arXiv subjects

Sean R. Muleady

Publications and source records attributed to Sean R. Muleady.

At least 19 recordsLinked to original sources

arXiv2026

Motional Kerr-Cat States of an Atom in an Optical Tweezer

Schr\"odinger cat states - quantum superpositions of classically or macroscopically distinct states - constitute a powerful resource for quantum computing, enhanced metrology, and probing coherence on large scales. Encoding such states in the phase space of an oscillator requires a nonlinearity, typically inherited from an auxiliary degree of freedom such as atomic spin or a Josephson junction. Neutral atoms trapped in reconfigurable optical tweezer arrays - a leading platform for quantum science and computing - provide an intrinsic nonlinearity via the motion of a single atom in a tightly focused trap. However, this self-Kerr mechanism has not previously been exploited for cat-state generation, and remains largely unexplored as a resource for motional-state control. Here we realize Schr\"odinger cat states in the quantized motion of a single neutral atom trapped in an optical tweezer. By modulating the depth and position, we demonstrate parity control of both Kerr-cat and Fock states alongside tunable nonlinearity, establishing a spin- and species-independent framework for controlling motion. We further show that the cat-state encoding is intrinsically robust against trap-frequency fluctuations that otherwise limit the fidelity of direct Fock-state transitions. These results establish Kerr-based control of neutral-atom motion as a new paradigm for cat-state and bosonic-state engineering in optical tweezers, providing a route toward quantum-error-correcting codes such as grid states, and toward quantum-enhanced sensing with arrays of non-Gaussian states.

quant-ph↗

arXiv2026

Multiparameter function estimation for general Hamiltonians

Estimation of physical parameters encoded in a Hamiltonian is a central task in quantum sensing and learning. While the ultimate precision limit for estimating a single parameter coupled to a single generator is well established, the corresponding bound for estimating a function of multiple parameters-each coupled to distinct and possibly non-commuting generators-remains unknown in general. Here, we derive the ultimate quantum limit and present an estimation protocol for any function of parameters in a general Hamiltonian that attains this bound. We show that, although the task is fundamentally a multiparameter problem, our tight bound reduces to an optimized single-parameter quantum Cramér-Rao bound, even for arbitrary generator sets. Our result unifies and extends previous works, providing a general framework for optimal function estimation in quantum systems.

quant-ph↗

arXiv2026

Unconventional entanglement scaling and quantum criticality in the long-range spin-one Heisenberg chain with single-ion anisotropy

Long-range interactions can fundamentally reshape the low-energy properties of low-dimensional quantum matter, altering both continuous symmetry breaking and topological phenomena. However, their impact on the quantum criticality separating these regimes remains poorly understood. We determine the ground-state phase diagram and critical properties of the spin-one Heisenberg chain with single-ion anisotropy and staggered antiferromagnetic power-law interactions, using matrix-product state (MPS) calculations complemented by high-order series expansions (pCUT+MC). Such long-range, non-frustrated interactions circumvent the Hohenberg-Mermin-Wagner theorem, thereby stabilizing continuous symmetry breaking (CSB) phases in direct competition with the Haldane phase. We map out the resulting phase diagram and analyze the entanglement entropy scaling behavior in the U(1) and SU(2) CSB phases, finding logarithmic corrections beyond the short-range, universal contributions expected from linearly dispersed Goldstone modes. We further characterize all critical boundaries through finite-size scaling of either the entanglement entropy or the staggered magnetization. In particular, the large-D-to-U(1)-CSB transition exhibits unconventional, continuously varying critical exponents as a function of the long-range decay exponent with a strong dependence on the imposed boundary conditions leading to distinct finite-size scalings for sufficiently long-range potentials. Remarkably, the Haldane-to-U(1)-CSB transition likewise displays unconventional quantum criticality with distinct continuously varying critical exponents. Our work positions this model as a target for near-term atomic platforms with tunable long-range couplings and exhibiting natural single-ion anisotropy, offering a minimal playground for exploring the interplay between long-range interactions, continuous symmetry breaking, and topology.

cond-mat.str-el↗

arXiv2026

Quantum simulation of the Dicke model in a two-dimensional ion crystal: chaos, quantum thermalization, and revivals

