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Saswata Roy

Publications and source records attributed to Saswata Roy.

14 recordsLinked to original sources

Exponential quantum advantage for learning signals with a single qubit

Quantum technology has the potential to transform scientific discovery, but quantum advantages often require processing capabilities well beyond the reach of experimental platforms. We show that coupling a single controllable qubit to an otherwise conventional sensor can exponentially reduce the number of measurements required to learn classical signals. These rigorous quantum advantages apply to fundamental sensing tasks, including learning Fourier coefficients, extracting temporal correlations from time-varying signals, and estimating transformations of physical observables. Using a superconducting cavity--qubit architecture, we experimentally demonstrate $10^7$-fold reductions in the number of measurements required for Fourier-amplitude and time-varying signal learning. Our $\textit{quantum feature sensing}$ algorithms further enable orders-of-magnitude improvements in simulations of weak-signal dark matter detection and wireless communication applications. These quantum advantages are derived from Quantum Phase-Space Inference (Q$\Psi$), a unifying theory of quantum-enhanced experiments that simultaneously converts a set of experimental objectives and constraints into tight lower bounds and optimal quantum-enhanced learning algorithms while producing a certificate of quantum advantage. Q$\Psi$ extends beyond the regimes captured by quantum Fisher information and provides a framework for systematically identifying rigorous quantum advantages in practical experimental tasks. Together, our results establish that near-term quantum technology can exponentially enhance our ability to learn from classical signals.

quant-ph

Quantum computational displacement sensing

Quantum computational sensing (QCS) combines quantum sensing with quantum computing to extract task-relevant information from the physical world. QCS can in principle achieve an accuracy advantage for specific tasks versus the alternative of raw-signal estimation using conventional quantum sensing followed by task-specific classical postprocessing. Here we report the experimental demonstration of quantum computational displacement sensing (QCDS) with a superconducting circuit comprising a qubit coupled to an oscillator. We consider binary classification sensing tasks, where the goal is to predict the class label of a single complex-valued displacement sensed once by the oscillator. Rather than estimating the displacement, our computational-sensing protocol -- using parameterized quantum circuits before and after sensing -- attempts to determine the binary class label using quantum processing and map it onto the ground or excited state of the qubit. A single measurement of the qubit directly outputs the prediction. We implemented circuits with up to 24 entangling gates and 38 free parameters, which were trained in silico. We show that increasing the circuit depth systematically improves expressivity and classification accuracy. We experimentally obtained an accuracy advantage over a suite of protocols that first use conventional quantum sensing to estimate the displacement before using classical postprocessing to perform prediction. For certain tasks, our protocol achieves a 15-percentage-points higher classification accuracy than most conventional approaches considered. Our results establish the feasibility of quantum computational sensing with noisy superconducting hardware and illustrate how integrating quantum computation with quantum sensing can enhance performance when the goal is to estimate a property or function of a signal rather than to estimate the signal.

quant-ph

Resist-free shadow deposition using silicon trenches for Josephson junctions in superconducting qubits

Superconducting qubit fabrication innovations continue to be explored to achieve higher performance. Despite improvements to base layer fabrication and processing, resist-based Josephson junction (JJ) schemes have largely remained unchanged. The polymer mask during deposition causes chemical contamination and limits in situ and ex situ surface preparation, junction materials, and scalability. Here, we demonstrate a resist-free approach to junction fabrication based on etched silicon trenches that is CMOS compatible and easily integrated into existing innovations in qubit base layer fabrication and chemical processing. We fabricate Al-AlOx-Al JJs and qubits using this method, measuring median energy relaxation times up to 184 microseconds. We find minimal contamination at the substrate-metal interface and fluctuations of energy relaxation on a 35 hour timescale that are narrow and normally distributed. The method widens the process window for substrate preparation and new materials platforms.

