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Samuele Grandi

Publications and source records attributed to Samuele Grandi.

At least 19 recordsLinked to original sources

Long-lived telecom-heralded single-photon storage in an absorptive spin-rephased quantum memory

Long-lived storage of single photons under the form of atomic excitations is at the foundation of long-distance entanglement distribution in quantum networks. To mitigate decoherence effects induced by the environment, rephasing of the hyperfine coherences using microwave pulses have been implemented in a variety of single-emitter and ensemble-based solid-state systems. However, the demonstration of storage of single photons in an absorptive quantum memory including such spin rephasing mechanism remains elusive. In this work, we show non-classical storage of telecom-heralded single photons in a Pr$^{3+}$:Y$_2$SiO$_5$ rare-earth ion doped crystal quantum memory using the atomic frequency comb (AFC) spin-wave protocol combined with a XY4 spin rephasing sequence. Long-lived AFC photon echoes are first observed in the classical regime for storage times of up to approximately 3 ms. We then demonstrate non-classical correlations between heralding photons and stored signal photons generated by a cavity-enhanced parametric photon-pair source for storage times of up to 180 $\mu$s and with measured cross-correlation values as high as 4.6(4). Together with the capacity of Pr$^{3+}$:Y$_2$SiO$_5$ QMs to support highly efficient and multiplexed storage, this result represents a significant step towards scalable long-distance quantum repeater links.

quant-ph

Heralded entanglement of on-demand spin-wave solid-state quantum memories for multiplexed quantum network links

The ability to distribute heralded entanglement between distant matter nodes is a primitive for the implementation of large-scale quantum networks. Some of the most crucial requirements for future applications include high heralding rates at telecom wavelengths, multiplexed operation and on-demand retrieval of stored excitations for synchronization of separate quantum links. Despite tremendous progress in various physical systems, the demonstration of telecom-heralded entanglement between quantum nodes featuring both multiplexed operation and on-demand retrieval remains elusive. In this work, we combine narrowband parametric photon-pair sources and solid-state quantum memories based on rare-earth doped crystals to demonstrate telecom heralded entanglement between spatially separated spin-wave quantum memories with fully adjustable recall time and temporal multiplexing of 15 modes. In a first experiment, the storage in the spin-state is conditioned on the entanglement heralding. We take advantage of the control over readout pulse phase to achieve feed-forward conditional phase-shifts on the stored photons depending on which heralding detector clicked. We exploit this effect to double the entanglement heralding rate for a given quantum state up to 510 cps, with an associated detection rate of 0.32 cps and measured positive concurrence by up to 6 standard deviations. In a second experiment, we simulate the communication time of a long-distance link by implementing an unconditional storage scheme with a dead-time of 100 $μ$s. We take advantage of temporal multiplexing to increase the entanglement rates by a factor of 15 with respect to single mode storage, reaching a value of 22 cps per heralding detector. These results establish our architecture as a prime candidate for the implementation of scalable high-rate quantum network links.

quant-ph

Quantum Storage of Qubits in an Array of Independently Controllable Solid-State Quantum Memories

Random-access quantum memories may offer computational advantages for quantum computers and networks. In this paper, we advance arrays of solid-state quantum memories towards their usage as random-access quantum memory. We perform quantum storage of path and time-bin qubits implemented with weak coherent states at the single-photon level, in an array of ten temporally-multiplexed memory cells with controllable addressing. The qubits can be stored in arbitrary combinations of memory cells, from which they are read-out on demand. We find average fidelities of $95_{-2}^{+2}\;\%$ for path qubits and $91^{+2}_{-2}\;\%$ for time-bin qubits. The measured fidelities violate the classical bounds for both encodings and for all ten cells. We also sequentially store a time-bin qubit in two different memory cells, maintain both qubits simultaneously in the array, and perform a collective read-out. The individual control paired with high storage fidelity represents a significant advance towards a solid-state random-access quantum memory for quantum repeaters and photonic quantum processors.

quant-ph

A solid-state temporally multiplexed quantum memory array at the single-photon level

The exploitation of multimodality in different degrees of freedom is one of the most promising ways to increase the rate of heralded entanglement between distant quantum nodes. In this paper, we realize a spatially-multiplexed solid-state quantum memory array with ten individually controllable spin-wave memory cells featuring on-demand read-out and temporal multiplexing. By combining spatial and temporal multiplexing, we store weak coherent pulses at the single-photon level in up to 250 spatio-temporal modes, with an average signal-to-noise ratio of 10(2). We perform a thorough characterization of the whole system, including its multiplexing and demultiplexing stage. We verify that the memory array exhibits low cross-talk even at the single-photon level. The measured performance indicates readiness for storing non-classical states and promises a speed-up in entanglement distribution rates.

