arXiv subjects

Scarlett S. Yu

Publications and source records attributed to Scarlett S. Yu.

9 recordsLinked to original sources

arXiv2026

High-fidelity entanglement of polar molecules by dynamic geometric control

In quantum information systems made of optical tweezer arrays of ultracold molecules, thermal motion of molecules degrades the coherence of their interactions, which limits entanglement fidelity and the concomitant scientific applicability of these systems. We show that by controlling the geometry of the dipolar interaction, even when a molecule occupies many motional states in the tweezer, coherence can be preserved. We characterize several geometries that suppress sensitivity to thermal fluctuations. We further use programmable, coherence-preserving motion of the molecules during entanglement to refocus dephasing from relative positional jitter of the tweezers, which is relevant even on the 10 nm scale. These methods yield substantially improved dipolar coherence and enable generation of two-molecule entanglement with a Bell state fidelity of $\mathcal{F}= 0.976^{+0.008}_{-0.011}$ in directly laser-cooled molecules.

physics.atom-ph↗

arXiv2025

Control of Dipolar Dynamics by Geometrical Programming

We propose and theoretically analyze methods for quantum many-body control through geometric reshaping of molecular tweezer arrays. Dynamic rearrangement during entanglement is readily available due to the extended coherence times of molecular rotational qubits. We show how motional dephasing can be suppressed and enhanced spin squeezing can be achieved in an actively rearranged short-range XY model. We also analyze in detail a specific static geometry that significantly suppresses decoherence. These general methods as applied to programmable quantum systems offer robust control modalities that are well suited to molecules.

quant-ph↗

arXiv2024

A conveyor-belt magneto-optical trap of CaF

We report the experimental realization of a conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) $μ$m and a peak number density of $3.6(5) \times 10^{10}$ cm$^{-3}$, a 600-fold increase over the conventional red-detuned MOTs of CaF, and the densest molecular MOT observed to date. Subsequent loading of these molecules into an optical dipole trap yields up to $2.6 \times 10^4$ trapped molecules at a temperature of 14(2) $μ$K with a peak phase-space density of $\sim 2.4 \times 10^{-6}$. This opens new possibilities for a range of applications utilizing high-density, optically trapped ultracold molecules.

physics.atom-ph↗

arXiv2023

Raman sideband cooling of molecules in an optical tweezer array to the 3-D motional ground state

Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the Standard Model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules. Further cooling of the molecules to near the motional ground state is crucial for reducing various dephasings in quantum and precision applications. In this work, we demonstrate Raman sideband cooling of CaF molecules in optical tweezers to near their motional ground state, with average motional occupation quantum numbers of $\bar{n}_{x}=0.16(12)$, $\bar{n}_{y}=0.17(17)$ (radial directions), $\bar{n}_{z}=0.22(16)$ (axial direction) and a 3-D motional ground state probability of $54\pm18\%$. This paves the way to increase molecular coherence times in optical tweezers for robust quantum computation and simulation applications.

physics.atom-ph↗

arXiv2022

Dipolar spin-exchange and entanglement between molecules in an optical tweezer array

Due to their intrinsic electric dipole moments and rich internal structure, ultracold polar molecules are promising candidate qubits for quantum computing and for a wide range of quantum simulations. Their long-lived molecular rotational states form robust qubits while the long-range dipolar interaction between molecules provides quantum entanglement. Using a molecular optical tweezer array, single molecules can be moved and separately addressed for qubit operations using optical and microwave fields, creating a scalable quantum platform. Here, we demonstrate long-range dipolar spin-exchange interactions in pairs of CaF molecules trapped in an optical tweezer array. We control the anisotropic interaction and realize the spin-$\frac{1}{2}$ quantum XY model by encoding an effective spin-$\frac{1}{2}$ system into the rotational states of the molecules. We demonstrate a two-qubit (two-molecule) gate to generate entanglement deterministically, an essential resource for all quantum information applications. Employing interleaved tweezer arrays, we demonstrate high fidelity single site molecular addressability.

physics.atom-ph↗

arXiv2022

Fast optical transport of ultracold molecules over long distances

Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these requirements are challenging to achieve in a magneto-optical trap (MOT) vacuum chamber that is connected to a cryogenic buffer gas beam source, as is the case for all molecule laser cooling experiments so far. Long distance transport of molecules greatly eases fulfilling these requirements as molecules are placed into a region separate from the MOT chamber. We realize a fast transport method for ultracold molecules based on an electronically focus-tunable lens combined with an optical lattice. The high transport speed is achieved by the 1D red-detuned optical lattice, which is generated by interference of a focus-tunable laser beam and a focus-fixed laser beam. Efficiency of 48(8)% is realized in the transport of ultracold calcium monofluoride (CaF) molecules over 46 cm distance in 50 ms, with a moderate heating from 32(2) μK to 53(4) μK. Positional stability of the molecular cloud allows for stable loading of an optical tweezer array with single molecules.

physics.atom-ph↗

arXiv2021

Rotational Coherence Times of Polar Molecules in Optical Tweezers

Qubit coherence times are critical to the performance of any robust quantum computing platform. For quantum information processing using arrays of polar molecules, a key performance parameter is the molecular rotational coherence time. We report a 93(7) ms coherence time for rotational state qubits of laser cooled CaF molecules in optical tweezer traps, over an order of magnitude longer than previous systems. Inhomogeneous broadening due to the differential polarizability between the qubit states is suppressed by tuning the tweezer polarization and applied magnetic field to a "magic" angle. The coherence time is limited by the residual differential polarizability, implying improvement with further cooling. A single spin-echo pulse is able to extend the coherence time to nearly half a second. The measured coherence times demonstrate the potential of polar molecules as high fidelity qubits.

physics.atom-ph↗

arXiv2021

Observation of Microwave Shielding of Ultracold Molecules

Harnessing the potential wide-ranging quantum science applications of molecules will require control of their interactions. Here, we use microwave radiation to directly engineer and tune the interaction potentials between ultracold calcium monofluoride (CaF) molecules. By merging two optical tweezers, each containing a single molecule, we probe collisions in three dimensions. The correct combination of microwave frequency and power creates an effective repulsive shield, which suppresses the inelastic loss rate by a factor of six, in agreement with theoretical calculations. The demonstrated microwave shielding shows a general route to the creation of long-lived, dense samples of ultracold molecules and evaporative cooling.

physics.atom-ph↗

arXiv2019

Suppressed spontaneous emission for coherent momentum transfer

Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We apply this technique to accelerate atoms, demonstrating up to an average of $19$ $\hbar k$ momentum transfers per spontaneous emission event. This represents more than an order of magnitude improvement in suppression of spontaneous emission compared to radiative scattering forces. For molecular beam slowing, this technique is capable of delivering a many-fold increase in the achievable time-averaged force to significantly reduce both the slowing distance and detrimental losses to dark vibrational states.

physics.atom-ph↗