arXiv subjects

Sebastiaan van Dijken

Publications and source records attributed to Sebastiaan van Dijken.

At least 19 recordsLinked to original sources

arXiv2026

Bismuth-substituted Lutetium Iron Garnet Films with Giant Visible-Range Magneto-Optical Sensitivity

Magneto-optical materials are indispensable across modern physics, serving as the foundation for precision magnetic sensing, nonreciprocal photonics, and optical isolation technologies. The continual pursuit of materials with high Verdet constants has driven the development of garnet-based compounds exhibiting giant magneto-optical sensitivity. In this work, we report the growth and comprehensive magneto-optical characterization of bismuth-substituted lutetium iron garnet (LuBiIG), a material that combines the large spin-orbit coupling of bismuth with the lattice stability of lutetium iron garnet. LuBiIG films with thicknesses between 85-220nm were grown by pulsed laser deposition and characterized at room temperature over the 500-820nm wavelength range. The films exhibit an exceptionally high Verdet constant of up to -1.37e8 degree/meter/Tesla, peaking in the visible spectral range near 520nm. These results position LuBiIG as a highly sensitive magneto-optical material suitable for advanced cryogenic detection and hybrid quantum applications.

cond-mat.mtrl-sci↗

arXiv2026

Brillouin Light Scattering Spectroscopy of Propagating Magnons at Sub-Kelvin Temperatures

Coupling light to magnetic excitations in the form of spin waves underpins both the optical study of magnetism and emerging schemes for quantum transduction, positioning the quanta of these excitations, magnons, as promising carriers for hybrid quantum networks. However, exploiting them in the quantum regime requires millikelvin temperatures to suppress thermal magnon populations, thereby confining such experiments to dilution refrigerators. There, magnons can already be excited and read out electrically, yet an optical interface required for microwave-to-optical photon conversion has been missing. Here, we demonstrate the first optical detection of coherently driven, propagating spin waves via Brillouin Light Scattering (BLS) spectroscopy inside a dilution refrigerator. By simultaneously recording the optical and electrical responses of the same spin-wave mode in a yttrium iron garnet film, we find that the BLS spectra track the electrically measured transmission across a range of applied magnetic fields. For the lowest optical power of 7.9 μW that still enabled spin-wave detection, we measured a global equilibrium sample temperature of 510 mK via a resistance thermometer, while numerical modelling of the laser-induced heating yields a maximum local temperature of 900 mK at the focal spot. This brings free-space optical access to magnons into the sub-kelvin regime, representing a milestone towards magnon-mediated quantum transduction in hybrid quantum systems.

cond-mat.other↗

arXiv2026

Spin-Wave Phase Shifter Controlled by a Domain Wall Racetrack

We propose a spin-wave phase shifter controlled using a domain-wall racetrack. The concept is demonstrated using micromagnetic simulations of a Permalloy domain-wall racetrack placed above a YIG film. The stray field from pinned domain walls modifies the internal magnetic field in the YIG region under the racetrack. This leads to a local change of the spin-wave wavelength and thereby enables control of the phase accumulated by Damon-Eshbach spin waves propagating through the region. Moving domain walls on the racetrack, the same physical structure can provide phase shifts of up to +/-90 degrees, without changing the waveguide geometry. A model based on the semiclassical approximation confirms that the phase shift is dominated by the domain-wall-induced stray field. These results suggest a route toward a compact programmable spin-wave phase shifter for interference-based magnonic circuits for information processing. Moreover, the demonstrated magnonic device integration with a magnetic domain-wall racetrack can lead to its application in in-memory computing.

cond-mat.mes-hall↗

arXiv2026

Spin-wave bandgap engineering via mode hybridization in dipolar-coupled YIG film/CoFeB nanodisk magnonic crystals

