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Salvatore Savasta

Publications and source records attributed to Salvatore Savasta.

At least 19 recordsLinked to original sources

Non-Hermitian Quantum Nonlinear Optics with Single Photons

Quantum nonlinear optics seeks to harness strong photon-photon interactions for scalable quantum technologies, although dissipative losses still pose a major barrier to near-unity conversion efficiency. Here, we bridge non-Hermitian physics with the quantum nonlinear domain by exploiting perfect absorption to identify and optimize few-photon nonlinear processes. We theoretically investigate two circuit QED systems, operating in the light-matter ultrastrong coupling regime. The first (i) enables simultaneous two-atom excitations by single photons, while the second (ii) realizes the strong coupling between a single-photon and a two-photon Fock states. We demonstrate that, since the strong optical nonlinearities cause quantum spectral features to emerge already at the level of linear response theory, the perfect absorption condition in $|S_{11}|$ enables near-deterministic single-photon down-conversion into (i) a qubit-qubit-correlated pair and (ii) a two-photon pair. We show that the conversion efficiency can be systematically optimized through experimentally accessible parameters, both linked to the emergence of Hermitian subspaces within the effective non-Hermitian Hamiltonians. These findings position non-Hermitian engineering as a broadly applicable route to optimizing quantum devices at the single-photon level, even beyond circuit-QED platforms.

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Interplay between photon condensation and electron-electron interactions in molecular systems

We investigate a minimal molecular model consisting of square planar plaquettes hosting multiple electrons, whose dynamics is governed by a tight-binding Hamiltonian supplemented by on-site Hubbard repulsion. By coupling this system to a spatially nonuniform cavity mode, we analyze the emergence of a magnetostatic instability, namely photon condensation, originating from the paramagnetic Van Vleck mechanism. The global behavior of the system is analyzed for different electronic filling factors, and we find that, except for the special cases of half-filling and single electron, where the transition, if it occurs, is necessarily a second order phase transition, the global system may also undergo a first order transition because of the action of the electron-electron interaction. The polaritonic excitation energies are analyzed, providing clear spectroscopic signatures of the magnetostatic instability and of its order.

cond-mat.mes-hall↗

Quantum Vacuum Radiation Near a Critical Point

Equilibrium quantum phase transitions profoundly reshape the ground state of light-matter systems; yet, the resulting quantum correlations, such as squeezing and entanglement, remain experimentally inaccessible since they involve virtual ground state excitations. We investigate how a nonadiabatic modulation of a Hamiltonian parameter can convert these virtual excitations into real photons, enabling quantum vacuum radiation. We show that proximity to the critical point strongly enhances the emitted photon flux and the non-classical nature of the emitted radiation, even when thermal fluctuations are expected to dominate. In addition, higher-order processes become relevant even for small modulation amplitudes, and we develop a framework that systematically incorporates them. Our results reveal that criticality can act as an efficient amplifier of vacuum fluctuations, offering new routes to probe and exploit quantum critical ground states.

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Superradiant Quantum Phase Transition in Open Systems: System-Bath Interaction at the Critical Point

The occurrence of a second-order quantum phase transition in the Dicke model is a well-established feature. On the contrary, a comprehensive understanding of the corresponding open system, particularly in the proximity of the critical point, remains elusive. When approaching the critical point, the system inevitably enters first the system-bath ultrastrong coupling regime and finally the deepstrong coupling regime, causing the failure of usual approximations adopted to describe open quantum systems. We study the interaction of the Dicke model with bosonic bath fields in the absence of additional approximations, which usually relies on the weakness of the system-bath coupling. We find that the critical point is not affected by the interaction with the environment. Moreover, the interaction with the environment is not able to affect the system ground-state condensates in the superradiant phase, whereas the bath fields are infected by the system and acquire macroscopic occupations. The obtained reflection spectra display lineshapes which become increasingly asymmetric, both in the normal and superradiant phases, when approaching the critical point.

