SearcharxivSearch

arXiv subjects

Salvatore Torquato

Publications and source records attributed to Salvatore Torquato.

At least 19 recordsLinked to original sources

Analysis of Conjectural Improvements to Minkowski's Lower Bound on the Sphere Packing Density

Torquato and Stillinger conjectured an exponential improvement of Minkowski's classical lower bound on the maximal density of sphere packings in $\mathbb{R}^d$, with exponential rate $2^{-(0.7786524795\ldots+o(1))d}$, using a pair-correlation-function optimization framework. Conditional on their realizability conjecture, we show that a simple family of hyperuniform pair correlation functions yields polynomial improvements over Minkowski's lower bound of the form $ϕ_{\max}\gtrsim d^β2^{-d}$ for every fixed $β>1$ in the high-$d$ limit. As the polynomial exponent increases with dimension, this family approaches the conjectured exponential improvement. We first give an explicit hyperuniform construction based on Gauss--Radau quadrature. It contains $\lfloor(d-1)/4\rfloor$ positive delta-function shells and has exponential rate $2^{-(0.622556248918\ldots+o(1))d}$, showing how growing radial complexity surpasses the Torquato--Stillinger rate. We then prove strong duality between the unrestricted pair-correlation program and its Cohn--Elkies dual: their optimal values coincide, with no duality gap. Combining this result with approximation by ordinary finite-band functions, we show that the unrestricted pair-correlation program attains the optimal Cohn--Elkies exponential rate $2^{-(0.6044005\ldots+o(1))d}$ in the high-$d$ limit, although this general result does not supply a comparable closed-form family. We further derive the Torquato--Stillinger exponential rate independently from the Cohn--Elkies dual linear-programming upper-bound formulation, showing that its radial objective test functions cannot asymptotically exclude packings with the Torquato--Stillinger density scaling. The agreement between these approaches provides evidence that exceptionally dense disordered sphere packings may exist in high dimensions and supports the Torquato--Stillinger conjectural lower bound.

math-ph

Quantifying translational and bond-orientational order metrics in hyperuniform and nonhyperuniform many-particle systems

Quantifying the degree of order/disorder in many-particle systems remains an outstanding problem in physics, materials science, and mathematics. To this end, we consider the translational order metric $τ_T$, defined as the squared $L^2$ norm of the total correlation function $h(\mathbf{r})$, and introduce its bond-orientational analogue $τ_O$, defined from the weighted total correlation function $h_{\mathbf{f}}(\mathbf{r})$ using local orientational weights (S. Torquato et al., Phys. Rev. X 16, 011042 (2026)). The pair $(τ_T,τ_O)$ places both forms of order on a common two-point statistical footing. We compute both metrics for two nonhyperuniform sphere-packing models in 2D and 3D as functions of packing fraction $ϕ$: 1) equilibrium hard particles and 2) nonequilibrium random sequential addition (RSA) packings. For the nonhyperuniform systems, bond-orientational order remains subdominant along the equilibrium-fluid and RSA configurations; however, its magnitude relative to the translational metric increases near the upper end of the equilibrium-fluid branches, much more strongly in 2D than in 3D, and the two metrics become comparable along the sampled crystal branches. At common packing fractions, equilibrium fluids and RSA packings trace distinct $(τ_T,τ_O)$ trajectories, revealing preparation-dependent differences in structural order. As a representative hyperuniform family, we study 2D disordered stealthy hyperuniform (SHU) ground states for $0<χ<1/2$, where $χ$ is the stealthiness parameter. Within the disordered SHU phase, bond-orientational order remains subdominant, but its magnitude relative to the translational metric increases toward the disorder-to-order threshold. In all three models, $τ_T$ and $τ_O$ are positively correlated beyond the Poisson-reference regime: $τ_O$ increases monotonically with $τ_T$ across the sampled state points.

cond-mat.stat-mech

Structural and physical properties of gyromorphs and disordered stealthy hyperuniform media

