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Sebastiaan L. D. ten Haaf

Publications and source records attributed to Sebastiaan L. D. ten Haaf.

18 recordsLinked to original sources

Cross-Platform Autonomous Control of Minimal Kitaev Chains

Contemporary quantum devices are reaching new limits in size and complexity, allowing for the experimental exploration of emergent quantum modes. However, this increased complexity introduces significant challenges in device tuning and control. Here, we demonstrate autonomous tuning of emergent Poor Man's Majorana zero modes in a minimal realization of a Kitaev chain. We achieve this task using cross-platform transfer learning. First, we train a tuning model on a theory model. Next, we retrain it using a Kitaev chain realization in a two-dimensional electron gas. Finally, we apply this model to tune a Kitaev chain realized in quantum dots coupled through a semiconductor-superconductor section in a one-dimensional nanowire. Utilizing a convolutional neural network, we predict the tunneling and Cooper pair splitting rates from differential conductance measurements, employing these predictions to adjust the electrochemical potential to a Poor Man's Majorana sweet spot. The algorithm successfully converges to an immediate vicinity of a sweet spot (within 1.5 mV in 67.6% of attempts and within 4.5 mV in 80.9% of cases), typically finding a sweet spot in 45 minutes or less. This advancement is a stepping stone towards autonomous tuning of emergent modes in interacting systems, and towards foundational tuning machine learning models that can be deployed across a range of experimental platforms.

cond-mat.mes-hall↗

Using Andreev bound states and spin to remove domain walls in a Kitaev chain

Quantum dot-superconductor hybrids have been established as a suitable platform for realizing Kitaev chains hosting Majorana bound states. Implementing these structures in a qubit architecture is expected to result in coherence times that scale exponentially with the lengths of the chains. To scale to longer systems, the phase differences between all superconducting segments in the chain need to be controlled. While this control has been demonstrated by using an external magnetic flux, ideally it can be achieved with control over intrinsic system parameters. In this work, we investigate whether the relevant phase differences can be tuned through the spin degree of freedom in each QD, or the chemical potential of the discrete bound states in the hybrid sections. We confirm that both these tuning knobs allow for controlling the phase difference in the couplings between neighbouring QDs, bypassing the requirement to tune an external flux. However, we find that the amplitude of the phase shifts can deviate from a discrete $π$-shift. We introduce a spatial variation in the spin-orbit field as a possible mechanism to explain the observed behaviour and comment on the consequences for experimentally creating long Kitaev chains.

cond-mat.mes-hall↗

Probing ground-state degeneracies of a strongly interacting Fermi-Hubbard model with superconducting correlations

The Fermi-Hubbard model and its rich phase diagram naturally emerges as a description for a wide range of electronic systems. Recent advances in semiconductor-superconductor hybrid quantum dot arrays have allowed to realize degenerate quantum systems in a controllable way, e.g., allowing to observe robust zero-bias peaks in Kitaev chains, indicative for Majorana bound states. In this work, we connect these two domains. Noting the strong on-site Coulomb repulsion within quantum dots, we study small arrays of spinful hybrid quantum dots implemented in a two-dimensional electron gas. This system constitutes a Fermi-Hubbard model with inter-site superconducting correlations. For two electronic sites, we find robust zero-bias peaks indicative of a strongly degenerate spectrum hosting emergent Majorana Kramers pairs or $\mathbb{Z}_3$-parafermions. Extending to three sites, we find that these spinful systems scale very differently compared to spinless Kitaev chains. When the sweet-spot conditions are satisfied pairwise, we find that the ground state degeneracy of the full three-site system is lifted. This degeneracy can be restored by tuning the superconducting phase difference between the hybrid segments. However, these states are not robust to quantum dot detuning. Our observations are a first step towards studying degeneracies in strongly interacting Fermi-Hubbard systems with superconducting correlations.

cond-mat.mes-hall↗

Gate reflectometry in a minimal Kitaev chain device

Hybrid quantum dot (QD)-superconductor system can be used to realize Majorana zero modes in artificial Kitaev chains. These chains provide a promising platform for the realization of Majorana qubits. Radio-frequency (RF) gate reflectometry is a fast, non-invasive, and sensitive technique that can be used to read out such qubits. In this work, we use gate reflectometry to probe two QDs coupled via a semiconductor-superconductor hybrid segment. We demonstrate that gate sensing can resolve charge stability diagrams and clearly distinguish between elastic cotunneling and crossed-Andreev reflection, the two key processes that allow one to form a Kitaev chain. Furthermore, we show that this information is accessible, even when the system is completely decoupled from the from the normal leads. In this closed regime, we show that the observed quantum capacitance signal is indicative of parity switching between the even and odd ground states. Our measurements in both open and closed regimes confirm that gate reflectometry captures the essential features of interdot coupling and parity dynamics.

