arXiv subjects

Sahand Mahmoodian

Publications and source records attributed to Sahand Mahmoodian.

At least 19 recordsLinked to original sources

arXiv2026

Dynamic stimulated emission for deterministic addition and subtraction of propagating photons

Photon subtraction and addition are essential non-Gaussian processes in quantum optics, where conventional methods using linear optics and number-resolving detection often suffer from low success probability. Here, we introduce the concept of \textit{dynamic stimulated emission}, whereby a quantum emitter undergoes stimulated emission with a time-dependent coupling. Despite interacting with a multimode photon field, we show that, for both two- and three-level emitters, their dynamics can mimic that of a single-mode Jaynes-Cummings model. This feature can be used to deterministically add or subtract a photon while maintaining a single propagating optical mode. We provide semi-analytic solutions to this problem for Fock states, enabling deterministic and unconditional photon addition and subtraction with fidelity ${\cal F}>0.996$. Our semi-analytic solutions are provided for both dynamically coupled two-level systems and for three-level systems whose dynamical coupling is controlled by a coherent laser drive. Moving beyond individual Fock states, we further showcase the ability to subtract and add single photons to photon-number superposition states. We show that Schr{ö}dinger cat states can be prepared from squeezed vacuum input via cascaded subtraction or cascaded addition. Finally, we show that our photon-addition process can be used to add a photon to any squeezed and displaced state with high success probability and fidelity ${\cal F}>0.99$, thereby potentially converting quantum emitters from single-photon sources to sources of single-photon-added Gaussian states without the need for inline squeezing. Our protocols provide a path towards integrating quantum emitters to construct efficient sources of single-mode non-Gaussian light beyond single photons.

quant-ph↗

arXiv2026

Efficient optical cat state generation using squeezed few-photon superposition states

Optical Schrödinger cat states are non-Gaussian states with applications in quantum technologies, such as for building error-correcting states in quantum computing. Yet the efficient generation of high-fidelity optical Schrödinger cat states is an outstanding problem in quantum optics. Here, we propose using squeezed superpositions of zero and two photons, $|θ\rangle = \cos{(θ/2)}|0\rangle + \sin{(θ/2)}|2\rangle$, as ingredients for protocols to efficiently generate high-fidelity cat states. We present a protocol using linear optics with success probability $P\gtrsim 50\%$ that can generate cat states of size $|α|^2=5$ with fidelity $F>0.99$. The protocol relies only on detecting single photons and is remarkably tolerant of loss, with $2\%$ detection loss still achieving $F>0.98$ for cats with $|α|^2=5$. We also show that squeezed $θ$ states are ideal candidates for nonlinear photon subtraction using a two-level system with near deterministic success probability and fidelity $F>0.98$ for cat states of size $|α|^2=5$. Schemes for generating $θ$ states using quantum emitters are also presented. Our protocols can be implemented with current state-of-the-art quantum optics experiments.

quant-ph↗

arXiv2026

Quantifying Pauli Errors in Single-Photon Resource-State Generation

We propose a scheme to compute Pauli error rates in photonics-based quantum error correction using experimental observables of single photons produced from quantum emitters. We show that first-order coherence measurements and first-order cross correlations, which can be implemented using photon counting, can extract single-photon and entangled single-photon wavefunctions in the presence of imperfections due to photon distinguishability, laser noise, and photon loss. Leveraging this, we show that the wavefunction of any entangled state of noisy photons produced from a single quantum emitter can be expressed in matrix-product-state form and can be used to analytically compute the expectation value of the stabilizer generators of the corresponding entangled state. From this we obtain analytic expressions for the Pauli error probabilities in terms of the photon noise parameters. Furthermore, we calculate Pauli error maps for entangled photons after undergoing Bell- state measurements in terms of these parameters. Our work provides a method to use experimental measurements to determine the required quality of photons produced from quantum emitters for fault-tolerant fusion-based photonics quantum computing.

