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Scott Diddams

Publications and source records attributed to Scott Diddams.

At least 19 recordsLinked to original sources
arXiv2025

Soft X-ray high-harmonic generation in an anti-resonant hollow core fiber driven by a 3 $\mu$m ultrafast laser

High-harmonic upconversion driven by a mid-infrared femtosecond laser can generate coherent soft X-ray beams in a tabletop-scale setup. Here, we report on a compact ytterbium-pumped optical parametric chirped pulse amplifier (OPCPA) laser system seeded by an all-fiber front-end and employing periodically-poled lithium niobate (PPLN) nonlinear media operated near the pulse fluence limits of current commercially available PPLN crystals. The OPCPA delivers 3 $\mu$m wavelength pulses with 775 $\mu$J energy at 1 kHz repetition rate, with transform-limited 120 fs pulse duration, diffraction-limited beam quality, and ultrahigh 0.33% rms energy stability over >18 hours. Using this laser, we generate soft X-ray high harmonics (HHG) in argon gas by focusing into a low-loss, high-pressure gas-filled anti-resonant hollow core fiber (ARHCF), generating coherent light at photon energies up to the argon L-edge (250 eV) and carbon K-edge (284 eV), with high beam quality and ~1% rms energy stability. This work demonstrates soft X-ray HHG in a high-efficiency guided-wave phase matched geometry, overcoming the high losses inherent to mid-IR propagation in unstructured waveguides, or the short interaction lengths of gas cells or jets. The ARHCF can operate long term without damage, and with the repetition rate, stability and robustness required for demanding applications in spectro-microscopy and imaging. Finally, we discuss routes for maximizing the soft X-ray HHG flux by driving He at higher laser intensities using either 1.5 $\mu$m or 3 $\mu$m - the signal and idler wavelengths of the laser.

physics.optics↗
arXiv2024

Gaia-4b and 5b: Radial Velocity Confirmation of Gaia Astrometric Orbital Solutions Reveal a Massive Planet and a Brown Dwarf Orbiting Low-mass Stars

Gaia astrometry of nearby stars is precise enough to detect the tiny displacements induced by substellar companions, but radial velocity data are needed for definitive confirmation. Here we present radial velocity follow-up observations of 28 M and K stars with candidate astrometric substellar companions, which led to the confirmation of two systems, Gaia-4b and Gaia-5b, and the refutation of 21 systems as stellar binaries. Gaia-4b is a massive planet ($M = 11.8 \pm 0.7 \:\mathrm{M_J}$) in a $P = 571.3 \pm 1.4\:\mathrm{day}$ orbit with a projected semi-major axis $a_0=0.312 \pm 0.040\:\mathrm{mas}$ orbiting a $0.644 \pm 0.02 \:\mathrm{M_\odot}$ star. Gaia-5b is a brown dwarf ($M = 20.9 \pm 0.5\:\mathrm{M_J}$) in a $P = 358.58 \pm 0.19\:\mathrm{days}$ eccentric $e=0.6412 \pm 0.0027$ orbit with a projected angular semi-major axis of $a_0 = 0.947 \pm 0.038\:\mathrm{mas}$ around a $0.34 \pm 0.03 \mathrm{M_\odot}$ star. Gaia-4b is one of the first exoplanets discovered via the astrometric technique, and is one of the most massive planets known to orbit a low-mass star.

astro-ph.EP↗
arXiv2024

Resonant EO combs: Beyond the standard phase noise model of frequency combs

A resonant electro-optic (EO) frequency comb is generated through electro-optic modulation of laser light within an optical resonator. Compared to cavity-less EO combs generated in a single pass through a modulator, resonant EO combs can produce broader spectra with lower radio frequency (RF) power and offer a measure of noise filtering beyond the cavity's linewidth. Understanding, measuring, and suppressing the sources of phase noise in resonant EO combs is crucial for their applications in metrology, astrophotonics, optical clock generation, and fiber-optic communication. According to the standard phase noise model of frequency combs, only two variables - the common mode offset and repetition rate phase noise - are needed to fully describe the phase noise of comb lines. However, in this work we demonstrate analytically, numerically, and experimentally that this standard model breaks down for resonant EO combs at short timescales (high frequencies) and under certain comb parameters. Specifically, a third phase noise component emerges. Consequently, resonant EO combs feature qualitatively different phase noise from their cavity-less counterparts and may not exhibit the anticipated noise filtering. A more complete description of the deviations from the standard phase noise model is critical to accurately predict the performance of frequency combs. The description presented here paves the way for improved designs tailored to applications such as super-continuum generation and optical communication.

