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Sara Marzban

Publications and source records attributed to Sara Marzban.

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Spectroscopy and Coherence of an Excited-State Transition in Tm$^{3+}$:YAlO$_3$ at Telecommunication Wavelength

We characterize spectroscopic and coherence properties of the 1451.37 nm excited-state zero-phonon line (ZPL) between the $^{3}F_{4}$ and the $^{3}H_{4}$ manifolds of a thulium-doped yttrium aluminum perovskite (Tm$^{3+}$:YAlO$_3$) crystal at temperatures around 1.5 K. We measure the absorption spectrum between the $^{3}H_{6}$ - $^{3}F_{4}$ and $^{3}F_{4}$ - $^{3}H_{4}$ manifolds, the inhomogeneous broadening of the $^{3}F_{4}$ - $^{3}H_{4}$ (excited-state) ZPL, and the lifetimes of the higher-lying and lower-lying excited states. We also investigate level shifts caused by the quadratic Zeeman interaction as well as spectral hole-burning spectra with varying magnetic fields, providing insights into hyperfine interactions. Using again spectral holes but also optical free induction decays (FIDs), we assess optical coherence times, finding a maximum of $4.75 \pm 0.07~μs$ at B=2T and low ion concentration in the $^{3}F_{4}$ level. Our results -- the first to demonstrate coherence of an excited-state transition in a rare-earth crystal -- suggest the possibility of exploiting such transitions for quantum technology.

quant-ph

Certification of linear optical quantum state preparation

Certification is important to guarantee the correct functioning of quantum devices. A key certification task is verifying that a device has produced a desired output state. In this work, we study this task in the context of photonic platforms, where single photons are propagated through linear optical interferometers to create large, entangled resource states for metrology, communication, quantum advantage demonstrations and for so-called linear optical quantum computing (LOQC). This setting derives its computational power from the indistinguishability of the photons, i.e., their relative overlap. Therefore, standard fidelity witnesses developed for distinguishable particles (including qubits) do not apply directly, because they merely certify the closeness to some fixed target state. We introduce a measure of fidelity suitable for this setting and show several different ways to witness it, based on earlier proposals for measuring genuine multi-photon indistinguishability. We argue that a witness based upon the discrete Fourier transform is an optimal choice. We experimentally implement this witness and certify the fidelity of several multi-photon states.

quant-ph

Bosonic statistics enhance Maxwell's demon in photonic experiment

Maxwell's demon elucidates the value of information in thermodynamics, using measurement and feedback: he evolves an equilibrated gas into a nonequilibrium state, from which one might extract work. The demon can evolve the system farther from equilibrium, on average, if the particles obey Bose-Einstein statistics than if they are distinguishable. We experimentally support this decade-and-a-half-old prediction by comparing indistinguishable with distinguishable photons. We use a fully programmable linear-optics platform, whose local photon statistics were shown recently to behave thermally. Our demon nondestructively measures the number of photons in a subset of the modes. Guided by the outcome, he conditionally interchanges the measured and unmeasured modes. This interchange creates a positive temperature difference between a mode in a particular subset and a mode in the other. The temperature difference is greater, on average, if the photons are indistinguishable. This result bolsters a long-standing prediction about the interplay among thermodynamics, information, and quantum particle statistics. Additionally, this work suggests a thermodynamic means of weakly validating boson-sampling platforms.

quant-ph

Experimental demonstration of boson sampling as a hardware accelerator for monte carlo integration

We present an experimental demonstration of boson sampling as a hardware accelerator for Monte Carlo integration. Our approach leverages importance sampling to factorize an integrand into a distribution that can be sampled using quantum hardware and a function that can be evaluated classically, enabling hybrid quantum-classical computation. We argue that for certain classes of integrals, this method offers a quantum advantage by efficiently sampling from probability distributions that are hard to simulate classically. We also identify structural criteria that must be satisfied to preserve computational hardness, notably the sensitivity of the classical post-processing function to high-order quantum correlations. To validate our protocol, we implement a proof-of-principle experiment on a programmable photonic platform to compute the first-order energy correction of a three-boson system in a harmonic trap under an Efimov-inspired three-body perturbation. The experimental results are consistent with theoretical predictions and numerical simulations, with deviations explained by photon distinguishability, discretization, and unitary imperfections. Additionally, we provide an error budget quantifying the impact of these same sources of noise. Our work establishes a concrete use case for near-term photonic quantum devices and highlights a viable path toward practical quantum advantage in scientific computing.

