arXiv subjects

Samir Lounis

Publications and source records attributed to Samir Lounis.

At least 19 recordsLinked to original sources

arXiv2026

Exact theory of chirality-dependent p-wave magnetism and Edelstein effect in spin spirals

Spin-momentum locking is widely regarded as a hallmark of relativistic spin-orbit coupling. Here we demonstrate analytically that it can instead emerge solely from magnetic chirality. Solving the minimal tight-binding model of electrons coupled to a spin spiral using a generalized Bloch theorem, we show that the spiral generates chirality-dependent p-wave magnetism characterized by the antisymmetric spin texture $\boldsymbol{s}(\boldsymbol{k})=-\boldsymbol{s}(-\boldsymbol{k})$. The exact solution further yields closed-form expressions for the electrical conductivity and the spin Edelstein susceptibility, revealing a microscopic mechanism by which magnetic chirality alone can generate spin polarization without spin-orbit coupling, with direct implications also for chirality-induced spin selectivity. In the strong exchange-coupling regime, the spin-dependent physics of the spin spiral becomes directly analogous to the orbital-dependent physics of electrons propagating through a non-magnetic helix. Our work establishes a minimal exactly solvable model of chirality-induced spin-momentum locking and spin-charge conversion beyond the conventional spin-orbit coupled paradigm.

cond-mat.mes-hall↗

arXiv2026

Coupled Spin-Orbital $p$-Wave Magnetism via Structural and Magnetic Chirality

Helical spin textures represent the minimal realization of $p$-wave magnetism which is characterized by momentum-odd spin polarization. Independently, structurally chiral crystals exhibit momentum-odd orbital polarization arising from broken inversion symmetry. Here, we demonstrate that spin-orbit coupling couples these two independent microscopic chirality degrees of freedom, allowing the orbital polarization of a chiral crystal to generate an additional contribution to the $p$-wave spin splitting. The resulting spin-orbital state is naturally classified by the relative chirality $\eta=\chi_{\mathrm c}\chi_{\mathrm m}$, giving rise to two symmetry-distinct $p$-wave phases corresponding to homochiral and heterochiral configurations which can be directly probed by the longitudinal conductivity. These phases exhibit distinct transport signatures, establishing a unified framework linking orbitronics and unconventional magnetism through coupled spin-orbital $p$-wave order.

cond-mat.mes-hall↗

arXiv2026

Chiral-Angle-Controlled Spin Splitting and Spin Transport in Nanotubes Rolled from d-wave Altermagnets

Altermagnets combine compensated collinear magnetic order with momentum-dependent spin splitting in the electronic band structure. Here, we show that rolling a two-dimensional (2D) $d$-wave altermagnet into a nanotube converts this momentum dependence into chiral-angle-controlled one-dimensional (1D) spin splitting through dimensional projection. A minimal tight-binding model reveals a characteristic nodal--antinodal dependence on the chiral angle $\theta$, with the central circumferential subband exhibiting a $\cos(2\theta)$ scaling and the projected spin splitting vanishing for the nodal orientation and reversing sign between orthogonal antinodal orientations. First-principles calculations for V$_2$O and representative symmetric and Janus systems demonstrate that this nodal--antinodal selection rule persists despite curvature-induced structural asymmetry and magnetic moment imbalance. We further show that the projected electronic structure produces chiral-angle-controlled spin-polarized transport: antinodal nanotubes exhibit spin-polarized transmission, whereas the nodal nanotube remains conducting with identical spin-channel transmission. These results demonstrate how dimensional projection can translate the momentum-space spin splitting of a 2D altermagnet into geometrically controlled electronic and transport properties in nanotubes.

cond-mat.mtrl-sci↗

arXiv2026

Chiral spin-textures in van der Waals heterostructures

Chiral spin textures such as skyrmions have attracted considerable attention due to their nontrivial topology, chirality, stability at the nanoscale, and potential for low-power spintronic devices. The recent discovery of intrinsic magnetism in van der Waals (vdW) materials and the ability to engineer their heterostructures has opened a new platform to study and manipulate such textures. In these layered systems, atomically sharp interfaces, strong spin-orbit coupling, and tunable symmetry breaking provide unique opportunities to stabilize and control chiral magnetic states. This review summarizes the fundamental mechanisms underlying the formation of chiral spin textures in vdW heterostructures, including the roles of exchange interactions, magnetic anisotropy, Dzyaloshinskii-Moriya interaction, and dipolar effects. We highlight key experimental advances in the observation and manipulation of chiral textures, discuss their dynamical properties and transport signatures, while overviewing selected theoretical investigations. Finally, we outline current challenges and future directions toward realizing robust, room-temperature chiral spin textures for practical spintronic technologies.

