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Sadamichi Maekawa

Publications and source records attributed to Sadamichi Maekawa.

At least 19 recordsLinked to original sources

Dipolar and quadrupolar spin supersolid states in a spin-1 triangular antiferromagnet

We present a systematic numerical study of the spin-1 antiferromagnetic Heisenberg model on the triangular lattice in an out-of-plane magnetic field, using Density Matrix Renormalization Group (DMRG) methods. By mapping out the quantum phase diagram as a function of the single-ion anisotropy $D_z$ and magnetic field, we identify distinct dipolar and quadrupolar spin supersolid states, characterized by spontaneous U(1) symmetry breaking with finite spin superfluid stiffness coexisting with longitudinal translational symmetry breaking. At zero field, the dipolar spin supersolid with a 'Y'-type spin configuration persists down to $D_z = 0$, whereas the quadrupolar spin supersolid prevails at large $D_z$. At intermediate fields, the phase diagram is dominated by an up-up-down phase. At high fields below saturation, a quadrupolar spin superfluid emerges in the large-$D_z$ regime, whereas a dipolar spin supersolid with a 'V'-type spin configuration dominates at small $D_z$. These phases are characterized through their order parameters and spin superfluid stiffness using calculations on various system sizes. Furthermore, the dynamical spin structure factor is obtained across the phase diagram, where characteristic spectral signatures of different phases are observed, including the gapless Goldstone mode and the roton-like minima. These features are directly accessible to inelastic neutron scattering experiments. Our results provide a theoretical understanding of the interplay between frustrations, anisotropy, and Zeeman interactions in driving distinct spin supersolid phases in the spin-1 system, which are relevant to various triangular-lattice antiferromagnets such as Na$_2$BaNi(PO$_4$)$_2$ and K$_2$Ni(SeO$_3$)$_2$.

cond-mat.str-el↗

Nonreciprocity reversal of magnetoacoustic attenuation in NiFe alloy thin films

Nonreciprocity, the asymmetry of transport, underlies technologies from the diode to the microwave isolator. In a ferromagnet, a surface acoustic wave generates an elliptical effective field with propagation-locked handedness, breaking the reciprocity of its propagation. Despite decades of study on this phenomenon, a method for controlling the sign of the nonreciprocity has remained elusive. Here we observe a sign reversal in Ni$_x$Fe$_{100-x}$ films. A 0.8 at.% change across Permalloy's zero-magnetostriction composition, where the magnetoelastic coefficient $b$ changes sign, reverses the handedness of the elliptical effective field and thereby the nonreciprocity, from 78.6% to -61.8%. Angle-dependent measurements and spin-wave-ellipticity modelling show that reversing the sign of $b$ reverses the handedness of the elliptically polarized effective field. Aided by cubic frequency scaling, we resolve the sign of $b$ down to -0.05 MPa in a 10-nm film, establishing nonreciprocity as a nanoscale probe of magnetoelastic coupling.

cond-mat.mtrl-sci↗

Dissipationless dynamics of spin supersolid states in a spin-1/2 triangular antiferromagnet with impurities

Motivated by recent experimental evidence for spin supersolid states in triangular-lattice compounds, we numerically investigate the dynamical properties of magnetic field-induced phases in the spin-1/2 easy-axis triangular antiferromagnetic Heisenberg model in the presence of magnetic impurities. In both weak- and strong-field spin supersolid states, the gapless Goldstone mode at the $K$ points remains robust against impurities, which is a direct manifestation of spin superfluidity. By contrast, at the same impurity density, impurities induce a splitting of the magnon bands in the conventional magnetic state, the so-called up-up-down state. In addition, the finite superfluid stiffness probed by the twisted phase in the spin supersolid states is consistent with the excitation spectrum. We argue that the excitation spectrum with impurities provides direct spectroscopic evidence for dissipationless spin dynamics in the spin supersolid states, which is experimentally accessible via inelastic neutron scattering.

cond-mat.str-el↗

A microscopic design rule for spin supersolids in triangular-lattice magnets

Spin supersolids emerge as a central topic in frustrated magnetism, motivating the search for realization in quantum materials. To this end, we study the origin of exchange anisotropy, $Δ$, in triangular-lattice cobaltate families $X_2$$Y$Co(PO$_4$)$_2$ and $X_2$Co(SeO$_3$)$_2$ ($X$ = Na, K, Rb, Cs; $Y$ = Mg, Ca, Sr, Ba) by tailoring realistic spin models. We show that $Δ$ is determined by the ratio of trigonal crystal field to spin-orbit coupling strength. This framework explains contrasting anisotropies in these families, predicts systematic trends in $Δ$ across $X/Y$-substitutions, and identifies candidate materials for spin supersolids. Our results establish trigonal field engineering as a microscopic route toward the design of spin supersolids.