Quantum many-body systems driven far from equilibrium can exhibit chaos, entanglement, and non-classical correlations, yet directly observing these phenomena in large, closed quantum systems remains challenging. Here we realize the Dicke model -- a fundamental description of light-matter interactions -- in a two-dimensional crystal of approximately 100 trapped ions. The ions' internal state is optically coupled to the center of mass vibrational mode via an optical spin-dependent force, enabling unitary many-body dynamics beyond the mean-field and few-body limits. In the integrable regime, where the phonons can be adiabatically eliminated, we observe a dynamical phase transition between ferromagnetic to paramagnetic spin phases. In contrast, when the spins and phonons are strongly coupled, we observe clear signatures of non-integrable chaotic dynamics, including erratic phase-space trajectories and the exponential growth of excitations and entanglement quantified by the one-body Rényi entropy. By quenching from an unstable fixed point in the near-integrable regime, quantum noise can generate correlated spin-phonon excitations. Our numerical calculations, in clear agreement with experiment, reveal the generation of two-mode spin-phonon squeezing, 2.6 dB below the standard quantum limit (4.6 dB relative to the initial thermal state), followed by generalized vacuum Rabi collapses and revivals. Our results establish large ion crystals as scalable analog quantum simulators of non-equilibrium light-matter dynamics and provide a controlled platform for experimental studies of information scrambling and entanglement in closed many-body systems.

quant-ph↗

arXiv2026

Interacting electrons in silicon quantum interconnects

Coherent interconnects between gate-defined silicon quantum processing units are essential for scalable quantum computation and long-range entanglement. We argue that one-dimensional electron channels formed in the silicon quantum well of a Si/SiGe heterostructure exhibit strong Coulomb interactions and realize strongly interacting Luttinger liquid physics. At low electron densities, the system enters a Wigner regime characterized by dominant 4kF correlations; increasing the electron density leads to a crossover from the Wigner regime to a Friedel regime with dominant 2kF correlations. We support these results through large-scale density matrix renormalization group (DMRG) simulations of the interacting ground state under both screened and unscreened Coulomb potentials. We propose experimental signatures of the Wigner-Friedel crossover via charge transport and charge sensing in both zero- and high-magnetic field limits. We also analyze the impact of short-range correlated disorder - including random alloy fluctuations and valley splitting variations - and identify that the Wigner-Friedel crossover remains robust until disorder levels of about 400 micro eV. Finally, we show that the Wigner regime enables long-range capacitive coupling between quantum dots across the interconnect, suggesting a route to create long-range entanglement between solid-state qubits. Our results position silicon interconnects as a platform for studying Luttinger liquid physics and for enabling architectures supporting nonlocal quantum error correction and quantum simulation.

cond-mat.mes-hall↗

arXiv2025

Hybrid qubit-oscillator module from motional states of two interacting atoms

We propose a qubit-oscillator platform based on the motional states of two interacting atoms in an optical tweezer. By stroboscopically modulating an engineered trap with tunable anharmonicity, we implement a complete set of bosonic operations and their qubit-controlled counterparts with high fidelity. This motional control enables accurate detection of magnetic dipolar interactions with $\sim10$ Hz sensitivity in one second, reaching sub-Hz resolution within a few minutes in a $20\times20$ tweezer array under realistic experimental imperfections. Our approach establishes a versatile platform for motional quantum control of two atoms, with applications to spin-boson physics and precision sensing of interaction potentials and trapping environments.

quant-ph↗

arXiv2025

Optimally learning functions in interacting quantum sensor networks

Estimating extensive combinations of local parameters in distributed quantum systems is a central problem in quantum sensing, with applications ranging from magnetometry to timekeeping. While optimal strategies are known for sensing non-interacting Hamiltonians in quantum sensor networks, fundamental limits in the presence of uncontrolled interactions remain unclear. Here, we establish optimal bounds and protocols for estimating a linear combination of local parameters of Hamiltonians with arbitrary, unknown interactions. In the process, we more generally establish bounds for learning any linear combination of Hamiltonian coefficients for arbitrary, commuting terms. Our results unify and extend existing bounds for non-interacting qubits and multimode interferometers, providing a general framework for distributed sensing and Hamiltonian learning in realistic many-body systems.

quant-ph↗

arXiv2025

Error mitigation of shot-to-shot fluctuations in analog quantum simulators

Analog quantum simulators have provided key insights into quantum many-body dynamics. However, in such systems, both coherent and incoherent errors limit their scalability, hindering simulations in regimes that challenge classical simulations. In this work, we introduce an error mitigation technique that addresses and effectively suppresses a key source of error in leading simulator platforms: shot-to-shot fluctuations in the parameters for the Hamiltonian governing the system dynamics. We rigorously prove that amplifying this shot-to-shot noise and extrapolating to the zero-noise limit recovers noiseless results for realistic noise distributions. Experimentally, we demonstrate this technique on a 27-ion trapped-ion quantum simulator, extending the two-qubit exchange oscillation lifetime threefold. Numerically, we predict a significant enhancement in the effective many-body coherence time for Rydberg atom arrays under realistic conditions. Our scheme provides a possible route towards extending the effective coherence time in analog quantum experiments, enabling deeper explorations of quantum many-body dynamics.