quant-ph

Telling different unravelings apart via nonlinear quantum-trajectory averages

The Gorini-Kossakowski-Sudarshan-Lindblad master equation (ME) governs the density matrix of open quantum systems (OQSs). When an OQS is subjected to weak continuous measurement, its state evolves as a stochastic quantum trajectory, whose statistical average solves the ME. The ensemble of such trajectories is termed an unraveling of the ME. We propose a method to operationally distinguish unravelings produced by the same ME in different measurement scenarios, using nonlinear averages of observables over trajectories. We apply the method to the paradigmatic quantum nonlinear system of resonance fluorescence in a two-level atom. We compare the Poisson-type unraveling, induced by direct detection of photons scattered from the two-level emitter, and the Wiener-type unraveling, induced by phase-sensitive detection of the emitted field. We show that a quantum-trajectory-averaged variance is able to distinguish these measurement scenarios. We evaluate the performance of the method, which can be readily extended to more complex OQSs, under a range of realistic experimental conditions.

quant-ph

Integrated thermo-optic phase shifters for laser-written photonic circuits operating at cryogenic temperatures

Integrated photonics offers compact and stable manipulation of optical signals in miniaturized chips, with the possibility of changing dynamically their functionality by means of integrated phase shifters. Cryogenic operation of these devices is becoming essential for advancing photonic quantum technologies, accommodating components like quantum light sources, single photon detectors and quantum memories operating at liquid helium temperatures. In this work, we report on a programmable glass photonic integrated circuit (PIC) fabricated through femtosecond laser waveguide writing (FLW) and controlled by thermo-optic phase shifters both in a room-temperature and in a cryogenic setting. By taking advantage of a femtosecond laser microstructuring process, we achieved reliable PIC operation with minimal power consumption and confined temperature gradients in both conditions. This advancement marks the first cryogenically-compatible programmable FLW PIC, paving the way for fully integrated quantum architectures realized on a laser-written photonic chip.

physics.optics

Towards the Intuitive Understanding of Quantum World: Sonification of Rabi Oscillations, Wigner functions, and Quantum Simulators

Recently, there has been considerable interest in "sonifying" scientific data; however, sonifying quantum processes using the newest quantum technologies, including Noise Intermediate Scale Quantum devices and quantum random number generators, is still an emerging area of research. Music technologists and composers employ the growing accessibility to diverse data from quantum mechanics as musical tools in the hope of generating new sound expressions. How different is the quantum world from the classical one, and is it possible to express the quantum world using sounds? Quantum phenomena are very different from those that we experience in our everyday lives. Thus, it is challenging to understand them intuitively. In this paper, we propose sonification as a method toward an intuitive understanding of various quantum mechanical phenomena, from Rabi oscillations and resonance fluorescence of a single atom through the generation of Schrödinger cat states in strong laser field physics to insulator-superfluid transition in quantum many-body systems. This paper illustrates various methods we experimented with in sonification and score representations of quantum data depending on the source data and performance settings.

quant-ph

Transmission of light-matter entanglement over a metropolitan network

We report on the transmission of telecom photons entangled with a multimode solid-state quantum memory over a deployed optical fiber in a metropolitan area. Photon pairs were generated through spontaneous parametric down-conversion, with one photon stored in a rare earth-based quantum memory, and the other, at telecommunication wavelengths, traveling through increasing distances of optical fibre, first in the laboratory and then outside in a deployed fibre loop. We measured highly-non-classical correlations between the stored and the telecom photons for storage times up to 25 $μ$s and for a fibre separation up to 50 km. We also report light-matter entanglement with a two-qubit fidelity up to 88$\%$, which remains constant within error bars for all fibre lengths, showing that the telecom qubit does not suffer decoherence during the transmission. Finally, we moved the detection stage of the telecom photons to a different location placed 17 km away, and confirmed the non-classical correlations between the two photons. Our system was adapted to provide the transmission of precise detection times and synchronization signals over long quantum communication channels, providing the first steps for a future quantum network involving quantum memories and non-classical states.