cond-mat.mes-hall↗

arXiv2026

$d$-wave Surface Altermagnetism in Centrosymmetric Collinear Antiferromagnets

Broken inversion symmetry at the surfaces of centrosymmetric collinear antiferromagnets lifts combined inversion and time-reversal symmetry ($PT$) and can, in principle, enable nonrelativistic d-wave spin splitting, termed surface altermagnetism. Combining symmetry analysis with first-principles calculations, we show that surface inversion breaking, while necessary, is not sufficient for this effect. Surface altermagnetism emerges only when no antiunitary symmetry survives at the surface that exchanges the two antiferromagnetically coupled surface sublattices and enforces spin degeneracy. We demonstrate this mechanism explicitly for the centrosymmetric G-type antiferromagnets V$_3$Al and BaMn$_2$Sb$_2$, and contrast it with MnPt, where a sublattice-exchanging symmetry survives at the surface in the form of translation-time-reversal symmetry ($tT$), thereby preserving spin degeneracy despite broken inversion symmetry. The mechanism is shown to apply across multiple classes of centrosymmetric antiferromagnets and remains robust against spin-orbit coupling, although relativistic spin mixing in heavier-element compounds may reduce the observable spin polarization. These results establish a symmetry-based route toward realizing robust nonrelativistic momentum-dependent spin polarization at antiferromagnetic surfaces and interfaces.

cond-mat.mtrl-sci↗

arXiv2025

Giant orbital Zeeman effects in a magnetic topological van der Waals interphase

Van der Waals (vdW) heterostructures allow the engineering of electronic and magnetic properties by the stacking different two-dimensional vdW materials. For example, orbital hybridisation and charge transfer at a vdW interface may result in electric fields across the interface that give rise to Rashba spin-orbit coupling. In magnetic vdW heterostructures, this in turn can drive the Dzyaloshinskii-Moriya interaction which leads to a canting of local magnetic moments at the vdW interface and may thus stabilise novel 2D magnetic phases. While such emergent magnetic "interphases" offer a promising platform for spin-based electronics, direct spectroscopic evidence for them is still lacking. Here, we report Zeeman effects with Land\'e $g$-factors up to $\approx230$ at the interface of graphene and the vdW ferromagnet Fe$_3$GeTe$_2$. They arise from a magnetic interphase in which local-moment canting and itinerant orbital moments generated by the non-trivial band topology of Fe$_3$GeTe$_2$ conspire to cause a giant asymmetric level splitting when a magnetic field is applied. Exploiting the inelastic phonon gap of graphene, we can directly access the buried vdW interface to the Fe$_3$GeTe$_2$ by scanning tunnelling spectroscopy. Systematically analyzing the Faraday-like screening of the tip electric field by the graphene, we demonstrate the tunability of the constitutional interface dipole, as well as the Zeeman effect, by tip gating. Our findings are supported by density functional theory and electrostatic modelling.

cond-mat.mes-hall↗

arXiv2025

Oxygen-driven altermagnetic symmetry inducing d-wave superconductivity in the cuprates and nickelates

Since the discovery of cuprate high-Tc superconductivity, numerous theoretical frameworks have been proposed to explain its mechanism; Anderson's RVB picture [Science 235, 1196-1198, 1987] and U(1) gauge theory [Phys. Rev. Lett. 76, 503-506, 1996] motivate a minimal one-band view that largely integrates out oxygen. By contrast, altermagnetism [Phys. Rev. X 12, 040501, 2022] yields a d-wave-like k-space magnetic texture from alternatingly rotated nonmagnetic cages; La2CuO4 (the parent of a high-Tc cuprate) is a prototypical example. As a proof of principle, we show in La2CuO4 that an alternating local pairing potential on the two Cu sublattices (plus/minus s(r)) produces a nodal, d-wave-like Delta(k). As orthorhombic tilts are, however, not the driver (and even suppress superconductivity in nickelates; [Nature 621, 493, (2023)], we then show that the in-plane oxygen sublattice of CuO2/NiO2 layers, ubiquitous in cuprates and nickelates, intrinsically realizes the same symmetry. Imposing an oxygen-centered, staggered s pairing yields a d-wave gap with perfect C4 symmetry, demonstrated self-consistently in NdNiO2 from first principles. While the underlying mechanism that drives this order is unclear, we outline possible origins. Further, this description of superconductivity enables mapping a real-space superconducting order parameter onto a lattice picture, allowing superconductivity and Hubbard physics to be treated on the same footing.

