bremsstrahlung emitted by electrons incident on free-atom targets only when k /Eo is approximately equal to 1. The experimental data are also in approximate agreement with the angular distribution predictions of the Monte Carlo program, PENELOPE.

physics.atom-ph↗

arXiv2012

Resonant Few-Photon Excitation of a Single-Ion Oscillator

We study the motion of an undamped single-ion harmonic oscillator, resonantly driven with a pulsed radiation pressure force. We demonstrate that a barium ion, initially cooled to the Doppler limit, quickly phase locks to the drive and builds up coherent oscillations above the thermal distribution after scattering of order one hundred photons. In our experiment, this seeded motion is subsequently amplified and then analyzed by Doppler velocimetry. Since the coherent oscillation is conditional upon the internal quantum state of the ion, this motional excitation technique could be useful in atomic or molecular single-ion spectroscopy experiments, providing a simple protocol for state readout of non-fluorescing ions with partially closed-cycle transitions.

physics.atom-ph↗

arXiv2011

Evidence for a spin-aligned neutron-proton paired phase from the level structure of $^{92}$Pd

The general phenomenon of shell structure in atomic nuclei has been understood since the pioneering work of Goeppert-Mayer, Haxel, Jensen and Suess.They realized that the experimental evidence for nuclear magic numbers could be explained by introducing a strong spin-orbit interaction in the nuclear shell model potential. However, our detailed knowledge of nuclear forces and the mechanisms governing the structure of nuclei, in particular far from stability, is still incomplete. In nuclei with equal neutron and proton numbers ($N = Z$), the unique nature of the atomic nucleus as an object composed of two distinct types of fermions can be expressed as enhanced correlations arising between neutrons and protons occupying orbitals with the same quantum numbers. Such correlations have been predicted to favor a new type of nuclear superfluidity; isoscalar neutron-proton pairing, in addition to normal isovector pairing (see Fig. 1). Despite many experimental efforts these predictions have not been confirmed. Here, we report on the first observation of excited states in $N = Z = 46$ nucleus $^{92}$Pd. Gamma rays emitted following the $^{58}$Ni($^{36}$Ar,2$n$)$^{92}$Pd fusion-evaporation reaction were identified using a combination of state-of-the-art high-resolution γ-ray, charged-particle and neutron detector systems. Our results reveal evidence for a spin-aligned, isoscalar neutron-proton coupling scheme, different from the previous prediction. We suggest that this coupling scheme replaces normal superfluidity (characterized by seniority coupling) in the ground and low-lying excited states of the heaviest N = Z nuclei. The strong isoscalar neutron- proton correlations in these $N = Z$ nuclei are predicted to have a considerable impact on their level structures, and to influence the dynamics of the stellar rapid proton capture nucleosynthesis process.

nucl-ex↗

arXiv2007

Intrinsic knotting and linking of almost complete graphs

We introduce new sufficient conditions for intrinsic knotting and linking. A graph on n vertices with at least 4n-9 edges is intrinsically linked. A graph on n vertices with at least 5n-14 edges is intrinsically knotted. We also classify graphs that are 0, 1, or 2 edges short of being complete partite graphs with respect to intrinsic linking and intrinsic knotting. In addition, we classify intrinsic knotting of graphs on 8 vertices.

math.GT↗

arXiv2002

Gamma ray Large Area Space Telescope (GLAST) Balloon Flight Engineering Model: Overview

The Gamma Ray Large Area Space Telescope (GLAST) Large Area Telescope (LAT) is a pair-production high-energy (>20 MeV) gamma-ray telescope being built by an international partnership of astrophysicists and particle physicists for a satellite launch in 2006, designed to study a wide variety of high-energy astrophysical phenomena. As part of the development effort, the collaboration has built a Balloon Flight Engineering Model (BFEM) for flight on a high-altitude scientific balloon. The BFEM is approximately the size of one of the 16 GLAST-LAT towers and contains all the components of the full instrument: plastic scintillator anticoincidence system (ACD), high-Z foil/Si strip pair-conversion tracker (TKR), CsI hodoscopic calorimeter (CAL), triggering and data acquisition electronics (DAQ), commanding system, power distribution, telemetry, real-time data display, and ground data processing system. The principal goal of the balloon flight was to demonstrate the performance of this instrument configuration under conditions similar to those expected in orbit. Results from a balloon flight from Palestine, Texas, on August 4, 2001, show that the BFEM successfully obtained gamma-ray data in this high-background environment.

astro-ph↗