quant-ph↗

arXiv2026

Theory of Three-Photon Transport Through a Weakly Coupled Atomic Ensemble

Understanding multi-photon interactions in non-equilibrium quantum systems is an outstanding challenge in quantum optics. In this work, we develop an analytical and diagrammatic framework to explore three-photon interactions in atomic ensembles weakly coupled to a one-dimensional waveguide. Taking advantage of the weak coupling, we use our diagrammatic framework to perform perturbation theory and calculate the leading-order contributions to the three-photon wavefunction, which would otherwise be intractable. We then compute the outgoing photon wavefunction of a resonantly driven atomic ensemble, with photon-photon interactions truncated up to three photons. Our formulation not only captures the individual transmission of photons but also isolates the connected S-matrix elements that embody genuine photon-photon correlations. Through detailed analysis, we obtain the analytic expressions of the connected third-order correlation function and the third-order electric-field-quadrature cumulant, which reveal non-Gaussian signatures emerging from the interplay of two- and three-photon processes. We also calculate the optical depth where non-Gaussian photon states can be observed. Numerical simulations based on a cascaded master equation validate our analytical predictions on a small-scale system. These results provide a formalism to further explore non-equilibrium quantum optics in atomic ensembles and extend this to the regime of non-Gaussian photon transport.

quant-ph↗

arXiv2026

Non-Gaussian Photon Correlations in Weakly Coupled Atomic Ensembles

We develop a scattering theory formalism and use it to predict that a resonantly driven atomic ensemble weakly coupled to an optical mode can generate light with non-Gaussian correlations. Our approach -- based on a perturbative diagrammatic expansion of multi-photon interactions -- shows that photon-photon interaction mediated by the emitters causes the transmitted light to have a non-vanishing connected third-order correlation function $g_c^{(3)}$. We explain the temporal pattern of $g_c^{(3)}$ using the interaction processes in our diagrammatic expansion. A quantitative comparison with cascaded master equation simulations for small ensembles with optical depth $\mathrm{OD}\leq 2$ confirms that the perturbative results remain accurate across experimentally relevant optical depths and for drive strengths large enough to make the predicted non-Gaussian signatures detectable. We anticipate that state-of-the-art nanofibre-coupled atomic ensembles can experimentally demonstrate our predictions.

quant-ph↗

arXiv2025

Emergence of unidirectionality and phase separation in optically dense emitter ensembles

The transmission of light through an ensemble of two-level emitters in a one-dimensional geometry is commonly described by one of two emblematic models of quantum electrodynamics (QED): the driven-dissipative Dicke model or the Maxwell-Bloch equations. Both exhibit distinct features of phase transitions and phase separations, depending on system parameters such as optical depth and external drive strength. Here, we explore the crossover between these models via a parent spin model from bidirectional waveguide QED, by varying positional disorder among emitters. Solving mean-field equations and employing a second-order cumulant expansion for the unidirectional model -- equivalent to the Maxwell-Bloch equations -- we study phase diagrams, the emitter's inversion, and transmission depending on optical depth, drive strength, and spatial disorder. We find in the thermodynamic limit the emergence of phase separation with a critical value that depends on the degree of spatial order but is independent of Doppler broadening effects. Even far from the thermodynamic limit, this critical value marks a special point in the emitter's correlation landscape of the unidirectional model and is also observed as a maximum in the magnitude of inelastically transmitted photons. We conclude that a large class of effective one-dimensional systems without tight control of the emitter's spatial ordering can be effectively modeled using a unidirectional waveguide approach.

quant-ph↗

arXiv2025

Using matrix-product states for time-series machine learning

Matrix-product states (MPS) have proven to be a versatile ansatz for modeling quantum many-body physics. For many applications, and particularly in one-dimension, they capture relevant quantum correlations in many-body wavefunctions while remaining tractable to store and manipulate on a classical computer. This has motivated researchers to also apply the MPS ansatz to machine learning (ML) problems where capturing complex correlations in datasets is also a key requirement. Here, we develop and apply an MPS-based algorithm, MPSTime, for learning a joint probability distribution underlying an observed time-series dataset, and show how it can be used to tackle important time-series ML problems, including classification and imputation. MPSTime can efficiently learn complicated time-series probability distributions directly from data, requires only moderate maximum MPS bond dimension $χ_{\rm max}$, with values for our applications ranging between $χ_{\rm max} = 20-160$, and can be trained for both classification and imputation tasks under a single logarithmic loss function. Using synthetic and publicly available real-world datasets, spanning applications in medicine, energy, and astronomy, we demonstrate performance competitive with state-of-the-art ML approaches, but with the key advantage of encoding the full joint probability distribution learned from the data, which is useful for analyzing and interpreting its underlying structure. This manuscript is supplemented with the release of a publicly available code package MPSTime that implements our approach. The effectiveness of the MPS-based ansatz for capturing complex correlation structures in time-series data makes it a powerful foundation for tackling challenging time-series analysis problems across science, industry, and medicine.