physics.optics↗
arXiv2024

Ultrastable vacuum-gap Fabry-P\'erot cavities operated in air

We demonstrate a vacuum-gap ultrastable optical reference cavity that does not require a vacuum enclosure. Our simple method of optical contact bonding in a vacuum environment allows for cavity operation in air while maintaining vacuum between the cavity mirrors. Vacuum is maintained long term, with no observed degradation in cavity stability for over 1 year after bonding. For a 1550 nm laser stabilized to a 9.7 mL in-vacuum bonded cavity, the measured Allan deviation is $2.4\times 10^{-14}$ at 1 s and its phase noise is thermal-noise-limited from 0.1 Hz to 10 kHz, reaching about -105 dBc/Hz at 10 kHz offset frequency. This represents the highest stability of any oscillator operated without a vacuum enclosure. Furthermore, we demonstrate a 0.5 mL in-vacuum bonded cavity created using microfabricated mirrors and cavity dicing, with phase noise reaching -95 dBc/Hz at 10 kHz offset frequency. By relieving the need for high-vacuum enclosures, we greatly enhance the portability and utility of low noise, compact cavity-stabilized lasers, with applications ranging from environmental sensing to mobile optical clocks to ultralow noise microwave generation.

physics.optics↗
arXiv2024

Element-specific and high-bandwidth ferromagnetic resonance spectroscopy with a coherent, extreme ultraviolet (EUV) source

We applied a tabletop, ultrafast, high-harmonic generation (HHG) source to measure the element-specific ferromagnetic resonance (FMR) in ultra-thin magnetic alloys and multilayers on an opaque Si substrate. We demonstrate a continuous wave bandwidth of 62 GHz, with promise to extend to 100 GHz or higher. This laboratory-scale instrument detects the FMR using ultrafast, extreme ultraviolet (EUV) light, with photon energies spanning the M-edges of most relevant magnetic elements. An RF frequency comb generator is used to produce a microwave excitation that is intrinsically synchronized to the EUV pulses with a timing jitter of 1.1 ps or better. We apply this system to measure the dynamics in a multilayer system as well as Ni-Fe and Co-Fe alloys. Since this instrument operates in reflection-mode, it is a milestone toward measuring and imaging the dynamics of the magnetic state and spin transport of active devices on arbitrary and opaque substrates. The higher bandwidth also enables measurements of materials with high magnetic anisotropy, as well as ferrimagnets, antiferromagnets, and short-wavelength (high wavevector) spinwaves in nanostructures or nanodevices. Furthermore, the coherence and short wavelength of the EUV will enable extending these studies using dynamic nanoscale lensless imaging techniques such as coherent diffractive imaging, ptychography, and holography.

cond-mat.mtrl-sci↗
arXiv2023

Complete reactants-to-products observation of a gas-phase chemical reaction with broad, fast mid-infrared frequency combs

Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing diagnostic approaches provide incomplete information. For example, mass spectrometry is optimized to gather snapshots of the presence of many chemical species, while conventional laser spectroscopy can quantify a single chemical species through time. Here we optimize for multiple objectives by introducing a high-speed and broadband, mid-infrared dual frequency comb absorption spectrometer. The optical bandwidth of >1000 cm-1 covers absorption fingerprints of many species with spectral resolution <0.03 cm-1 to accurately discern their absolute quantities. Key to this advance are 1 GHz pulse repetition rate frequency combs covering the 3-5 um region that enable microsecond tracking of fast chemical process dynamics. We demonstrate this system to quantify the abundances and temperatures of each species in the complete reactants-to-products breakdown of 1,3,5-trioxane, which exhibits a formaldehyde decomposition pathway that is critical to modern low temperature combustion systems. By maximizing the number of observed species and improving the accuracy of temperature and concentration measurements, this spectrometer advances understanding of chemical reaction pathways and rates and opens the door for novel developments such as combining high-speed chemistry with machine learning.