cond-mat.supr-con↗

arXiv2025

Electronic properties of Kagome metal YbV$_3$Sb$_4$: A First-Principles Study

We have investigated the vanadium-based Kagome metal YbV$_3$Sb$_4$ using density functional theory (DFT) combined with the Wannier function analysis. We explore the electronic properties, de Haas-van Alphen (dHvA) effect and Fermi surface. The inclusion of spin-orbit coupling SOC induces the splitting of Yb-4f states, while its impact on the V-3d states is moderate. Furthermore, we have incorporated SOC+U, where U being the Hubbard parameter, which drastically changes the Yb-4f states creating additional splitting leading to three distinct peaks in the density of states (DOS). The V-3d atoms with the Kagome lattice contribute maximum to the transport properties, exhibits flat bands near the EF while being protected under SOC and U+SOC. Herein, we report the vulnerability of the Yb-4f states under SOC and U+SOC. Furthurmore, The Fermi surface is found to comprise of quasi-2D cylindrical sheets centered at the Gamma-point, along with smaller pockets near the Brillouin zone boundaries, which under combined U+SOC, a small spherical pocket emerges and the cylindrical sheet exhibits slight deformations. The dHvA frequencies reach as high as 70 kilotesla, which increase with tilt angle, exhibiting a nearly parabolic trend as expected for cylindrical orbits, while a low-frequency branch remains below 1 kT. Only the U+SOC case shows noticeable modification in both the Fermi surface and the dHvA oscillation. Crucially, the $Z_2$ invariant calculation identifies YbV$_3$Sb$_4$ as a strong topological metal ($r_0 = 1$). These findings not only advance our understanding of the underlying quantum phenomena in rare-earth Kagome systems, but also establish YbV$_3$Sb$_4$ as a compelling and promising platform for exploring intertwined topology and electron correlations in kagome lattices, thereby offering valuable insights for engineering quantum phases in layered materials.

cond-mat.str-el↗

arXiv2025

Effect of applied pressure on the non-relativistic spin-splitting (NRSS) of FeSb2 altermagnet: A first-principles study

We have investigated the pressure-dependent electronic structure, phonon stability, and anomalous Hall response of the recently discovered altermagnet FeSb2 from density functional theory (DFT) and Wannier function analysis. From density functional perturbation theory (DFPT) calculations, we have found that FeSb2 remains dynamically stable up to 10 GPa, evidenced by positive phonon frequencies. Our spin-polarised band structure shows that the node of band crossing between spin-up and spin-down bands around the Fermi energy exactly lies at the Gamma and A-symmetry points. The Fermi crossing is mostly exhibited by band-24, band-25 and band-26. The non-relativistic spin-splitting (NRSS) along M'-Gamma-M and A-Z-A' symmetry is attributed to the broken time-reversal (PT ) symmetry. There are significant changes in the band profile under applied pressure, as one can see the shifting of the node of band-24 and band-26 towards the lower energy side. The NRSS exhibited by band-24 along M'-Gamma-M symmetry is notably small. Although the strength of NRSS of band-26 along A-Z-A' symmetry is significant but reduces under applied pressure. The anomalous Hall conductivity (AHC) values are prominent in -1 to 1 eV range. A sharp peaked and positive AHC values at ambient pressure, becomes spectrally broadened and negative at 10 GPa due to pressure-induced band crossings and redistribution of Berry curvature near the Fermi level. We have observed that the values of spin hall conductivity (SHC) are around 2-2.5 times lower as compared to AHC and prominent in between -1.0 eV to 1.0 eV. Our results establish FeSb2 as a tunable altermagnetic candidate where pressure can modulate both topological transport and dynamic stability, offering opportunities for strain-engineered Hall responses in compensated magnetic systems.

cond-mat.str-el↗

arXiv2025

Ab-initio exploration of Gd monolayer interfaced with WSe$_2$: from electronic and magnetic properties to the anomalous Hall effect

Heterostructures involving transition metal dichalcogenides (TMDs) have attracted significant research interest due to the richness and versatility of the underlying physical phenomena. In this work, we investigate a heterostructure consisting of a rare-earth material, specifically a Gd monolayer, interfaced with WSe$_2$. We explore its electronic structure, magnetic properties, and transport behavior, with particular emphasis on the emergence of the anomalous Hall effect (AHE). Both Gd and W are heavy elements, providing strong spin-orbit coupling (SOC), which plays a crucial role in triggering the AHE. The combination of strong SOC and inversion symmetry breaking leads to pronounced asymmetries between the $\Gamma-K$ and $\Gamma-K^\prime$ directions in the Brillouin zone. Our calculations reveal a substantial anomalous Hall conductivity (AHC) at the ferromagnetic interface, primarily originating from numerous avoided crossings involving the d-states of both Gd and W near the Fermi level. Moreover, we demonstrate that the AHC is highly tunable, either by adjusting the in-plane lattice constant or by reducing the separation between Gd and WSe$_2$.