quant-ph

Experimental validation of boson sampling using detector binning

We experimentally demonstrate a testing strategy for boson samplers that is based on efficiently computable expressions for the output photon counting distributions binned over multiple optical modes. We apply this method to validate boson sampling experiments with three photons on a reconfigurable photonic chip, which implements a four-mode interferometer, analyzing 50 Haar-random unitary transformations while tuning photon distinguishability via controlled delays. We show that for high values of indistinguishability, the experiment accurately reproduces the ideal boson sampling binned-mode distributions, which exhibit variations that depend both on the specific interferometer implemented as well as the choice of bin, confirming the usefulness of the method to diagnose imperfections such as partial distinguishability or imperfect chip control. Finally, we analyze the behavior of Haar-averaged binned-mode distributions with partial distinguishability and demonstrate analytically that its variance is proportional to the average of the square of the photons' indistinguishability parameter. These findings highlight the central role of binning in boson sampling validation, offering a scalable and efficient framework for assessing multiphoton interference and experimental performance.

quant-ph

Optical Investigations of Coherence and Relaxation Dynamics of a Thulium-doped Yttrium Gallium Garnet Crystal at sub-Kelvin Temperatures for Optical Quantum Memory

Rare-earth ion-doped crystals are of great interest for quantum memories, a central component in future quantum repeaters. To assess the promise of 1$\%$ Tm$^{3+}$-doped yttrium gallium garnet (Tm:YGG), we report measurements of optical coherence and energy-level lifetimes of its $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$ transition at a temperature of around 500 mK and various magnetic fields. Using spectral hole burning, we find hyperfine ground-level (Zeeman level) lifetimes of several minutes at magnetic fields of less than 1000 G. We also measure coherence time exceeding one millisecond using two-pulse photon echoes. Three-pulse photon echo and spectral hole burning measurements reveal that due to spectral diffusion, the effective coherence time reduces to a few $μ$s over a timescale of around two hundred seconds. Finally, temporal and frequency-multiplexed storage of optical pulses using the atomic frequency comb protocol is demonstrated. Our results suggest Tm:YGG to be promising for multiplexed photonic quantum memory for quantum repeaters.

quant-ph

Frequency tunable, cavity-enhanced single erbium quantum emitter in the telecom band

Single quantum emitters embedded in solid-state hosts are an ideal platform for realizing quantum information processors and quantum network nodes. Among the currently-investigated candidates, Er$^{3+}$ ions are particularly appealing due to their 1.5 $μ$m optical transition in the telecom band as well as their long spin coherence times. However, the long lifetimes of the excited state -- generally in excess of 1 ms -- along with the inhomogeneous broadening of the optical transition result in significant challenges. Photon emission rates are prohibitively small, and different emitters generally create photons with distinct spectra, thereby preventing multi-photon interference -- a requirement for building large-scale, multi-node quantum networks. Here we solve this challenge by demonstrating for the first time linear Stark tuning of the emission frequency of a single Er$^{3+}$ ion. Our ions are embedded in a lithium niobate crystal and couple evanescently to a silicon nano-photonic crystal cavity that provides an up to 143 increase of the measured decay rate. By applying an electric field along the crystal c-axis, we achieve a Stark tuning greater than the ion's linewidth without changing the single-photon emission statistics of the ion. These results are a key step towards rare earth ion-based quantum networks.

quant-ph

A long-lived solid-state optical quantum memory for high-rate quantum repeaters

We argue that long optical storage times are required to establish entanglement at high rates over large distances using memory-based quantum repeaters. Triggered by this conclusion, we investigate the $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$ transition at 795.325 nm of Tm:Y$_3$Ga$_5$O$_{12}$ (Tm:YGG). Most importantly, we show that the optical coherence time can reach 1.1 ms, and, using laser pulses, we demonstrate optical storage based on the atomic frequency comb protocol up to 100 $μ$s as well as a memory decay time T$_M$ of 13.1 $μ$s. Possibilities of how to narrow the gap between the measured value of T$_m$ and its maximum of 275 $μ$s are discussed. In addition, we demonstrate quantum state storage using members of non-classical photon pairs. Our results show the potential of Tm:YGG for creating quantum memories with long optical storage times, and open the path to building extended quantum networks.

quant-ph

The observation of photon echoes from evanescently coupled rare-earth ions in a planar waveguide

We report the measurement of the inhomogeneous linewidth, homogeneous linewidth and spin state lifetime of Pr3+ ions in a novel waveguide architecture. The TeO2 slab waveguide deposited on a bulk Pr3+:Y2SiO5 crystal allows the 3H4 - 1D2 transition of Pr3+ ions to be probed by the optical evanescent field that extends into the substrate. The 2 GHz inhomogeneous linewidth, the optical coherence time of 70 +- 5 us, and the spin state lifetime of 9.8 +- 0.3 s indicate that the properties of ions interacting with the waveguide mode are consistent with those of bulk ions. This result establishes the foundation for large, integrated and high performance rare-earth-ion quantum systems based on a waveguide platform.

quant-ph