arXiv subjects

Sebastian Hofferberth

Publications and source records attributed to Sebastian Hofferberth.

At least 19 recordsLinked to original sources

arXiv2026

Direct laser-written optomechanical double membranes in an optical microcavity

Optomechanical membrane-in-the-middle systems that comprise several coupled compliant membranes offer enhanced optomechanical coupling and collective dynamics. Recent realizations were fundamentally restricted to two membranes and to limited structural optimization of the involved membranes due to their intricate fabrication and experimental integration. Here, we present a fiber-based Fabry-Perot microcavity incorporating monolithically integrated double-membrane resonators fabricated by 3D direct laser writing. We realize controllable mechanical mode hybridization of membranes with coupling rates of up to $J_{\mathrm{mech}}/2\pi = 0.16$ MHz, exceeding the mechanical linewidths. We demonstrate enhanced collective optomechanical coupling of the membrane stack's breathing mode, reaching collective coupling strengths of up to $g_{\mathrm{col}}^{(-)}/2\pi \approx 0.1$ MHz. Our transfer-matrix calculations predict further substantial enhancements with realistic reductions of membrane thickness and spacing, and a larger number of membranes. Our results establish direct laser-written membrane arrays as a scalable platform for multimode cavity optomechanics, combining tunable mechanical interactions, enhanced collective optomechanical coupling, and scalability towards larger mechanically coupled resonator systems.

physics.optics↗

arXiv2026

Spatial correlations of photons interacting via transverse Rydberg blockade

We develop a theory of the transverse spatial dynamics of two interacting photons in a Rydberg nonlinear medium. Extending the well-studied one-dimensional case, we explore both longitudinal and transverse correlations of photons propagating as Rydberg polaritons. We identify distinct behaviors and scaling laws for these correlations, arising from fundamentally different mechanisms in the two directions: diffraction for transverse correlations and diffusion for longitudinal correlations. We develop a model incorporating a Gaussian optical beam and an inhomogeneous atomic density distribution, from which we derive quantitative predictions for correlation functions in both directions. We further show that the propagation equations can be reduced to a single Schr\"odinger-like equation, allowing approximate solutions that are supported by full numerical results. Our findings indicate that the transverse correlation length is determined primarily by the blockade radius, whereas the longitudinal correlation length is limited by bandwidth. These results establish transverse Rydberg blockade as a distinct and measurable correlation mechanism and show that spatial photon correlations provide a direct means of measuring the blockade radius.

quant-ph↗

arXiv2026

Accurate Modeling of Rydberg Atoms and Their Interactions: Theory and Implementation in PairInteraction

Rydberg atoms provide a powerful platform for exploring strongly interacting quantum systems, both in free space and in structured electromagnetic environments, with growing applications in quantum technology. Accurately modeling their single-atom properties and mutual interactions is essential for interpreting experiments and designing new architectures. We present a unified theoretical framework for Rydberg atoms and their interactions based on multi-channel quantum defect theory (MQDT) and static electromagnetic Green's tensors. MQDT provides a precise description of Rydberg states of divalent atoms such as strontium and ytterbium, while the Green's tensor formalism provides a general and flexible approach for calculating interactions between two Rydberg atoms in arbitrary geometries, including modifications induced by nearby surfaces. We implement this framework in an updated version of the open-source PairInteraction software [Weber et al., J.~Phys.~B~50 (2017)]. The implementation leverages high-performance libraries and achieves speedups of one order of magnitude for pair-potential calculations compared to prior software. We demonstrate the capabilities of the framework through example applications to divalent atoms and show excellent agreement with experimental data for an exemplary Stark map of $^{174}$Yb. The modular software architecture enables the community to extend it further.

physics.atom-ph↗

arXiv2025

Revealing electron-ytterbium interactions through Rydberg molecular spectroscopy

Divalent atoms have emerged as powerful alternatives to alkalis in ultracold atom platforms, offering unique advantages arising from their two-electron structure. Among these species, ytterbium (Yb) is especially promising, yet its anionic properties and its Rydberg spectrum remain comparatively unexplored. In this work, we perform a first and comprehensive experimental and theoretical investigation of ultralong-range Rydberg molecules (ULRMs) of $^{174}$Yb in $6sns\,^1S_0$ Rydberg states across nearly two decades in principal quantum number $n$ and three orders of magnitude in molecular binding energy. Using the Coulomb Green's function formalism, we compute Born-Oppenheimer molecular potentials describing the Rydberg atom in the presence of a ground-state perturber and achieve quantitative agreement with high-resolution molecular spectra. This enables the extraction of low-energy electron-Yb scattering phase shifts, including the zero-energy $s$-wave scattering length and the positions of two spin-orbit split $p$-wave shape resonances. Our results provide strong evidence that the Yb$^{-}$ anion exists only as a metastable resonance.% We additionally show the sensitivity of ULRM spectra to the atomic quantum defects, using this to determine the quantum defect of the $6s23f\, ^1F_3$ state. Together, these findings establish Yb ULRMs as a powerful probe of electron-Yb interactions and lay essential groundwork for future Rydberg experiments with divalent atoms.