quant-ph↗

arXiv2025

Lieb-Mattis states for robust entangled differential phase sensing

We explore a two-node, entanglement-enhanced sensor network for differential phase sensing that exploits decoherence-free subspaces to suppress common-mode noise, a primary limitation of many state-of-the-art quantum sensors. We identify a class of entangled states that, while not strictly optimal, achieve the same asymptotic sensitivity scaling as optimal states and can be prepared efficiently from initially unentangled atomic ensembles. Importantly, the preparation time decreases with increasing system size. This makes the states compatible with realistic noise processes in present-day quantum sensors that operate with large particle numbers but lack full error correction. We illustrate these ideas using two cavity-mediated preparation protocols: (i) coherent, unitary entanglement generation analogous to bosonic two-mode squeezing, yielding Heisenberg scaling; and (ii) dissipative preparation via collective emission into a shared cavity mode, providing a square-root improvement beyond the standard quantum limit. Numerical simulations show that both approaches remain effective at experimentally realistic cavity cooperativities, establishing a practical path toward scalable, quantum-enhanced differential phase sensing.

quant-ph↗

arXiv2025

Observation of generalized t-J spin dynamics with tunable dipolar interactions

Long-range and anisotropic dipolar interactions profoundly modify the dynamics of particles hopping in a periodic lattice potential. We report the realization of a generalized t-J model with dipolar interactions using a system of ultracold fermionic molecules with spin encoded in the two lowest rotational states. We independently tuned the dipolar Ising and spin-exchange couplings and the molecular motion and studied their interplay on coherent spin dynamics. Using Ramsey spectroscopy, we observed and modeled interaction-driven contrast decay that depends strongly both on the strength of the anisotropy between Ising and spin-exchange couplings and on motion. This study paves the way for future exploration of kinetic spin dynamics and quantum magnetism with highly tunable molecular platforms in regimes that are challenging for existing numerical and analytical methods.

cond-mat.quant-gas↗

arXiv2025

Enhancement of Rydberg Blockade via Microwave Dressing

Experimental control over the strength and angular dependence of interactions between atoms is a key capability for advancing quantum technologies. Here, we use microwave dressing to manipulate and enhance Rydberg-Rydberg interactions in an atomic ensemble. By varying the cloud length relative to the blockade radius and measuring the statistics of the light retrieved from the ensemble, we demonstrate a clear enhancement of the interaction strength due to microwave dressing. These results are successfully captured by a theoretical model that accounts for the excitation dynamics, atomic density distribution, and the phase-matched retrieval efficiency. Our approach offers a versatile platform for further engineering interactions by exploiting additional features of the microwave fields, such as polarization and detuning, opening pathways for new quantum control strategies.

physics.atom-ph↗

arXiv2024

Efficient preparation of Dicke states

We present an algorithm utilizing mid-circuit measurement and feedback that prepares Dicke states with polylogarithmically many ancillas and polylogarithmic depth. Our algorithm uses only global mid-circuit projective measurements and adaptively-chosen global rotations. This improves over prior work that was only efficient for Dicke states of low weight, or was not efficient in both depth and width. Our algorithm can also naturally be implemented in a cavity QED context using polylogarithmic time, zero ancillas, and atom-photon coupling scaling with the square root of the system size.

quant-ph↗

arXiv2024

Measuring bipartite spin correlations of lattice-trapped dipolar atoms

We demonstrate a bipartition technique using a super-lattice architecture to access correlations between alternating planes of a mesoscopic array of spin-3 chromium atoms trapped in a 3D optical lattice. Using this method, we observe that out-of-equilibrium dynamics driven by long-range dipolar interactions lead to spin anti-correlations between the two spatially separated subsystems. Our bipartite measurements reveal a subtle interplay between the anisotropy of the 3D dipolar interactions and that of the lattice structure, without requiring single-site addressing. We compare our results to theoretical predictions based on a truncated cumulant expansion and a new cluster semi-classical method that we use to investigate correlations at the microscopic scale. Comparison with a high-temperature analytical model reveals quantum thermalization at a high negative spin temperature.

cond-mat.quant-gas↗

arXiv2023

Validating phase-space methods with tensor networks in two-dimensional spin models with power-law interactions

Using a recently developed extension of the time-dependent variational principle for matrix product states, we evaluate the dynamics of 2D power-law interacting XXZ models, implementable in a variety of state-of-the-art experimental platforms. We compute the spin squeezing as a measure of correlations in the system, and compare to semiclassical phase-space calculations utilizing the discrete truncated Wigner approximation (DTWA). We find the latter efficiently and accurately captures the scaling of entanglement with system size in these systems, despite the comparatively resource-intensive tensor network representation of the dynamics. We also compare the steady-state behavior of DTWA to thermal ensemble calculations with tensor networks. Our results open a way to benchmark dynamical calculations for two-dimensional quantum systems, and allow us to rigorously validate recent predictions for the generation of scalable entangled resources for metrology in these systems.