Disordered stealthy hyperuniform materials combine liquid-like statistical isotropy with crystal-like homogeneity, suppressed density fluctuations at large length scales, bounded holes, and an isotropic structure factor that vanishes for a finite range of wavevectors. This combination yields unusual physical properties, including optical transparency, effective delocalization, ultrafast spreadability, optimal conductivity, and complete isotropic photonic bandgaps. Gyromorphs, point patterns whose structure factor includes rings of Bragg-like peaks arranged with discrete $G$-fold rotational symmetry, were recently introduced as counterexamples: disordered media that can somehow achieve the same physical properties, in some cases with higher performance, without stealthiness or hyperuniformity. In this paper, we resolve the puzzle of how gyromorphs fit consistently with the stealthy hyperuniform studies. We first show that gyromorphs are actually hyperuniform and, in the large-$G$ limit where they become nearly isotropic, belong to the weakest form of hyperuniformity, known as Class III. Thus, gyromorphs should have comparatively degraded physical properties compared to stealthy hyperuniform media, which belong to the strongest form of hyperuniformity, known as Class I. We verify this expectation using the rigorous spectral Green's matrix method for the calculation of the density of states (DOS) and Purcell factors in large arrays of electric dipoles. We find that gyromorphs display size-dependent pseudogaps richly populated by localized states rather than smooth band gaps like those found for highly stealthy hyperuniform materials or in deterministic structures such as Vogel spiral and triangular lattices. Furthermore, we predict similar disorder-induced degradation relative to stealthy hyperuniformity with regard to transparency, spreadability and diffusion properties.

physics.optics

Inferring stealthy hyperuniform correlations from quantum transport

Stealthy hyperuniform disordered systems exhibit strongly suppressed long-wavelength fluctuations, producing correlated disorder with unusual consequences for wave propagation. A central quantity characterizing these systems is the stealthiness parameter $χ$, which controls the range of excluded Fourier components in the disorder spectrum. However, in realistic settings, the microscopic disorder configuration may not be directly accessible, making it challenging to determine $χ$ from structural information alone. Here, we propose a conductance-based inverse protocol to recover stealthy hyperuniform correlations from transport data. As a proof of concept, we study spinless fermions in a one-dimensional tight-binding chain connected to clean semi-infinite leads, with on-site disorder generated by imposing a stealthy spectrum $S(k)=Θ(|k|-K)$, where $K=2πχ$. The energy-dependent transmittance is computed using a recursive Green's function method and compared with target spectra through a misfit function defined over an energy window. We show that the position of the sharp drop separating high- and low-transmittance regions is strongly controlled by $χ$, while the disorder strength $W$ mainly affects the absolute magnitude of the transmittance. As a result, the misfit function displays a clear minimum close to the target stealthy parameter. Our results demonstrate that transmittance spectra can serve as fingerprints of stealthy hyperuniform disorder, providing a practical route to infer correlated-disorder parameters from transport measurements.

cond-mat.mes-hall

Predictive Formulas for Scattering Mean Free Path for General Disordered Dielectric Media Beyond the Long-Wavelength Regime

We derive predictive formulas for the scattering mean free path $\ell_s$ of statistically homogeneous two-phase dielectric media in dimensions $d=1,2,3$. Unlike Mie-based estimates limited to identical circular or spherical scatterers, the formulas apply to arbitrarily shaped and polydisperse particulate media as well as nonparticulate media, with microstructure entering through the spectral density. The formulas are based on the exact strong-contrast expansion for the effective dynamic dielectric constant. We apply them to five nonhyperuniform and hyperuniform models and validate selected cases using finite-difference time-domain simulations. For $k_1/s \lesssim 1$, where $k_1$ is the incident wavenumber and $s$ is the specific surface, the predictions agree well with simulations and are consistent with Mie theory where applicable, while improving accuracy for two-dimensional transverse-magnetic polarization. Mie estimates become more accurate for $k_1/s \gtrsim 1$. For hyperuniform media with $\widetildeχ_V(k)\sim k^α$ at small $k$, the theory predicts $\ell_s\sim k_1^{-(d+1+α)}$; stealthy hyperuniform media are transparent over a finite wavenumber interval. These results provide a microstructure-based route to predict and design wave transport in general disordered dielectric materials.