cond-mat.mes-hall↗

Probing Majorana localization of a phase-controlled three-site Kitaev chain with an additional quantum dot

Few-site implementations of the Kitaev chain offer a minimal platform to study the emergence and stability of Majorana bound states. Here, we realize two- and three-site chains in semiconducting quantum dots coupled via superconductors, and tune them to the sweet spot where zero-energy Majorana modes appear at the chain ends. We demonstrate control of the superconducting phase through both magnetic field and sweet-spot selection, and fully characterize the excitation spectrum under local and global perturbations. All spectral features are identified using the ideal Kitaev chain model. To assess Majorana localization, we couple the system to an additional quantum dot. The absence of energy splitting at the sweet spot confirms the high quality of the Majorana modes, despite the minimal size of the chains.

cond-mat.mes-hall↗

Observation of edge and bulk states in a three-site Kitaev chain

A chain of quantum dots (QDs) in semiconductor-superconductor hybrid systems can form an artificial Kitaev chain hosting Majorana bound states (MBSs). These zero-energy states are expected to be localised on the edges of the chain, at the outermost QDs. The remaining QDs, comprising the bulk, are predicted to host an excitation gap that protects the MBSs at the edges from local on-site perturbations. Here we demonstrate this connection between the bulk and edges in a minimal system, by engineering a three-site Kitaev chain in a two-dimensional electron gas. Through direct tunneling spectroscopy on each site, we show that the appearance of stable zero-bias conductance peaks at the outer QDs is correlated with the presence of an excitation gap in the middle QD. Furthermore, we show that this gap can be controlled by applying a superconducting phase difference between the two hybrid segments and that the MBSs are robust only when the excitation gap is present. We find a close agreement between experiments and the original Kitaev model, thus confirming key predictions for MBSs in a three-site chain.

cond-mat.mes-hall↗

Interaction-induced strong zero modes in short quantum dot chains with time-reversal symmetry

We theoretically explore the emergence of strong zero modes in a two-site chain consisting of two quantum dots coupled due to a central dot that mediates electron hopping and singlet superconducting pairing. In the presence of time-reversal symmetry, the on-site Coulomb interaction leads to a three-fold ground-state degeneracy when tuning the system to a sweet spot as a function of the inter-dot couplings. This degeneracy is protected against changes of the dot energies in the same way as "poor man's'' Majorana bound states in short Kitaev chains. In the limit of strong interactions, this protection is maximal and the entire spectrum becomes triply degenerate, indicating the emergence of a ''poor man's'' version of a strong zero mode. We explain the degeneracy and protection by constructing corresponding Majorana Kramers-pair operators and $\mathbb{Z}_3$-parafermion operators. The strong zero modes share many properties of Majorana bound states in short Kitaev chains, including the stability of zero-bias peaks in the conductance and the behavior upon coupling to an additional quantum dot. However, they can be distinguished through finite-bias spectroscopy and the exhibit a different behavior when scaling to longer chains.

cond-mat.mes-hall↗

A flux-controlled two-site Kitaev chain

In semiconducting-superconducting hybrid devices, Andreev bound states (ABSs) can mediate the coupling between quantum dots (QDs), allowing for the realisation of artificial Kitaev chains. In order to engineer Majorana bound states (MBSs) in these systems, one must control the energy of the ABSs. In this work, we show how extended ABSs in a flux tunable Josephson junction can be used to control the coupling between distant quantum dots separated by $\approx$ 1 $\mathrmμ$m. In particular, we demonstrate that the combination of electrostatic control and phase control over the ABSs significantly increases the parameter space in which MBSs are observed. Finally, by employing an additional spectroscopic probe in the hybrid region between the QDs, we gain information about the spatial distribution of the Majorana wave function in a two-site Kitaev chain.

cond-mat.mes-hall↗

Scaling up a sign-ordered Kitaev chain without magnetic flux control

Quantum dot-superconductor arrays have emerged as a new and promising material platform for realizing topological Kitaev chains. So far, experiments have implemented a two-site chain with limited protection. Here we propose an experimentally feasible protocol for scaling up the chain in order to enhance the protection of the Majorana zero modes. To this end, we make use of the fact that the relative sign of normal and superconducting hoppings mediated by an Andreev bound state can be changed by electrostatic gates. In this way, our method only relies on the use of individual electrostatic gates on hybrid regions, quantum dots, and tunnel barriers, respectively, without the need for individual magnetic flux control, greatly simplifying the device design. Our work provides guidance for realizing a topologically protected Kitaev chain, which is the building block of error-resilient topological quantum computation.

cond-mat.mes-hall↗

Triplet correlations in Cooper pair splitters realized in a two-dimensional electron gas

