arXiv subjects

Sander A. Mann

Publications and source records attributed to Sander A. Mann.

14 recordsLinked to original sources

arXiv2026

Chiral thermal fluctuations and enhanced refrigeration in a nonreciprocal nanomechanical system

Understanding how the breaking of reciprocity influences thermal flows and microscopic thermodynamic processes such as refrigeration and energy conversion is of broad current interest. We report experimental measurements of thermal flows and refrigeration in nanomechanical resonator networks in which nonreciprocity is controlled through an optically-induced synthetic magnetic flux. Time-modulated optomechanical interactions allow controlled coupling, gauge fields, and refrigeration processes through nanomechanical frequency conversion. We quantify nonequilibrium heat flows between resonators coupled to dissipative baths of different occupation and image heat and effective temperature in networks through measuring correlations of fluctuations. Synthetic magnetism is shown to imprint chirality on thermal fluctuations in a loop of resonators, leading to pronounced chiral flows with different handedness in distinct frequency bands. We find that the heat flows in a non-equilibrium system are tuned by the synthetic magnetic flux, which redistributes energy in the thermal steady-state. Specifically, we illustrate how nonreciprocity enhances the refrigeration of a resonator in the strong coupling regime, reducing its temperature below the bound that applies to time-reversal symmetric networks. These results experimentally demonstrate the impact of nonreciprocity on thermodynamic machines, and provide new methods to characterize them at the microscopic level.

cond-mat.mes-hall↗

arXiv2026

A generalized Kirchhoff's law of thermal radiation for Floquet media

Kirchhoff's law fundamentally relates thermal emission to absorption. For linear, static, reciprocal media, it equates the emissivity and absorptivity for each direction and frequency, while in nonreciprocal systems emission and absorption are equal when the bias is time-reversed. In time-varying media, however, temporal modulation breaks time-translation invariance, converts frequencies, and enables energy exchange with the modulation drive. As a result, a same-frequency relation between absorptivity and emissivity can no longer be expected. Here, we derive a generalized Kirchhoff's law for linear time-varying Floquet media. We show that the emissivity at a given frequency equals a weighted sum of harmonic-resolved absorptivities of the adjoint system, with weights accounting for thermal occupation and photon-flux conversion. This relation has both practical and fundamental consequences. In practical terms, it allows emissivity to be calculated from absorption, simplifying the design of time-varying thermal emitters. More fundamentally, it reveals thermal radiation regimes inaccessible in static media. In particular, we identify time-varying structures that exhibit strong emission with negligible absorption at the same frequency for all directions, yielding a near-maximal violation of the conventional form of Kirchhoff's law.

physics.optics↗

arXiv2026

Optical Modulation Due to Energy Exchange Between Photonic and Exciton Modes in the Intermediate Coupling Regime

Actively tunable photonic devices are vital for next-generation optoelectronics requiring rapid switching and high bandwidth. Although organic optoelectronic devices have found wide application, their use as optical modulators has been limited by low absorption in the critical near-infrared (NIR) region, slow response time, and weak nonlinearities. To address these limitations, we developed a scheme based on intermediate exciton-photon coupling in a NIR absorbing squaraine-dye based photonic structure. Using energy-momentum resolved pump-probe spectroscopy, we show that the sign and magnitude of the optical response of our system depends strongly on the energy detuning between the excitonic and photonic modes. These data are analyzed using temporal coupled-mode theory to show that near resonance, a distinct energy exchange process emerges in the cross-over regime between strong and weak light-matter coupling. This effect enables dynamical control over the photoinduced response, providing a pathway for broadband optical signal modulation extending into the NIR spectral region.