cond-mat.dis-nn

Towards stealthy hyperuniform networks with optimal isotropic complete photonic band gaps using a novel inverse design procedure

We present a two-stage inverse design procedure for producing disordered stealthy hyperuniform trivalent photonic networks in two dimensions with isotropic complete photonic band gaps (PBGs) blocking light regardless of direction or polarization (TE or TM) over a wide frequency range. Most ordinary disordered systems fail to maintain complete PBGs as system size increases. The only known exceptions that remain open in the largest simulations have been generated by mapping stealthy hyperuniform point patterns into trivalent networks. However, the resulting networks are not truly stealthy hyperuniform two-phase media. Although their PBGs remain open, they are relatively narrow due to limited overlap between the TE and TM band gaps and broad band tails caused by localized defect states. By contrast, our two-stage inverse design aims to make the final network itself stealthy hyperuniform, achieving unprecedented near-optimal overlap between the TE and TM band gaps and a small defect state density at the band edges. We obtain not only single realizations with large PBGs, but a striking homogeneity across a large ensemble, effectively probing a network with 100,000 vertices. This ensemble-based band gap is comparable in width to the complete PBG of an anisotropic honeycomb photonic crystal with the same network parameters and nearly an order of magnitude wider than the previously widest known isotropic complete PBGs. Our designs can be fabricated using additive manufacturing, offering new pathways to manipulate electromagnetic waves for photonic technologies.

physics.optics

Precise Determination of the Long-Time Asymptotics of the Diffusion Spreadability of Two-Phase Media

The time-dependent diffusion spreadability $\mathcal{S}(t)$ is a powerful dynamical probe of the microstructure of two-phase heterogeneous media across length scales [Torquato, S., \emph{Phys. Rev. E.}, 104 054102 (2021)]. It has been shown that when the spectral density takes the power-law form $\tildeχ_{_V}(\mathbf{k})\sim |\mathbf{k}|^α$ as the wavenumber $|\mathbf{k}|$ tends to zero, the normalized excess spreadability $\mathscr{s}^{ex}(t)$ [proportional to $\mathcal{S}(\infty)-\mathcal{S}(t)$] scales as $\mathscr{s}^{ex}(t)\sim t^{-\frac{d+α}{2}}$ in the long-time limit $t\to\infty$, enabling one to determine the infinite-wavelength scaling exponent $α$. An algorithm that allows one to reliably extract the exponent $α$ from long-time spreadability data was previously devised [Wang, H., Torquato, S., \emph{Phys. Rev. Appl.}, 17 034022 (2022)]. In this paper, we further improve this procedure to obtain $α$ even more accurately by incorporating higher-order correction terms to the long-time asymptotics and by utilizing analyticity properties of $\tildeχ_{_V}(k)$ at the origin. We illustrate our procedure by analyzing hyperuniform ($α> 0$), typical nonhyperuniform ($α=0$), and antihyperuniform ($-d < α<0$) models of two-phase media. In addition, by combining the large-$t$ asymptotic expansion of $\mathscr{s}^{ex}(t)$ with the small-$t$ expansion, we have devised a two-point Padé approximant to approximate $\mathscr{s}^{ex}(t)$ for all $t$ with just a few parameters. Our findings facilitate the characterization of the microstructure of two-phase media across length scales as obtained from numerical spreadability data or experimental data obtained from NMR relaxation measurements. Our work can also be applied in the inverse design of two-phase microstructures with targeted spreadability behaviors.