Cooper pairs occupy the ground state of superconductors and are typically composed of maximally entangled electrons with opposite spin. In order to study the spin and entanglement properties of these electrons, one must separate them spatially via a process known as Cooper pair splitting (CPS). Here we provide the first demonstration of CPS in a semiconductor two-dimensional electron gas (2DEG). By coupling two quantum dots to a superconductor-semiconductor hybrid region we achieve efficient Cooper pair splitting, and clearly distinguish it from other local and non-local processes. When the spin degeneracy of the dots is lifted, they can be operated as spin-filters to obtain information about the spin of the electrons forming the Cooper pair. Not only do we observe a near perfect splitting of Cooper pairs into opposite-spin electrons (i.e. conventional singlet pairing), but also into equal-spin electrons, thus achieving triplet correlations between the quantum dots. Importantly, the exceptionally large spin-orbit interaction in our 2DEGs results in a strong triplet component, comparable in amplitude to the singlet pairing. The demonstration of CPS in a scalable and flexible platform provides a credible route to study on-chip entanglement and topological superconductivity in the form of artificial Kitaev chains.

cond-mat.mes-hall↗

A two-site Kitaev chain in a two-dimensional electron gas

Artificial Kitaev chains can be used to engineer Majorana bound states (MBSs) in superconductor-semiconductor hybrids. In this work, we realize a two-site Kitaev chain in a two-dimensional electrongas by coupling two quantum dots through a region proximitized by a superconductor. We demonstrate systematic control over inter-dot couplings through in-plane rotations of the magnetic field and via electrostatic gating of the proximitized region. This allows us to tune the system to sweet spots in parameter space, where robust correlated zero bias conductance peaks are observed in tunnelling spectroscopy. To study the extent of hybridization between localized MBSs, we probe the evolution of the energy spectrum with magnetic field and estimate the Majorana polarization, an important metric for Majorana-based qubits. The implementation of a Kitaev chain on a scalable and flexible 2D platform provides a realistic path towards more advanced experiments that require manipulation and readout of multiple MBSs.

cond-mat.mes-hall↗

Signatures of Majorana protection in a three-site Kitaev chain

Majorana zero modes (MZMs) are non-Abelian excitations predicted to emerge at the edges of topological superconductors. One proposal for realizing a topological superconductor in one dimension involves a chain of spinless fermions, coupled through $p$-wave superconducting pairing and electron hopping. This concept is also known as the Kitaev chain. A minimal two-site Kitaev chain has recently been experimentally realized using quantum dots (QDs) coupled through a superconductor. In such a minimal chain, MZMs are quadratically protected against global perturbations of the QD electrochemical potentials. However, they are not protected from perturbations of the inter-QD couplings. In this work, we demonstrate that extending the chain to three sites offers greater protection than the two-site configuration. The enhanced protection is evidenced by the stability of the zero-energy modes, which is robust against variations in both the coupling amplitudes and the electrochemical potential variations in the constituent QDs. While our device offers all the desired control of the couplings it does not allow for superconducting phase control. Our experimental observations are in good agreement with numerical simulated conductances with phase averaging. Our work pioneers the development of longer Kitaev chains, a milestone towards topological protection in QD-based chains.

cond-mat.supr-con↗

Enhancing the excitation gap of a quantum-dot-based Kitaev chain

Connecting double quantum dots via a semiconductor-superconductor hybrid segment offers a platform for creating a two-site Kitaev chain that hosts a pair of "poor man's Majoranas" at a finely tuned sweet spot. However, the effective couplings, which are mediated by Andreev bound states in the hybrid, are generally weak in the tunneling regime. As a consequence, the excitation gap is limited in size, presenting a formidable challenge for using this platform to demonstrate non-Abelian statistics of Majoranas and realizing error-resilient topological quantum computing. In this work, we systematically study the effects of increasing the coupling between the dot and the hybrid segment. In particular, the proximity effect transforms the dot orbitals into Yu-Shiba-Rusinov states, forming a new spinless fermion basis for a Kitaev chain, and we derive a theory for their effective coupling. As the coupling strength between the dots and the hybrid segment increases, we find a significant enhancement of the excitation gap and reduced sensitivity to local perturbations. Although the hybridization of the Majorana wave function with the central Andreev bound states increases strongly with increasing coupling, the overlap of Majorana modes on the outer dots remains small, which is a prerequisite for potential qubit experiments. We discuss how the strong-coupling regime shows in experimentally accessible quantities, such as the local and non-local conductance, and provide a protocol for tuning a double-dot system into a sweet spot with a large excitation gap.