We investigate spin-wave transport in hybrid two-dimensional magnonic crystals comprising a low-damping yttrium iron garnet (YIG) film coupled to a periodic array of CoFeB nanodisks. Using propagating spin-wave spectroscopy, super-Nyquist magneto-optical Kerr effect microscopy, and micromagnetic simulations, we demonstrate the formation of pronounced and tunable bandgaps that do not originate from conventional Bragg scattering. Instead, these gaps arise from hybridization between the fundamental magnonic-crystal mode and in-plane transverse standing modes induced by the periodic nanodisk array. The spectral position and width of these gaps are controlled by geometric parameters and by the magnetic state of the nanodisks, including their vortex configuration, which governs both static and dynamic dipolar coupling. For larger lattice periods, additional gaps emerge through hybridization with modes quantized both transverse and parallel to the spin-wave propagation direction, reflecting dispersion folding in two dimensions. Our results establish mode hybridization as a versatile mechanism for engineering spin-wave band structures beyond the constraints of Bragg scattering and provide a pathway toward reconfigurable magnonic devices based on dipolar-coupled hybrid architectures.

cond-mat.mes-hall↗

arXiv2026

Realization of the Tellegen Effect in Resonant Optical Metasurfaces

The nonreciprocal magnetoelectric effect in Tellegen materials enables exotic phenomena such as axion-modified electrodynamics and fosters the development of magnet-free nonreciprocal media. As the nonreciprocal counterpart to the well-known chiral electromagnetic response, it offers a parallel framework in which many concepts developed for chiral materials can be translated to Tellegen media, potentially unlocking new avenues for fundamental studies and applications. Although predicted over 75 years ago and observed in only a handful of natural materials with very low strength, the strong optical Tellegen effect has remained experimentally elusive. Here, we report the first experimental demonstration of a resonant optical diagonal Tellegen effect in a metasurface, showcasing a response that is 100 times greater than that of any known natural material. This optical metasurface, consisting of randomly distributed cobalt-silicon nanoscatterers with strong shape anisotropy, utilizes spontaneous magnetization to achieve a robust Tellegen effect without the need for an external magnetic field. In addition to the Tellegen response, the metasurface exhibits both gyroelectric and gyromagnetic effects, contributing to nonreciprocal cross-polarized light reflection. We introduce a technique to independently extract the amplitudes of these three effects using conventional magneto-optical single-side-illumination measurements. The observation of the resonant Tellegen effects in the optical frequency range may lead to the experimental observation of axionic electrodynamics and compact bias-free nonreciprocal optical devices.

physics.optics↗

arXiv2026

Nonlinear dynamics in magnonic Fabry-Pérot resonators: Low-power neuron-like activation and transmission suppression

We report on nonlinear spin-wave dynamics in magnonic Fabry-Pérot resonators composed of yttrium iron garnet (YIG) films coupled to CoFeB nanostripes. Using super-Nyquist sampling magneto-optical Kerr effect microscopy and micromagnetic simulations, we observe a systematic downshift of the spin-wave transmission gaps as the excitation power increases. This nonlinear behavior occurs at low power levels, reduced by a strong spatial concentration of spin waves within the resonator. The resulting power-dependent transmission enables neuron-like activation behavior and frequency-selective nonlinear spin-wave absorption. Our results highlight magnonic Fabry-Pérot resonators as compact low-power nonlinear elements for neuromorphic magnonic computing architectures.

cond-mat.mtrl-sci↗

arXiv2025

Reservoir computing in a lithium-based magneto-ionic device

In-materio computing exploits the intrinsic physical dynamics of materials to perform complex computations, enabling low-power, real-time data processing by embedding computation directly within physical layers. Here, we demonstrate a voltage-controlled magneto-ionic device that functions as a reservoir computer capable of forecasting chaotic time series. The device consists of a crossbar structure with a Ta/CoFeB/Ta/MgO/Ta bottom electrode and a LiPON/Pt top electrode. A chaotic Mackey-Glass time series is encoded into a voltage signal applied to the device, while 2D Fourier transforms of voltage-dependent magnetic domain patterns form the output. Performance is influenced by the input rate, smoothing of the output, the number of elements in the reservoir state vector, and the training duration. We identify two distinct computational regimes: short-term prediction is optimized using smoothed, low-dimensional states with minimal training, whereas prediction around the Mackey-Glass delay time benefits from unsmoothed, high-dimensional states and extended training. Reservoir computing metrics reveal that slower input rates are more tolerant to output smoothing, while faster input rates degrade both memory capacity and nonlinear processing. These findings demonstrate the potential of magneto-ionic systems for neuromorphic computing and offer design principles for tuning performance in response to input signal characteristics.