cond-mat.mtrl-sci

Two-dimensional stealthy hyperuniform polycrystalline disk packings

Polycrystals consist of grains of local crystalline order separated by grain boundaries. Their structure is not hyperuniform, even though perfect crystals are, because polycrystals consist of randomly sized and oriented grains that generate appreciable long-wavelength density fluctuations. In this paper, we use a collective-coordinate optimization procedure to generate two-dimensional polycrystalline packings composed of identical disks arranged in a pattern that is ultradense, stealthy, and hyperuniform (hereafter named SHU). We compare them with polycrystalline disk packings obtained via a modified Lubachevsky--Stillinger rapid compression algorithm (hereafter named LS), a molecular dynamics protocol that serves as a standard reference model describing realistic, nonhyperuniform polycrystalline microstructures. We carry out an extensive comparison of polycrystalline SHU and LS packings that includes differences in two-point statistics, grain size, specific surface area, diffusion spreadability, and optical response as quantified by the imaginary part of the effective dynamic dielectric constant. We find that the polycrystalline SHU packings exhibit a distinctive grain-size distribution, a consequence of long-range correlations between different grains that is absent in the nonhyperuniform case. Within the nonlocal strong-contrast expansion, we confirm that polycrystalline SHU packings made of dielectric material are perfectly transparent to electromagnetic waves at small wave vectors, in contrast to LS packings. Moreover, polycrystalline SHU packings offer enhanced diffusion spreadability. Although polycrystalline SHU packings are not expected to form spontaneously in nature, they may be created for applications as metamaterials via nanolithography or 3D printing that take advantage of their distinctive optical and transport properties.

cond-mat.mtrl-sci

Percolation and Criticality in Hyperuniform Networks

Hyperuniform many-particle systems, which encompass crystals, quasicrystals and certain exotic disordered systems, exhibit an anomalous suppression of density fluctuations on macroscopic length scales relative to those of conventional disordered systems. Here we investigate the percolation behaviors of disordered stealthy hyperuniform systems (SHU), a subclass of hyperuniform configurations for which the structure factor vanishes for a finite range of wavevectors near the origin, with the degree of stealthiness controlled via a parameter $χ$. We construct Delaunay triangulation networks derived from SHU configurations with varying $χ$ as well as Poisson point configurations for the purpose of comparison. We investigate a non-uniform bond percolation process, in which bond occupation probabilities decrease with the Euclidean distance between the connected vertices. In this setting, percolation is induced by varying a tuning parameter $z$. We estimate the percolation thresholds $z_c$ and critical exponents of the networks via finite-size scaling and the Newman-Ziff algorithm. We find that SHU networks exhibit lower percolation thresholds than Poisson networks. Notably, the percolation threshold of SHU networks decreases with the stealthiness parameter $χ$, indicating that global connectivity emerges more readily as short-range order increases. Moreover, we show that SHU networks with large $χ$ belong to the same universality class as lattices, while Poisson and low-$χ$ systems show deviations. We relate the shift in critical exponents to the degree of suppression of density fluctuations in the point configurations. Our work extends previous studies on transport properties of SHU systems from continuum two-phase media to networks. These results open new avenues for optimizing the resilience of statistically homogeneous disordered networks.

cond-mat.stat-mech

Hyperuniformity of Weighted Particle Systems

Hyperuniform particle arrangements are characterized by a local number variance that grows more slowly than the volume of the observation window. We generalize this concept to describe particle systems in which particles carry weights: internal degrees of freedom such as scalars, vectors, pseudovectors, directors, tensors, or extrinsic local attributes. Our generalization extends hyperuniformity from fluctuations in particle positions to fluctuations in the spatial distribution of weights. We derive generalized weighted pair correlation, autocovariance, and spectral functions, and show their relation to the local variance in weighted many-particle systems. Applying this formalism to bond-orientational ordered phases, dipolar liquid water, Voronoi-cell volumes, and certain ionic liquids, we demonstrate that hyperuniformity in the particle system does not necessarily translate to hyperuniformity of the weighted system. In fact, cases exist where a hyperuniform particle system becomes antihyperuniform when weighted, and others where nonhyperuniform or antihyperuniform particle systems yield hyperuniform weighted systems. This theoretical framework provides a road map for quantifying large-scale fluctuations in weighted many-particle systems, offering a powerful tool for identifying systems with novel physical properties.

cond-mat.stat-mech

Communication: Modeling layered mosaic perovskite alloy microstructures across length scales via a packing algorithm