physics.optics↗

arXiv2026

Finite-Size Effects in Nonlocal Metasurfaces

Metasurfaces leveraging nonlocal resonances enable narrowband spectral control and strong near-fields, with applications spanning augmented reality, biosensing, and nonlinear optics. However, the large spa- tial extent of these modes also poses new challenges: finite-size effects often deteriorate the performance of practical, footprint-limited devices. Here, we develop a spatiotemporal coupled-mode theory model that intuitively and quantitatively captures how finite size affects the scattering response of nonlocal metasurfaces. This reveals that, when the modal propagation length becomes constrained by the phys- ical interaction length, the scattered field shows strong interference fringes and linewidth broadening. We derive an expression for the quality factor that incorporates an additional edge-loss channel, demon- strating that the stored energy and effective lifetime scale exponentially with the interaction length. We validate these predictions experimentally using position- and momentum-resolved spectroscopy on a 30-micron-wide metasurface. Overall, this work formalizes the impact of finite size on the scattering re- sponse of nonlocal photonic systems, and provides handles on how to minimize the impact of finite-size effects in metasurface design.

physics.optics↗

arXiv2026

Enhanced Interband Optical Nonlinearities from Coupled Quantum Wells

The recent, rapid advances in nonlinear chipscale nanophotonics in the visible and near-infrared have been largely driven by manipulating the local dielectric environment proximate to decades-old workhorse bulk nonlinear optical materials, rather than increasing the inherent strength of their nonlinear response. While proposed decades ago, we demonstrate the first experimental realization of a new class of designer nonlinear materials that leverage the interband optical transition in asymmetric structures to provide strong second order susceptibility, $χ^{(2)}$. Using simple AlGaAs/GaAs coupled quantum wells operating in the near-infrared as a prototype, we observed strong second harmonic generation enhancement of 1550 nm to 775 nm over bulk controls. Extracted $χ^{(2)}$ values were as high as 2750 pm/V, which is $>$7x that of bulk GaAs. Furthermore, measured susceptibilities agreed well with quantum mechanical calculations of $χ^{(2)}$ using layer profiles extracted from electron microscopy. Growth interruptions were employed to improve interfacial abruptness in response to electron microscopy characterization, resulting in increased $χ^{(2)}$ toward the simulation predictions for ideal heterointerfaces. More complex layer designs showed predicted $χ^{(2)}$ up to 7 nm/V. Such materials are anticipated to find myriad applications, including entangled photon generation at telecommunications wavelengths for chipscale quantum information processing.

physics.optics↗

arXiv2025

Nonreciprocity in Quantum Technology

Nonreciprocity-the ability to transmit signals in one direction while blocking them in the reverse-has become a powerful resource in quantum technologies, enabling directional amplification, routing of quantum information, and topologically protected quantum states. Recent experimental advances have demonstrated nonreciprocal behavior in low-loss, fully integrated devices operating with weak or no magnetic bias, enabled by synthetic gauge fields, optomechanical interactions, and chiral light-matter coupling. These achievements overcome the limitations of more traditional approaches, making nonreciprocity compatible with superconducting circuits and scalable quantum photonic architectures as well as an integral part of the next generation of modular quantum computers, distributed quantum networks, and precision metrology. Here we highlight the key concepts for engineering nonreciprocity in quantum systems and describe how this functionality can be employed for high-fidelity qubit readout, robust quantum state transfer, and boosting the sensitivity of quantum sensors.

quant-ph↗

arXiv2024

Million-Q Free Space Meta-Optical Resonator at Visible Wavelengths

High-quality (Q)-factor optical resonators with extreme temporal coherence are of both technological and fundamental importance in optical metrology, continuous-wave lasing, and semiconductor quantum optics. Despite extensive efforts in designing high-Q resonators across different spectral regimes, the experimental realization of very large Q-factors at visible wavelengths remains challenging due to the small feature size that is sensitive to fabrication imperfections, and thus is typically implemented in integrated photonics. In the pursuit of free-space optics with the benefits of large space-bandwidth product and massive parallel operations, here we design and fabricate a visible-wavelength etch-free metasurface with minimized fabrication defects and experimentally demonstrate a million-scale ultrahigh-Q resonance. A new laser-scanning momentum-space-resolved spectroscopy technique with extremely high spectral and angular resolution is developed to characterize the record-high Q-factor as well as the dispersion of the million-Q resonance in free space. By integrating monolayer WSe2 into our ultrahigh-Q meta-resonator, we further demonstrate laser-like highly unidirectional and narrow-linewidth exciton emission, albeit without any operating power density threshold. Under continuous-wave laser pumping, we observe pump-power-dependent linewidth narrowing at room temperature, indicating the potential of our meta-optics platform in controlling coherent quantum light-sources. Our result also holds great promise for applications like optical sensing, spectral filtering, and few-photon nonlinear optics.

