SearcharxivSearch

arXiv subjects

Sandra Stroj

Publications and source records attributed to Sandra Stroj.

15 recordsLinked to original sources

Cascaded Metasurface Interferometer for Multipath Interference with Classical and Quantum Light

Beamsplitters represent fundamental components in both classical and quantum optical systems, enabling the distribution of light, as well as the generation of interference, superposition and entanglement. However, optical networks constructed from conventional bulk 2x2-beamsplitters encounter inherent scalability issues, as the number of required beamsplitters scales quadratically with the number of optical modes for a fully connected network. Metasurfaces offer a promising route to overcome these constraints. By manipulating light at the wavelength scale compact optical components with advanced functionalities can be constructed, which address several modes simultaneously. In this work, we design and experimentally utilize a metasurface as a multiport beamsplitter. Furthermore, we realize a multimode interferometer composed of two cascaded metasurfaces. We characterize the individual and cascaded metasurfaces using classical light, showing controllable splitting ratios through tunable phase relations. We then expand the approach to quantum light, employing single photons to demonstrate second- and third-order photon correlations, as well as single photon interference across multiple spatial paths. These results establish metasurface-based multiport beamsplitters as a scalable and reconfigurable platform bridging classical and quantum photonics.

physics.optics

A complete fs-laser-ablation route to miniaturized single-crystal PMN-PT piezoelectric actuators

This article presents a novel fabrication route for miniaturized piezoelectric actuators that relies exclusively on processes based on femtosecond (fs) laser ablation. Previous work has already demonstrated that fs-lasers are uniquely suited for the fabrication of piezoelectric actuators based on PMN-PT, which are required for multiaxial strain-tuning of quantum dots (QDs) to enable, e.g. the generation of highly entangled photon pairs. Building on these foundations, the present work advances actuator performance and capabilities by introducing a local thinning strategy. This approach allows the realization of smaller devices, which in turn enables lower operating voltages, while simultaneously offering the possibility of integrating multiple quantum light sources on a single chip. The article provides a detailed description of the full fabrication chain, entirely based on fs-laser processing steps, from substrate thinning to metal layer structuring and final device definition. A particular focus is placed on the final cutting process, where the implementation of a third-harmonic ultraviolet (UV) fs-laser wavelength significantly improves edge quality and shape definition compared to the second harmonic (SH) wavelength used in previous work. The device fabricated through the combination of local thinning and UV-based cutting promises not only to enhance the efficiency of strain transfer but also to ensure the mechanical stability required for practical applications. These results establish fs-laser-based fabrication as a versatile and scalable method for next-generation piezoelectric actuators, paving the way for advanced strain-engineering approaches in semiconductor quantum optics and integrated quantum photonics.

physics.app-ph

All-photonic entanglement swapping with remote quantum dots

Entanglement swapping is a protocol that details how to create entanglement between previously uncorrelated particles. Its all-photonic version - mediated by the interference of photon pairs generated by separate quantum systems-finds disparate applications in quantum networks. So far, all-photonic entanglement swapping between remote systems has been implemented only using sources that operate probabilistically. However, the scaling up of quantum networks requires deterministic quantum emitters that do not suffer from a trade-off between degree of entanglement and photonpair generation rate. Here, we demonstrate all-photonic entanglement swapping using photon-pairs generated by two separate GaAs quantum dots. The emitters are deterministically embedded in hybrid semiconductor-piezoelectric devices that make the entangled-photons from two dissimilar quantum dots nearly identical. Entanglement swapping is demonstrated with a fidelity as high as 0.71(2), more than 10 standard deviations above the classical limit. The experimental data are quantitatively explained by a theoretical model that also suggests how to boost the protocol performances. Our work opens the path to the exploitation of quantum dot entangled-photon sources in quantum repeater networks.

quant-ph

Ability of entanglement and purity to help to detect systematic experimental errors