Layered "mosaic" metal-halide perovskite materials display a wide-variety of microstructures that span the order-disorder spectrum and can be tuned via the composition of their constituent B-site octahedral species. Such materials are typically modeled using computationally expensive ab initio methods, but these approaches are greatly limited to small sample sizes. Here, we develop a highly efficient hard-particle packing algorithm to model large samples of these layered complex alloys that enables an accurate determination of the geometrical and topological properties of the B-site arrangements within the plane of the inorganic layers across length scales. Our results are in good agreement with various experiments, and therefore our algorithm bypasses the need for full-blown ab initio calculations. The accurate predictive power of our algorithm demonstrates how our minimalist hard-particle model effectively captures complex interactions and dynamics like incoherent thermal motion, out of plane octahedral tilting, and bond compression/stretching. We specifically show that the composition-dependent miscibility predicted by our algorithm for certain silver-iron and copper-indium layered alloys are consistent with previous experimental observations. We further quantify the degree of mixing in the simulated structures across length scales using our recently developed sensitive "mixing" metric. The large structural snapshots provided by our algorithm also shed light on previous experimentally measured magnetic properties of a copper-indium system. The generalization of our algorithm to model 3D perovskite alloys is also discussed. In summary, our packing model and mixing metric enable one to accurately explore the enormous space of hypothetical layered mosaic alloy compositions and identify materials with potentially desirable optoelectronic and magnetic properties.

cond-mat.mtrl-sci

Effective delocalization in the one-dimensional Anderson model with stealthy disorder

We study analytically and numerically the Anderson model in one dimension with "stealthy" disorder, defined as having a power spectrum that vanishes in a continuous band of wave numbers. Motivated by recent studies on the optical transparency properties of stealthy hyperuniform layered media, we compute the localization length using a perturbative expansion of the self-energy. We find that, for fixed energy and small but finite disorder strength $W$, there exists for any finite length system a range of stealthiness $χ$ for which the localization length exceeds the system size. This kind of "effective delocalization" is the result of the novel kind of correlated disorder that spans a continuous range of length scales, a defining characteristic of stealthy systems. Unlike uncorrelated disorder, for which the localization length $ξ$ scales as $W^{-2}$ to leading order for small W, the leading order terms in the perturbation expansion of $ξ$ for stealthy disordered systems vanish identically for a progressively large number of terms as $χ$ increases such that $ξ$ scales as $W^{-2n}$ with arbitrarily large $n$. Moreover, we support our analytical results with numerical simulations. Our results introduce stealthy disorder into quantum tight-binding models and show that enforcing a low-$k$ spectral gap markedly alters the scattering landscape, enabling localization lengths that exceed the system size at fixed disorder strength. Since this mechanism relies only on the spectral properties of the disorder, it carries over directly to photonic and phononic wave systems.

cond-mat.dis-nn

Quantifying when hyperuniformity of a many-particle system leads to uniformity across length scales

Hyperuniform systems are distinguished by an unusually strong suppression of large-scale density fluctuations and, consequently, display a high degree of uniformity at the largest length scales. In some cases, however, enhanced uniformity is expected to be present even at intermediate and possibly small length scales. There exist three different classes of hyperuniform systems, where class I and class III are the strongest and weakest forms, respectively. We utilize the local number variance $σ_N^2(R)$ associated with a window of radius $R$ as a diagnostic to quantify the approach to the asymptotic large-$R$ hyperuniform scaling of a variety of class I, II, and III systems. We find, for all class I systems we analyzed, including crystals, quasicrystals, disordered stealthy hyperuniform systems, and the one-component plasma, a faster approach to the asymptotic scaling of $σ_N^2(R)$, governed by corrections with integer powers of $1/R$. Thus, we conclude this represents the highest degree of effective uniformity from small to large length scales. Class II systems, such as Fermi-sphere point processes, are characterized by logarithmic $1/\ln(R)$ corrections and, consequently, a lower degree of local uniformity. Class III systems, such as perturbed lattice patterns, present an asymptotic scaling of $1/R^α$, $0 < α< 1$, implying, curiously, an intermediate degree of local uniformity. In addition, our study provides insight into when experimental and numerical finite systems are representative of large-scale behavior. Our findings may thereby facilitate the design of hyperuniform systems with enhanced physical properties arising from local uniformity.

