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S. Yu. Gavrilkin

Publications and source records attributed to S. Yu. Gavrilkin.

At least 19 recordsLinked to original sources

3D- (H-theta-phi) magnetic phase diagram of antiferromagnetic metal GdB6 with electron and lattice instability

The origin of charge transport and magnetization anisotropy was studied in GdB6, an antiferromagnetic (AF) metal (N\'eel temperature TN ~ 15.5 K) with cubic lattice and Gd S-type magnetic ions. Both small static Jahn-Teller distortions and nanoscale electronic instabilities (dynamic charge stripes) were found in precise low temperature X-ray diffraction measurements. The detailed magnetic field (H) vs temperature (T) phase diagrams were constructed with two main magnetic phases AF(I) and AF(II). Using the angular phi-dependences of magnetoresistance and magnetization, impeller-type patterns of the H-phi magnetic phase diagrams in the (110) and (111) planes were found at helium temperatures, which included the AF phases I and II separated from each other by radial and circular boundaries. The results argue in favor of the important role of the spin density wave 5d- component in the magnetic structure of AF(II) state. Charge fluctuations in stripes are proposed to be responsible for the suppression of the Ruderman-Kittel-Kasuya-Yoshida (RKKY) indirect exchange between the first and second neighboring Gd3+ ions located along the <100> and <110> directions. These dynamic charge stripes and vibrationally coupled Gd-Gd pairs produce unusual anisotropy of charge scattering and the impeller-type diagrams in GdB6 with S-type magnetic ion.

cond-mat.str-el

Magnetoresistance in the helical itinerant magnets MnSi and Mn$_{1-x}$Co$_x$Si

We studied the longitudinal and transverse magnetoresistance of helical magnets, MnSi and Mn$_{1-x}$Co$_x$Si, at temperatures between 1.8 and 100~K and in magnetic fields up to 9 Tesla. All substances exhibited negative longitudinal and transverse magnetoresistance at temperatures above 4~K, which is most likely related to the suppression of spin fluctuations by the magnetic field. Note that in contrast to our finding, the longitudinal magnetoresistance of ferromagnetic metals was found to be positive. The unique positive and anisotropic magnetoresistance of pure MnSi at low temperatures (1.8 and 4~K) in the induced ferromagnetic phase shows effective suppression of fluctuations by the magnetic field. The significant difference in behavior between pure MnSi and doped MnSi lies in the specifics of the latter material, which forms a sort of helical fluctuation cloud and reveals quantum critical properties at low temperatures. The observed isotropic magnetoresistance in MnSi and Mn$_{1-x}$Co$_x$Si at higher temperatures can tentatively be attributed to the shortening of the mean free path of electrical carriers due to scattering on magnetic fluctuations and impurities, which results in a suppression of Lorentz force effects.

cond-mat.str-el

Linear and isotropic magnetoresistance of Co$_{1-x}$Fe$_x$Si at x=0.2; 0.4; 0.65

We studied the magnetoresistance (MR) of well-characterized samples of Co$_{1-x}$Fe$_x$Si at x=0.2, 0.4, and 0.65 at temperatures between 1.8 and 100~K and magnetic fields of 9~T. The quasilinear dependence of MR on the magnetic field at low temperatures and the practically isotropic properties of MR in these compounds are tentatively attributed to the specifics of Weyl electron spectra and general disorder of the materials.

cond-mat.str-el

Magnetic Phase Diagrams of Antiferromagnet DyB12 with Jahn-Teller Lattice Instability and Electron Phase Separation

The origin of charge transport and magnetization anisotropy was studied in DyB12, an antiferromagnetic (AF) metal with Neel temperature TN = 16.3 K that exhibits both cooperative Jahn-Teller distortions of the fcc crystal structure and nanoscale electronic instabilities (dynamic charge stripes). Based on the results obtained the magnetic field (H) vs temperature (T) phase diagrams have been constructed. Moreover, from angle dependent magnetoresistance and magnetization measurements the butterfly-type patterns of the H-phi magnetic phase diagram in the (110) plane were created, which include a number of different magnetic phases separated from each other by radial and circular boundaries. Several positive and negative contributions to magnetoresistance were separated and analyzed, providing arguments in favor of the important role of the spin density wave 5d-component in the magnetic structure of AF state. We argue that charge fluctuations in stripes are responsible for the suppression of the Ruderman-Kittel-Kasuya-Yoshida (RKKY) indirect exchange between the nearest neighbored Dy3+ ions located along the same 110 directions, as these dynamic charge stripes produce the magnetic phase diversity and the butterfly-type anisotropy in DyB12.