stat.ML↗

arXiv2023

Broadband terahertz near-field excitation and detection of silicon photonic crystal modes

Chip-based terahertz (THz) devices are emerging as versatile tools for manipulating mm-wave frequencies in the context of integrated high-speed communication technologies for potential sixth-generation (6G) wireless applications. The characterization of THz devices is typically performed using far-field techniques that provide limited information about the underlying physical mechanisms producing them. As the library of chip-based functionalities expands, e.g., for tailoring the emission and directional propagation properties of THz antennas and waveguides, novel characterization techniques will likely be beneficial for observing subtle effects that are sensitive to a device's structural parameters. Here we present near-field measurements showing the emission properties of a broadband THz emitter placed in the vicinity of a photonic crystal (PHC) slab. These experiments reveal long-predicted emission properties, but which to our knowledge have yet to be experimentally observed at THz frequencies. We demonstrate three distinct effects between 0.3-0.5 THz: (i) field suppression at frequencies corresponding to quasi-TE bandgaps (ii) a frequency-dependent directed emission along two distinct pathways for two neighboring frequencies, resulting in a local field concentration; (iii) a re-direction of the emission, achieved by rotating the PHC with respect to the dipole orientation. Simulations reveal that the observed behavior can be predicted from the underlying band structure. Our results highlight the opportunities that PHCs can potentially provide for alignment-free, chip-based 6G technologies. Our experimental technique extends the applicability realms of THz spectroscopy and will find use for characterizing the THz modes supported by true samples, whose inherent imperfections cannot realistically be accounted for by simulations, particularly in highly dispersive frequency bands.

physics.optics↗

arXiv2022

Higher-order mean-field theory of chiral waveguide QED

Waveguide QED with cold atoms provides a potent platform for the study of non-equilibrium, many-body, and open-system quantum dynamics. Even with weak coupling and strong photon loss, the collective enhancement of light-atom interactions leads to strong correlations of photons arising in transmission, as shown in recent experiments. Here we apply an improved mean-field theory based on higher-order cumulant expansions to describe the experimentally relevant, but theoretically elusive, regime of weak coupling and strong driving of large ensembles. We determine the transmitted power, squeezing spectra and the degree of second-order coherence, and systematically check the convergence of the results by comparing expansions that truncate cumulants of few-particle correlations at increasing order. This reveals the important role of many-body and long-range correlations between atoms in steady state. Our approach allows to quantify the trade-off between anti-bunching and output power in previously inaccessible parameter regimes. Calculated squeezing spectra show good agreement with measured data, as we present here.

quant-ph↗

arXiv2022

Direct observation of photon bound states using a single artificial atom

The interaction between photons and a single two-level atom constitutes a fundamental paradigm in quantum physics. The nonlinearity provided by the atom means that the light-matter interaction depends strongly on the number of photons interacting with the two-level system within its emission lifetime. This nonlinearity results in the unveiling of strongly correlated quasi-particles known as photon bound states, giving rise to key physical processes such as stimulated emission and soliton propagation. While signatures consistent with the existence of photon bound states have been measured in strongly interacting Rydberg gases, their hallmark excitation-number-dependent dispersion and propagation velocity have not yet been observed. Here, we report the direct observation of a photon-number-dependent time delay in the scattering off a single semiconductor quantum dot coupled to an optical cavity. By scattering a weak coherent pulse off the cavity-QED system and measuring the time-dependent output power and correlation functions, we show that single photons, and two- and three-photon bound states incur different time delays of 144.02\,ps, 66.45\,ps and 45.51\,ps respectively. The reduced time delay of the two-photon bound state is a fingerprint of the celebrated example of stimulated emission, where the arrival of two photons within the lifetime of an emitter causes one photon to stimulate the emission of the other from the atom.