quant-ph

Error semitransparent universal control of a bosonic logical qubit

Bosonic codes offer hardware-efficient approaches to logical qubit construction and hosted the first demonstration of beyond-break even logical quantum memory. However, such accomplishments were done for idling information, and realization of fault-tolerant logical operations remains a critical bottleneck for universal quantum computation in scaled systems. Error-transparent (ET) gates offer an avenue to resolve this issue, but experimental demonstrations have been limited to phase gates. Here, we introduce a framework based on dynamic encoding subspaces that enables simple linear drives to accomplish universal gates that are error semi-transparent (EsT) to oscillator photon loss. With an EsT logical gate set of {X, H, T}, we observe a five-fold reduction in infidelity conditioned on photon loss, demonstrate extended active-manipulation lifetimes with quantum error correction, and construct a composite EsT non-Clifford operation using a sequence of eight gates from the set. Our approach is compatible with methods for detectable ancilla errors, offering an approach to error-mitigated universal control of bosonic logical qubits with the standard quantum control toolkit.

quant-ph

Krypton-sputtered tantalum films for scalable high-performance quantum devices

Superconducting qubits based on tantalum (Ta) thin films have demonstrated the highest-performing microwave resonators and qubits. This makes Ta an attractive material for superconducting quantum computing applications, but, so far, direct deposition has largely relied on high substrate temperatures exceeding \SI{400}{\celsius} to achieve the body-centered cubic phase, BCC (\textalpha-Ta). This leads to compatibility issues for scalable fabrication leveraging standard semiconductor fabrication lines. Here, we show that changing the sputter gas from argon (Ar) to krypton (Kr) promotes BCC Ta synthesis on silicon (Si) at temperatures as low as \SI{200}{\celsius}, providing a wide process window compatible with back-end-of-the-line fabrication standards. Furthermore, we find these films to have substantially higher electronic conductivity, consistent with clean-limit superconductivity. We validated the microwave performance through coplanar waveguide resonator measurements, finding that films deposited at \SI{250}{\celsius} and \SI{350}{\celsius} exhibit a tight performance distribution at the state of the art. Higher temperature-grown films exhibit higher losses, in correlation with the degree of Ta/Si intermixing revealed by cross-sectional transmission electron microscopy. Finally, with these films, we demonstrate transmon qubits with a relatively compact, \SI{20}{\micro\meter} capacitor gap, achieving a median quality factor up to 14 million.

quant-ph

Frozonium: Freezing Anharmonicity in Floquet Superconducting Circuits

Floquet engineering is a powerful method that can be used to modify the properties of interacting many-body Hamiltonians via the application of periodic time-dependent drives. Here we consider the physics of an inductively shunted superconducting Josephson junction in the presence of Floquet drives in the fluxonium regime and beyond, which we dub the frozonium artificial atom. We find that in the vicinity of special ratios of the drive amplitude and frequency, the many-body dynamics can be tuned to that of an effectively linear bosonic oscillator, with additional nonlinear corrections that are suppressed in higher powers of the drive frequency. By analyzing the inverse participation ratios between the time-evolved frozonium wavefunctions and the eigenbasis of a linear oscillator, we demonstrate the ability to achieve a novel dynamical control using a combination of numerical exact diagonalization and Floquet-Magnus expansion. We discuss the physics of resonances between quasi-energy states induced by the drive, and ways to mitigate their effects. We also highlight the enhanced protection of frozonium against external sources of noise present in experimental setups. This work lays the foundation for future applications in quantum memory and bosonic quantum control using superconducting circuits.

cond-mat.mes-hall

A Mathematical Structure for Amplitude-Mixing Error-Transparent Gates for Binomial Codes

Bosonic encodings of quantum information offer hardware-efficient, noise-biased approaches to quantum error correction relative to qubit register encodings. Implementations have focused in particular on error correction of stored, idle quantum information, whereas quantum algorithms are likely to desire high duty cycles of active control. Error-transparent operations are one way to preserve error rates during operations, but, to the best of our knowledge, only phase gates have so far been given an explicitly error-transparent formulation for binomial encodings. Here, we introduce the concept of 'parity nested' operations, and show how these operations can be designed to achieve continuous amplitude-mixing logical gates for binomial encodings that are fully error-transparent to the photon loss channel. For a binomial encoding that protects against l photon losses, the construction requires $\lfloor$l/2$\rfloor$ + 1 orders of generalized squeezing in the parity nested operation to fully preserve this protection. We further show that error-transparency to all the correctable photon jumps, but not the no-jump errors, can be achieved with just a single order of squeezing. Finally, we comment on possible approaches to experimental realization of this concept.