Measurements are central in all quantitative sciences, and a fundamental challenge is to make observations without systematic measurement errors. This holds in particular for quantum information processing, where other error sources, such as noise and decoherence, are unavoidable. Consequently, methods for detecting systematic errors have been developed, but the required quantum state properties are yet unexplored. We theoretically develop a direct and efficient method to detect systematic errors in quantum experiments and demonstrate it experimentally using quantum state tomography of photon pairs emitted from a semiconductor quantum dot. Our method can be scaled to multi-qubit systems, and we find that entanglement and quantum states with high purity can help identify systematic errors.

quant-ph

Quantum teleportation with dissimilar quantum dots over a hybrid quantum network

Photonic quantum information processing in metropolitan quantum networks lays the foundation for cloud quantum computing [1, 2], secure communication [3, 4], and the realization of a global quantum internet [5, 6]. This paradigm shift requires on-demand and high-rate generation of flying qubits and their quantum state teleportation over long distances [7]. Despite the last decade has witnessed an impressive progress in the performances of deterministic photon sources [8-11], the exploitation of distinct quantum emitters to implement all-photonic quantum teleportation among distant parties has remained elusive. Here, we overcome this challenge by using dissimilar quantum dots whose electronic and optical properties are engineered by light-matter interaction [12], multi-axial strain [13] and magnetic fields [14] so as to make them suitable for the teleportation of polarization qubits. This is demonstrated in a hybrid quantum network harnessing both fiber connections and 270 m free-space optical link connecting two buildings of the University campus in the center of Rome. The protocol exploits GPS-assisted synchronization, ultra-fast single photon detectors as well as stabilization systems that compensate for atmospheric turbulence. The achieved teleportation state fidelity reaches up to 82+-1%, above the classical limit by more than 10 standard deviations. Our field demonstration of all-photonic quantum teleportation opens a new route to implement solid-state based quantum relays and builds the foundation for practical quantum networks.

quant-ph

Wavevector-resolved polarization entanglement from radiative cascades

The generation of entangled photons from radiative cascades has enabled milestone experiments in quantum information science with several applications in photonic quantum technologies. Significant efforts are being devoted to pushing the performances of near-deterministic entangled-photon sources based on single quantum emitters often embedded in photonic cavities, so to boost the flux of photon pairs. The general postulate is that the emitter generates photons in a nearly maximally entangled state of polarization, ready for application purposes. Here, we demonstrate that this assumption is unjustified. We show that in radiative cascades there exists an interplay between photon polarization and emission wavevector, strongly affecting quantum correlations when emitters are embedded in micro-cavities. We discuss how the polarization entanglement of photon pairs from a biexciton-exciton cascade in quantum dots strongly depends on their propagation wavevector, and it can even vanish for large emission angles. Our experimental results, backed by theoretical modelling, yield a brand-new understanding of cascaded emission for various quantum emitters. In addition, our model provides quantitative guidelines for designing optical microcavities that retain both a high degree of entanglement and collection efficiency, moving the community one step further towards an ideal source of entangled photons for quantum technologies.

quant-ph

Strain-induced dynamic control over the population of quantum emitters in two-dimensional materials

The discovery of quantum emitters (QEs) in two-dimensional materials (2D) has triggered a surge of research to assess their suitability for quantum photonics. While their microscopic origin is still the subject of intense studies, position-controlled QEs are routinely fabricated using static strain gradients, which are used to drive excitons towards localized regions of the crystal where quantum light emission takes place. However, the use of strain in a dynamic fashion to control the brightness of single-photon sources in 2D materials has not been explored so far. In this work, we address this challenge by introducing a novel hybrid semiconductorpiezoelectric device in which WSe2 monolayers are integrated onto piezoelectric pillars that provide both static and dynamic strains. The static strains are first used to induce the formation of QEs, whose emission shows photon anti-bunching. Their energy and brightness are then controlled via the application of voltages to the piezoelectric pillars. Numerical simulations combined with drift-diffusion equations show that these effects are due to a strain-induced modification of the confining-potential landscape, which in turn leads to a net redistribution of excitons among the different QEs. Our work provides a method to dynamically control the brightness of single photon sources based on 2D materials.

