arXiv subjects

Sanshui Xiao

Publications and source records attributed to Sanshui Xiao.

At least 55 records · Page 3Linked to original sources

arXiv2012

Surface-enhanced Raman spectroscopy (SERS): nonlocal limitations

Giant field enhancement and field singularities are a natural consequence of the commonly employed local-response framework. We show that a more general nonlocal treatment of the plasmonic response leads to new and possibly fundamental limitations on field enhancement with important consequences for our understanding of SERS. The intrinsic length scale of the electron gas serves to smear out assumed field singularities, leaving the SERS enhancement factor finite even for geometries with infinitely sharp features. For silver nano-groove structures, mimicked by periodic arrays of half-cylinders (up to 120 nm in radius), we find no enhancement factors exceeding ten orders of magnitude (10^10).

physics.optics↗

arXiv2010

Field enhancement at metallic interfaces due to quantum confinement

We point out an apparently overlooked consequence of the boundary conditions obeyed by the electric displacement vector at air-metal interfaces: the continuity of the normal component combined with the quantum mechanical penetration of the electron gas in the air implies the existence of a surface on which the dielectric function vanishes. This, in turn, leads to an enhancement of the normal component of the total electric field. We study this effect for a planar metal surface, with the inhomogenous electron density accounted for by a Jellium model. We also illustrate the effect for equilateral triangular nanoislands via numerical solutions of the appropriate Maxwell equations, and show that the field enhancement is several orders of magnitude larger than what the conventional theory predicts.

cond-mat.mes-hall↗

arXiv2010

Nearly-zero transmission through periodically modulated ultrathin metal films

Transmission of light through an optically ultrathin metal film with a thickness comparable to its skin depth is significant. We demonstrate experimentally nearly-zero transmission of light through a film periodically modulated by a one-dimensional array of subwavelength slits. The suppressed optical transmission is due to the excitation of surface plasmon polaritons and the zero-transmission phenomenon is strongly dependent on the polarization of the incident wave.

physics.optics↗

arXiv2009

Material Limitations on the Detection Limit in Refractometry

We discuss the detection limit for refractometric sensors relying on high-Q optical cavities and show that the ultimate classical detection limit is given by min{Dn} > eta with n+i*eta being the complex refractive index of the material under refractometric investigation. Taking finite Q factors and filling fractions into account, the detection limit declines. As an example we discuss the fundamental limits of silicon-based high-Q resonators, such as photonic crystal resonators, for sensing in a bio-liquid environment, such as a water buffer. In the transparency window of silicon the detection limit becomes almost independent on the filling fraction, while in the visible, the detection limit depends strongly on the filling fraction because silicon absorbs strongly.

physics.optics↗

arXiv2009

Enhanced transmission of transverse electric waves through periodic arrays of structured subwavelength apertures

Transmission through sub-wavelength apertures in perfect metals is expected to be strongly suppressed. However, by structural engineering of the apertures, we numerically demonstrate that the transmission of transverse electric waves through periodic arrays of subwavelength apertures in a thin metallic film can be significantly enhanced. Based on equivalent circuit theory analysis, periodic arrays of square structured subwavelength apertures are obtained with a 1900-fold transmission enhancement factor when the side length $a$ of the apertures is 10 times smaller than the wavelength ($a/λ=0.1$). By examining the induced surface currents and investigating the influence of the lattice constant and the incident angle to the resonant frequency, we show that the enhancement is due to the excitation of the strong localized resonant modes of the structured apertures.

physics.optics↗

arXiv2008

Limits of slow-light in photonic crystals

While ideal photonic crystals would support modes with a vanishing group velocity, state-of-the art structures have still only provided a slow-down by roughly two orders of magnitude. We find that the induced density of states caused by lifetime broadening of the electromagnetic modes results in the group velocity acquiring a finite value above zero at the band gap edges, while attaining superluminal values within the band gap. Simple scalings of the minimum and maximum group velocities with the imaginary part of the dielectric function or, equivalently, the linewidth of the broadened states, are presented. The results obtained are entirely general and may be applied to any effect which results in a broadening of the electromagnetic states, such as loss, disorder, finite-size effects, etc. This significantly limits the reduction in group velocity attainable via photonic crystals.