cond-mat.mtrl-sci↗

arXiv2025

Influence of Interlayer Stacking on Optical Behavior in WSe$_{2}$/MoS$_{2}$ van der Waals Heterostructures

We investigate the impact of crystal alignment on excitonic behavior in WSe$_{2}$/MoS$_{2}$ van der Waals heterostructures by comparing eclipsed (AA) and staggered (AB) stacking configurations. Our first-principles and symmetry-based analysis reveal that interlayer stacking symmetry plays a central role in determining the nature of electron-hole pairs. We uncover a rich variety of excitonic states, including spatially confined two-dimensional (2D) excitons, delocalized three-dimensional (3D) excitons, and charge-transfer (CT) excitons with interlayer character. The dimensionality and optical activity of these excitons are governed by the interplay among orbital character, interlayer hybridization, and symmetry-imposed selection rules. Our findings establish general principles for engineering excitonic properties in van der Waals heterostructures through controlled layer orientation and stacking order.

cond-mat.str-el↗

arXiv2025

Three-dimensional topological orbital Hall effect caused by magnetic hopfions

Magnetic hopfions are non-collinear spin textures that are characterized by an integer topological invariant, called Hopf index. The three-dimensional magnetic solitons can be thought of as a tube with a twisted magnetization that has been closed at both ends to form a torus. The tube consists of a magnetic whirl called in-plane skyrmion or bimeron. Although hopfions have been observed by microscopy techniques, their detection remains challenging as they lack an electronic hallmark so far. Here we predict a three-dimensional orbital Hall effect caused by hopfion textures: When an electric field is applied, the hopfion generates a transverse current of orbital angular momentum. The effect arises due to the local emergent field that gives rise to in-plane and out-of-plane orbital Hall conductivities. This orbital Hall response can be seen as a hallmark of hopfions and allows us to distinguish them from other textures, like skyrmioniums, that look similar in real-space microscopy experiments. While the two-dimensional topological invariant of a skyrmion determines its topological Hall transport, the unique three-dimensional topological orbital Hall effect can be identified with the three-dimensional topological invariant that is the Hopf index. Our results make hopfions attractive for spin-orbitronic applications because their orbital signatures allow for their detection in devices and give rise to large orbital torques.

cond-mat.mes-hall↗

arXiv2025

Chirality-induced selectivity of angular momentum by orbital Edelstein effect in carbon nanotubes

Carbon nanotubes (CNTs) are promising materials exhibiting exceptional strength, electrical conductivity, and thermal properties, making them promising for various technologies. Besides achiral configurations with a zigzag or armchair edge, there exist chiral CNTs with a broken inversion symmetry. Here, we demonstrate that chiral CNTs exhibit chirality-induced orbital selectivity (CIOS), which is caused by the orbital Edelstein effect and could be detected as chirality-induced spin selectivity (CISS). We find that the orbital Edelstein susceptibility is an odd function of the chirality angle of the nanotube and is proportional to its radius. For metallic CNTs close to the Fermi level, the orbital Edelstein susceptibility increases quadratically with energy. This makes the CISS and CIOS of metallic chiral nanotubes conveniently tunable by doping or applying a gate voltage, which allows for the generation of spin- and orbital-polarized currents. The possibility of generating large torques makes chiral CNTs interesting candidates for technological applications in spin-orbitronics and quantum computing.

cond-mat.mes-hall↗

arXiv2025

Unlocking Hidden Potential in Electron Holography of Non-Collinear Spin Textures

Due to their particle-like properties, three-dimensional (3D) spin textures have garnered significant interest, particularly for their potential applications in next-generation information storage devices. However, efficiently identifying these textures remains a major challenge. Here, we approach this problem from a new perspective. Rather than relying solely on the magnetic stray field, which vanishes in antiferromagnets, we use multiple-scattering theory to demonstrate that spin textures carry nontrivial charges due to the noncollinearity of magnetic moments. This induced charge encodes magnetic information driven by spin-mixing and spin-orbit interactions. We propose leveraging electron holography to extract this information by reconstructing phase images obtained from transmission electron microscopy (TEM). To quantify this effect, we systematically calculate and compare the contributions of both conventional and newly identified mechanisms to the phase images, considering different electronic structure parameters. Our findings mark a significant milestone in advancing the exploration and possible application of 3D spin textures in next-generation spintronic devices.