cond-mat.str-el

Two-gap superconductor ZrB$_{12}$ with dynamic stripes and charge density waves: Crystal structure, physical properties and pairing mechanism

A review of long-term studies of ZrB$_{12}$ and LuB$_{12}$ superconductors with very similar conduction bands and phonon spectra, but with radically different (by a factor of 15-20) critical temperatures and magnetic fields is presented. A detailed analysis of well-known studies in combination with new results of structural, thermodynamic and charge transport measurements obtained here for these metallic dodecaborides with Jahn-Teller instability of the rigid boron network and with dynamic charge stripes allows us to conclude in favor of the primary role of nanoscale effects of electron phase separation, leading to the formation of one-dimensional dynamic chains with different configurations of fluctuating charges, which in the case of ZrB$_{12}$ are predominantly $2p$-states, and for LuB$_{12}$-$5d$-$2p$ states. We propose a new plasmon-phonon pairing mechanism in ZrB$_{12}$, which may be common to different classes of high-$T_c$ superconductors.

cond-mat.supr-con

Evidence for spin droplets (ferrons) formation in the heavy fermion metal CeB$_6$ with dynamic charge stripes

The presented studies of resistivity (R), thermal conductivity (k) and specific heat (C) at low temperature 1.8-7 K in magnetic field up to 90 kOe made it possible to detect for the first time the exponential field dependences R(H), 1/k(H), $C(H) \sim \exp(-μ_{\rm eff}H/kBT)$ of the charge transport and thermal characteristics in the so-called antiferroquadrupole (AFQ) phase of the archetypal heavy-fermion CeB$_6$ hexaboride. From magnetoresistance measurements it is shown that in the AFQ state the effective magnetic moment varies in the range $μ_{\rm eff}(T) = 1.4$-1.9$μ$B, and its value is very close to $μ_{\rm eff}(τ)(T) = 2μ$B, derived from the field dependence of the relaxation time $|tau(H)$ observed in the heat capacity and thermal conductivity experiments. The phenomenological model proposed here allowed us to attribute the magnetic moments to spin droplets (ferrons), that appear in the bulk AFQ phase of CeB$_6$ crystals. The relevant electron phase separation at the nanoscale, manifested by dynamic charge stripes, that leads to the formation of ferrons, was revealed from the analysis of low-temperature X-ray diffraction experiments using the maximum entropy method. We argue that the Jahn-Teller collective mode of B$_6$ clusters is responsible for the charge stripe formation, which subsequently induces transverse quasi-local vibrations of Ce ions in the form of pairs and triples. These lead to 4f-5d spin fluctuations providing spin-polarons (ferrons) in the CeB$_6$ matrix.

cond-mat.str-el

Magnetoresistance of a bulk sample of FeSi

The magnetoresistance, MR of a well-characterized bulk FeSi sample was studied. It is shown that after a chaotic behavior at temperatures below 6 K, the magnetoresistance of FeSi becomes regular functions of temperature and magnetic field. The observations suggest that the mean free path of carriers defines along with the unknown negative component the negative values of magnetoresistance of FeSi then approaching zero values at high temperatures.

cond-mat.str-el

Physical properties of MnSi at extreme doping with Co: Quantum criticality

The samples of (Mn$_{1-x}$Co$_x$)Si with $x=0.15$ and $x=0.17$ were grown and their physical properties: magnetization and magnetic susceptibility, resistivity and heat capacity were studied. The data analysis included also the previous results at $x=0.057, 0.063, 0.09$. The indicated doping MnSi with Co completely destroys the helical phase transition whereas basically saves the helical fluctuation area normally situated slightly above the phase transition temperature. This area spreading from $\sim$5 to 0 K is not changed much with doping and forms some sort of helical fluctuation cloud revealing the quantum critical properties: $C_p/T\rightarrow\infty$ at $T\rightarrow0$.

