arXiv subjects

Santiago Tarrago Velez

Publications and source records attributed to Santiago Tarrago Velez.

5 recordsLinked to original sources

arXiv2024

Strong coupling at room temperature with a centimeter-scale quartz crystal

Brillouin-based optomechanical systems with high-frequency acoustic modes provide a promising platform for implementing quantum-information processing and wavelength conversion applications, and for probing macroscopic quantum effects. Achieving strong coupling through electrostrictive Brillouin interaction is essential for coupling the massive mechanical mode to an optical field, thereby controlling and characterizing the mechanical state. However, achieving strong coupling at room temperature has proven challenging due to fast mechanical decay rates, which increase the pumping power required to surpass the coupling threshold. Here, we report an optomechanical system with independent control over pumping power and frequency detuning to achieve and characterize the strong-coupling regime of a bulk acoustic-wave resonator. Through spectral analysis of the cavity reflectivity, we identify clear signatures of strong coupling, i.e., normal-mode splitting and an avoided crossing in the detuned spectra, while estimating the mechanical linewidth $Γ_m/2π~=~7.13MHz$ and the single-photon coupling rate $g_0/2π~=~7.76Hz$ of our system. Our results provide valuable insights into the performances of room-temperature macroscopic mechanical systems and their applications in hybrid quantum devices.

quant-ph↗

arXiv2022

Measurement-Induced Collective Vibrational Quantum Coherence under Spontaneous Raman Scattering in a Liquid

Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered field lacks any predictable phase relationship with the incoming field. When probing an ensemble of molecules, the question therefore arises: What quantum state should be used to describe the molecular ensemble following spontaneous Stokes scattering? We experimentally address this question by measuring time-resolved Stokes--anti-Stokes two-photon coincidences on a molecular liquid consisting of several sub-ensembles with slightly different vibrational frequencies. When spontaneously scattered Stokes photons and subsequent anti-Stokes photons are detected into a single spatiotemporal mode, the observed dynamics is inconsistent with a statistical mixture of individually excited molecules. Instead, we show that the data are reproduced if Stokes--anti-Stokes correlations are mediated by a collective vibrational quantum, i.e. a coherent superposition of all molecules interacting with light. Our results demonstrate that the degree of coherence in the vibrational state of the liquid is not an intrinsic property of the material system, but rather depends on the optical excitation and detection geometry.

quant-ph↗

arXiv2021

Bell correlations between light and vibration at ambient conditions

Time-resolved Raman spectroscopy techniques offer various ways to study the dynamics of molecular vibrations in liquids or gases and optical phonons in crystals. While these techniques give access to the coherence time of the vibrational modes, they are not able to reveal the fragile quantum correlations that are spontaneously created between light and vibration during the Raman interaction. Here, we present a scheme leveraging universal properties of spontaneous Raman scattering to demonstrate Bell correlations between light and a collective molecular vibration. We measure the decay of these hybrid photon-phonon Bell correlations with sub-picosecond time resolution and find that they survive over several hundred oscillations at ambient conditions. Our method offers a universal approach to generate entanglement between light and molecular vibrations. Moreover, our results pave the way for the study of quantum correlations in more complex solid-state and molecular systems in their natural state.

quant-ph↗

arXiv2019

Preparation and decay of a single quantum of vibration at ambient conditions

A single quantum of excitation of a mechanical oscillator is a textbook example of the principles of quantum physics. Mechanical oscillators, despite their pervasive presence in nature and modern technology, do not generically exist in an excited Fock state. In the past few years, careful isolation of GHz-frequency nano-scale oscillators has allowed experimenters to prepare such states at milli-Kelvin temperatures. These developments illustrate the tension between the basic predictions of quantum mechanics that should apply to all mechanical oscillators existing even at ambient conditions, and the complex experiments in extreme conditions required to observe those predictions. We resolve the tension by creating a single Fock state of a vibration mode of a crystal at room temperature using a technique that can be applied to any Raman-active system. After exciting a bulk diamond with a femtosecond laser pulse and detecting a Stokes-shifted photon, the 40~THz Raman-active internal vibrational mode is prepared in the Fock state $|1>$ with $98.5\%$ probability. The vibrational state is read out by a subsequent pulse, which when subjected to a Hanbury-Brown-Twiss intensity correlation measurement reveals the sub-Poisson number statistics of the vibrational mode. By controlling the delay between the two pulses we are able to witness the decay of the vibrational Fock state over its $3.9$ ps lifetime at room temperature. Our technique is agnostic to specific selection rules, and should thus be applicable to any Raman-active medium, opening a new generic approach to the experimental study of quantum effects related to vibrational degrees of freedom in molecules and solid-state systems.

quant-ph↗

arXiv2018

Two-Color Pump-Probe Measurement of Photonic Quantum Correlations Mediated by a Single Phonon

We propose and demonstrate a versatile technique to measure the lifetime of the one-phonon Fock state using two-color pump-probe Raman scattering and spectrally-resolved, time-correlated photon counting. Following pulsed laser excitation, the $n=1$ phonon Fock state is probabilistically prepared by projective measurement of a single Stokes photon. The detection of an anti-Stokes photon generated by a second, time-delayed laser pulse probes the phonon population with sub-picosecond time resolution. We observe strongly non-classical Stokes--anti-Stokes correlations, whose decay maps the single phonon dynamics. Our scheme can be applied to any Raman-active vibrational mode. It can be modified to measure the lifetime of $n \geq 1$ Fock states or the phonon quantum coherences through the preparation and detection of two-mode entangled vibrational states.

quant-ph↗