physics.optics↗

arXiv2024

Intersubband polaritonic metasurfaces for high-contrast ultra-fast power limiting and optical switching

Nonlinear intersubband polaritonic metasurfaces support one of the strongest known ultrafast nonlinear responses in the mid-infrared frequency range across all condensed matter systems. Beyond harmonic generation and frequency mixing, these nonlinearities can be leveraged for ultrafast optical switching and power limiting, based on tailored transitions from strong to weak polaritonic coupling. Here, we demonstrate synergistic optimization of materials and photonic nanostructures to achieve large reflection contrast in ultrafast polaritonic metasurface limiters. The devices are based on optimized semiconductor heterostructure materials that minimize the intersubband transition linewidth and reduce absorption in optically saturated nanoresonators, achieving a record-high reflection contrast of 54% experimentally. We also discuss opportunities to further boost the metrics of performance of this class of ultrafast limiters, showing that reflection contrast as high as 94% may be realistically achieved using all-dielectric intersubband polaritonic metasurfaces.

physics.optics↗

arXiv2023

Spatio-Temporal Coupled Mode Theory for Nonlocal Metasurfaces

Diffractive nonlocal metasurfaces have recently opened a broad range of exciting developments in nanophotonics research and applications, leveraging spatially extended (yet locally patterned) resonant modes to control light with new degrees of freedom. While conventional grating responses are elegantly captured by temporal coupled mode theory (TCMT), TCMT is not well equipped to capture the more sophisticated responses observed in the nascent field of nonlocal metasurfaces. Here, we introduce spatio-temporal coupled mode theory (STCMT), capable of elegantly capturing the key features of the resonant response of wavefront-shaping nonlocal metasurfaces. This framework can quantitatively guide nonlocal metasurface design, and is compatible with local metasurface frameworks, making it a powerful tool to rationally design and optimize a broad class of ultrathin optical components. We validate this STCMT framework against full-wave simulations of various nonlocal metasurfaces, demonstrating that this tool offers a powerful semi-analytical framework to understand and model the physics and functionality of these devices, without the need for computationally intense full-wave simulations. We also discuss how this model may shed physical insights into nonlocal phenomena in photonics and into the functionality of the resulting devices. As a relevant example, we showcase STCMT's flexibility by applying it to study and rapidly prototype nonlocal metasurfaces that spatially shape thermal emission.

physics.optics↗

arXiv2023

Lower Bounds to the Q factor of Electrically Small Resonators through Quasistatic Modal Expansion

The problem of finding the optimal current distribution supported by small radiators yielding the minimum quality (Q) factor is a fundamental problem in electromagnetism. Q factor bounds constrain the maximum operational bandwidth of devices including antennas, metamaterials, and nanoresonators, and have been featured in seminal papers in the past decades. Here, we determine the lower bounds of Q factors of small-size plasmonic and high-permittivity dielectric resonators, which are characterized by quasi-electrostatic and quasi-magnetostatic natural modes, respectively. We expand the induced current density field in the resonator in terms of these modes, leading to closed-form analytical expressions for the electric and magnetic polarizability tensors, whose largest eigenvalue is directly linked to the minimum Q factor. Our results allow also to determine in closed form the corresponding optimal current density field. In particular, when the resonator exhibits two orthogonal reflection symmetries the minimum Q factor can be simply obtained from the Q factors of the single current modes with non-vanishing dipole moments aligned along the major axis of the resonator. Overall, our results open exciting opportunities in the context of nano-optics and metamaterials, facilitating the analysis and design of optimally shaped resonators for enhanced and tailored light-matter interactions.

