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Scott D. Baalrud

Publications and source records attributed to Scott D. Baalrud.

At least 37 records · Page 2Linked to original sources

Effects of Coulomb Coupling on Stopping Power and a Link to Macroscopic Transport

Molecular dynamics simulations are used to assess the influence of Coulomb coupling on the energy evolution of charged projectiles in the classical one-component plasma. The average projectile kinetic energy is found to decrease linearly with time when $ν_α/ω_{p} \lesssim 10^{-2}$, where $ν_{α}$ is the Coulomb collision frequency between the projectile and the medium, and $ω_{p}$ is the plasma frequency. Stopping power is obtained from the slope of this curve. In comparison to the weakly coupled limit, strong Coulomb coupling causes the magnitude of the stopping power to increase, the Bragg peak to shift to several times the plasma thermal speed, and for the stopping power curve to broaden substantially. The rate of change of the total projectile kinetic energy averaged over many independent simulations is shown to consist of two measurable components: a component associated with a one-dimensional friction force, and a thermal energy exchange rate. In the limit of a slow and massive projectile, these can be related to the macroscopic transport rates of self-diffusion and temperature relaxation in the plasma. Simulation results are compared with available theoretical models for stopping power, self-diffusion coefficients, and temperature relaxation rates.

physics.plasm-ph↗

The Barkas Effect in Plasma Transport

Molecular dynamics simulations reveal that a fundamental symmetry of plasma kinetic theory is broken at moderate to strong Coulomb coupling: the collision rate depends on the signs of the colliding charges. This symmetry breaking is analogous to the Barkas effect observed in charged-particle stopping experiments and gives rise to significantly enhanced electron-ion collision rates. It is expected to affect any neutral plasma with moderate to strong Coulomb coupling such as ultracold neutral plasmas (UNP) and the dense plasmas of ICF and laser-matter interaction experiments. The physical mechanism responsible is screening of binary collisions by the correlated plasma medium, which causes an asymmetry in the dynamics of large-angle scattering. Because the effect pertains only to close interactions, it is not predicted by traditional transport models based on cut-off Coulomb collisions or linear dielectric response. A model for the effective screened interaction potential is presented that is suitable for the coupling strengths achieved in UNP experiments. Transport calculations based on this potential and the effective potential kinetic theory agree with simulated relaxation rates and predict that the Barkas effect can cause up to a 70% increase in the electron-ion collision rate at the conditions of present UNP experiments. The influence of the Barkas effect in other transport processes is also considered.

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Transport formulas for multi-component plasmas within the effective potential theory framework

The recently proposed effective potential theory [Phys. Rev. Lett. 110, 235001 (2013)] allows evaluating transport in coupled plasmas with the well-developed formalisms for systems with binary collisions. To facilitate practical implementation of this concept in fluid models of multi-component plasmas, compact expressions for the transport coefficients in terms the generalized Coulomb logarithms are summarized from existing prescriptions. For weakly coupled plasmas, characterized by Debye-shielded Coulomb interaction potential, expressions become fully analytical. In coupled plasmas the generalized Coulomb logarithms need to be evaluated numerically. Routines implementing the described formalisms are included as supplemental material.

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Collisionless Kinetic Theory of Oblique Tearing Instabilities

The linear dispersion relation for collisionless kinetic tearing instabilities is calculated for a Harris equilibrium. In contrast to the conventional 2D geometry, which considers only modes at the center of the current sheet, modes can span the current sheet in 3D. Modes at each resonant surface have a unique angle ($θ$) with respect to the guide field direction. Both kinetic simulations and numerical eigenmode solutions of the linearized Vlasov-Maxwell equations have recently revealed that standard analytic theories vastly overestimate the growth rate of oblique modes ($θ\neq 0$). We find that this stabilization is associated with the density-gradient-driven diamagnetic drift. The analytic theories miss this drift stabilization because the inner tearing layer broadens at oblique angles sufficiently far that the assumption of scale separation between the inner and outer regions of boundary-layer theory breaks down. The dispersion relation obtained by numerically solving a single second order differential equation is found to approximately capture the drift stabilization predicted by solutions of the full integro-differential eigenvalue problem. A simple analytic estimate for the stability criterion is provided.