cond-mat.stat-mech

Transparency versus Anderson localization in one-dimensional disordered stealthy hyperuniform layered media

We present numerical simulations of disordered stealthy hyperuniform layered media ranging up to 10,000 thin slabs of high-dielectric constant separated by intervals of low dielectric constant that show no apparent evidence of Anderson localization of electromagnetic waves or deviations from transparency for a continuous band of frequencies ranging from zero up to some value $ω_T$. The results are consistent with the strong-contrast formula including its tight upper bound on $ω_T$ and with previous simulations on much smaller systems. We utilize a transfer matrix method to compute the Lyaponov exponents, which we show is a more reliable method for detecting Anderson localization by applying it to a range of systems with common types of disorder known to exhibit localization, such as perturbed periodic lattices. The Lyaponov exponents for these systems with ordinary disorder show clear evidence of localization, in contrast to the cases of perfectly periodically spaced slabs and disordered stealthy hyperuniform layered systems. As with any numerical study, one should be cautious about drawing definitive conclusions. There remains the challenge of determining whether one-dimensional disordered stealthy hyperuniform layered media possess a finite localization length on some scale much larger than our already large system size or, alternatively, are exceptions to the standard Anderson localization theorems.

cond-mat.dis-nn

Existence of Nonequilibrium Glasses in the Degenerate Stealthy Hyperuniform Ground-State Manifold

Stealthy interactions are an emerging class of nontrivial, bounded long-ranged oscillatory pair potentials with classical ground states that can be disordered, hyperuniform, and infinitely degenerate. Their hybrid crystal-liquid nature endows them with novel physical properties with advantages over their crystalline counterparts. Here, we show the existence of nonequilibrium hard-sphere glasses within this unusual ground-state manifold as the stealthiness parameter $χ$ tends to zero that are remarkably configurationally extremely close to hyperuniform 3D maximally random jammed (MRJ) sphere packings. The latter are prototypical glasses since they are maximally disordered, perfectly rigid, and perfectly nonergodic. Our optimization procedure, which leverages the maximum cardinality of the infinite ground-state set, not only guarantees that our packings are hyperuniform with the same structure-factor scaling exponent as the MRJ state, but they share other salient structural attributes, including a packing fraction of $0.638$, a mean contact number per particle of 6, gap exponent of $0.44(1)$, and pair correlation functions $g_2(r)$ and structures factors $S(k)$ that are virtually identical to one another for all $r$ and $k$, respectively. Moreover, we demonstrate that stealthy hyperuniform packings can be created within the disordered regime ($0 < χ<1/2$) with heretofore unattained maximal packing fractions. As $χ$ increases from zero, they always form interparticle contacts, albeit with sparser contact networks as $χ$ increases from zero, resulting in linear polymer-like chains of contacting particles with increasingly shorter chain lengths. The capacity to generate ultradense stealthy hyperuniform packings for all $χ$ opens up new materials applications in optics and acoustics.

cond-mat.dis-nn

Dynamical properties of particulate composites derived from ultradense stealthy hyperuniform sphere packings

Stealthy hyperuniform (SHU) many-particle systems are distinguished by a structure factor that vanishes not only at zero wavenumber (as in ``standard'' hyperuniform systems) but also across an extended range of wavenumbers near the origin. We generate disordered SHU packings of identical and `nonoverlapping' spheres in $d$-dimensional Euclidean space using a modified collective-coordinate optimization algorithm that incorporates a soft-core repulsive potential between particles in addition to the standard stealthy pair potential. These SHU packings are ultradense, spanning a broad spectrum of structures depending on the stealthiness parameter $χ$. We consider two-phase media composed of hard particles derived from ultradense SHU packings embedded in a matrix phase, with varying stealthiness parameter $χ$ and packing fractions $ϕ$. Our main objective is the estimation of the dynamical physical properties of such two-phase media, namely, the effective dynamic dielectric constant and the time-dependent diffusion spreadability, which is directly related to nuclear magnetic relaxation in fluid-saturated porous media. We show through spreadability that two-phase media derived from ultradense SHU packings exhibit faster interphase diffusion due to the higher packing fractions achievable compared to media obtained without soft-core repulsion. The imaginary part of the effective dynamic dielectric constant of SHU packings vanishes at a small wavenumber, implying perfect transparency for the corresponding wavevectors. We also obtain cross-property relations between transparency characteristics and long-time behavior of the spreadability for such two-phase media. Our results demonstrate that disordered two-phase media derived from ultradense SHU packings exhibit advantageous transport and optical behaviors of both theoretical and experimental significance.