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Strong coupling between a single-photon and a two-photon Fock state

The realization of strong nonlinear coupling between single photons has been a long-standing goal in quantum optics and quantum information science, promising wide impact applications, such as all-optical deterministic quantum logic and single-photon frequency conversion. Here, we report an experimental observation of the strong coupling between a single-photon and a two-photon Fock state in an ultrastrongly-coupled circuit-QED system. This strong nonlinear interaction is realized by introducing a detuned flux qubit working as an effective coupler between two modes of a superconducting coplanar waveguide resonator. The ultrastrong light--matter interaction breaks the excitation number conservation, and an external flux bias breaks the parity conservation. The combined effect of the two enables the strong one--two-photon coupling. Quantum Rabi-like avoided crossing is resolved when tuning the two-photon resonance frequency of the first mode across the single-photon resonance frequency of the second mode. Within this new photonic regime, we observe the thresholdless second harmonic generation for a mean photon number below one. Our results represent a key step towards a new regime of quantum nonlinear optics, where individual photons can deterministically and coherently interact with each other in the absence of any stimulating fields.

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Noise Protected Logical Qubit in a Open Chain of Superconducting Qubits with Ultrastrong Interactions

To achieve a fault-tolerant quantum computer, it is crucial to increase the coherence time of quantum bits. In this work, we theoretically investigate a system consisting of a series of superconducting qubits that alternate between XX and YY ultrastrong interactions. By considering the two-lowest energy eigenstates of this system as a {\it logical} qubit, we demonstrate that its coherence is significantly enhanced: both its pure dephasing and relaxation times are extended beyond those of individual {\it physical} qubits. Specifically, we show that by increasing either the interaction strength or the number of physical qubits in the chain, the logical qubit's pure dephasing rate is suppressed to zero, and its relaxation rate is reduced to half the relaxation rate of a single physical qubit. Single qubit and two-qubit gates can be performed with a high fidelity.

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Observation of Perfect Absorption in Hyperfine Levels of Molecular Spins with Hermitian Subspaces

We investigate Perfect Absorption (PA) of radiation, in which incoming energy is entirely dissipated, in a system consisting of molecular spin centers coherently coupled to a planar microwave resonator operated at milliKelvin temperature and in the single photon regime. This platform allows us to fine tune the spin-photon coupling and to control the effective dissipation of the two subsystems towards the environment, thus giving us the opportunity to span over a wide space of parameters. Our system can be effectively described by a non-Hermitian Hamiltonian exhibiting distinct Hermitian subspaces. We experimentally show that these subspaces, linked to the presence of PA, can be engineered through the resonator-spin detuning, which controls the composition of the polaritons in terms of photon and spin content. In such a way, the required balance between the feeding and the loss rates is effectively recovered even in the absence of PT-symmetry. We show that Hermitian subspaces influence the overall aspect of coherent spectra of cavity QED systems and enlarge the possibility to explore non-Hermitian effects in open quantum systems. We finally discuss how our results can be potentially exploited for applications, in particular as single-photon switches and modulators.

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From Few to Many Emitters Cavity QED: Energy Levels and Emission Spectra From Weak to Deep-Strong Coupling

We present a systematic study of the properties of systems composed of $N$ two-level quantum emitters coupled to a single cavity mode, for light-matter interaction strengths ranging from the weak to the ultrastrong and deep-strong coupling regimes. Beginning with an analysis of the energy spectrum as a function of the light-matter coupling strength, we examine systems with varying numbers of emitters, from a pair to large collections, approaching the thermodynamic limit ($N \to \infty$). Additionally, we explore the emission properties of these systems under incoherent excitation of the emitters, employing a general theoretical framework for open cavity-QED systems, which is valid across all light-matter interaction regimes and preserves gauge invariance within truncated Hilbert spaces. Furthermore, we study the influence of the emitter-environment interaction on the spectral properties of the system. Specifically, when each emitter interacts independently with its own reservoir, we observe the emergence of an emission peak at the cavity's resonant frequency for even values of $N$. Our analysis also clarify the evolution of the system as the number of emitters increases, ultimately converging towards an equivalent system composed of two interacting single-mode bosonic fields.