cond-mat.str-el

Checkerboard-type patterns of charge stripes in two-gap superconductor ZrB12

Inhomogeneous superconductivity in the high quality single crystals of ZrB12 (Tc = 6 K) has been studied using the heat capacity and x-ray diffraction (XRD) data. Evidence of two-band superconductivity with two branches of upper critical field Hc2(Tc) is obtained in a magnetic field applied along the [110] axis of the crystal. On the contrary, at H //[100], the only dependence Hc2(Tc) is observed. This finding is supplemented with the checkerboard-type patterns of the charge stripes in ZrB12 deduced from the detailed analysis of XRD data. These patterns are compared to the structure of the charge stripes in the weakly bound superconductor LuB12, whose Tc is 15 times lower than that of ZrB12. Probable nature of the two-gap superconductivity in ZrB12 with strongly enhanced characteristics is discussed.

cond-mat.supr-con

Spin state crossover in Co3BO5

The magnetic contribution of the Co3+ ions in Co3BO5 has been investigated using the Co (K-edge) XMCD, dc magnetic susceptibility, and heat capacity measurements. The crystal structure of Co3BO5 single crystal has been solved in detail at the T range 296-703 K. The results have been supplemented by the GGA+U calculations.

cond-mat.mtrl-sci

Electronic Band Structure and Superconducting Properties of SnAs

We report comprehensive study of physical properties of the binary superconductor compound SnAs. The electronic band structure of SnAs was investigated using both angle-resolved photoemission spectroscopy (ARPES) in a wide binding energy range and density functional theory (DFT) within generalized gradient approximation (GGA). The DFT/GGA calculations were done including spin-orbit coupling for both bulk and (111) slab crystal structures. Comparison of the DFT/GGA band dispersions with ARPES data shows that (111) slab much better describes ARPES data than just bulk bands. Superconducting properties of SnAs were studied experimentally by specific heat, magnetic susceptibility, magnetotransport measurements and Andreev reflection spectroscopy. Temperature dependences of the superconducting gap and of the specific heat were found to be well consistent with those expected for the single band BCS superconductors with an isotropic s-wave order parameter. Despite spin-orbit coupling is present in SnAs, our data shows no signatures of a potential unconventional superconductivity, and the characteristic BCS ratio $2Δ/T_c = 3.48 - 3.73$ is very close to the BCS value in the weak coupling limit.

cond-mat.supr-con

Maltese Cross anisotropy in Ho0.8Lu0.2B12 antiferromagnetic metal with dynamic charge stripes

The model strongly correlated electron system Ho0.8Lu0.2B12 which demonstrates a cooperative Jahn-Teller instability of the boron sub-lattice in combination with rattling modes of Ho(Lu) ions, dynamic charge stripes and unusual antiferromagnetic (AF) ground state has been studied in detail at low temperatures by magnetoresistance, magnetization and heat capacity measurements. Based on received results it turns out that the angular H-fi-T magnetic phase diagrams of this non-equilibrium AF metal can be reconstructed in the form of a Maltese cross. The dramatic AF ground state symmetry lowering of this dodecaboride with fcc crystal structure can be attributed to the redistribution of conduction electrons which leave the RKKY oscillations of the electron spin density to participate in the dynamic charge stripes providing with extraordinary changes in the indirect exchange interaction between magnetic moments of Ho3+ ions and resulting in the emergence of a number of various magnetic phases. It is also shown that the two main contributions to magnetoresistance in the complex AF phase, the (i) positive linear on magnetic field and the (ii) negative quadratic component can be separated and analyzed quantitatively, correspondingly, in terms of charge carrier scattering on spin density wave (5d) component of the magnetic structure and on local 4f-5d spin fluctuations of holmium sites.

cond-mat.str-el

Superconducting gap symmetry in BaFe$_{1.9}$Ni$_{0.1}$As$_{2}$ superconductor

We report on the Andreev spectroscopy and specific heat of high-quality single crystals BaFe$_{1.9}$Ni$_{0.1}$As$_{2}$. The intrinsic multiple Andreev reflection spectroscopy reveals two anisotropic superconducting gaps $Δ_L \approx 3.2 \textendash 4.5$\,meV, $Δ_S \approx 1.2 \textendash 1.6$\,meV (the ranges correspond to the minimum and maximum value of the coupling energy in the $k_xk_y$-plane). The $25 \textendash 30 \%$ anisotropy shows the absence of nodes in the superconducting gaps. Using a two-band model with s-wave-like gaps $Δ_L \approx 3.2$\,meV and $Δ_S \approx 1.6$\,meV, the temperature dependence of the electronic specific heat can be well described. A linear magnetic field dependence of the low-temperature specific heat offers a further support of s-wave type of the order parameter. We find that a d-wave or single-gap BCS theory under the weak-coupling approach cannot describe our experiments.