cond-mat.mtrl-sci

A source of entangled photons based on a cavity-enhanced and strain-tuned GaAs quantum dot

A quantum-light source that delivers photons with a high brightness and a high degree of entanglement is fundamental for the development of efficient entanglement-based quantum-key distribution systems. Among all possible candidates, epitaxial quantum dots are currently emerging as one of the brightest sources of highly entangled photons. However, the optimization of both brightness and entanglement currently requires different technologies that are difficult to combine in a scalable manner. In this work, we overcome this challenge by developing a novel device consisting of a quantum dot embedded in a circular Bragg resonator, in turn, integrated onto a micromachined piezoelectric actuator. The resonator engineers the light-matter interaction to empower extraction efficiencies up to 0.69(4). Simultaneously, the actuator manipulates strain fields that tune the quantum dot for the generation of entangled photons with corrected fidelities to a maximally entangled state up to 0.96(1). This hybrid technology has the potential to overcome the limitations of the key rates that plague QD-based entangled sources for entanglement-based quantum key distribution and entanglement-based quantum networks.

quant-ph

Beyond the four-level model: Dark and hot states in quantum dots degrade photonic entanglement

Entangled photon pairs are essential for a multitude of photonic quantum applications. To date, the best performing solid-state quantum emitters of entangled photons are semiconductor quantum dots operated around liquid-helium temperatures. To favor the widespread deployment of these sources, it is important to explore and understand their behavior at temperatures accessible with compact Stirling coolers. Here we study the polarization entanglement among photon pairs from the biexciton-exciton cascade in GaAs quantum dots at temperatures up to 65 K. We observe entanglement degradation accompanied by changes in decay dynamics, which we ascribe to thermal population and depopulation of hot and dark states in addition to the four levels relevant for photon pair generation. Detailed calculations considering the presence and characteristics of the additional states and phonon-assisted transitions support the interpretation. We expect these results to guide the optimization of quantum dots as sources of highly entangled photons at elevated temperatures.

quant-ph

Signatures of the Optical Stark Effect on Entangled Photon Pairs from Resonantly-Pumped Quantum Dots

Two-photon resonant excitation of the biexciton-exciton cascade in a quantum dot generates highly polarization-entangled photon pairs in a near-deterministic way. However, the ultimate level of achievable entanglement is still debated. Here, we observe the impact of the laser-induced AC-Stark effect on the quantum dot emission spectra and on entanglement. For increasing pulse-duration/lifetime ratios and pump powers, decreasing values of concurrence are recorded. Nonetheless, additional contributions are still required to fully account for the observed below-unity concurrence.

quant-ph

Experimental Multi-state Quantum Discrimination in the Frequency Domain with Quantum Dot Light

The quest for the realization of effective quantum state discrimination strategies is of great interest for quantum information technology, as well as for fundamental studies. Therefore, it is crucial to develop new and more efficient methods to implement discrimination protocols for quantum states. Among the others, single photon implementations are more advisable, because of their inherent security advantage in quantum communication scenarios. In this work, we present the experimental realization of a protocol employing a time-multiplexing strategy to optimally discriminate among eight non-orthogonal states, encoded in the four-dimensional Hilbert space spanning both the polarization degree of freedom and photon energy. The experiment, built on a custom-designed bulk optics analyser setup and single photons generated by a nearly deterministic solid-state source, represents a benchmarking example of minimum error discrimination with actual quantum states, requiring only linear optics and two photodetectors to be realized. Our work paves the way for more complex applications and delivers a novel approach towards high-dimensional quantum encoding and decoding operations.