physics.app-ph↗

arXiv2025

Magnetic and structural properties of epitaxial Er-substituted yttrium iron garnet films grown by pulsed laser deposition

Er-substituted yttrium iron garnet (Er:YIG) holds the potential of combining the low magnetic damping of YIG with the telecom-band optical transitions of $\text{Er}^{3+}$ ions, making it a suitable material for hybrid optomagnonic devices and microwave-to-optical quantum transduction. We report the epitaxial growth of $\text{Er}_{x}\text{Y}_{3-x}\text{Fe}_{5}\text{O}_{12}$ films with $x=0.008-0.20$ on (111)-oriented gadolinium gallium garnet (GGG) substrates using pulsed laser deposition. X-ray diffraction, reciprocal space mapping, and scanning transmission electron microscopy confirm single-phase, fully coherent growth with atomically sharp interfaces across the entire substitution range. Magnetometry reveals a gradual decrease in saturation magnetization with increasing Er content, consistent with antiparallel coupling between Er$^{3+}$ spins and the net Fe$^{3+}$ moments, along with the emergence of an in-plane uniaxial magnetic anisotropy. The ferromagnetic resonance broadens with Er concentration due to increased Gilbert damping and inhomogeneous linewidth broadening. Films with low Er content ($x=0.008$), most relevant for optomagnonic applications, retain nearly isotropic magnetization and exhibit a damping parameter only slightly higher than that of undoped YIG. These results identify growth and substitution conditions that preserve YIG's low-loss magnetic properties while introducing optical functionality, establishing Er:YIG as a viable platform for hybrid quantum magnonics and microwave-to-optical transduction.

cond-mat.mtrl-sci↗

arXiv2025

Spin-wave propagation at low temperatures in YIG thin films on YSGG substrates

The use of spin waves in magnetic thin films at cryogenic temperatures has long been hindered by the lack of a suitable material platform. Yttrium iron garnet (YIG) is the leading candidate, yet it is typically grown on gadolinium gallium garnet (GGG) substrates, which develop a large paramagnetic moment at low temperatures. This substrate effect limits spin-wave propagation. In this work, we demonstrate that thin YIG films grown on yttrium scandium gallium garnet (YSGG) substrates support robust spin-wave propagation in the Damon-Eshbach geometry, measurable down to 2 K under applied magnetic fields up to 150 mT. Compared with YIG/GGG, YIG/YSGG films exhibit narrower ferromagnetic resonance (FMR) linewidths at low temperatures and are free from the atomic interdiffusion effects that degrade the performance of YIG/GGG systems. These results establish YIG/YSGG thin films as a promising low-temperature platform, overcoming the intrinsic limitations of YIG/GGG and opening new opportunities for scalable magnonic and hybrid quantum devices operating under cryogenic conditions.

cond-mat.mes-hall↗

arXiv2024

A magneto-ionic synapse for reservoir computing

Neuromorphic computing aims to revolutionize large-scale data processing by developing efficient methods and devices inspired by neural networks. Among these, the control of magnetism through ion migration has emerged as a promising approach due to the inherent memory and nonlinearity of ionically conducting and magnetic materials. In this work, we present a lithium-ion-based magneto-ionic device that uses applied voltages to control the magnetic domain state of a perpendicularly magnetized ferromagnetic layer. This behavior emulates the analog and non-volatile properties of biological synapses and enables the creation of a simple reservoir computing system. To illustrate its capabilities, the device is used in a waveform classification task, where the voltage amplitude range and magnetic bias field are tuned to optimize the recognition accuracy.