physics.chem-ph↗
arXiv2023

An extreme test case for planet formation: a close-in Neptune orbiting an ultracool star

In current theories of planet formation, close-orbiting planets as massive as Neptune are expected to be very rare around low-mass stars. We report the discovery of a Neptune-mass planet orbiting the `ultracool' star LHS 3154, which is nine times less massive than the Sun. The planet's orbital period is 3.7 days and its minimum mass is 13.2 Earth masses, giving it the largest known planet-to-star mass ratio among short-period planets ($<$\,100 days) orbiting ultracool stars. Both the core accretion and gravitational instability theories for planet formation struggle to account for this system. In the core-accretion scenario, in particular, the dust mass of the protoplanetary disk would need to be an order of magnitude higher than typically seen in protoplanetary disk observations of ultracool stars.

astro-ph.EP↗
arXiv2022

1-GHz mid-infrared frequency comb spanning 3 to 13 {\mu}m

Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously combine the high-speed, high spectral resolution, and broad optical bandwidth needed to accurately study complex, transient events in chemistry, combustion, and microscopy. However, such a spectrometer has not yet been demonstrated due to the lack of GHz MIR frequency combs with broad and full spectral coverage. Here, we introduce the first broadband MIR frequency comb laser platform at 1 GHz repetition rate that achieves spectral coverage from 3 to 13 {\mu}m. This frequency comb is based on a commercially available 1.56 {\mu}m mode-locked laser, robust all-fiber Er amplifiers and intra-pulse difference frequency generation (IP-DFG) of few-cycle pulses in \c{hi}(2) nonlinear crystals. When used in a dual comb spectroscopy (DCS) configuration, this source will simultaneously enable measurements with {\mu}s time resolution, 1 GHz (0.03 cm-1) spectral point spacing and a full bandwidth of >5 THz (>166 cm-1) anywhere within the MIR atmospheric windows. This represents a unique spectroscopic resource for characterizing fast and non-repetitive events that are currently inaccessible with other sources.

physics.optics↗
arXiv2021

Single-cycle all-fiber frequency comb

Single-cycle pulses with deterministic carrier-envelope phase enable the study and control of light-matter interactions at the sub-cycle timescale, as well as the efficient generation of low-noise multi-octave frequency combs. However, current single-cycle light sources are difficult to implement and operate, hindering their application and accessibility in a wider range of research. In this paper, we present a single-cycle 100 MHz frequency comb in a compact, turn-key, and reliable all-silica-fiber format. This is achieved by amplifying 2 $\mu$m seed pulses in heavily-doped Tm:fiber, followed by cascaded self-compression to yield 6.8 fs pulses with 215 kW peak power and 374 mW average power. The corresponding spectrum covers more than two octaves, from below 700 nm up to 3500 nm. Driven by this single-cycle pump, supercontinuum with 180 mW of integrated power and a smooth spectral amplitude between 2100 and 2700 nm is generated directly in silica fibers. To broaden applications,few-cycle pulses extending from 6 $\mu$m to beyond 22 $\mu$m with long-term stable carrier-envelope phase are created using intra-pulse difference frequency, and electro-optic sampling yields comb-tooth-resolved spectra. Our work demonstrates the first all-fiber configuration that generates single-cycle pulses, and provides a practical source to study nonlinear optics on the same timescale.

physics.optics↗
arXiv2020

EarthFinder Probe Mission Concept Study: Characterizing nearby stellar exoplanet systems with Earth-mass analogs for future direct imaging