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Reduction of electron heating by magnetizing ultracold neutral plasma

Electron heating in an ultracold neutral plasma is modeled using classical molecular dynamics simulations in the presence of an externally applied magnetic field. A sufficiently strong magnetic field is found to reduce disorder induced heating and three body recombination heating of electrons by constraining electron motion, and therefore heating, to the single dimension aligned with the magnetic field. A strong and long-lasting temperature anisotropy develops, and the overall kinetic electron temperature is effectively reduced by a factor of three. These results suggest that experiments may increase the effective electron coupling strength using an applied magnetic field.

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Transport Regimes Spanning Magnetization-Coupling Phase Space

The manner in which transport properties vary over the entire parameter-space of coupling and magnetization strength is explored for the first time. Four regimes are identified based on the relative size of the gyroradius compared to other fundamental length scales: the collision mean free path, Debye length, distance of closest approach and interparticle spacing. Molecular dynamics simulations of self-diffusion and temperature anisotropy relaxation spanning the parameter space are found to agree well with the predicted boundaries. Comparison with existing theories reveals regimes where they succeed, where they fail, and where no theory has yet been developed.

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Influence of coupling on thermal forces and dynamic friction in plasmas with multiple ion species

The recently proposed effective potential theory [Phys. Rev. Lett. 110, 235001 (2013)] is used to investigate the influence of coupling on inter-ion-species diffusion and momentum exchange in multi-component plasmas. Thermo-diffusion and the thermal force are found to diminish rapidly as strong coupling onsets. For the same coupling parameters, the dynamic friction coefficient is found to tend to unity. These results provide an impetus for addressing the role of coupling on diffusive processes in inertial confinement fusion experiments.

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Pair Correlation Functions of Strongly Coupled Two-Temperature Plasma

Using molecular dynamics simulations, we perform the first direct tests of three proposed models for the pair correlation functions of strongly coupled plasmas with species of unequal temperature. The models are all extensions of the Ornstein-Zernike/hypernetted-chain theory used to good success for equilibrium plasmas. Each theory is evaluated at several coupling strengths, temperature ratios, and mass ratios for a model plasma in which the electrons are positively charged. We show that the model proposed by Seuferling, Vogel, and Teopffer [Phys. Rev. A 40, 323 (1989)] agrees well with molecular dynamics over a wide range of mass and temperature ratios, as well as over a range of coupling strength similar to that of the equilibrium HNC theory. The SVT model also correctly predicts the strength of interspecies correlations and exhibits physically reasonable long-wavelength limits of the static structure factors. Comparisons of the SVT model with the Yukawa OCP model are used to show that ion-ion pair correlations are well described by the YOCP model up to $Γ_e \approx 1$, beyond which it rapidly breaks down.

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Temperature Anisotropy Relaxation of the One-Component Plasma

The relaxation rate of a Maxwellian velocity distribution function that has an initially anisotropic temperature $(T_\parallel \neq T_\perp)$ is an important physical process in space and laboratory plasmas. It is also a canonical example of an energy transport process that can be used to test theory. Here, this rate is evaluated using molecular dynamics simulations of the one-component plasma. Results are compared with the predictions of four kinetic theories; two treating the weakly coupled regime (1) the Landau equation, and (2) the Lenard-Balescu equation, and two that attempt to extend the theory into the strongly coupled regime (3) the effective potential theory and (4) the generalized Lenard-Balescu theory. The role of dynamic screening is studied, and is found to have a negligible influence on this transport rate. Oscillations and a delayed relaxation onset in the temperature profiles are observed at strong coupling, which are not described by the kinetic theories.

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Thermodynamic State Variables in Quasi-Equilibrium Ultracold Neutral Plasma

The pressure and internal energy of an ultracold plasma in a state of quasi-equilibrium are evaluated using classical molecular dynamics simulations. Coulomb collapse is avoided by modeling electron-ion interactions using an attractive Coulomb potential with a repulsive core. We present a method to separate the contribution of classical bound states, which form due to recombination, from the contribution of free charges when evaluating these thermodynamic state variables. It is found that the contribution from free charges is independent of the choice of repulsive core length-scale when it is sufficiently short-ranged. The partial pressure associated with the free charges is found to closely follow that of the one-component plasma model, reaching negative values at strong coupling, while the total system pressure remains positive. This pseudo-potential model is also applied to Debye-Hückel theory to describe the weakly coupled regime.