cond-mat.soft

Ultradense Sphere Packings Derived From Disordered Stealthy Hyperuniform Ground States

Disordered stealthy hyperuniform (SHU) packings are an emerging class of exotic amorphous two-phase materials endowed with novel physical properties. Such packings of identical spheres have been created from SHU point patterns via a modified collective-coordinate optimization scheme that includes a soft-core repulsion, besides the standard `stealthy' pair potential. Using the distributions of minimum pair distances and nearest-neighbor distances, we find that when the stealthiness parameter $χ$ is lower than 0.5, the maximal values of $ϕ$, denoted by $ϕ_{\max}$, decrease to zero on average as the particle number $N$ increases if there are no soft-core repulsions. By contrast, the inclusion of soft-core repulsions results in very large $ϕ_{\max}$ independent of $N$, reaching up to $ϕ_{\max}=1.0, 0.86, 0.63$ in the zero-$χ$ limit and decreasing to $ϕ_{\max}=1.0, 0.67, 0.47$ at $χ=0.45$ for $d=1,2,3$, respectively. We obtain explicit formulas for $ϕ_{\max}$ as functions of $χ$ and $N$ for a given $d$. For $d=2,3$, our soft-core SHU packings for small $χ$ become configurationally very close to the jammed hard-particle packings created by fast compression algorithms, as measured by the pair statistics. As $χ$ increases beyond $0.20$, the packings form fewer contacts and linear polymer-like chains. The resulting structure factors $S(k)$ and pair correlation functions $g_2(r)$ reveal that soft-core repulsions significantly alter the short- and intermediate-range correlations in the SHU ground states. We also compute the spectral density $\tildeχ_{_V}(k)$, which can be used to estimate various physical properties (e.g., electromagnetic properties, fluid permeability, and mean survival time) of SHU two-phase dispersions. Our results offer a new route for discovering novel disordered hyperuniform two-phase materials with unprecedentedly high density.

cond-mat.soft

From point patterns to networks: to what extent does the Delaunay triangulation reproduce key spatial and density information?

It is important that a spatial network's construction algorithm reproduces the structural properties of the original physical embedding. Here, we assess the Delaunay triangulation as a spatial network construction algorithm for seven different types of 2D point patterns, including hyperuniform systems. The latter are characterized by completely suppressed normalized infinite-wavelength density fluctuations. We demonstrate that the quartile coefficients of dispersion of multiple centrality measures are capable of rank-ordering hyperuniform and nonhyperuniform systems independently, but they cannot distinguish a system that is nearly hyperuniform from hyperuniform systems. Thus, we investigate the local densities of the point pattern and of the network. We reveal that there is a strong correlation between local densities in the point pattern and network in nonhyperuniform systems, but there is no such correlation in hyperuniform systems. When calculating the pair-correlation function and local density covariance function on the point pattern and network, the point pattern and network functions are similar only in nonhyperuniform systems. In hyperuniform systems, the triangulation has a positive covariance of local network densities in pairs of nodes that are close together that is not present in the point patterns. Thus, we demonstrate that the Delaunay triangulation accurately captures the density fluctuations of the point pattern only when the point pattern possesses a positive local density covariance at small distances. Such positive correlation is seen in most real-world systems, so the Delaunay triangulation is generally an effective tool for building a spatial network from a 2D point pattern, but there are situations (i.e., disordered hyperuniform systems) where we caution that the Delaunay triangulation would not be effective at capturing the underlying physical embedding.

cond-mat.stat-mech