cond-mat.str-el↗

Emergent Spin Supersolids in Frustrated Quantum Materials

Recent years have witnessed the emergence of spin supersolids in frustrated quantum magnets, establishing a material-based platform for supersolidity beyond its original context in solid helium. A spin supersolid is characterized by the coexistence of longitudinal spin order that breaks lattice translational symmetry and transverse spin order associated with the spontaneous breaking of the spin U(1) symmetry. Extensive experimental investigations, together with advanced numerical studies, have now revealed a coherent and internally consistent picture of these phases, substantially deepening our understanding of supersolidity in quantum magnetic materials. Beyond their fundamental interest as exotic quantum states, potential applications in highly efficient demagnetization cooling have been supported by a giant magnetocaloric effect observed in candidate materials. Moreover, the possible dissipationless spin supercurrents could open promising perspectives for spin transport and spintronic applications. This review summarizes recent progress on emergent spin supersolids in frustrated triangular-lattice quantum antiferromagnets, surveys experimental evidence from thermodynamic and spectroscopic measurements, and compares these results with theoretical studies of minimal models addressing global phase diagrams, ground state properties, and collective excitations. In addition, this review discusses characteristic spin-transport phenomena and outlines future directions for exploring spin supersolids as functional quantum materials.

cond-mat.str-el↗

Josephson diode effect via a non-equilibrium Rashba system

A non-equilibrium state in a Rashba system under an in-plane magnetic field is identified as the origin of the Josephson diode effect. This state is induced by a current bias--necessary for measuring the current-voltage characteristics--which shifts the Fermi momentum away from equilibrium. This essential mechanism has been overlooked in previous studies. This oversight stems from the implicit assumption that the equilibrium-based formulations are sufficient to describe Josephson effect. We formulate the Josephson coupling via the non-equilibrium Rashba system under current bias using a tunneling Hamiltonian, where the Rashba system is modeled as one-dimensional. When the magnetic field is applied perpendicular to the current, the Josephson coupling becomes asymmetric, giving rise to the diode effect. The magnitude and sign of this effect depend on the distance between the superconducting electrodes $d$, the in-plane magnetic field, and the spin-orbit coupling strength. Our results clarify the microscopic origin of the Josephson diode effect, which can be optimized by tuning $d$.

cond-mat.supr-con↗

Electromagnetic evanescent field associated with surface acoustic wave: Response of metallic thin films

Surface acoustic waves (SAWs), coherent vibrational modes localized at solid surfaces, have been employed to manipulate and detect electronic and magnetic states in condensed-matter systems via strain. SAWs are commonly excited in a piezoelectric material, often the substrate. In such systems, SAWs not only generate strain but also electric field at the surface. Conventional analysis of the electric field accompanying the SAW invokes the electrostatic approximation, which may fall short in fully capturing its essential characteristics by neglecting the effect of the magnetic field. Here we study the electric and magnetic fields associated with SAWs without introducing the electrostatic approximation. The plane wave solution takes the form of an evanescent field that decays along the surface normal with a phase velocity equal to the speed of sound. If a metallic film is placed on the piezoelectric substrate, a time- and space-varying electric field permeates into the film with a decay length along the film normal defined by the skin depth and the SAW wavelength. For films with high conductivity, the phase of the electric field varies along the film normal. The emergence of the evanescent field is a direct consequence of dropping the electrostatic approximation, providing a simple but critical physical interpretation of the SAW-induced electromagnetic field.

cond-mat.mes-hall↗

Spin Seebeck Effect of Triangular-lattice Spin Supersolid

Using thermal tensor-network approach, we investigate the spin Seebeck effect (SSE) of the triangular-lattice quantum antiferromagnet hosting spin supersolid phase. We focus on the low-temperature scaling behaviors of the normalized spin current across the interface. For the 1D Heisenberg chain, we find a negative spinon spin in the bulk current with algebraic temperature scaling; at low fields, boundary effects induce a second sign reversal at lower temperatures. These benchmark results are consistent with field-theoretical analysis. On the triangular lattice, spin frustration dramatically enhances the low-temperature SSE, with distinct spin-current signatures -- particularly the sign reversal and characteristic temperature dependence -- distinguishing different spin states. Remarkably, we discover a persistent, negative spin current in the spin supersolid phase, which saturates to a non-zero value in the low-temperature limit and can be ascribed to the Goldstone-mode-mediated spin supercurrents. Moreover, a universal scaling $T^{d/z}$ is found at the U(1)-symmetric polarization quantum critical points. These distinct quantum spin transport traits provide sensitive spin current probes for spin supersolid states in quantum magnets such as Na$_2$BaCo(PO$_4$)$_2$. Furthermore, our results also establish spin supersolids as a tunable quantum platform for spin caloritronics in the ultralow-temperature regime.