quant-ph

Micromachining of PMN-PT Crystals with Ultrashort Laser Pulses

Lead-magnesium niobate lead-titanate (PMN-PT) has been proven as an excellent material for sensing and actuating applications. The fabrication of advanced ultra-small PMN-PT-based devices relies on the availability of sophisticated procedures for the micro-machining of PMN-PT thin films or bulk substrates. Approaches reported up to date include chemical etching, excimer laser ablation and ion milling. To ensure an excellent device performance, a key mandatory feature for a micro-machining process is to preserve as far as possible the crystalline quality of the substrates; in other words, the fabrication method must induce a low density of cracks and other kind of defects. In this work, we demonstrate a relatively fast procedure for the fabrication of high-quality PMN-PT micro-machined actuators employing green femtosecond laser pulses. The fabricated devices feature absence of extended cracks and well defined edges with relatively low roughness, which is advantageous for the further integration of nanomaterials onto the piezoelectric actuators.

physics.app-ph

Strain-Tuning of the Optical Properties of Semiconductor Nanomaterials by Integration onto Piezoelectric Actuators

The tailoring of the physical properties of semiconductor nanomaterials by strain has been gaining increasing attention over the last years for a wide range of applications such as electronics, optoelectronics and photonics. The ability to introduce deliberate strain fields with controlled magnitude and in a reversible manner is essential for fundamental studies of novel materials and may lead to the realization of advanced multi-functional devices. A prominent approach consists in the integration of active nanomaterials, in thin epitaxial films or embedded within carrier nanomembranes, onto Pb(Mg1/3Nb2/3)O3-PbTiO3-based piezoelectric actuators, which convert electrical signals into mechanical deformation (strain). In this review, we mainly focus on recent advances in strain-tunable properties of self-assembled InAs quantum dots embedded in semiconductor nanomembranes and photonic structures. Additionally, recent works on other nanomaterials like rare-earth and metal-ion doped thin films, graphene and MoS2 or WSe2 semiconductor two-dimensional materials are also reviewed. For the sake of completeness, a comprehensive comparison between different procedures employed throughout the literature to fabricate such hybrid piezoelectric-semiconductor devices is presented. Very recently, a novel class of micro-machined piezoelectric actuators have been demonstrated for a full control of in-plane stress fields in nanomembranes, which enables producing energy-tunable sources of polarization-entangled photons in arbitrary quantum dots. Future research directions and prospects are discussed.

cond-mat.mes-hall

Reversible Control of In-plane Elastic Stress Tensor in Nanomembranes

Strain engineering allows the physical properties of materials and devices to be widely tailored, as paradigmatically demonstrated by strained transistors and semiconductor lasers employed in consumer electronics. For this reason, its potential impact on our society has been compared to that of chemical alloying. Although significant progress has been made in the last years on strained nanomaterials, strain fields (which are of tensorial nature, with six independent components) are still mostly used in a "scalar" and/or static fashion. Here we present a new class of strain actuators which allow the three components of the in-plane stress tensor in a nanomembrane to be independently and reversibly controlled. The actuators are based on monolithic piezoelectric substrates, which are micro-machined via femtosecond-laser processing. Their functionality is demonstrated by "programming" arbitrary stress states in a semiconductor layer, whose light emission is used as a local and sensitive strain gauge. The results shown in this work open a new route to investigate and make use of strain effects in materials and devices.

cond-mat.mtrl-sci

Scalable Sources of Entangled Photons with Wavelength on Demand

The prospect of using the quantum nature of light for secure communication keeps spurring the search and investigation of suitable sources of entangled-photons. Semiconductor quantum dots are arguably the most attractive. They can generate indistinguishable entangled-photons deterministically, and are compatible with current photonic-integration technologies, a set of properties not shared by any other entanglement resource. However, as no two quantum dots are identical, they emit entangled-photons with random energies. This hinders their exploitation in communication protocols requiring entangled-states with well-defined energies. Here, we introduce scalable quantum-dot-based sources of polarization-entangled-photons whose energy can be controlled via dynamic strain-engineering without degrading the degree of entanglement of the source. As a test-bench, we interface quantum dots with clouds of atomic vapours, and we demonstrate slow-entangled-photons from a single quantum emitter. These results pave the way towards the implementation of hybrid quantum networks where entanglement is distributed among distant parties using scalable optoelectronic devices.

cond-mat.mes-hall