EarthFinder is a NASA Astrophysics Probe mission concept selected for study as input to the 2020 Astrophysics National Academies Decadal Survey. The EarthFinder concept is based on a dramatic shift in our understanding of how PRV measurements should be made. We propose a new paradigm which brings the high precision, high cadence domain of transit photometry as demonstrated by Kepler and TESS to the challenges of PRV measurements at the cm/s level. This new paradigm takes advantage of: 1) broad wavelength coverage from the UV to NIR which is only possible from space to minimize the effects of stellar activity; 2) extremely compact, highly stable, highly efficient spectrometers (R>150,000) which require the diffraction-limited imaging possible only from space over a broad wavelength range; 3) the revolution in laser-based wavelength standards to ensure cm/s precision over many years; 4) a high cadence observing program which minimizes sampling-induced period aliases; 5) exploiting the absolute flux stability from space for continuum normalization for unprecedented line-by-line analysis not possible from the ground; and 6) focusing on the bright stars which will be the targets of future imaging missions so that EarthFinder can use a ~1.5 m telescope.

astro-ph.IM↗
arXiv2020

A Mini-Neptune and a Venus-Zone Planet in the Radius Valley Orbiting the Nearby M2-dwarf TOI-1266: Validation with the Habitable-zone Planet Finder

We report on the validation of two planets orbiting the nearby (36pc) M2 dwarf TOI-1266 observed by the TESS mission. The inner planet is sub-Neptune-sized ($R=2.46 \pm 0.08 R_\oplus$) with an orbital period of 10.9 days. The outer planet has a radius of $1.67_{-0.11}^{+0.09} R_\oplus$ and resides in the exoplanet Radius Valley---the transition region between rocky and gaseous planets. With an orbital period of 18.8 days, the outer planet receives an insolation flux of 2.4 times that of Earth, similar to the insolation of Venus. Using precision near-infrared radial velocities with the Habitable-zone Planet Finder Spectrograph, we place upper mass limits of $15.9 M_\oplus$ and $6.4 M_\oplus$ at 95% confidence for the inner and outer planet, respectively. A more precise mass constraint of planet c, achievable with current RV instruments given the host star brightness (V=12.9, J=9.7), will yield further insights into the dominant processes sculpting the exoplanet Radius Valley.

astro-ph.EP↗
arXiv2020

Mid-infrared frequency combs at 10 GHz

We demonstrate mid-infrared (MIR) frequency combs at 10 GHz repetition rate via intra-pulse difference-frequency generation (DFG) in quasi-phase-matched nonlinear media. Few-cycle pump pulses ($\mathbf{\lesssim}$15 fs, 100 pJ) from a near-infrared (NIR) electro-optic frequency comb are provided via nonlinear soliton-like compression in photonic-chip silicon-nitride waveguides. Subsequent intra-pulse DFG in periodically-poled lithium niobate waveguides yields MIR frequency combs in the 3.1--4.1 $\mu$m region, while orientation-patterned gallium phosphide provides coverage across 7--11 $\mu$m. Cascaded second-order nonlinearities simultaneously provide access to the carrier-envelope-offset frequency of the pump source via in-line f-2f nonlinear interferometry. The high-repetition rate MIR frequency combs introduced here can be used for condensed phase spectroscopy and applications such as laser heterodyne radiometry.

physics.optics↗
arXiv2019

Precision frequency-comb terahertz spectroscopy on pure quantum states of a single molecular ion

Spectroscopy is a powerful tool for studying molecules and is commonly performed on large thermal molecular ensembles that are perturbed by motional shifts and interactions with the environment and one another, resulting in convoluted spectra and limited resolution. Here, we use generally applicable quantum-logic techniques to prepare a trapped molecular ion in a single quantum state, drive terahertz rotational transitions with an optical frequency comb, and read out the final state non-destructively, leaving the molecule ready for further manipulation. We resolve rotational transitions to 11 significant digits and derive the rotational constant of CaH+ to be B_R = 142501777.9(1.7) kHz. Our approach suits a wide range of molecular ions, including polyatomics and species relevant for tests of fundamental physics, chemistry, and astrophysics.