physics.app-ph↗

arXiv2024

Magnonic Fabry-Pérot resonators as programmable phase shifters

We explore the use of magnonic Fabry-Pérot resonators as programmable phase shifters for spin-wave computing. The resonator, composed of a yttrium iron garnet (YIG) film coupled with a CoFeB nanostripe, operates through dynamic dipolar coupling, leading to wavelength downconversion and the formation of a magnonic cavity. Using super-Nyquist sampling magneto-optical Kerr effect (SNS-MOKE) microscopy and micromagnetic simulations, we demonstrate that these resonators can induce a $π$ phase shift in the transmitted spin wave. The phase shift is highly sensitive to the magnetization alignment within the resonator, allowing for on-demand control via magnetic switching. This feature, combined with low-loss transmission, positions the magnonic Fabry-Pérot resonator as a promising component for reconfigurable magnonic circuits and spin-wave computing devices.

cond-mat.mtrl-sci↗

arXiv2024

Tuning of perpendicular magnetic anisotropy in Bi-substituted yttrium iron garnet films by He$^+$ ion irradiation

We report the continuous tuning of magnetic anisotropy in perpendicularly magnetized bismuth-substituted yttrium iron garnet (Bi-YIG) films via He$^+$ ion irradiation. Our findings indicate that the magnetization direction of epitaxial Bi-YIG films on sGGG substrates transitions from out-of-plane in the as-grown state to in-plane after He+ ion irradiation at a fluence exceeding $2\times 10^{14}$ ions/cm$^2$. The reorientation is attributed to the relaxation of tensile film strain, which reduces the perpendicular magnetic anisotropy without affecting the saturation magnetization. The Gilbert damping parameter and the inhomogeneous broadening of the ferromagnetic resonance linewidth show only minimal increases with ion irradiation. Additionally, at a fluence of $5\times 10^{13}$ ions/cm$^2$, we observe the formation of magnetic bubble domains in the Bi-YIG films. Micromagnetic simulations estimate a Dzyaloshinskii-Moriya interaction of 0.006 mJ/m$^2$, which is insufficient for stabilizing Néel-type skyrmions. Finally, we demonstrate that the effects of He$^+$ ion irradiation can be largely reversed through thermal annealing in an oxygen atmosphere.

cond-mat.mtrl-sci↗

arXiv2023

Solid-state lithium-ion supercapacitor for voltage control of skyrmions

Ionic control of magnetism gives rise to high magneto-electric coupling efficiencies at low voltages, which is essential for low-power magnetism-based non-conventional computing technologies. However, for on-chip applications, magneto-ionic devices typically suffer from slow kinetics, poor cyclability, impractical liquid architectures or strong ambient effects. As a route to overcoming these problems, we demonstrate an LiPON-based solid-state ionic supercapacitor with a magnetic Pt/Co$_{40}$Fe$_{40}$B$_{20}$/Pt thin-film electrode which enables voltage control of a magnetic skyrmion state. Skyrmion nucleation and annihilation are caused by Li ion accumulation and depletion at the magnetic interface under an applied voltage. The skyrmion density can be controlled through dc applied fields or through voltage pulses. The skyrmions are nucleated by single 60-$μ$s voltage pulses and devices are cycled 750,000 times without loss of electrical performance. Our results demonstrate a simple and robust approach to ionic control of magnetism in spin-based devices.

cond-mat.mtrl-sci↗

arXiv2023

Electric field control of RKKY coupling through solid-state ionics

Placing a suitable spacer layer between two magnetic layers can lead to an interaction between the magnetic layers known as Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling. Controlling RKKY coupling, particularly the ability to switch between ferromagnetic and antiferromagnetic coupling, would enable novel magnetic data storage devices. By combining solid-state Li ion battery technology with an out-of-plane magnetized Co/Pt-based stack coupled through a Ru interlayer we investigate the effects of the insertion of Li ions on the magnetic properties of the stack. The RKKY coupling and its voltage dependence is measured as a function of the Ru interlayer thickness, along with the effects of repeated voltage cycling. The Li ions both change the amplitude of the RKKY coupling and its phase, leading to the ability to switch the RKKY coupling between ferromagnetic and antiferromagnetic with applied voltages.