cond-mat.supr-con

Probing Bulk Superconducting Order Parameter in Ba(K)Fe$_2$As$_2$ by Four Complementary Techniques

Using four different experimental techniques, we performed comprehensive studies of the bulk superconductive properties of single crystals of the nearly optimally doped $Ba_{1-x}K_xFe_2As_2$ ($T_{c} \approx 36\,K$), a typical representative of the 122 family. We investigated temperature dependencies of the (i) specific heat $C_{el}(T)$, (ii) first critical magnetic field $H_{c1}(T)$, (iii) intrinsic multiple Andreev reflection effect (IMARE), and (iv) infrared reflectivity spectra. All data clearly show the presence of (at least) two superconducting nodeless gaps. The quantitative data on the superconducting spectrum obtained by four different techniques are consistent with each other: (a) the small energy gap $Δ_S(0) \approx 1.8 - 2.5\,meV$, and the large gap energy $Δ_L(0) \approx 9.5 - 11.3\,meV$ that demonstrates the signature of an extended s-wave symmetry ($\sim~33 \%$ in-plane anisotropy), (b) the characteristic ratio $2Δ_L/k_BT_C$ noticeably exceeds the BCS value.

cond-mat.supr-con

Vortex Structure and Anisotropic Superconducting Gaps in Ba[Fe(Ni)]$_2$As$_2$

We studied nearly optimally Ni-substituted BaFe$_{2-x}$Ni$_x$As$_2$ (BFNA) single crystals with $T_C \approx 18.5$\,K. In irreversible magnetization measurements, we determined the field dependence of the critical-current density and discuss the nature of observed strong bulk pinning. Using intrinsic multiple Andreev reflections effect (IMARE) spectroscopy, we directly determine two distinct superconducting gaps and resolve their moderate anisotropy in the momentum space. The BCS-ratio for the large gap $2Δ_L/k_BT_C > 4.1$ evidences for a strong coupling in the $Δ_L$-bands.

cond-mat.supr-con

Suppression of Superconductivity in Lu$_x$Zr$_{1-x}$B$_{12}$ : Evidence of Static Magnetic Moments Induced by Non-Magnetic Impurities

Based on low temperature resistivity, heat capacity and magnetization investigations we show that the unusually strong suppression of superconductivity in Lu$_x$Zr$_{1-x}$B$_{12}$ BSC-type superconductors in the range $x$$<$0.08 is caused by the emergence of static spin polarization in the vicinity of non-magnetic lutetium impurities. The analysis of received results points to a formation of static magnetic moments with $μ_{eff}$$\approx$$3μ_B$ per Lu-ion. The size of these spin polarized nanodomains was estimated to be about 5 $Å$.

cond-mat.str-el

Uniaxial anisotropy and low-temperature antiferromagnetism of Mn2BO4 single crystal

The Mn2BO4 single crystals have been grown using the flux technique. The careful study crystal structure and magnetic properties have been carried out. The antiferromagnet transition at TN = 26 K has been traced through the dc magnetization and specific heat temperature dependences. The magnetic uniaxial anisotropy has been detected with easy axis of magnetization lying in ab-plane. A reduction of the effective magnetic moment value is assigned to the non-quenched orbital moment of Jahn-Teller Mn3+ ions. Based on the superexchange interactions calculations the magnetic behavior is discussed.

cond-mat.str-el

Quantum degradation of the second order phase transition

The specific heat, magnetization and thermal expansion of single crystals of antiferromagnetic insulator EuTe, measured at temperatures down to 2 K and in magnetic fields up to 90 kOe, demonstrate non trivial properties. The Neel temperature, being 9.8 K at H=0, decreases with magnetic field and tends to zero at 76 kOe, therefore forming a quantum critical point. The heat capacity and thermal expansion coefficient reveal lambda-type anomalies at the second order magnetic phase transition at low magnetic fields, evolving to simple jumps at high magnetic fields and low temperatures, well described in a fluctuation free mean-field theory. The experimental data and the corresponding analysis favor the quantum concept of effective increasing space dimensionality at low temperatures that suppresses a fluctuation divergence at a second order phase transition.

cond-mat.str-el