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Effective Potential Theory for Diffusion in Binary Ionic Mixtures

Self-diffusion and interdiffusion coefficients of binary ionic mixtures are evaluated using the Effective Potential Theory (EPT), and the predictions are compared with the results of molecular dynamics simulations. We find that EPT agrees with molecular dynamics from weak coupling well into the strong coupling regime, which is a similar range of coupling strengths as previously observed in comparisons with the one-component plasma. Within this range, typical relative errors of approximately 20% and worst-case relative errors of approximately 40% are observed. We also examine the Darken model, which approximates the interdiffusion coefficients based on the self-diffusion coefficients.

physics.plasm-ph↗

Electron Preheaths: The Outsized Influence of Positive Boundaries on Plasmas

Electron sheaths form near the surface of objects biased more positive than the plasma potential, such as in the electron saturation region of a Langmuir probe trace. Generally, the formation of electron sheaths requires that the electron-collecting area be sufficiently smaller ($\sqrt{2.3m_e/M}$ times) than the ion-collecting area. They are commonly thought to be local phenomena that collect the random thermal electron current, but do not otherwise perturb a plasma. Here, using experiments on an electrode embedded in a wall, particle-in-cell simulations and theory, it is shown that under low temperature plasma conditions ($T_e \gg T_i$) electron sheaths are far from local. Instead, a long presheath region (in excess of 70 $λ_D$) extends into the plasma where electrons are accelerated via a pressure gradient to a flow speed exceeding the electron thermal speed at the sheath edge. This fast flow is found to excite instabilities, causing strong fluctuations near the sheath edge.

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Particle-in-cell study of the ion-to-electron sheath transition

The form of a sheath near a small electrode, with bias changing from below to above the plasma potential is studied using 2D particle-in-cell (PIC) simulations. Five cases are studied: (A) an electrode biased more than the electron temperature ($T_e/e$) below the plasma potential, (B) an electrode biased less than $T_e/2e$ below the plasma potential, (C) an electrode biased nearly at the plasma potential, (D) an electrode biased more than $T_i/2e$ but less than $T_e/2e$ above the plasma potential, and (E) an electrode biased much greater than $T_e/2e$ above the plasma potential. In case (A), the electron velocity distribution function (EVDF) is observed to be Maxwellian with a Boltzmann-type exponential density decay through the ion sheath and presheath. In cases (B) and (C), the EVDFs exhibit a loss-cone type truncation due to fast electrons overcoming the small potential difference between the electrode and plasma. No sheath is present in this regime, and the plasma remains quasineutral up to the electrode. The EVDF truncation leads to a presheath-like density and flow velocity gradient. In case (D) an electron sheath is present, and essentially all ions are repelled. Here the truncation driven behavior persists, but is accompanied by a shift in the maximum value of the EVDF that is not present in the negative bias cases. In case (E), the flow shift becomes greater and the loss-cone moves further into the tail of the EVDF. In this case the flow moment has significant contributions from both the flow shift of the EVDF maximum, and the loss-cone truncation.

physics.plasm-ph↗

Theory of the Electron Sheath and Presheath

Electron sheaths are commonly found near Langmuir probes collecting the electron saturation current. The common assumption is that the probe collects the random flux of electrons incident on the sheath, which tacitly implies that there is no electron presheath and that the flux collected is due to a velocity space truncation of the electron velocity distribution function (EVDF). This work provides a dedicated theory of electron sheaths, which suggests that they are not so simple. Motivated by EVDFs observed in Particle-In-Cell (PIC) simulations, a 1D model for the electron sheath and presheath is developed. In the model, under low temperature plasma conditions ($T_e\gg T_i$), an electron pressure gradient accelerates electrons in the presheath to a flow velocity that exceeds the electron thermal speed at the sheath edge. This pressure gradient generates large flow velocities compared to what would be generated by ballistic motion in response to the electric field. It is found that in many situations, under common plasma conditions, the electron presheath extends much further into the plasma than an analogous ion presheath. PIC simulations reveal that the ion density in the electron presheath is determined by a flow around the electron sheath and that this flow is due to 2D aspects of the sheath geometry. Simulations also indicate the presence of ion acoustic waves excited by the differential flow between electrons and ions in the presheath which result in sheath edge fluctuations. The 1D model and time averaged PIC simulations are compared and it is shown that the model provides a good description of the electron sheath and presheath.