quant-ph

Detection of single ions in a nanoparticle coupled to a fiber cavity

Many quantum information protocols require the storage and manipulation of information over long times, and its exchange between nodes of a quantum network across long distances. Implementing these protocols requires an advanced quantum hardware, featuring, for example, a register of long-lived and interacting qubits with an efficient optical interface in the telecommunication band. Here we present the Purcell-enhanced detection of single solid-state ions in erbium-doped nanoparticles placed in a fiber cavity, emitting photons at 1536 nm. The open-access design of the cavity allows for complete tunability both in space and frequency, selecting individual particles and ions. The ions are confined in a volume two orders of magnitude smaller than in previous realizations, increasing the probability of finding ions separated only by a few nanometers which could then interact. We report the detection of individual spectral features presenting saturation of the emission count rate and linewidth, as expected for two-level systems. We also report an uncorrected $g^{(2)} \left ( 0 \right )$ of 0.24(5) for the emitted field, confirming the presence of a single emitter. Our fully fiber-integrated system is an important step towards the realization of the initially envisioned quantum hardware.

quant-ph

Long-distance multiplexed quantum teleportation from a telecom photon to a solid-state qubit

Quantum teleportation is an essential capability for quantum networks, allowing the transmission of quantum bits (qubits) without a direct exchange of quantum information. Its implementation between distant parties requires teleportation of the quantum information to matter qubits that store it for long enough to allow users to perform further processing. Here we demonstrate long distance quantum teleportation from a photonic qubit at telecom wavelength to a matter qubit, stored as a collective excitation in a solid-state quantum memory. Our system encompasses an active feed-forward scheme, implementing a phase shift on the qubit retrieved from the memory, therefore completing the protocol. Moreover, our approach is time-multiplexed, allowing for an increase in the teleportation rate, and is directly compatible with the deployed telecommunication networks, two key features for its scalability and practical implementation, that will play a pivotal role in the development of long-distance quantum communication.

quant-ph

Multimode capacity of atomic-frequency comb quantum memories

Ensemble-based quantum memories are key to developing multiplexed quantum repeaters, able to overcome the intrinsic rate limitation imposed by finite communication times over long distances. Rare-earth ion doped crystals are main candidates for highly multimode quantum memories, where time, frequency and spatial multiplexing can be exploited to store multiple modes. In this context the atomic frequency comb (AFC) quantum memory provides large temporal multimode capacity, which can readily be combined with multiplexing in frequency and space. In this article, we derive theoretical formulas for quantifying the temporal multimode capacity of AFC-based memories, for both optical memories with fixed storage time and spin-wave memories with longer storage times and on-demand read out. The temporal multimode capacity is expressed in key memory parameters, such as AFC bandwidth, fixed-delay storage time, memory efficiency, and control field Rabi frequency. Current experiments in europium- and praseodymium-doped Y$_2$SiO$_5$ are analyzed within this theoretical framework, and prospects for higher temporal capacity in these materials are considered. In addition we consider the possibility of spectral and spatial multiplexing to further increase the mode capacity, with examples given for both rare earh ions.

quant-ph

Storage and analysis of light-matter entanglement in a fibre-integrated system

The deployment of a fully-fledged quantum internet poses the challenge of finding adequate building-blocks for entanglement distribution between remote quantum nodes. An ideal system would combine propagation in optical fibres with quantum memories for light, leveraging on the existing communication network while featuring the scalability required to extend to network sizes. Here we demonstrate a fiber-integrated quantum memory entangled with a photon at telecommunication wavelength. The storage device is based on a fiber-pigtailed laser written waveguide in a rare-earth doped solid and allows an all-fiber stable adressing of the memory. The analysis of the entanglement is performed using fibre-based interferometers. Our results feature orders of magnitude advances in terms of storage time and efficiency for integrated storage of light-matter entanglement, and constitute a significant step forward towards quantum networks using integrated devices.

quant-ph

Entanglement between a telecom photon and an on-demand multimode solid-state quantum memory

Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand read-out and multimode operation are additional precious assets that will benefit the communication rate. In this work we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely non-degenerate parametric down-conversion, featuring energy-time entanglement between the telecom-wavelength idler and a visible signal photon. The latter is stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal as a spin wave using the full Atomic Frequency Comb scheme. We then recall the stored signal photon and analyze the entanglement using the Franson scheme. We measure conditional fidelities of $92(2)\%$ for excited-state storage, enough to violate a CHSH inequality, and $77(2)\%$ for spin-wave storage. Taking advantage of the on-demand read-out from the spin state, we extend the entanglement storage in the quantum memory for up to 47.7~$μ$s, which could allow for the distribution of entanglement between quantum nodes separated by distances of up to 10 km.