physics.optics↗

arXiv2008

Resonant-tunnelling-assisted crossing for subwavelength plasmonic slot waveguides

We theoretically investigate the properties of crossing for two perpendicular subwavelength plasmonic slot waveguides. We show that, when encountering nano intersection, the crosstalk for the direct crossing is around 25%, almost same as throughout. In terms of symmetry considerations and resonant-tunnelling effect, we design compact cavity-based structures. Our results show that the crosstalk is eliminated and the throughput reaches the unity on resonance. Simulations results are in agreement with those from the coupled-model theory. When taking into account of the material loss, due to the unchanged symmetry properties of the modes, the crosstalk is still suppressed. Our results may open a way to construct nanoscale crossings for high-density nanoplasmonic integration circuits.

physics.optics↗

arXiv2008

Nanostructure design for surface-enhanced Raman spectroscopy - prospects and limits

Surface-enhanced Raman spectroscopy (SERS) allows single-molecule detection due to the strong field localization occurring at sharp bends or kinks of the metal-vacuum interface. An important question concerns the limits of the signal enhancement that can be achieved via a judicious design of the surface. By using a specific example of a technologically realizable nanopatterned surface, we demonstrate that while very high enhancement factors (~10^12) can be found for an ideal surface, these are unlikely to be achieved in laboratory samples, because even a minute, inevitable rounding-off strongly suppresses the enhancement, as well as shifts the optimal frequency. Our simulations indicate that the geometric enhancement factors are unlikely to exceed ~10^8 for real samples, and that it is necessary to consider the geometric uncertainty to reliably predict the frequency for maximum enhancement.

physics.optics↗

arXiv2008

Slow-light enhanced absorption for bio-chemical sensing applications: potential of low-contrast lossy materials

Slow-light enhanced absorption in liquid-infiltrated photonic crystals has recently been proposed as a route to compensate for the reduced optical path in typical lab-on-a-chip systems for bio-chemical sensing applications. A simple perturbative expression has been applied to ideal structures composed of lossless dielectrics. In this work we study the enhancement in structures composed of lossy dielectrics such as a polymer. For this particular sensing application we find that the material loss has an unexpected limited drawback and surprisingly, it may even add to increase the bandwidth for low-index contrast systems such as polymer devices.

physics.optics↗

arXiv2007

Liquid-infiltrated photonic crystals - enhanced light-matter interactions for lab-on-a-chip applications

Optical techniques are finding widespread use in analytical chemistry for chemical and bio-chemical analysis. During the past decade, there has been an increasing emphasis on miniaturization of chemical analysis systems and naturally this has stimulated a large effort in integrating microfluidics and optics in lab-on-a-chip microsystems. This development is partly defining the emerging field of optofluidics. Scaling analysis and experiments have demonstrated the advantage of micro-scale devices over their macroscopic counterparts for a number of chemical applications. However, from an optical point of view, miniaturized devices suffer dramatically from the reduced optical path compared to macroscale experiments, e.g. in a cuvette. Obviously, the reduced optical path complicates the application of optical techniques in lab-on-a-chip systems. In this paper we theoretically discuss how a strongly dispersive photonic crystal environment may be used to enhance the light-matter interactions, thus potentially compensating for the reduced optical path in lab-on-a-chip systems. Combining electromagnetic perturbation theory with full-wave electromagnetic simulations we address the prospects for achieving slow-light enhancement of Beer-Lambert-Bouguer absorption, photonic band-gap based refractometry, and high-Q cavity sensing.

physics.optics↗

arXiv2007

Enhanced transmission through arrays of subwavelength holes in gold films coated by a finite dielectric layer