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Influence of Ion Streaming Instabilities on Transport Near Plasma Boundaries

Plasma boundary layers are susceptible to electrostatic instabilities driven by ion flows in presheaths and, when present, these instabilities can influence transport. In plasmas with a single species of positive ion, ion-acoustic instabilities are expected under conditions of low pressure and large electron-to-ion temperature ratio ($T_e/T_i \gg 1$). In plasmas with two species of positive ions, ion-ion two-stream instabilities can also be excited. The stability phase-space is characterized using the Penrose criterion and approximate linear dispersion relations. Predictions for how these instabilities affect ion and electron transport in presheaths, including rapid thermalization due to instability-enhanced collisions and an instability-enhanced ion-ion friction force, are also briefly reviewed. Recent experimental tests of these predictions are discussed along with research needs required for further validation. The calculated stability boundaries provide a guide to determine the experimental conditions at which these effects can be expected.

physics.plasm-ph↗

Modified Enskog Kinetic Theory for Strongly Coupled Plasmas

Concepts underlying the Enskog kinetic theory of hard-spheres are applied to include short-range correlation effects in a model for transport coefficients of strongly coupled plasmas. The approach is based on an extension of the effective potential transport theory [S.~D.~Baalrud and J.~Daligault, Phys.~Rev.~Lett.~{\bf 110}, 235001 (2013)] to include an exclusion radius surrounding individual charged particles that is associated with Coulomb repulsion. This is obtained by analogy with the finite size of hard spheres in Enskog's theory. Predictions for the self-diffusion and shear viscosity coefficients of the one-component plasma are tested against molecular dynamics simulations. The theory is found to accurately capture the kinetic contributions to the transport coefficients, but not the potential contributions that arise at very strong coupling ($Γ\gtrsim 30$). Considerations related to a first-principles generalization of Enskog's kinetic equation to continuous potentials are also discussed.

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Extensions and Applications of the Bohm Criterion

The generalized Bohm criterion is revisited in the context of incorporating kinetic effects of the electron and ion distribution functions into the theory. The underlying assumptions and results of two different approaches are compared: The conventional `kinetic Bohm criterion' and a fluid-moment hierarchy approach. The former is based on the asymptotic limit of an infinitely thin sheath ($λ_D/l =0$), whereas the latter is based on a perturbative expansion of a sheath that is thin compared to the plasma ($λ_D/l \ll 1$). Here $λ_D$ is the Debye length, which characterizes the sheath length scale, and $l$ is a measure of the plasma or presheath length scale. The consequences of these assumptions are discussed in terms of how they restrict the class of distribution functions to which the resulting criteria can be applied. Two examples are considered to provide concrete comparisons between the two approaches. The first is a Tonks-Langmuir model including a warm ion source [Robertson 2009 \textit{Phys.\ Plasmas} {\bf 16} 103503]. This highlights a substantial difference between the conventional kinetic theory, which predicts slow ions dominate at the sheath edge, and the fluid moment approach, which predicts slow ions have little influence. The second example considers planar electrostatic probes biased near the plasma potential using model equations and particle-in-cell simulations. This demonstrates a situation where electron kinetic effects alter the Bohm criterion, leading to a subsonic ion flow at the sheath edge.

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Effective Potential Theory: A Practical Way to Extend Plasma Transport Theory to Strong Coupling

The effective potential theory is a physically motivated method for extending traditional plasma transport theories to stronger coupling. It is practical in the sense that it is easily incorporated within the framework of the Chapman-Enskog or Grad methods that are commonly applied in plasma physics and it is computationally efficient to evaluate. The extension is to treat binary scatterers as interacting through the potential of mean force, rather than the bare Coulomb or Debye-screened Coulomb potential. This allows for aspects of many-body correlations to be included in the transport coefficients. Recent work has shown that this method accurately extends plasma theory to orders of magnitude stronger coupling when applied to the classical one-component plasma model. The present work shows that similar accuracy is realized for the Yukawa one-component plasma model and it provides a comparison with other approaches.

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