SearcharxivSearch

arXiv subjects

Sebastian Dehe

Publications and source records attributed to Sebastian Dehe.

4 recordsLinked to original sources

Solutocapillary bubble centering in a confined ethanol plume in water

This study investigates the radial centering of gas bubbles within a buoyant plume of ethanol injected into a co-flowing water sheath flow in a vertical capillary. Bubbles nucleate in the ethanol stream due to CO$_2$ supersaturation and rapidly migrate toward the plume axis via solutocapillary (Marangoni) forces driven by interfacial tension gradients in the ethanol-water mixture. Experiments reveal that bubbles of varying sizes reliably align along the plume centerline, facilitated by steep radial concentration gradients near the plume boundary. A reduced-order model supports robust centering across a wide range of bubble radii. For larger bubbles, axial Marangoni effects modulate ascent velocities and can even induce upstream migration under transient conditions, highlighting the complex feedback between bubble dynamics and plume distortion. The results demonstrate that solutocapillary migration provides a reliable mechanism for contact-free bubble focusing, with implications for bubble manipulation in microfluidics, reactors, and phase-separation processes.

physics.flu-dyn

Upstream motion of oil droplets in co-axial Ouzo flow due to Marangoni forces

To explore the physicochemical hydrodynamics of phase-separating ternary liquids (Ouzo-type), a binary oil-ethanol mixture is introduced into a co-flowing stream of water. Oil droplets nucleate at the interface between the two liquids, leading to a larger oil droplet interacting with the ethanol-rich jet. Although buoyancy forces and hydrodynamic drag forces push the droplet in downstream direction, we observe an upstream motion. Using computational fluid dynamics simulations of a simplified model system, we identify the nucleation zone for oil droplets and uncover Marangoni forces to be responsible for the upstream motion of the droplet. A semi-analytical model allows us to identify the key parameters governing this effect. A general conclusion is that Marangoni stresses can reverse the motion of droplets through channels, where the surrounding liquid is a multi-component mixture. The insights from this work are not only relevant for channel flow, but more generally, for the physicochemical hydrodynamics of multiphase, multi-component systems.

physics.flu-dyn

Controlling the electrostatic Faraday instability using superposed electric fields

When the interface between a dielectric and a conducting liquid is excited by an oscillatory electric field, electrostatic Faraday waves can be induced. Here, we study the response of the interface to an AC electric field, which is superposed by either a second AC field of different frequency, or by a DC field. An algorithm based on light refraction at the fluidic interface is used to obtain the spatio-temporal response of the Faraday waves, and the critical voltage corresponding to onset of instability, the interfacial oscillation frequency and the dominant wavelengths are determined. The influence of the mixing ratio, which denotes the relative amplitudes of the different components of the driving signal, is analyzed, and the experimental results are compared with theoretical predictions. For AC/AC driving, gradual variations of the mixing ratio can induce a jump of the pattern wavelength, which is a result of the transition from harmonic to a subharmonic oscillation. For AC/DC driving, the interface oscillates either harmonically or subharmonically, and the response wavelength can be tuned continuously by adjusting the admixture of the DC component. For both driving modes, the experiments show good agreement with theory.

physics.flu-dyn

Deformation modes of an oil-water interface under a local electric field: From Taylor cones to surface dimples

Fluidic interfaces disintegrate under sufficiently strong electric fields, leading to electrohydrodynamic (EHD) tip streaming. Taylor cones, which emit charged droplets from the tip of a conical cusp, are among the most prominent and well-studied examples of EHD instabilities. In liquid-liquid systems, more complex interface deformation modes than simple Taylor cones can be observed, with the interface being pushed away from the electrode, and additional cone structures emerging from the rim of the dimple. In this article, we investigate the mechanisms behind these deformation modes experimentally and numerically, and demonstrate that the presence of droplets triggers the dimple at the interface. In order to characterize the underlying processes, we replace the pin electrode by a hollow metallic needle with a prescribed electrolyte volume flow. The submerged electrospray introduces droplets of an aqueous KCl solution with varying ion concentrations into silicone oils with varying viscosities. By measuring the corresponding electric current and by optical investigation of the interface deformation, we study the system response to variations of the ionic concentration, viscosity, applied voltage as well as flow rate. In addition to the experiments, we use a finite element solver and compute the charge transport due to the droplets in the oil phase. Further, we compute the electric potential distribution, flow field and interface deformation. After calibration of our model with particle tracking velocimetry data of the flow inside the oil phase, we reproduce the experimentally observed dimple at the liquid-liquid interface. In summary, this work highlights the importance of charged droplets for the complex dynamic modes observed when a liquid-liquid interface is exposed to a local electric field.

physics.flu-dyn