quant-ph

Microwave signal processing using an analog quantum reservoir computer

Quantum reservoir computing (QRC) has been proposed as a paradigm for performing machine learning with quantum processors where the training is efficient in the number of required runs of the quantum processor and takes place in the classical domain, avoiding the issue of barren plateaus in parameterized-circuit quantum neural networks. It is natural to consider using a quantum processor based on superconducting circuits to classify microwave signals that are analog -- continuous in time. However, while theoretical proposals of analog QRC exist, to date QRC has been implemented using circuit-model quantum systems -- imposing a discretization of the incoming signal in time, with each time point input by executing a gate operation. In this paper we show how a quantum superconducting circuit comprising an oscillator coupled to a qubit can be used as an analog quantum reservoir for a variety of classification tasks, achieving high accuracy on all of them. Our quantum system was operated without artificially discretizing the input data, directly taking in microwave signals. Our work does not attempt to address the question of whether QRCs could provide a quantum computational advantage in classifying pre-recorded classical signals. However, beyond illustrating that sophisticated tasks can be performed with a modest-size quantum system and inexpensive training, our work opens up the possibility of achieving a different kind of advantage than a purely computational advantage: superconducting circuits can act as extremely sensitive detectors of microwave photons; our work demonstrates processing of ultra-low-power microwave signals in our superconducting circuit, and by combining sensitive detection with QRC processing within the same system, one could achieve a quantum sensing-computational advantage, i.e., an advantage in the overall analysis of microwave signals comprising just a few photons.

quant-ph

Synthetic high angular momentum spin dynamics in a microwave oscillator

Spins and oscillators are foundational to much of physics and applied sciences. For quantum information, a spin 1/2 exemplifies the most basic unit, a qubit. High angular momentum spins (HAMSs) and harmonic oscillators provide multi-level manifolds (e.g., qudits) which have the potential for hardware-efficient protected encodings of quantum information and simulation of many-body quantum systems. In this work, we demonstrate a new quantum control protocol that conceptually merges these disparate hardware platforms. Namely, we show how to modify a harmonic oscillator on-demand to implement a continuous range of generators associated to resonant driving of a harmonic qudit, which we can interpret as accomplishing linear and nonlinear control over a harmonic HAMS degree of freedom. The spin-like dynamics are verified by demonstration of linear spin coherent (SU(2)) rotations, nonlinear spin control, and comparison to other manifolds like simply-truncated oscillators. Our scheme allows the first universal control of such a harmonic qudit encoding: we use linear operations to accomplish four logical gates, and further show that nonlinear harmonicity-preserving operations complete the logical gate set. Our results show how motion on a closed Hilbert space can be useful for quantum information processing and opens the door to superconducting circuit simulations of higher angular momentum quantum magnetism.

quant-ph

Non-Linear Hall Effect in Multi-Weyl Semimetals

In the presence of time reversal symmetry, a non-linear Hall effect can occur in systems without an inversion symmetry. One of the prominent candidates for detection of such Hall signals are Weyl semimetals. In this article, we investigate the Berry curvature induced second and third order Hall effect in multi-Weyl semimetals with topological charges $n =1, 2, 3$. We use low energy effective models to obtain general analytical expressions and discover the presence of a large Berry curvature dipole in multi-Weyl semimetals. We also study the Berry curvature dipole in a realistic tight-binding lattice model and observe two different kinds of variation with increasing topological charge -- these can be attributed to different underlying Berry curvature components. We provide estimates of the signatures of second harmonic of Hall signal in multi-Weyl semimetals, which can be detected experimentally. Furthermore, we predict the existence of a third order Hall signal in multi-Weyl semimetals. We derive the analytical expressions of Berry connection polarizability tensor, which is responsible for third order effects, using a low energy model and estimate the measurable conductivity. Our work can help guide experimental discovery of Berry curvature multipole physics in multi-Weyl semimetals.