physics.atom-ph↗

arXiv2025

Entanglement of mechanical oscillators mediated by a Rydberg tweezer chain

Mechanical systems provide a unique test bed for studying quantum phenomena at macroscopic length scales. However, realizing quantum states that feature quantum correlations among macroscopic mechanical objects remains an experimental challenge. Here, we propose a quantum system in which two micro-electromechanical oscillators interact through a chain of Rydberg atoms confined in optical tweezers. We demonstrate that the coherent dynamics of the system generate entanglement between the oscillators. Furthermore, we utilize the tunability of the radiative decay of the Rydberg atoms for dissipative entanglement generation. Our results highlight the potential to exploit the flexibility and tunability of Rydberg atom chains to generate nonclassical correlations between distant mechanical oscillators.

quant-ph↗

arXiv2024

Magic running- and standing-wave optical traps for Rydberg atoms

Magic trapping of ground and Rydberg states, which equalizes the AC Stark shifts of these two levels, enables increased ground-to-Rydberg state coherence times. We measure via photon storage and retrieval how the ground-to-Rydberg state coherence depends on trap wavelength for two different traps and find different optimal wavelengths for a one-dimensional optical lattice trap and a running wave optical dipole trap. Comparison to theory reveals that this is caused by the Rydberg electron sampling different potential landscapes. The observed difference increases for higher principal quantum numbers, where the extent of the Rydberg electron wave function becomes larger than the optical lattice period. Our analysis shows that optimal magic trapping conditions depend on the trap geometry, in particular for optical lattices and tweezers.

physics.atom-ph↗

arXiv2024

Two-color Ytterbium MOT in a compact dual-chamber setup

We present an experimental scheme for producing ultracold Ytterbium atoms in a compact dual-chamber setup. A dispenser-loaded two-dimensional (2D) magneto-optical trap (MOT) using permanent magnets and operating on the broad $^1S_0\to {}^1P_1$ singlet transition delivers over $10^7$ atoms per second through a differential pumping stage into a three-dimensional (3D) MOT. The two-color 3D MOT uses the broad singlet transition to accumulate $\sim\!2\times 10^7$ atoms of $^{174}\text{Yb}$ within $2.5~\text{s}$ and subsequently the narrow $^1S_0\to {}^3P_1$ intercombination line to cool the atomic cloud to below $10~\mathrm{\mu K}$. We report optimized parameters for each stage of the atom collection sequence, achieving high transfer efficiency. We find that shelving into the triplet state during the broad-transition MOT almost doubles the number of trapped atoms.

physics.atom-ph↗

arXiv2024

Engineering Rydberg-pair interactions in divalent atoms with hyperfine-split ionization thresholds

Quantum information processing with neutral atoms relies on Rydberg excitation for entanglement generation. While the use of heavy divalent or open-shell elements, such as strontium or ytterbium, has benefits due to their optically active core and a variety of possible qubit encodings, their Rydberg structure is generally complex. For some isotopes in particular, hyperfine interactions are relevant even for highly excited electronic states. We employ multi-channel quantum defect theory to infer the Rydberg structure of isotopes with non-zero nuclear spin and perform non-perturbative Rydberg-pair interaction calculations. We find that due to the high level density and sensitivities to external fields, experimental parameters must be precisely controlled. Specifically in ${}^{87}$Sr, we study an intrinsic F\"orster resonance, unique to divalent atoms with hyperfine-split thresholds, which simultaneously provides line stability with respect to external field fluctuations and enhanced long-range interactions. Additionally, we provide parameters for pair states that can be effectively described by single-channel Rydberg series. The explored pair states provide exciting opportunities for applications in the blockade regime as well as for more exotic long-range interactions such as largely flat, distance-independent potentials.

physics.atom-ph↗

arXiv2024

Nonreciprocal recovery of electromagnetically induced transparency by wavenumber mismatch in hot atoms

For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atom velocity and the wavenubmer mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and $k_{p} < k_{c}$, with $k_{p}$ and $k_{c}$ being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, opening promising avenues for example for realization of magnetic-field free optical isolators. In this tutorial we discuss the theoretical derivation of this effect and show the underlying mechanism to be an avoided crossing of the states dressed by the coupling laser as a function of atomic velocities when $k_{p}<k_{c}$. We investigate how the non-reciprocity scales with wavelength mismatch and show how to experimentally demonstrate the effect in a simple Rydberg-EIT system using thermal Rubidium atoms.

quant-ph↗

arXiv2023

Quantum Optics with Rydberg Superatoms

Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.

