arXiv subjects

Satoshi Ashihara

Publications and source records attributed to Satoshi Ashihara.

6 recordsLinked to original sources

arXiv2026

Cooperative effects of membrane confinement and gelation on PEG crystallization pathway

Lipid-coated microscale hydrogels provide confined, hydrated environments in which polymer phase behavior can differ markedly from that in bulk. Here, we investigate the crystallization pathway of poly(ethylene glycol) (PEG) encapsulated in lipid-coated agarose microgels. Surprisingly, polarized-light microscopy reveals birefringence in the microgels under conditions where PEG remains non-crystalline in the corresponding bulk solution. The birefringence disappears upon heating and spontaneously reappears after further cooling or upon local mechanical stimulation. Infrared microspectroscopy demonstrates that the birefringent microgels contain crystalline PEG, whereas non-birefringent microgels contain PEG in an amorphous-like state, indicating the existence of a metastable precursor prior to crystallization. Furthermore, cooling below the phase-separation temperature produces PEG-rich domains preferentially near the membrane, suggesting that membrane wetting governs the spatial distribution of PEG before crystallization. Together, these results indicate that membrane confinement and agarose gelation cooperatively alter the local hydration environment of PEG, thereby stabilizing an amorphous-like precursor and redirecting the subsequent crystallization pathway. Our findings identify the coupling of membrane wetting and gelation as a key factor governing PEG crystallization in confined soft materials.

cond-mat.soft↗

arXiv2026

Transverse spin texture in optical non-Hermitian skin modes

In structured electromagnetic fields, polarization textures are often closely linked to the spatial variation of the energy flow. However, this familiar picture has been established mainly for lossless and isotropic settings, and concrete examples showing how it is modified in media with gain and loss remain limited. Here, we demonstrate that optical skin modes associated with the non-Hermitian skin effect (NHSE) carry a finite transverse circular-polarization texture and further show that the accompanying in-plane electric-field spin texture deviates from the familiar lossless spin-flow picture. Using exact TE mode solutions, we separate the common exponential skin envelope from the oscillatory component. This decomposition shows that the circular-polarization texture is not generated by the skin envelope itself but by the oscillatory interference component modified by non-Hermiticity. It also reveals a handedness bias and a reshaped spatial relation between circularity and intensity. Finite-element calculations confirm that these features remain robust in loss-biased anisotropic media. These results show that gain and loss provide additional freedom for engineering electric-field spin textures beyond conventional lossless photonic settings.

physics.optics↗

arXiv2025

Selective Enhancement of Optical Chirality and Spin Angular Momentum in Plasmonic Near-Field

The interaction between circularly polarized (CP) light and matter is governed by two fundamental quantities: spin angular momentum (SAM) and optical chirality (OC). While these quantities are inseparable in free space, they can be selectively enhanced in plasmonic near-field regions through appropriately designed structures. We demonstrate that the excitation of circular plasmonic nanostructures with CP light enables selective or simultaneous enhancement of SAM and OC through the excitation of rotating plasmon modes. Electromagnetic field analysis reveals that SAM enhancement originates from transverse SAM induced by unidirectional evanescent waves, whereas OC enhancement is governed by the interference between the plasmonic electric field and incident magnetic field. The finite element method simulations confirm that circular dichroism signals arising from these enhanced near fields clearly depend on the SAM and OC of the local fields, underscoring the importance of structural design in the detection and enhancement of optically active phenomena at the nanoscale.

physics.optics↗

arXiv2024

Designing rotational motion of charges on plasmonic nanostructures excited by circularly polarized light

Rotational motion of charges in plasmonic nanostructures plays an important role in transferring angular momentum between light and matter on the nanometer scale. Although sophisticated control of rotational charge motion has been achieved using spatially structured light, its extension to simultaneous excitation of the same charge motion in multiple nanostructures is not straightforward. In this study, we perform model calculations to show that spatially homogeneous circularly polarized (CP) light can excite rotational charge motions with a high degrees of freedom by exploiting the rotational symmetry of the plasmonic structure and that of the plasmon mode. Finite-difference time-domain simulations demonstrate selective excitation of rotational charge motion for both isolated nanoplates and periodic array structures, showing that complex charge rotations can be manipulated by plane CP waves in a wide range of plasmonic structures.

physics.optics↗

arXiv2024

Frequency-Modulation Mode-Locked Laser with GHz Spectral Width Tunable in the 2-3 um Region

A narrow-bandwidth actively mode-locked laser using a Cr:ZnS gain medium has been successfully demonstrated. A free-space electro-optic phase modulator is employed in the solid-state laser resonator to achieve frequency-modulation (FM) mode-locking, which achieves a narrow spectral width of ~1 GHz and a pulse duration of ~500 ps over a wide tuning range of 1947-2445 nm. The operation frequency of the modulator determines the repetition rate of the mode-locked pulse train and can stabilize it to millihertz-level without any additional feedback loop systems. We also study the theoretical expression of pulse duration and spectral width in a FM mode-locking in a laser cavity that contains considerable group-delay dispersion. The results indicates that larger intracavity dispersion can only stabilize the laser operation by avoiding mode switching, but also narrow the spectral width and increase the pulse duration. The proposed laser features a narrow spectral width at a desired mid-infrared wavelength and a comb-like spectral structure with stabilized longitudinal mode spacing, providing a powerful tool for sensing and control of molecules.

physics.optics↗

arXiv2023

Rotationally displaced electric field intensity distribution around square nanoantennas induced by circularly polarized light

An optical field around regular polygon metal nanostructures excited by circularly polarized light can exhibit rotationally displaced intensity distributions. Although this phenomenon has been recognized, its underlying mechanisms has not been sufficiently explained. Herein, finite-difference time-domain simulations and model analyses reveal that the rotationally displaced optical intensity distribution can be generated when each of the linear polarization components that constitute circular polarization excites a superposition of multiple modes. The proposed model reasonably explains the rotationally displaced patterns for a square nanoantenna and other regular-polygon nanoantennas.

physics.optics↗