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Santanu Manna

Publications and source records attributed to Santanu Manna.

At least 19 recordsLinked to original sources

Planar metal-semiconductor Yagi-Uda type antennas for tunable narrow-linewidth quantum dot emitters

Tunable photonic architectures that improve the extraction efficiency of light from embedded epitaxial quantum dots across a wide spectral range are key enablers for developing bright sources of single and indistinguishable photons. In this study, we experimentally demonstrate planar multilayer antenna structures consisting of epitaxially grown AlGaAs and InGaAs membranes containing quantum dots sandwiched between metallic Au (or Ag) reflector and director layers together with Al$_2$O$_3$ spacer layers. We show that the linewidths and fine-structure splitting of the neutral exciton emission remain comparable to those measured in the corresponding unprocessed samples, demonstrating that the fabrication process preserves the optical quality of the emitters. In addition to broadband operation, we demonstrate that the planar architecture is compatible with electrical tuning via integrated diode structures, and strain tuning using piezoelectric actuators. In spite of limitations related to optical losses in the ultrathin metallic layers, the demonstrated fabrication simplicity, scalability, and compatibility with tunable quantum emitters establish planar antennas as a promising platform for solid-state quantum photonic devices.

physics.optics

Towards Stirling cooler operable single-photon sources based on low-noise GaAs quantum dots

For photonic quantum technology applications, sources capable of emitting photons with indistinguishability close to unity are essential. Ideally, these sources should not require demanding cooling systems. Here, we present temperature-dependent two-photon-interference measurements on photons produced by the radiative decay of the negative trion in a low-noise GaAs quantum dot, which are in quantitative agreement with theoretical calculations accounting for carrier-phonon interactions and coupling to excited states. While at at the lowest explored temperatures the emission linewidth reaches values only 6(2) % above the Fourier limit and the indistinguishability I between subsequently emitted photons reaches 0.966(6), the latter drops to 0.05(4) at 55 K. We show that this loss can be explained with the coupling with energetically close excited trion states and suggest that the photon indistinguishability at elevated temperatures can be increased by employing Purcell enhancement of the emission rate or by increasing the energy separation of the excited states. Using cavity-enhanced emission, we experimentally verify the first route and demonstrate an improvement in photon indistinguishability from 0.314(25) to 0.80(3) at 32 K, which - to our knowledge - is the highest reported value at such temperature.

quant-ph

A diode nanocavity for fast, efficient and tunable emission of highly entangled photon pairs and Fourier-transform-limited single photons

Deterministic sources of entangled photon pairs and indistinguishable photons are expected to play a key role in photonic quantum technologies. Semiconductor quantum dots are promising candidates due to their on-demand emission and compatibility with nanophotonic structures. However, current implementations face trade-offs between extraction efficiency, Purcell enhancement, as well as charge noise that causes blinking and degrades indistinguishability. Here we demonstrate a tunable nano-optoelectronic device based on a quantum dot embedded in a p-i-n diode circular-Bragg-grating-resonator and featuring extraction efficiencies up to 0.55(6) and Purcell-factor of $\sim$8. The device generates wavelength-tunable entangled photon pairs with suppressed blinking and raw (corrected) concurrence > 0.89 (0.91) over a range of 1.6 nm. The very same source also emits single, nearly Fourier-limited and highly indistinguishable photons with raw (corrected) $\mathcal{V}_{\text{HOM}}$ = 0.951(4) (0.988(6)). These results demonstrate a viable platform for semiconductor quantum photonics.

quant-ph

Low-density InGaAs/AlGaAs Quantum Dots in Droplet-Etched Nanoholes

Over the past two decades, epitaxial semiconductor quantum dots (QDs) have demonstrated very promising properties as sources of single photons and entangled photons on-demand. Among different growth methods, droplet etching epitaxy has allowed the growth of almost strain-free QDs, with low and controllable surface densities, small excitonic fine structure splitting (FSS), and fast radiative decays. Here, we extend the local droplet etching technique to In(Ga)As QDs in AlGaAs, thereby increasing the achievable emission wavelength range beyond that accessible to GaAs/AlGaAs QDs, while benefiting from the aforementioned advantages of this growth method. We observe QD densities of $\sim 0.2\ μ\mathrm{m}^{-2}$, FSS values as small as $3\ μ\mathrm{eV}$, and short radiative lifetimes of $\sim 300\ \mathrm{ps}$, while extending the achievable emission range to $\sim 920\ \mathrm{nm}$ at cryogenic temperatures. We envision these QDs to be particularly suitable for integrated quantum photonics applications.