quant-ph↗

arXiv2021

Unraveling two-photon entanglement via the squeezing spectrum of light traveling through nanofiber-coupled atoms

We observe that a weak guided light field transmitted through an ensemble of atoms coupled to an optical nanofiber exhibits quadrature squeezing. From the measured squeezing spectrum we gain direct access to the phase and amplitude of the energy-time entangled part of the two-photon wavefunction which arises from the strongly correlated transport of photons through the ensemble. For small atomic ensembles we observe a spectrum close to the lineshape of the atomic transition, while sidebands are observed for sufficiently large ensembles, in agreement with our theoretical predictions. Furthermore, we vary the detuning of the probe light with respect to the atomic resonance and infer the phase of the entangled two-photon wavefunction. From the amplitude and the phase of the spectrum, we reconstruct the real- and imaginary part of the time-domain wavefunction. Our characterization of the entangled two-photon component constitutes a diagnostic tool for quantum optics devices.

quant-ph↗

arXiv2020

Dynamics of many-body photon bound states in chiral waveguide QED

We theoretically study the few- and many-body dynamics of photons in chiral waveguides. In particular, we examine pulse propagation through a system of $N$ two-level systems chirally coupled to a waveguide. We show that the system supports correlated multi-photon bound states, which have a well-defined photon number $n$ and propagate through the system with a group delay scaling as $1/n^2$. This has the interesting consequence that, during propagation, an incident coherent state pulse breaks up into different bound state components that can become spatially separated at the output in a sufficiently long system. For sufficiently many photons and sufficiently short systems, we show that linear combinations of $n$-body bound states recover the well-known phenomenon of mean-field solitons in self-induced transparency. For longer systems, however, the solitons break apart through quantum correlated dynamics. Our work thus covers the entire spectrum from few-photon quantum propagation, to genuine quantum many-body (atom and photon) phenomena, and ultimately the quantum-to-classical transition. Finally, we demonstrate that the bound states can undergo elastic scattering with additional photons. Together, our results demonstrate that photon bound states are truly distinct physical objects emerging from the most elementary light-matter interaction between photons and two-level emitters. Our work opens the door to studying quantum many-body physics and soliton physics with photons in chiral waveguide QED.

quant-ph↗

arXiv2019

A wave-function ansatz method for calculating field correlations and its application to the study of spectral filtering and quantum dynamics of multi-emitter systems

We develop a formalism based on a time-dependent wave-function ansatz to study correlations of photons emitted from a collection of two-level quantum emitters. We show how to simulate the system dynamics and evaluate the intensity of the scattered photons and the second-order correlation function $g^{(2)}$ in terms of the amplitudes of the different components of the wave function. Our approach is efficient for considering systems that contain up to two excitations. To demonstrate this we first consider the example of spectral filtering of photons emitted from a single quantum emitter. We show how our formalism can be used to study spectral filtering of the two-photon component of the emitted light from a single quantum emitter for various kinds of filters. Furthermore, as a general application of our formalism, we show how it can be used to study photon-photon correlations in an optically dense ensemble of two-level quantum emitters. In particular we lay out the details of simulating correlated photon transport in such ensembles reported recently by S. Mahmoodian {\it et.al.} [Phys. Rev. Lett. {\bf 121}, 143601 (2018)]. Compared to other existing techniques, the advantage of our formalism is that it is applicable to any generic spectral filter and quantum many-body systems involving a large number of quantum emitters while requiring only a modest computational resource.

quant-ph↗

arXiv2019

Correlating photons using the collective nonlinear response of atoms weakly coupled to an optical mode

Photons in a nonlinear medium can repel or attract each other, resulting in a strongly correlated quantum many-body system. Typically, such strongly correlated states of light arise from the extreme nonlinearity granted by quantum emitters that are strongly coupled to a photonic mode. However, in these approaches, unavoidable dissipation, like photon loss, blurs nonlinear quantum effects. Here, we generate strongly correlated photon states using only weak coupling and taking advantage of dissipation. We launch light through an ensemble of non-interacting waveguide-coupled atoms, which induce correlations between simultaneously arriving photons through collectively enhanced nonlinear interactions. These correlated photons then experience less dissipation than the uncorrelated ones. Depending on the number of atoms, we experimentally observe strong photon bunching or anti-bunching of the transmitted light. This realization of a collectively enhanced nonlinearity may turn out transformational for quantum information science and opens new avenues for generating nonclassical light, covering frequencies from the microwave to the X-ray regime.