cond-mat.mtrl-sci↗

arXiv2022

Wideband Brillouin light scattering analysis of spin waves excited by a white-noise RF generator

Spin waves are studied intensively for their intriguing properties and potential use in future technology platforms for the transfer and processing of information and microwave signals. The development of devices and materials for spin-wave systems requires a lot of measurement time and effort, and thus increasing the measurement throughput by extending the instrumentation capabilities is of the essence. In this letter, we report on a new and straightforward approach to increase the measurement throughput by fully exploiting the wideband detection nature of the Brillouin light scattering technique in single-shot experiments using a white-noise RF generator.

cond-mat.mes-hall↗

arXiv2022

Direct observation of a dynamical glass transition in a nanomagnetic artificial Hopfield network

Spin glasses, generally defined as disordered systems with randomized competing interactions, are a widely investigated complex system. Theoretical models describing spin glasses are broadly used in other complex systems, such as those describing brain function, error-correcting codes, or stock-market dynamics. This wide interest in spin glasses provides strong motivation to generate an artificial spin glass within the framework of artificial spin ice systems. Here, we present the experimental realization of an artificial spin glass consisting of dipolar coupled single-domain Ising-type nanomagnets arranged onto an interaction network that replicates the aspects of a Hopfield neural network. Using cryogenic x-ray photoemission electron microscopy (XPEEM), we performed temperature-dependent imaging of thermally driven moment fluctuations within these networks and observed characteristic features of a two-dimensional Ising spin glass. Specifically, the temperature dependence of the spin glass correlation function follows a power law trend predicted from theoretical models on two-dimensional spin glasses. Furthermore, we observe clear signatures of the hard to observe rugged spin glass free energy in the form of sub-aging, out of equilibrium autocorrelations and a transition from stable to unstable dynamics.

cond-mat.dis-nn↗

arXiv2021

Magnetic on-off switching of a plasmonic laser

The nanoscale mode volumes of surface plasmon polaritons have enabled plasmonic lasers and condensates with ultrafast operation. Most plasmonic lasers are based on noble metals, rendering the optical mode structure inert to external fields. Here, we demonstrate active magnetic-field control over lasing in a periodic array of Co/Pt multilayer nanodots immersed in an IR-140 dye solution. We exploit the magnetic nature of the nanoparticles combined with mode tailoring to control the lasing action. Under circularly polarized excitation, angle-resolved photoluminescence measurements reveal a transition between lasing action and non-lasing emission as the nanodot magnetization is reversed. Our results introduce magnetization as a means of externally controlling plasmonic nanolasers, complementary to the modulation by excitation, gain medium, or substrate. Further, the results show how effects of magnetization on light that are inherently weak can be observed in the lasing regime, inspiring studies of topological photonics.

physics.optics↗

arXiv2021

Thermal motion of skyrmion arrays in granular films

Magnetic skyrmions are topologically-distinct swirls of magnetic moments which display particle-like behaviour, including the ability to undergo thermally-driven diffusion. In this paper we study the thermally activated motion of arrays of skyrmions using temperature dependent micromagnetic simulations where the skyrmions form spontaneously. In particular, we study the interaction of skyrmions with grain boundaries, which are a typical feature of sputtered ultrathin films used in experimental devices. We find the interactions lead to two distinct regimes. For longer lag times the grains lead to a reduction in the diffusion coefficient, which is strongest for grain sizes similar to the skyrmion diameter. At shorter lag times the presence of grains enhances the effective diffusion coefficient due to the gyrotropic motion of the skyrmions induced by their interactions with grain boundaries. For grain sizes significantly larger than the skyrmion diameter clustering of the skyrmions occurs in grains with lower magnetic anisotropy.

cond-mat.mes-hall↗