physics.app-ph

Few-electron spin qubits in optically active GaAs quantum dots

The knowledge of the energy spectrum completely defines the dynamics of a quantum system for a given initial state. This makes spectroscopy a key characterization technique when studying or designing qubits and complex quantum systems. In semiconductor quantum dots, the electronic quantum states can be probed through charge transport spectroscopy, but the electric current itself disrupts the fragile quantum system, and the technique is practically limited to gate-defined quantum dots. Epitaxial quantum dots benefit from excellent optical properties, but are usually incompatible with charge transport, while alternative spectroscopy techniques provide only limited information. Here we demonstrate a spectroscopy technique which utilizes nuclear spins as a non-invasive probe. By using spin currents instead of the charge currents we achieve near-equilibrium probing. Experiments are conducted on low-strain GaAs/AlGaAs epitaxial dots, revealing energy spectra for charge configurations with up to seven electrons and the subtle properties of the multi-electron states. The rich variety of observations includes long-lived spin-qubit states in s and p shells, ground-state phase transitions, strong spin-orbit coupling regimes, and anomalously fast nuclear spin diffusion. Experiments are backed up by good agreement with the first-principles configuration-interaction numerical modelling. Our work uncovers few-electron states as a new operating regime for optically active quantum dots. Accurate control and probing of many-body states offers a test-bed system for fundamental physics studies, while prospective technological applications include electron spin qubits with extended coherence and scalable electrical control.

cond-mat.mes-hall

Electric-field control of photon indistinguishability in cascaded decays in quantum dots

Photon indistinguishability, entanglement, and antibunching are key ingredients in quantum optics and photonics. Decay cascades in quantum emitters offer a simple method to create entangled photon-pairs with negligible multi-pair generation probability. However, the degree of indistinguishability of the photons emitted in a cascade is intrinsically limited by the lifetime ratio of the involved transitions. Here we show that, for the biexciton-exciton cascade in a quantum dot, this ratio can be widely tuned by an applied electric field. Hong-Ou-Mandel interference measurements of two subsequently emitted biexciton photons show that their indistinguishability increases with increasing field, following the theoretically predicted behavior. At the same time, the emission linewidth stays close to the transform-limit, favoring applications relying on the interference among photons emitted by different sources.

quant-ph

Passive Demultiplexed Two-photon State Generation from a Quantum Dot

High-purity multi-photon states are essential for photonic quantum computing. Among existing platforms, semiconductor quantum dots offer a promising route to scalable and deterministic multi-photon state generation. However, to fully realize their potential we require a suitable optical excitation method. Current approaches of multi-photon generation rely on active polarization-switching elements (e.g., electro-optic modulators, EOMs) to spatio-temporally demultiplex single photons. Yet, the achievable multi-photon rate is fundamentally limited by the switching speed of the EOM. Here, we introduce a fully passive demultiplexing technique that leverages a stimulated two-photon excitation process to achieve switching rates that are only limited by the quantum dot lifetime. We demonstrate this method by generating two-photon states from a single quantum dot without requiring any active switching elements. Our approach significantly reduces the cost of demultiplexing while shifting it to the excitation stage, enabling loss-free demultiplexing and effectively doubling the achievable multi-photon generation rate when combined with existing active demultiplexing techniques.

quant-ph

Storing quantum coherence in a quantum dot nuclear spin ensemble for over 100 milliseconds

States with long coherence are a crucial requirement for qubits and quantum memories. Nuclear spins in epitaxial quantum dots are a great candidate, offering excellent isolation from external environments and on-demand coupling to optical flying qubits. However, coherence times are limited to $\lesssim1$ ms by the dipole-dipole interactions between the nuclei and their quadrupolar coupling to inhomogeneous crystal strain. Here, we combine strain engineering of the nuclear spin ensemble and tailored dynamical decoupling sequences to achieve nuclear spin coherence times exceeding 100 ms. Recently, a reversible transfer of quantum information into nuclear spin ensembles has been demonstrated in quantum dots. Our results provide a path to develop this concept into a functioning solid-state quantum memory suitable for quantum repeaters in optical quantum communication networks.

cond-mat.mes-hall

Refining Boundary Value Problems in Non-local Micropolar Mechanics

This research explores refined boundary conditions for a traction-free surface in a non-local micropolar half-space, combining non-local and micropolar elasticity effects to study Rayleigh wave propagation in an isotropic, homogeneous medium. This study revisits the solution for Rayleigh waves obtained within the framework of Eringen's non-local differential model. It highlights that the equivalence between the non-local differential and integral formulations breaks down for a micropolar half-space and can only be restored under specific additional boundary conditions. For mathematical tractability, equivalence is assumed for a defined subset of stresses. Asymptotic analysis is further employed to capture the effects of the boundary layer within the non-local micropolar half-space. This technique finally derives the refined boundary conditions for micropolar media.