physics.atom-ph↗
arXiv2019

A versatile digital approach to laser frequency comb stabilization

We demonstrate the use of a flexible digital servo system for the optical stabilization of both the repetition rate and carrier-envelope offset frequency of a laser frequency comb. The servo system is based entirely on a low-cost field programmable gate array, simple electronic components, and existing open-source software. Utilizing both slow and fast feedback actuators of a commercial mode-locked laser frequency comb, we maintain cycle-slip free locking of optically-derived beatnotes over a 30 hour period, and measure residual phase noise at or below ~0.1 rad, corresponding to <100 attosecond timing jitter on the optical phase locks. This stability is sufficient for high-precision frequency comb applications, and indicates comparable performance to existing frequency control systems. The modularity of this system allows for it to be easily adapted to suit the servo actuators of a wide variety of laser frequency combs and continuous-wave lasers, reducing cost and complexity barriers, and enabling digital phase control in a wide range of settings.

physics.ins-det↗
arXiv2019

Optical-Clock-Based Time Scale

A time scale is a procedure for accurately and continuously marking the passage of time. It is exemplified by Coordinated Universal Time (UTC), and provides the backbone for critical navigation tools such as the Global Positioning System (GPS). Present time scales employ microwave atomic clocks, whose attributes can be combined and averaged in a manner such that the composite is more stable, accurate, and reliable than the output of any individual clock. Over the past decade, clocks operating at optical frequencies have been introduced which are orders of magnitude more stable than any microwave clock. However, in spite of their great potential, these optical clocks cannot be operated continuously, which makes their use in a time scale problematic. In this paper, we report the development of a hybrid microwave-optical time scale, which only requires the optical clock to run intermittently while relying upon the ensemble of microwave clocks to serve as the flywheel oscillator. The benefit of using clock ensemble as the flywheel oscillator, instead of a single clock, can be understood by the Dick-effect limit. This time scale demonstrates for the first time sub-nanosecond accuracy for a few months, attaining a fractional frequency uncertainty of 1.45*10-16 at 30 days and reaching the 10-17 decade at 50 days, with respect to UTC. This time scale significantly improves the accuracy in timekeeping and could change the existing time-scale architectures.

physics.app-ph↗
arXiv2018

Tunable mid-infrared generation via wide-band four wave mixing in silicon nitride waveguides

We experimentally demonstrate wide-band (>100 THz) frequency down-conversion of near-infrared (NIR) femtosecond-scale pulses from an Er:fiber laser to the mid-infrared (MIR) using four-wave-mixing (FWM) in photonic-chip silicon-nitride waveguides. The engineered dispersion in the nanophotonic geometry, along with the wide transparency range of silicon nitride, enables large-detuning FWM phase-matching and results in tunable MIR from 2.6-3.6 um on a single chip with 100-pJ-scale pump-pulse energies. Additionally, we observe > 20 dB broadband parametric gain for the NIR pulses when the FWM process is operated in a frequency up-conversion configuration. Our results demonstrate how integrated photonic circuits could realize multiple nonlinear optical phenomena on the same chip and lead to engineered synthesis of broadband, tunable, and coherent light across the NIR and MIR wavelength bands from fiber-based pumps.

physics.app-ph↗
arXiv2018

Thermal and Nonlinear Dissipative-Soliton Dynamics in Kerr Microresonator Frequency Combs

We explore the dynamical response of dissipative Kerr solitons to changes in pump power and detuning and show how thermal and nonlinear processes couple these parameters to the frequency-comb degrees of freedom. Our experiments are enabled by a Pound-Drever-Hall (PDH) stabilization approach that provides on-demand, radiofrequency control of the frequency comb. PDH locking not only guides Kerr-soliton formation from a cold microresonator, but opens a path to decouple the repetition and carrier-envelope-offset frequencies. In particular, we demonstrate phase stabilization of both Kerr-comb degrees-of-freedom to a fractional frequency precision below 10^-16, compatible with optical-timekeeping technology. Moreover, we investigate the fundamental role that residual laser-resonator detuning noise plays in the spectral purity of microwave generation with Kerr combs.

physics.optics↗