quant-ph↗

arXiv2019

Chiral Light--Matter Interaction Beyond the Rotating-Wave Approximation

I introduce and analyse chiral light--matter interaction in the ultrastrong coupling limit where the rotating-wave approximation cannot be made. Within this limit, a two-level system (TLS) with a circularly polarized transition dipole interacts with a copolarized mode through rotating-wave terms. However, the counter-rotating terms allow the TLS to couple to a counter-polarized mode with the same coupling strength, i.e., one that is completely decoupled within the rotating-wave approximation. Although such a Hamiltonian is not particle number conserving, the conservation of angular momentum generates a $U(1)$ symmetry which allows constructing an ansatz. The eigenstates and dynamics of this novel model are computed for single-cavity interactions and for a many-mode system. The form of the ansatz provides significant analytic insight into the physics of the ground state and the dynamics, e.g., it indicates that the ground states are two-mode squeezed. This work has significant implications for engineering light--matter interaction and novel quantum many-body dynamics beyond the rotating-wave approximation.

quant-ph↗

arXiv2018

Spatially Adiabatic Frequency Conversion in Optoelectromechanical Arrays

Faithful conversion of quantum signals between microwave and optical frequency domains is crucial for building quantum networks based on superconducting circuits. Optoelectromechanical systems, in which microwave and optical cavity modes are coupled to a common mechanical oscillator, are a promising route towards this goal. In these systems, efficient, low-noise conversion is possible using a mechanically dark mode of the fields but the conversion bandwidth is limited to a fraction of the cavity linewidth. Here, we show that an array of optoelectromechanical transducers can overcome this limitation and reach a bandwidth that is larger than the cavity linewidth. The coupling rates are varied in space throughout the array so that the mechanically dark mode of the propagating fields adiabatically changes from microwave to optical or vice versa. This strategy also leads to significantly reduced thermal noise with the collective optomechanical cooperativity being the relevant figure of merit. Finally, we demonstrate that, quite surprisingly, the bandwidth enhancement per transducer element is largest for small arrays; this feature makes our scheme particularly attractive for state-of-the-art experimental setups.

quant-ph↗

arXiv2018

Strongly correlated photon transport in waveguide QED with weakly coupled emitters

We show that strongly correlated photon transport can be observed in waveguides containing optically dense ensembles of emitters. Remarkably, this occurs even for weak coupling efficiencies. Specifically, we compute the photon transport properties through a chirally coupled system of $N$ two-level systems driven by a weak coherent field, where each emitter can also scatter photons out of the waveguide. The photon correlations arise due to an interplay of nonlinearity and coupling to a loss reservoir, which creates a strong effective interaction between transmitted photons. The highly correlated photon states are less susceptible to losses than uncorrelated photons and have a power-law decay with $N$. This is described using a simple universal asymptotic solution governed by a single scaling parameter which describes photon bunching and power transmission. We show numerically that, for randomly placed emitters, these results hold even in systems without chirality. The effect can be observed in existing tapered fiber setups with trapped atoms.

quant-ph↗

arXiv2017

Spin-photon interface and spin-controlled photon switching in a nanobeam waveguide

Access to the electron spin is at the heart of many protocols for integrated and distributed quantum-information processing [1-4]. For instance, interfacing the spin-state of an electron and a photon can be utilized to perform quantum gates between photons [2,5] or to entangle remote spin states [6-9]. Ultimately, a quantum network of entangled spins constitutes a new paradigm in quantum optics [1]. Towards this goal, an integrated spin-photon interface would be a major leap forward. Here we demonstrate an efficient and optically programmable interface between the spin of an electron in a quantum dot and photons in a nanophotonic waveguide. The spin can be deterministically prepared with a fidelity of 96\%. Subsequently the system is used to implement a "single-spin photonic switch", where the spin state of the electron directs the flow of photons through the waveguide. The spin-photon interface may enable on-chip photon-photon gates [2], single-photon transistors [10], and efficient photonic cluster state generation [11].

quant-ph↗