cond-mat.mes-hall↗

arXiv2025

Triple-Q state in magnetic breathing kagome lattice

Magnetic frustration in two-dimensional spin lattices with triangular motifs underpins a series of exotic states, ranging from multi-Q configurations to disordered spin-glasses. The antiferromagnetic kagome lattice, characterized by its network of corner-sharing triangles, represents a paradigmatic frustrated system exhibiting macroscopic degeneracy. Expanding upon the kagomerization mechanism, we focus on the magnetic breathing kagome lattice formed by a Mn monolayer deposited on a heavy metal substrate and capped with h-BN. The Mn kagome arrangement induces pronounced magnetic frustration, as evidenced by the nearly flat bands derived from spin spiral energy calculations. Including further-neighbor interactions reveals a spin spiral energy minimum along the $\Gamma$-K line and an intriguing triple-Q state with nonzero topological charge, potentially leading to highly nonlinear Hall effects. Furthermore, the flat band properties can further give rise to an even more complex spin configuration, marked by several Q-pockets in the spin structure factor. These results present a fertile ground for advancing the study of multi-Q states and exploring emergent topological phenomena.

cond-mat.mtrl-sci↗

arXiv2024

Confinement-induced altermangetism in RuO$_2$ thin films

The magnetic properties of bulk RuO$_2$ remain a subject of active debate, despite its pivotal role in the emergence of altermagnetism. The latter is a novel paradigm in magnetic phases, characterized by the absence of net magnetization due to anti-parallel alignment of magnetic moments, yet displaying finite spin-splitting in the electronic band structure. This unique behavior unlocks opportunities for advanced applications in information technology devices. Recent experimental and theoretical investigations suggest that bulk RuO$_2$, contrary to prior assumptions, is non-magnetic. In this work, we propose the fabrication of RuO$_2$ thin films to robustly stabilize the altermagnetic phase. Unlike their bulk counterparts, thin films experience substantial strain relaxation, leading to a dramatic impact on the electronic structure that triggers a transition towards an altermagnetic behavior, which mimics the impact of an artificially applied Hubbard-U correction to account for electronic correlations. Our findings promote the use and exploration of thin films for the realization of spintronic devices based on altermagnets.

cond-mat.mtrl-sci↗

arXiv2024

Frustrated magnetism in Mn films on Ag(111) surface: from chiral in-plane N\'eel state to row-wise antiferromagnetism

We conduct a comprehensive density functional theory (DFT) study to explore the intricate magnetic properties of frustrated Mn monolayer on the Ag(111) surface. Spin-polarized scanning tunneling microscopy demonstrates that a N\'eel magnetic state characterizes such an interface, which contradicts systematic ab-initio predictions made in the last two decades indicating that the ground state is collinear row-wise antiferromagnetic (RW-AFM) state. Here, we employ the all-electron full-potential Korringa-Kohn-Rostoker Green function (KKR) method and find that the ground state is a chiral magnetic N\'eel state, with magnetic moments rotating in the surface plane following a unique sense of rotation, as dictated by the underlying in-plane magnetic anisotropy and Dzyaloshinskii-Moriya interaction. Once allowing disordered magnetic states, as described within the disordered local moment (DLM) approach, we reveal the possibility of stabilization of a RW-AFM state. We conjecture that at low temperatures, the chiral N\'eel state prevails, while at higher temperatures, the magnetic exchange interactions are modified by magnetic disorder, which can then induce a transition towards a RW-AFM state. Our work addresses a long term experimental-theoretical controversy and provides significant insights into the magnetic interactions and stability of Mn films on noble metal substrates, contributing to the broader understanding of the different magnetic facets of frustrated magnetism in thin films.

cond-mat.mtrl-sci↗

arXiv2024

Newly discovered magnetic phase: A brief review on Altermagnets

Recently, a new magnetic phase, termed altermagnetism, has caught the attention of the magnetism and spintronics community. This newly discovered magnetic phenomenon differs from traditional ferromagnetism and antiferromagnetic. It generally lacks net magnetization and is characterized by unusual non-relativistic spin-splitting and broken time-reversal symmetry. This leads to novel transport properties such as the anomalous Hall effect, the crystal Nernst effect, and spin-dependent phenomena that cannot be fully explained by traditional magnetic theories. Spin-dependent phenomena such as spin currents, spin-splitter torques, and high-frequency dynamics emerge as key characteristics in altermagnets. This paper reviews the main aspects pertaining to altermagnets by providing an overview of theoretical investigations and experimental realizations. We discuss the most recent developments in altermagnetism, its comparison to other magnetic orders, and future prospects for exploiting its unique properties in next-generation devices.

cond-mat.str-el↗