math-ph

Optically Pumped Terahertz Amplitude Modulation in Type-II Ge QD/Si heterostructures grown via Molecular Beam Epitaxy

This article exploits group-IV germanium (Ge) quantum dots (QDs) on Silicon-on-Insulator (SOI) grown by molecular beam epitaxy (MBE) in order to explore its optical behaviour in the Terahertz (THz) regime. In this work, Ge QDs, pumped by an above bandgap near infrared wavelength, exhibit THz amplitude modulation in the frequency range of 0.1-1.0 THz. The epitaxial Ge QDs outperform reference SOI substrate in THz amplitude modulation owing to higher carrier generation in weakly confined dots compared to its bulk counterpart. This is further corroborated using theoretical model based on the non-equilibrium Green's function (NEGF) method. This model enables the calculation of photo carriers generated (PCG) and their confinement in the Ge QD region. Our model also reroutes the calculation from PCG to corresponding plasma frequency and hence to refractive index and THz photo-conductivity. Moreover, the photo-generated confined holes accumulation at the Ge QDs-Si interface is elevated after optical illumination, leading to a decreased THz photo-conductivity. This augmentation in THz photo-conductivity contributes to a significant enhancement of THz modulation depth ~77% at Ge QDs-Si interfaces compared to bare SOI at 0.1 THz.

physics.optics

Tuning the coherent interaction of an electron qubit and a nuclear magnon

A central spin qubit interacting coherently with an ensemble of proximal spins can be used to engineer entangled collective states or a multi-qubit register. Making full use of this many-body platform requires tuning the interaction between the central spin and its spin register. GaAs quantum dots offer a model realization of the central spin system where an electron qubit interacts with multiple ensembles of $\sim 10^{4}$ nuclear spins. In this work, we demonstrate tuning of the interaction between the electron qubit and the nuclear many-body system in a GaAs quantum dot. The homogeneity of the GaAs system allows us to perform high-precision and isotopically selective nuclear sideband spectroscopy, which reveals the single-nucleus electronic Knight field. Together with time-resolved spectroscopy of the nuclear field, this fully characterizes the electron-nuclear interaction for a priori control. An algorithmic feedback sequence selects the nuclear polarization precisely, which adjusts the electron-nuclear exchange interaction in situ via the electronic g-factor anisotropy. This allows us to tune directly the activation rate of a collective nuclear excitation (magnon) and the coherence time of the electron qubit. Our method is applicable to similar central-spin systems and enables the programmable tuning of coherent interactions in the many-body regime.

quant-ph

Many-body quantum register for a spin qubit

Quantum networks require quantum nodes with coherent optical interfaces and multiple stationary qubits. In terms of optical properties, semiconductor quantum dots are highly compelling, but their adoption as quantum nodes has been impaired by the lack of auxiliary qubits. Here, we demonstrate a functional quantum register in a semiconductor quantum dot leveraging the dense, always-present nuclear spin ensemble. We prepare 13,000 host nuclear spins into a single many-body dark state to operate as the register logic state $|0\rangle$. The logic state $|1\rangle$ is defined as a single nuclear magnon excitation, enabling controlled quantum-state transfer between the electron spin qubit and the nuclear magnonic register. Using 130-ns SWAP gates, we implement a full write-store-retrieve-readout protocol with 68.6(4)% raw overall fidelity and a storage time of 130(16) $μ$s in the absence of dynamical decoupling. Our work establishes how many-body physics can add step-change functionality to quantum devices, in this case transforming quantum dots into multi-qubit quantum nodes with deterministic registers.

quant-ph

A source of entangled photons based on a cavity-enhanced and strain-tuned GaAs quantum dot

A quantum-light source that delivers photons with a high brightness and a high degree of entanglement is fundamental for the development of efficient entanglement-based quantum-key distribution systems. Among all possible candidates, epitaxial quantum dots are currently emerging as one of the brightest sources of highly entangled photons. However, the optimization of both brightness and entanglement currently requires different technologies that are difficult to combine in a scalable manner. In this work, we overcome this challenge by developing a novel device consisting of a quantum dot embedded in a circular Bragg resonator, in turn, integrated onto a micromachined piezoelectric actuator. The resonator engineers the light-matter interaction to empower extraction efficiencies up to 0.69(4). Simultaneously, the actuator manipulates strain fields that tune the quantum dot for the generation of entangled photons with corrected fidelities to a maximally entangled state up to 0.96(1). This hybrid technology has the potential to overcome the limitations of the key rates that plague QD-based entangled sources for entanglement-based quantum key distribution and entanglement-based quantum networks.