cond-mat.str-el↗

Harmonic and Subharmonic Magnon Generation in a Surface Acoustic Wave Resonator

We experimentally observe the generation of magnon harmonics and subharmonics in an on-chip surface acoustic wave resonator incorporating a thin Co$_{20}$Fe$_{60}$B$_{20}$ film, using micro-focused Brillouin light scattering. In our devices, rotating the in-plane magnetic field allows continuous tuning of the magnon-phonon coupling from weak to strong within the same resonator. In the weak coupling regime, we only observe fundamental magnetoelastic wave signal at $f_{1}$. Conversely, in the strong coupling regime, in addition to the fundamental magnetoelastic wave, we observe subharmonic and harmonic signals at $3/2f_{1}$, $2f_{1}$, and $3f_{1}$, which are well reproduced by our analytical model. Our results establish phonons as a means to generate and control nonlinear magnons in the strong coupling regime, providing a new route for magnonic signal processing.

cond-mat.mes-hall↗

Controlling spin currents with magnon interference in a canted antiferromagnet

Controlling spin current lies at the heart of spintronics and its applications. The sign of spin currents is monotonous in ferromagnets once the current direction is determined. Spin currents in antiferromagnets can possess opposite polarization, but requires enormous magnetic fields to lift the degeneracy. Controlling spin currents with different polarization is urgently demanded but remains hitherto elusive. Here, we demonstrate the control of spin currents at room temperature by magnon interference in a canted antiferromagnet, hematite recently also classified as an altermagnet. Magneto-optical characterization by Brillouin light scattering revealed that the spatial periodicity of the beating patterns was tunable via the microwave frequency. The inverse spin-Hall voltage changed sign as the frequency was scanned, i.e., a frequency-controlled switching of polarization in pure spin currents was obtained. Our work marks the use of antiferromagnetic magnon interference to control spin currents, which substantially extends the horizon for the emerging field of coherent antiferromagnetic spintronics.

cond-mat.mes-hall↗

Spin current generation by acousto-electric evanescent wave

We experimentally demonstrate that a spin current can be induced by the acousto-electric evanescent wave, an electric field associated with surface acoustic waves (SAWs) that decay along the surface normal. A previous study showed that a magnetic-field-dependent dc voltage (acoustic voltage) emerges in heavy metal (HM)/ferromagnet (FM) bilayers under excitation of SAWs. The effect, referred to as the acoustic spin Hall effect, was understood by assuming a SAW-induced ac spin current rectified by the oscillation of the FM layer magnetization and the inverse spin Hall effect. However, the mechanism of the spin current generation remained unidentified. Here we measure the acoustic voltage as a function of the SAW propagation direction relative to the crystalline orientation of a LiNbO$_3$ substrate. We find that the magnetic field angle dependence of the acoustic voltage exhibits a phase shift depending on the SAW propagation direction. The result is consistently explained in terms of the acousto-electric evanescent wave generating the spin current in HM layer via the spin Hall effect, thus clarifies the origin of the acoustic spin Hall effect.

cond-mat.mes-hall↗

Observation of nonreciprocal diffraction of surface acoustic wave

Rectification phenomenon caused by the simultaneous breaking of time reversal and spatial inversion symmetries has been extended to a wide range of (quasi)particles and waves; however, the nonreciprocal diffraction, which is the imbalance of upward and downward deflections, was previously observed only for photons and remained to be extended to other (quasi)particles. In this study, we present evidence of the nonreciprocal diffraction of surface acoustic wave (SAW) utilizing a magnetoelastic grating on a SAW device. Asymmetric diffraction intensities were observed when the ferromagnetic resonance was acoustically excited. Based on a theoretical model, we attribute the microscopic origin of this phenomenon to the resonant scattering involving ferromagnetic resonance excitations. The novel property may pave an avenue to further development of SAW devices for various purposes, including microwave communications and quantum engineering applications.