quant-ph

Topical White Paper: A Case for Quantum Memories in Space

It has recently been theoretically shown that Quantum Memories (QM) could enable truly global quantum networking when deployed in space thereby surpassing the limited range of land-based quantum repeaters. Furthermore, QM in space could enable novel protocols and long-range entanglement and teleportation applications suitable for Deep-Space links and extended scenarios for fundamental physics tests. In this white paper we will make the case for the importance of deploying QMs to space, and also discuss the major technical milestones and development stages that will need to be considered.

quant-ph

Applications of Quantum Randomness: From Rabi Oscillations to Fourier Axis Controlling the Musical Timbre

Randomness has attracted great interest in the field of music composition for quite some time. As early as 1962, Iannis Xenakis started exploring a stochastic approach to randomness by using computer-based interlinking probability functions to determine compositional structure, pitches and their durations. Soon after, composers and music technologists started to explore randomness with various methods of algorithmic compositions, sometimes with the help of artificial intelligence. However, in most cases, the source of randomness they used was in fact deterministic in nature. That is to say, the random numbers that they employed are imperfect in the strict sense (simply put, perfect random numbers never have repeating patterns). Moreover, the method in which they produced such randomness was extrinsic to the method in which randomness was applied. In this project, we attempt to take a further step by directly producing sound events from the genuine quantum true randomness of quantum physical systems. Through this method, we aim at achieving a new sense of aesthetic effect in music which derives from the true randomness that prevails in the natural quantum world.

quant-ph

Telecom-heralded entanglement between remote multimode solid-state quantum memories

Future quantum networks will enable the distribution of entanglement between distant locations and allow applications in quantum communication, quantum sensing and distributed quantum computation. At the core of this network lies the ability of generating and storing entanglement at remote, interconnected quantum nodes. While remote physical systems of various nature have been successfully entangled, none of these realisations encompassed all of the requirements for network operation, such as telecom-compatibility and multimode operation. Here we report the demonstration of heralded entanglement between two spatially separated quantum nodes, where the entanglement is stored in multimode solid-state quantum memories. At each node a praseodymium-doped crystal stores a photon of a correlated pair, with the second photon at telecommunication wavelengths. Entanglement between quantum memories placed in different labs is heralded by the detection of a telecom photon at a rate up to 1.4 kHz and is stored in the crystals for a pre-determined storage time up to 25 microseconds. We also show that the generated entanglement is robust against loss in the heralding path, and demonstrate temporally multiplexed operation, with 62 temporal modes. Our realisation is extendable to entanglement over longer distances and provides a viable route towards field-deployed, multiplexed quantum repeaters based on solid-state resources.

quant-ph

Single-photon-level sub-Doppler pump-probe spectroscopy of rubidium

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe lasers are independently tunable in frequency, with the probe operating at the single-photon-level. The two-dimensional spectrum measured as the laser frequencies are scanned shows fluorescence, Doppler-broadened absorption dips and sub-Doppler features. The detuning between the pump and probe lasers allows compensation of the Doppler shift for all atomic velocities in the room temperature vapor, meaning we observe sub-Doppler features for all atoms in the beam. We detail a theoretical model of the system which incorporates fluorescence, saturation effects and optical pumping and compare this with the measured spectrum, finding a mean absolute percentage error of 4.17\%. In the future this technique could assist in frequency stabilization of lasers, and the single-photon-level probe could be replaced by a single photon source.

physics.atom-ph

Hybrid plasmonic waveguide coupling of photons from a single molecule

We demonstrate the emission of photons from a single molecule into a hybrid gap plasmon waveguide (HGPW). Crystals of anthracene, doped with dibenzoterrylene (DBT), are grown on top of the waveguides. We investigate a single DBT molecule coupled to the plasmonic region of one of the guides, and determine its in-plane orientation, excited state lifetime and saturation intensity. The molecule emits light into the guide, which is remotely out-coupled by a grating. The second-order auto-correlation and cross-correlation functions show that the emitter is a single molecule and that the light emerging from the grating comes from that molecule. The coupling efficiency is found to be $β_{WG}=11.6(1.5)\%$. This type of structure is promising for building new functionality into quantum-photonic circuits, where localised regions of strong emitter-guide coupling can be interconnected by low-loss dielectric guides.

quant-ph