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Renormalization and Low-Energy Effective Models in Cavity and Circuit QED

The quantum Rabi model (QRM) is a cornerstone in the study of light-matter interactions within cavity and circuit quantum electrodynamics (QED). It effectively captures the dynamics of a two-level system coupled to a single-mode resonator, serving as a foundation for understanding quantum optical phenomena in a great variety of systems. However, this model may produce inaccurate results for large coupling strengths, even in systems with high anharmonicity. Moreover, issues of gauge invariance further undermine its reliability. In this work, we introduce a renormalized QRM that incorporates the effective influence of higher atomic energy levels, providing a significantly more accurate representation of the system while still maintaining a two-level description. To demonstrate the versatility of this approach, we present two different examples: an atom in a double-well potential and a superconducting artificial atom (fluxonium qubit). This procedure opens new possibilities for precisely engineering and understanding cavity and circuit QED systems, which are highly sought-after, especially for quantum information processing.

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Bilateral photon emission from a vibrating mirror and multiphoton entanglement generation

Entanglement plays a crucial role in the development of quantum-enabled devices. One significant objective is the deterministic creation and distribution of entangled states, achieved, for example, through a mechanical oscillator interacting with confined electromagnetic fields. In this study, we explore a cavity resonator containing a two-sided perfect mirror. Although the mirror separates the cavity modes into two independent confined electromagnetic fields, the radiation pressure interaction gives rise to high-order effective interactions across all subsystems. Depending on the chosen resonant conditions, which are also related to the position of the mirror, we study $2n$-photon entanglement generation and bilateral photon pair emission. Demonstrating the non-classical nature of the mechanical oscillator, we provide a pathway to control these phenomena, opening potential applications in quantum technologies. Looking ahead, similar integrated devices could be used to entangle subsystems across vastly different energy scales, such as microwave and optical photons.

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Circuit QED Spectra in the Ultrastrong Coupling Regime: How They Differ from Cavity QED

Cavity quantum electrodynamics (QED) studies the interaction between resonator-confined radiation and natural atoms or other formally equivalent quantum excitations, under conditions where the quantum nature of photons is relevant. Phenomena studied in cavity QED can also be explored using superconducting artificial atoms and microwave photons in superconducting resonators. These circuit QED systems offer the possibility to reach the ultrastrong coupling regime with individual artificial atoms, unlike their natural counterparts. In this regime, the light-matter coupling strength reaches a considerable fraction of the bare resonance frequencies in the system. Here, we provide a careful analysis of both incoherent and coherent spectra in circuit QED systems consisting of a flux qubit interacting with an LC resonator. Despite these systems can be effectively described by the quantum Rabi model, as the corresponding cavity QED ones, we find distinctive features, depending on how the system is coupled to the output port, which become evident in the ultrastrong coupling regime.

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Phonon Pumping by Modulating the Ultrastrong Vacuum

The vacuum (i.e., the ground state) of a system in ultrastrong light-matter coupling contains particles that cannot be emitted without any dynamical perturbation and is thus called virtual. We propose a protocol for inducing and observing real mechanical excitations of a mirror enabled by the virtual photons in the ground state of a tripartite system, where a resonant optical cavity is ultrastrongly coupled to a two-level system (qubit) and, at the same time, optomechanically coupled to a mechanical resonator. Real phonons are coherently emitted when the frequency of the two-level system is modulated at a frequency comparable to that of the mechanical resonator and, therefore much lower than the optical frequency. We demonstrate that this hybrid effect is a direct consequence of the virtual photon population in the ground state. Within a classical physics analogy, attaching a weight to a spring only changes its resting position, whereas dynamically modulating the weight makes the system oscillate. In our case, however, the weight is the vacuum itself. We propose and accurately characterize a hybrid superconducting-optomechanical setup based on available state-of-the-art technology, where this effect can be experimentally observed.

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Quantum Phase Transitions in Many-Dipole Light-Matter Systems

A potential phase transition between a normal ground state and a photon-condensed ground state in many-dipole light-matter systems is a topic of considerable controversy, exasperated by conflicting no-go and counter no-go theorems and often ill-defined models. We clarify this long-lasting debate by analyzing two specific arrangements of atoms, including a 3D cubic lattice and a cavity-embedded square lattice layer, which provides a physical model for single-mode cavity QED with coupled dipoles in the thermodynamic limit. These models are shown to significantly differ from the standard Dicke model and, in the thermodynamic limit, give rise to renormalized Hopfield models. We show that a ferroelectric phase transition can (in principle) still occur and the description of the abnormal phase beyond the critical point requires the inclusion of nonlinear terms in the Holstein-Primakoff mapping. We also show how our model agrees with recent experiments.