cond-mat.mes-hall↗

Spin and spin current -- From fundamentals to recent progress

Along with the progress of spin science and spintronics research, the flow of electron spins, (i.e. spin current), has attracted interest. New phenomena and electronic states were explained in succession using the concept of spin current. Moreover, as many of the conventionally known spintronics phenomena became well organized based on spin current, it has rapidly been recognized as an essential concept in a wide range of condensed matter physics. In this article, we focus on recent developments in the physics of spin, spin current, and their related phenomena, where the conversion between spin angular momentum and different forms of angular momentum plays an essential role. Starting with an introduction to spin current, we first discuss the recent progress in spintronic phenomena driven by spin-exchange coupling: spin pumping, topological Hall torque, and emergent inductor. We, then, extend our discussion to the interaction/interconversion of spins with heat, lattice vibrations, and charge current and address recent progress and perspectives on the spin Seebeck and Peltier effects. Next, we review the interaction between mechanical motion and electron/nuclear spins and argue the difference between the Barnett field and rotational Doppler effect. We show that the Barnett effect reveals the angular momentum compensation temperature, at which the net angular momentum is quenched in ferrimagnets.

cond-mat.mtrl-sci↗

Strongly Coupled Spin Waves and Surface Acoustic Waves at Room Temperature

Here, we report the observation of strong coupling between magnons and surface acoustic wave (SAW) phonons in a thin CoFeB film constructed in an on-chip SAW resonator by analyzing SAW phonon dispersion anticrossings. Our device design provides the tunability of the film thickness with a fixed phonon wavelength, which is a departure from the conventional approach in strong magnon--phonon coupling research. We detect a monotonic increase in the coupling strength by expanding the film thickness, which agrees with our theoretical model. Our work offers a significant way to advance fundamental research and the development of devices based on magnon--phonon hybrid quasiparticles.

cond-mat.mes-hall↗

Electron Hydrodynamics by Spin Hall Effect

Electron hydrodynamics is currently known to emerge only when electron-electron interaction dominates over the momentum-nonconserving scatterings of electrons, where the electron transport is described by a hydrodynamic equation. Here we show that electron transport in electron systems with the spin Hall effect is also given by the hydrodynamic equation, whose kinetic viscosity is determined by the spin diffusion length and the transport lifetime. The electric current vorticity is proportional to the spin accumulation due to the spin Hall effect in two-dimensional systems. We demonstrate by solving the hydrodynamic equation in a two-dimensional system with a cavity, combined with micromagnetic simulation for an attached chiral magnetic insulator, that the spin accumulated near the boundary of the cavity creates a magnetic skyrmion. Our findings and demonstration shed light on a novel aspect of electron hydrodynamics and spin transport.

cond-mat.mes-hall↗

Acoustically driven magnon-phonon coupling in a layered antiferromagnet

Harnessing the causal relationships between mechanical and magnetic properties of van der Waals materials presents a wealth of untapped opportunity for scientific and technological advancement, from precision sensing to novel memories. This can, however, only be exploited if the means exist to efficiently interface with the magnetoelastic interaction. Here, we demonstrate acoustically-driven spin-wave resonance in a crystalline antiferromagnet, chromium trichloride, via surface acoustic wave irradiation. The resulting magnon-phonon coupling is found to depend strongly on sample temperature and external magnetic field orientation, and displays a high sensitivity to extremely weak magnetic anisotropy fields in the few~mT range. Our work demonstrates a natural pairing between power-efficient strain-wave technology and the excellent mechanical properties of van der Waals materials, representing a foothold towards widespread future adoption of dynamic magneto-acoustics.

cond-mat.mes-hall↗

Shapiro steps in charge-density-wave states driven by ultrasound

We show that ultrasound can induce the Shapiro steps (SS) in the charge-density-wave (CDW) state. When ultrasound with frequency $ω$ and a dc voltage are applied, the SS occur at the current $I$ $\propto$ $nω$ with integer $n$. Even and odd multiples of SS are represented by two couplings between the CDW and ultrasound. Although an ac voltage bias with frequency $ω$ induces the SS at $I\propto nω$, the ultrasound bias enhances the odd multiples more strongly than the even ones. This is the difference between the ultrasound and the ac voltage. Since the SS cause abrupt peaks in the $dV/dI$, the extreme changes in the $I$-$V$ curve will be applied to a very sensitive ultrasound detector.

cond-mat.mes-hall↗

Derivation of Interacting Two-Qubit Dynamics from Spin-Boson Model

We derive damping equations of motion for interacting two-spin states from a spin-boson model in order to examine qubit dynamics in quantum computers. On the basis of the composite operator method, we develop the Caldeira-Leggett approach for open quantum systems so that the entanglement dynamics originated from the two-spin correlation can be taken. We demonstrate numerical results for time dependence on the two-spin dynamics. We find that the relaxation of the total spin is described by a quantum version of the Landau-Lifshitz-Gilbert equation for magnetic materials. We also find that a two-spin composite mode keeps oscillation even after the total spin has been fully relaxed. We thus conclude that the two-spin correlation due to the presence of the composite mode is stable against dissipation. We consider the mechanism of why the correlation is maintained.

quant-ph↗