cond-mat.mes-hall

Tunable Topology and Berry Curvature Dipole in Transition Metal Dichalcogenide Janus Monolayers

Janus transition metal dichalcogenides, with intrinsic mirror asymmetry, exhibit a wide array of interesting properties. In this work, we study Janus monolayers derived from WTe$_2$ using first-principles and tight-binding calculations. We discover that WSeTe and WSTe are topologically trivial, in contrast to the parent quantum spin Hall insulator WTe$_2$. Motivated by the growing interest in non-linear Hall effect, which also requires asymmetric structures, we investigate the Berry curvature and its dipole in these Janus systems and find that they exhibit strikingly large values of Berry curvature dipole, despite being in the topologically trivial phase. We track down the origin of this behaviour and put forth a low-energy massive Dirac model to understand the central features of our ab initio computations. Our predictions introduce Janus monolayers as promising new platforms for exploring as well as engineering non-linear Hall effect.

cond-mat.mes-hall

Different Flavors of Exact-Factorization-Based Mixed Quantum-Classical Methods for Multistate Dynamics

The exact factorization approach has led to the development of new mixed quantum-classical methods for simulating coupled electron-ion dynamics. We compare their performance for dynamics when more than two electronic states are occupied at a given time, and analyze: (1) the use of coupled versus auxiliary trajectories in evaluating the electron-nuclear correlation terms, (2) the approximation of using these terms within surface-hopping and Ehrenfest frameworks, and (3) the relevance of the exact conditions of zero population transfer away from nonadiabatic coupling regions and total energy conservation. Dynamics through the three-state conical intersection in the uracil radical cation as well as polaritonic models in one dimension are studied.

quant-ph

Curing the Divergence in Time-Dependent Density Functional Quadratic Response Theory

The adiabatic approximation in time-dependent density functional theory (TDDFT) is known to give an incorrect pole structure in the quadratic response function, leading to unphysical divergences in excited state-to-state transition probabilities and hyperpolarizabilties. We find the form of the exact quadratic response kernel and derive a practical and accurate approximation that cures the divergence. We demonstrate our results on excited state-to-state transition probabilities of a model system and of the LiH molecule.

physics.chem-ph

Analytical Gradients for Nuclear-Electronic Orbital Time-Dependent Density Functional Theory: Excited State Geometry Optimizations and Adiabatic Excitation Energies

The computational investigation of photochemical processes often entails the calculation of excited state geometries, energies, and energy gradients. The nuclear-electronic orbital (NEO) approach treats specified nuclei, typically protons, quantum mechanically on the same level as the electrons, thereby including the associated nuclear quantum effects and non-Born-Oppenheimer behavior into quantum chemistry calculations. The multicomponent density functional theory (NEO-DFT) and time-dependent DFT (NEO-TDDFT) methods allow efficient calculations of ground and excited states, respectively. Herein, the analytical gradients are derived and implemented for the NEO-TDDFT method and the associated Tamm-Dancoff approximation (NEO-TDA). The programmable equations for these analytical gradients, as well as the NEO-DFT analytical Hessian, are provided. The NEO approach includes the anharmonic zero-point energy and density delocalization associated with the quantum protons, as well as vibronic mixing, in geometry optimizations and energy calculations of ground and excited states. The harmonic zero-point energy associated with the other nuclei can be computed via the NEO Hessian. This approach is used to compute the 0-0 adiabatic excitation energies for a set of nine small molecules with all protons quantized, exhibiting slight improvement over the conventional electronic approach. Geometry optimizations of two excited state intramolecular proton transfer systems are performed with one and two quantized protons, respectively. The NEO calculations for these systems produce electronically excited state geometries with stronger intramolecular hydrogen bonds and similar relative stabilities compared to conventional electronic methods. This work provides the foundation for nonadiabatic dynamics simulations of fundamental processes such as photoinduced proton transfer and proton-coupled electron transfer.

physics.chem-ph