physics.optics↗

arXiv2021

On the bandwidth of singular plasmonic resonators in relation to the Chu limit

Plasmonic nanostructures with singular geometries can exhibit a broadband scattering response that at first glance appears to violate the lower bounds for the radiation quality (Q) factor of small radiators, known as the Chu limit. Here we explore this apparent contradiction, investigating the Q factor of the resonant modes supported by two nearly touching cylinders, and analyze how their fractional bandwidth fares in relation to the Chu limit. We first derive lower bounds for the radiation Q factors of two-dimensional objects of arbitrary cross-section. We then discuss the dissipation and radiation Q factors associated with the plasmonic resonances of a cylinder dimer as a function of its gap size. We show that the radiation Q factor is always larger than the minimum Q and, as long as the peaks in the scattering spectrum are well separated, their bandwidth is equal to the inverse of their Q factor. In the limit of touching cylinders, the resonance spectra transition from discrete to a continuum around an accumulation point, yielding a broadband response for any finite level of material loss. Within any given frequency interval, the response is the result of a multitude of plasmon resonances, each individually obeying the Chu limit. Nevertheless, the connection between the Q factor and the overall bandwidth of the scattering response is lost. Our study sheds light onto the exotic resonant phenomena emerging when plasmonic materials are shaped in singular geometries, and outlines their opportunities and limitations for nanophotonics.

physics.optics↗

arXiv2018

Nonreciprocal Cavities and the Time-Bandwidth Limit

The time-bandwidth limit inherently relates the lifetime of a resonance and its spectral bandwidth, with direct implications on the maximum storage time of a pulse versus its frequency content. It has been recently argued that nonreciprocal cavities may overcome this constraint, by breaking the strict equality of their incoupling and outcoupling coefficients. Here, we generally study the implications of nonreciprocity on resonant cavities and derive general relations, stemming from microscopic reversibility, that govern their dynamics. We show that nonreciprocal cavities do not provide specific advantages in terms of the time-bandwidth limit, but they may have other attractive properties for nanophotonic systems.

physics.optics↗

arXiv2017

Imaging a Nitrogen-Vacancy Center with a Diamond Immersion Metalens

Solid-state quantum emitters have emerged as robust single-photon sources and addressable spins: key components in rapidly developing quantum technologies for broadband magnetometry, biological sensing, and quantum information science. Performance in these applications, be it magnetometer sensitivity or quantum key generation rate, is limited by the number of photons detected. However, efficient collection of a quantum emitter's photoluminescence (PL) is challenging as its atomic scale necessitates diffraction-limited imaging with nanometer-precision alignment, oftentimes at cryogenic temperatures. In this letter, we image an individual quantum emitter, an isolated nitrogen-vacancy (NV) center in diamond, using a dielectric metalens composed of subwavelength pillars etched into the diamond's surface. The metalens eliminates the need for an objective by operating as a high-transmission-efficiency immersion lens with a numerical aperture (NA) greater than 1.0. This design provides a scalable approach for fiber coupling solid-state quantum emitters that will enable the development of deployable quantum devices.

physics.optics↗

arXiv2016

Indirect to direct bandgap transition in methylammonium lead halide perovskite

Methylammonium lead iodide perovskites are considered direct bandgap semiconductors. Here we show that in fact they present a weakly indirect bandgap 60 meV below the direct bandgap transition. This is a consequence of spin-orbit coupling resulting in Rashba-splitting of the conduction band. The indirect nature of the bandgap explains the apparent contradiction of strong absorption and long charge carrier lifetime. Under hydrostatic pressure from ambient to 325 MPa, Rashba splitting is reduced due to a pressure induced ordering of the crystal structure. The nature of the bandgap becomes increasingly more direct, resulting in five times faster charge carrier recombination, and a doubling of the radiative efficiency. At hydrostatic pressures above 325 MPa, MAPI undergoes a reversible phase transition resulting in a purely direct bandgap semiconductor. The pressure-induced changes suggest epitaxial and synthetic routes to higher efficiency optoelectronic devices.

cond-mat.mtrl-sci↗