cond-mat.mes-hall↗

Realization of a minimal Kitaev chain in coupled quantum dots

Majorana bound states constitute one of the simplest examples of emergent non-Abelian excitations in condensed matter physics. A toy model proposed by Kitaev shows that such states can arise at the ends of a spinless $p$-wave superconducting chain. Practical proposals for its realization require coupling neighboring quantum dots in a chain via both electron tunneling and crossed Andreev reflection. While both processes have been observed in semiconducting nanowires and carbon nanotubes, crossed-Andreev interaction was neither easily tunable nor strong enough to induce coherent hybridization of dot states. Here we demonstrate the simultaneous presence of all necessary ingredients for an artificial Kitaev chain: two spin-polarized quantum dots in an InSb nanowire strongly coupled by both elastic co-tunneling and crossed Andreev reflection. We fine-tune this system to a sweet spot where a pair of Poor Man's Majorana states is predicted to appear. At this sweet spot, the transport characteristics satisfy the theoretical predictions for such a system, including pairwise correlation, zero charge and stability against local perturbations. While the simple system presented here can be scaled to simulate a full Kitaev chain with an emergent topological order, it can also be used imminently to explore relevant physics related to non-Abelian anyons.

cond-mat.mes-hall↗

Singlet and triplet Cooper pair splitting in hybrid superconducting nanowires

In most naturally occurring superconductors, electrons with opposite spins are paired up to form Cooper pairs. This includes both conventional $s$-wave superconductors such as aluminum as well as high-$T_\text{c}$, $d$-wave superconductors. Materials with intrinsic $p$-wave superconductivity, hosting Cooper pairs made of equal-spin electrons, have not been conclusively identified, nor synthesized, despite promising progress. Instead, engineered platforms where $s$-wave superconductors are brought into contact with magnetic materials have shown convincing signatures of equal-spin pairing. Here, we directly measure equal-spin pairing between spin-polarized quantum dots. This pairing is proximity-induced from an $s$-wave superconductor into a semiconducting nanowire with strong spin-orbit interaction. We demonstrate such pairing by showing that breaking a Cooper pair can result in two electrons with equal spin polarization. Our results demonstrate controllable detection of singlet and triplet pairing between the quantum dots. Achieving such triplet pairing in a sequence of quantum dots will be required for realizing an artificial Kitaev chain.

cond-mat.mes-hall↗

Crossed Andreev reflection and elastic co-tunneling in a three-site Kitaev chain nanowire device

The formation of a topological superconducting phase in a quantum-dot-based Kitaev chain requires nearest neighbor crossed Andreev reflection and elastic co-tunneling. Here we report on a hybrid InSb nanowire in a three-site Kitaev chain geometry - the smallest system with well-defined bulk and edge - where two superconductor-semiconductor hybrids separate three quantum dots. We demonstrate pairwise crossed Andreev reflection and elastic co-tunneling between both pairs of neighboring dots and show sequential tunneling processes involving all three quantum dots. These results are the next step towards the realization of topological superconductivity in long Kitaev chain devices with many coupled quantum dots.

cond-mat.mes-hall↗

Controlled crossed Andreev reflection and elastic co-tunneling mediated by Andreev bound states

A short superconducting segment can couple attached quantum dots via elastic co-tunneling (ECT) and crossed Andreev reflection (CAR). Such coupled quantum dots can host Majorana bound states provided that the ratio between CAR and ECT can be controlled. Metallic superconductors have so far been shown to mediate such tunneling phenomena, albeit with limited tunability. Here we show that Andreev bound states formed in semiconductor-superconductor heterostructures can mediate CAR and ECT over mesoscopic length scales. Andreev bound states possess both an electron and a hole component, giving rise to an intricate interference phenomenon that allows us to tune the ratio between CAR and ECT deterministically. We further show that the combination of intrinsic spin-orbit coupling in InSb nanowires and an applied magnetic field provides another efficient knob to tune the ratio between ECT and CAR and optimize the amount of coupling between neighboring quantum dots.

cond-mat.mes-hall↗

Supported lipid membranes with designed geometry

The membrane curvature of cells and intracellular compartments continuously adapts to enable cells to perform vital functions, from cell division to signal trafficking. Understanding how membrane geometry affects these processes in vivo is challenging because of the membrane complexity as well as the short time and small length scales involved. By contrast, in vitro model membranes with engineered curvature provide a versatile platform for this investigation and applications to biosensing and biocomputing. However, a general route to the fabrication of lipid membranes with prescribed curvature and high spatial resolution is still missing. Here, we present a strategy that overcomes these challenges and achieve lipid membranes with designed shape by combining 3D micro-printing and replica-molding lithography to create scaffolds with virtually any geometry and high spatial resolution. The resulting supported lipid membranes are homogeneous, fluid, and can form chemically distinct lipid domains. These features are essential for understanding curvature-dependent cellular processes and developing programmable bio-interfaces for living cells and nanostructures.

cond-mat.soft↗