quant-ph↗

arXiv2023

Comparison of Spontaneous Emission in Trapped Ion Multiqubit Gates at High Magnetic Fields

Penning traps have been used for performing quantum simulations and sensing with hundreds of ions and provide a promising route toward scaling up trapped ion quantum platforms because of the ability to trap and control up to thousands of ions in 2D and 3D crystals. A leading source of decoherence in laser-based multiqubit operations on trapped ions is off-resonant spontaneous emission. While many trapped ion quantum computers or simulators utilize clock qubits, other systems rely on Zeeman qubits, which require a more complex calculation of this decoherence. We examine theoretically the impacts of spontaneous emission on quantum gates performed with trapped ions in a high magnetic field. We consider two types of gates -- light-shift and Molmer-Sorensen gates -- and compare the decoherence errors in each. We also compare different detunings, polarizations, and required intensities of the laser beams used to drive the gates. We show that both gates can have similar performance at their optimal operating conditions and examine the experimental feasibility of various operating points. By examining the magnetic field dependence of each gate, we demonstrate that when the $P$ state fine structure splitting is large compared to the Zeeman splittings, the theoretical performance of the Molmer-Sorensen gate is significantly better than that of the light-shift gate. Additionally, for the light-shift gate, we make an approximate comparison between the fidelities that can be achieved at high fields with the fidelities of state-of-the-art two-qubit trapped ion quantum gates. We show that, with regard to spontaneous emission, the achievable infidelity of our current configuration is about an order of magnitude larger than that of the best low-field gates, but we also discuss alternative configurations with potential error rates that are comparable with state-of-the-art trapped ion gates.

quant-ph↗

arXiv2023

Quantum-enhanced sensing on an optical transition via emergent collective quantum correlations

The control over quantum states in atomic systems has led to the most precise optical atomic clocks to date. Their sensitivity is currently bounded by the standard quantum limit, a fundamental floor set by quantum mechanics for uncorrelated particles, which can nevertheless be overcome when operated with entangled particles. Yet demonstrating a quantum advantage in real world sensors is extremely challenging and remains to be achieved aside from two remarkable examples, LIGO and more recently HAYSTAC. Here we illustrate a pathway for harnessing scalable entanglement in an optical transition using 1D chains of up to 51 ions with state-dependent interactions that decay as a power-law function of the ion separation. We show our sensor can be made to behave as a one-axis-twisting (OAT) model, an iconic fully connected model known to generate scalable squeezing. The collective nature of the state manifests itself in the preservation of the total transverse magnetization, the reduced growth of finite momentum spin-wave excitations, the generation of spin squeezing comparable to OAT (a Wineland parameter of $-3.9 \pm 0.3$ dB for only N = 12 ions) and the development of non-Gaussian states in the form of atomic multi-headed cat states in the Q-distribution. The simplicity of our protocol enables scalability to large arrays with minimal overhead, opening the door to advances in timekeeping as well as new methods for preserving coherence in quantum simulation and computation. We demonstrate this in a Ramsey-type interferometer, where we reduce the measurement uncertainty by $-3.2 \pm 0.5$ dB below the standard quantum limit for N = 51 ions.

quant-ph↗

arXiv2022

Enhancing spin squeezing using soft-core interactions

We propose a new protocol for preparing spin squeezed states in controllable atomic, molecular, and optical systems, with particular relevance to emerging optical clock platforms compatible with Rydberg interactions. By combining a short-ranged, soft-core potential with an external drive, we can transform naturally emerging Ising interactions into an XX spin model while opening a many-body gap. The gap helps maintain the system within a collective manifold of states where metrologically useful spin squeezing can be generated at a level comparable to the spin squeezing generated in systems with genuine all-to-all interactions. We examine the robustness of our protocol to experimentally-relevant decoherence and show favorable performance over typical protocols lacking gap protection.

quant-ph↗

arXiv2022

Fast generation of spin squeezing via resonant spin-boson coupling

We propose protocols for the creation of useful entangled states in a system of spins collectively coupled to a bosonic mode, directly applicable to trapped-ion and cavity QED setups. The protocols use coherent manipulations of the spin-boson interactions naturally arising in these systems to prepare spin squeezed states exponentially fast in time. We demonstrate the robustness of the protocols by analyzing the effects of natural sources of decoherence in these systems and show their advantage compared to more standard slower approaches where entanglement is generated algebraically with time.

quant-ph↗