quant-ph

Quantum non-demolition measurement of an electron spin qubit through its low-energy many-body spin environment

The measurement problem dates back to the dawn of quantum mechanics. Here, we measure a quantum dot electron spin qubit through off-resonant coupling with thousands of redundant nuclear spin ancillae. We show that the link from quantum to classical can be made without any "wavefunction collapse", in agreement with the Quantum Darwinism concept. Large ancilla redundancy allows for single-shot readout with high fidelity $\approx99.85\%$. Repeated measurements enable heralded initialization of the qubit and probing of the equilibrium electron spin dynamics. Quantum jumps are observed and attributed to burst-like fluctuations in a thermally populated phonon bath.

cond-mat.mes-hall

Approaching a fully-polarized state of nuclear spins in a semiconductor quantum dot

Magnetic noise of atomic nuclear spins is a major problem for solid state spin qubits. Highly-polarized nuclei would not only overcome this obstacle, but also make nuclear spins a useful quantum information resource. However, achieving sufficiently high nuclear polarizations has remained an evasive goal. Here we implement a nuclear spin polarization protocol which combines strong optical pumping and fast electron tunneling. Polarizations well above 95% are generated in GaAs semiconductor quantum dots on a timescale of 1 minute. The technique is compatible with standard quantum dot device designs, where highly-polarized nuclear spins can simplify implementations of quantum bits and memories, as well as offer a testbed for studies of many-body quantum dynamics and magnetism.

cond-mat.mes-hall

Beyond the four-level model: Dark and hot states in quantum dots degrade photonic entanglement

Entangled photon pairs are essential for a multitude of photonic quantum applications. To date, the best performing solid-state quantum emitters of entangled photons are semiconductor quantum dots operated around liquid-helium temperatures. To favor the widespread deployment of these sources, it is important to explore and understand their behavior at temperatures accessible with compact Stirling coolers. Here we study the polarization entanglement among photon pairs from the biexciton-exciton cascade in GaAs quantum dots at temperatures up to 65 K. We observe entanglement degradation accompanied by changes in decay dynamics, which we ascribe to thermal population and depopulation of hot and dark states in addition to the four levels relevant for photon pair generation. Detailed calculations considering the presence and characteristics of the additional states and phonon-assisted transitions support the interpretation. We expect these results to guide the optimization of quantum dots as sources of highly entangled photons at elevated temperatures.

quant-ph

Nuclear spin diffusion in the central spin system of a GaAs/AlGaAs quantum dot

The spin diffusion concept provides a classical description of a purely quantum-mechanical evolution in inhomogeneously polarized many-body systems such as nuclear spin lattices. The central spin of a localized electron alters nuclear spin diffusion in a way that is still poorly understood. In contrast to previous predictions, we show experimentally that in GaAs/AlGaAs quantum dots the electron spin accelerates nuclear spin diffusion, without forming any Knight field gradient barrier. Such acceleration is present even at high magnetic fields, which we explain as a result of electron spin-flip fluctuations. Diffusion-limited nuclear spin lifetimes range between 1 and 10 s, providing plenty of room for recent proposals seeking to store and process quantum information using quantum dot nuclear spins.

cond-mat.mes-hall

Ideal refocusing of an optically active spin qubit under strong hyperfine interactions

Combining highly coherent spin control with efficient light-matter coupling offers great opportunities for quantum communication and networks, as well as quantum computing. Optically active semiconductor quantum dots have unparalleled photonic properties, but also modest spin coherence limited by their resident nuclei. Here, we demonstrate that eliminating strain inhomogeneity using lattice-matched GaAs-AlGaAs quantum dot devices prolongs the electron spin coherence by nearly two orders of magnitude, beyond 0.113(3) ms. To do this, we leverage the 99.30(5)% fidelity of our optical pi-pulse gates to implement dynamical decoupling. We vary the number of decoupling pulses up to N = 81 and find a coherence time scaling of N^{0.75(2)}. This scaling manifests an ideal refocusing of strong interactions between the electron and the nuclear-spin ensemble, holding the promise of lifetime-limited spin coherence. Our findings demonstrate that the most punishing material science challenge for such quantum-dot devices has a remedy, and constitute the basis for highly coherent spin-photon interfaces.

cond-mat.mes-hall