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Sean E. Tilton

Publications and source records attributed to Sean E. Tilton.

3 recordsLinked to original sources

Nonlinear Photoemission for Bright Beams in X-Band Photoinjectors

The ongoing development of low-cost and compact x-ray light sources is vital for increasing the number of experiments that can be performed at the atomic scale. Smaller sources can be operated in blow-out mode, in which a high-charge, short-bunch length electron beam self compresses into a uniformly ellipsoidal shape. This mode necessitates a photoinjector whose laser has a pulse duration on the order of $10^2$ fs. In this case, linear photoemission with an ultraviolet laser presents significant technical challenges, as many optical substrates degrade at these wavelengths. In this paper, we present an alternative design that uses nonlinear photoemission to produce electron beams with high charge and short bunch length. This photoinjector design produces an electron beam with a bunch charge of up to $200$ pC, an RMS bunch length of $140$ fs, a normalized transverse emittance of $1$ to $1.4$ mm$\cdot$mrad, and an energy spread of $10^{-4}$. This results in a beam brightness of $9.74\times10^{18}$ A/m$^2$, which is bright enough for our beamline's purposes. Ongoing efforts are aimed at further increasing the electron beam brightness by using a spatial light modulator to shape the laser

physics.optics

Ultrafast x-ray scattering reveals composite amplitude collective mode in the Weyl charge density wave material (TaSe$_4$)$_2$I

We report ultrafast x-ray scattering experiments of the quasi-1D charge density wave (CDW) material (TaSe$_4$)$_2$I following photoexcitation with femtosecond infrared laser pulses. From the time-dependent diffraction signal at the CDW sidebands we identify an amplitude mode derived primarily from the transverse acoustic component of the CDW static distortion. The dynamics of this acoustic amplitude mode are described well by a model of a displacive excitation, which we interpret as mediated through a coupling to the optical phonon component associated with the tetramerization of the Ta chains.

cond-mat.mtrl-sci

Temperature-dependent photoluminescence in Ge: experiment and theory

We report a photoluminescence study of high-quality Ge samples at temperatures 12 K $\leq$ T $\leq$ 295 K, over a spectral range that covers phonon-assisted emission from the indirect gap (between the lowest conduction band at the L point of the Brillouin zone and the top of the valence band at the $Γ$ point), as well as direct gap emission (from the local minimum of the conduction band at the $Γ$ point). The spectra display a rich structure with a rapidly changing lineshape as a function of T. A theory is developed to account for the experimental results using analytical expressions for the contributions from LA, TO, LO, and TA phonons. Coupling of states exactly at the $Γ$ and L points is forbidden by symmetry for the latter two phonon modes, but becomes allowed for nearby states and can be accounted for using wave-vector dependent deformation potentials. Excellent agreement is obtained between predicted and observed photoluminescence lineshapes. A decomposition of the predicted signal in terms of the different phonon contributions implies that near room temperature indirect optical absorption and emission are dominated by forbidden processes, and the deformation potentials for allowed processes are smaller than previously assumed.

cond-mat.mtrl-sci