Enhanced transmissions through a gold film with arrays of subwavelength holes are theoretically studied, employing the rigid full vectorial three dimensional finite difference time domain method. Influence of air-holes shape to the transmission is firstly studied, which confirms two different resonances attributing to the enhanced transmission: the localized waveguide resonance and periodic surface plasmon resonances. For the film coated with dielectric layers, calculated results show that in the wavelength region of interest the localized waveguide resonant mode attributes to sensing rather than the periodic gold-glass surface plasmon mode. Although the detected peak is fairly broad and the shift is not too pronounced, we emphasize the contribution for sensing from the localized waveguide resonant mode, which may opens up new ways to design surface plasmon based sensors.

physics.optics↗

arXiv2007

Slow-light enhancement of Beer-Lambert-Bouguer absorption

We theoretically show how slow light in an optofluidic environment facilitates enhanced light-matter interactions, by orders of magnitude. The proposed concept provides strong opportunities for improving existing miniaturized chemical absorbance cells for Beer-Lambert-Bouguer absorption measurements widely employed in analytical chemistry.

physics.optics↗

arXiv2007

Proposal of highly sensitive optofluidic sensors based on dispersive photonic crystal waveguides

Optofluidic sensors based on highly dispersive two-dimensional photonic crystal waveguides are theoretically studied. Results show that these structures are strongly sensitive to the refractive index of the infiltrated liquid (nl), which is used to tune dispersion of the photonic crystal waveguide. Waveguide mode-gap edge shifts about 1.2 nm for dnl=0.002. The shifts can be explained well by band structure theory combined with first-order perturbation theory. These devices are potentially interesting for chemical sensing applications.

physics.optics↗

arXiv2007

Liquid-infiltrated photonic crystals: Ohmic dissipation and broadening of modes

The pronounced light-matter interactions in photonic crystals make them interesting as opto-fludic "building blocks" for lab-on-a-chip applications. We show how conducting electrolytes cause dissipation and smearing of the density-of-states, thus altering decay dynamics of excited bio-molecules dissolved in the electrolyte. Likewise, we find spatial damping of propagating modes, of the order dB/cm, for naturally occurring electrolytes such as drinking water or physiological salt water.

physics.optics↗

arXiv2006

Highly dispersive photonic band-gap-edge optofluidic biosensors

Highly dispersive photonic band-gap-edge optofluidic biosensors are studied theoretically. We demonstrate that these structures are strongly sensitive to the refractive index of the liquid, which is used to tune dispersion of the photonic crystal. The upper frequency band-gap edge shifts about 1.8 nm for dn=0.002, which is quite sensitive. Results from transmission spectra agree well with those obtained from the band structure theory.

physics.optics↗

arXiv2006

Mesoscopic magnetism in dielectric photonic crystal meta materials: topology and inhomogeneous broadening

We consider meta materials made from a two-dimensional dielectric rod-type photonic crystal. The magnetic response is studied within the recently developed homogenization theory and we in particular study the effects of topology and inhomogeneous broadening. While topology itself mainly affects the Mie resonance frequency we find that the dispersion in the topological radius R of the dielectric rods may lead to significant inhomogeneous broadening and suppression of the negative-mu phenomena for dR/R0 >> epsilon''/epsilon', with epsilon=epsilon'+i*epsilon'' being the relative dielectric function of the rods.

cond-mat.mes-hall↗

arXiv2006

Resonator channel drop filters in a plasmon-polaritons metal

Channel drop filters in a plasmon-polaritons metal are studied. It shows that light can be efficiently dropped. Results obtained by the FDTD method are consistent with those from coupled mode theory. It also shows, without considering the loss of the metal, that the quality factor for the channel drop system reaches 4000. The quality factor decreases significantly if we take into account the loss, which also leads to a weak drop efficiency.

physics.optics↗

arXiv2005

Study of transmission properties for waveguide bends by use of a circular photonic crystal

We study the transmission properties for the waveguide bends composed by a circular photonic crystal. Two types (Y and U type) of the waveguide bends utilizing the circular photonic crystal are studied. It has been shown, compared with the conventional photonic crystal waveguide bends, transmission properties for these bends can be significantly improved. Over a 6.4% bandwidth, less than 1-dB loss/bend are observed. U bent waveguide, i.e., $180^o$ bend, can be easily realized with low loss using the circular photonic crystal.

physics.optics↗