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Photon condensation, Van Vleck paramagnetism, and chiral cavities

We introduce a gauge-invariant model of planar, square molecules coupled to a quantized spatially-varying cavity electromagnetic vector potential A(r). Specifically, we choose a temporally chiral cavity hosting a uniform magnetic field B, as this is the simplest instance in which a transverse spatially-varying A(r) is at play. We show that when the molecules are in the Van Vleck paramagnetic regime, an equilibrium quantum phase transition to a photon condensate state occurs.

cond-mat.mes-hall↗

Ultrastrong Magnon-Photon Coupling Achieved by Magnetic Films in Contact with Superconducting Resonators

Coherent coupling between spin wave excitations (magnons) and microwave photons in a cavity may disclose new paths to unconventional phenomena as well as for novel applications. Here, we present a systematic investigation on YIG (Yttrium Iron Garnet) films on top of coplanar waveguide resonators made of superconducting YBCO. We first show that spin wave excitations with frequency higher than the Kittel mode can be excited by putting in direct contact a 5~$μ$m thick YIG film with the YBCO coplanar resonator (cavity frequency $ω_c/2 π= 8.65$~GHz). With this configuration, we obtain very large values of the collective coupling strength $λ/2 π\approx 2$~GHz and cooperativity $C=5 \times 10^4$. Transmission spectra are analyzed by a modified Hopfield model for which we provide an exact solution that allows us to well reproduce spectra by introducing a limited number of free parameters. It turns out that the coupling of the dominant magnon mode with photons exceeds 0.2 times the cavity frequency, thus demonstrating the achievement of the ultrastrong coupling regime with this architecture. Our analysis also shows a vanishing contribution of the diamagnetic term which is a peculiarity of pure spin systems.

cond-mat.mes-hall↗

Probing the symmetry breaking of a light--matter system by an ancillary qubit

Hybrid quantum systems in the ultrastrong, and even more in the deep-strong, coupling regimes can exhibit exotic physical phenomena and promise new applications in quantum technologies. In these nonperturbative regimes, a qubit--resonator system has an entangled quantum vacuum with a nonzero average photon number in the resonator, where the photons are virtual and cannot be directly detected. The vacuum field, however, is able to induce the symmetry breaking of a dispersively coupled probe qubit. We experimentally observe the parity symmetry breaking of an ancillary Xmon artificial atom induced by the field of a lumped-element superconducting resonator deep-strongly coupled with a flux qubit. This result opens a way to experimentally explore the novel quantum-vacuum effects emerging in the deep-strong coupling regime.

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Gauge-Independent Emission Spectra and Quantum Correlations in the Ultrastrong Coupling Regime of Open System Cavity-QED

A quantum dipole interacting with an optical cavity is one of the key models in cavity quantum electrodynamics (cavity-QED). To treat this system theoretically, the typical approach is to truncate the dipole to two levels. However, it has been shown that in the ultrastrong-coupling regime, this truncation naively destroys gauge invariance. By truncating in a manner consistent with the gauge principle, we introduce master equations {for open systems} to compute gauge-invariant emission spectra, photon flux rates, and quantum correlation functions which show significant disagreement with previous results obtained using the standard quantum Rabi model. Explicit examples are shown using both the dipole gauge and the Coulomb gauge.

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Flying atom back-reaction and mechanically generated photons from vacuum

We investigate the dynamics of a two-level atom flying through a photonic cavity when the light-matter interaction is in the ultrastrong coupling regime. We adopt a closed full quantum description that takes into account the quantization of the atom center-of-mass motion in addition to its internal degree of freedom and to the quantized photonic cavity field. We find that multiple qualitatively different dynamical regimes are achievable according to two key figures of merit: the ratio between the kinetic energy and the bare excitation energies, and the product of these bare energies with the time the atom takes to fly through the cavity. According to the values of those figures of merit, the atom can be reflected by the \emph{dressed} vacuum, or can convert part of its kinetic energy into real excitations which might be emitted out of the cavity. In the first case, the atom experiences a \emph{quantum regenerative braking} mechanism, based on temporary storage of energy into virtual excitations.

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