quant-ph↗

arXiv2023

Photothermal gas detection using a miniaturized fiber Fabry-Perot cavity

We demonstrate a robust and miniaturized fiber Fabry-Perot cavity-based sensor for photothermal spectroscopic signal retrieval. The proof-of-concept experiment involved the use of a near-infrared pump laser to detect methane molecules on an isolated overtone 2.3 R(4) transition located at 6057.1 cm-1. The photothermal-related modulation of the gas refractive index was induced at the center of the interferometer, which was filled with the sample. Subsequently, the phase change of the resonating probe beam was measured as a shift in the reflected beam intensity, which was proportional to the methane concentration. A normalized noise equivalent absorption coefficient of 7.06 x 10-8 cm-1 W Hz-1/2 was achieved, suggesting significant potential for the design of small and versatile gas detectors with excellent detectivity. We discuss future improvements of the proposed photothermal gas detection approach.

physics.optics↗

arXiv2022

Direct laser-written optomechanical membranes in fiber Fabry-Perot cavities

Integrated micro and nanophotonic optomechanical experiments enable the manipulation of mechanical resonators on the single phonon level. Interfacing these structures requires elaborate techniques limited in tunability, flexibility, and scaling towards multi-mode systems. Here, we demonstrate a cavity optomechanical experiment using 3D-laser-written polymer membranes inside fiber Fabry-Perot cavities. Vacuum coupling strengths of ~ 30 kHz to the fundamental megahertz mechanical mode are reached. We observe optomechanical spring tuning of the mechanical resonator by tens of kHz exceeding its linewidth at cryogenic temperatures. The extreme flexibility of the laser writing process allows for a direct integration of the membrane into the microscopic cavity. The direct fiber coupling, its scaling capabilities to coupled resonator systems, and the potential implementation of dissipation dilution structures and integration of electrodes make it a promising platform for fiber-tip integrated accelerometers, optomechanically tunable multi-mode mechanical systems, or directly fiber-coupled systems for microwave to optics conversion.

physics.optics↗

arXiv2022

Interplay between optomechanics and the dynamical Casimir effect

We develop a model of a quantum field confined within a cavity with a movable wall where the position of the wall is quantized. We obtain a full description of the dynamics of both the quantum field and the confining wall depending on the initial state of the whole system. Both the reaction and back-reaction of the field on the wall, and the wall on the field, can be taken into account, as well as external driving forces on both the cavity and the wall. The model exactly reproduces the resonant cavity mode stimulation due to the periodic motion of the mirror (dynamical Casimir effect), as well as the standard radiation pressure effects on the quantized wall(optomechanics). The model also accounts for the interplay of the two scenarios. Finally, the time evolution of the radiation force shows the interplay between the static and dynamical Casimir effect.

quant-ph↗

arXiv2022

Creation of non-classical states of light in a chiral waveguide

Creating non-classical states of light from simple quantum systems together with classical resources is a challenging problem. We show how chiral emitters under a coherent drive can generate non-classical photon states. For our analysis, we select a specific temporal mode in the transmitted light field, resulting in a coupled master equation for the relevant mode and the chiral emitters. We characterise the mode's state by its Wigner function and show that the emission from the system predominantly produces mixtures of few-photon-added coherent states. We argue that these non-classical states are experimentally accessible and show their application for quantum metrology.

quant-ph↗

arXiv2022

Non-exponential decay of a collective excitation in an atomic ensemble coupled to a one-dimensional waveguide

We study the dynamics of a single excitation coherently shared amongst an ensemble of atoms and coupled to a one-dimensional wave guide. The coupling between the matter and the light field gives rise to collective phenomena such as superradiant states with an enhanced initial decay rate, but also to the coherent exchange of the excitation between the atoms. We find that the competition between the two phenomena provides a characteristic dynamics for the decay of the excitations, and remarkably exhibits an algebraic behavior, instead of the expected standard exponential one, for a large number of atoms. The analysis is first performed for a chiral waveguide, where the problem can be solved analytically, and then is extended to the bidirectional waveguide.

quant-ph↗

arXiv2022

Achievements and Perspectives of Optical Fiber Fabry-Perot Cavities

Fabry-Perot interferometers have stimulated numerous scientific and technical applications ranging from high resolution spectroscopy over metrology, optical filters to interfaces of light and matter at the quantum limit and more. End facet machining of optical fibers has enabled the miniaturization of optical Fabry-Perot cavities. Integration with fiber wave guide technology allows for small yet open devices with favorable scaling properties including mechanical stability and compact mode geometry. These Fiber Fabry-Perot Cavities (FFPCs) are stimulating extended applications in many fields including cavity quantum electrodynamics, optomechanics, sensing, nonlinear optics and more. Here we summarize the state of the art of devices based on Fiber Fabry-Perot Cavities, provide an overview of applications and conclude with expected further research activities.

physics.optics↗

arXiv2021

Polaritons in two-dimensional parabolic waveguides

The suite of highly confined polaritons supported by two-dimensional (2D) materials constitutes a versatile platform for nano-optics, offering the means to channel light on deep-subwavelength scales. Graphene, in particular, has attracted considerable interest due to its ability to support long-lived plasmons that can be actively tuned via electrical gating. While the excellent optoelectronic properties of graphene are widely exploited in plasmonics, its mechanical flexibility remains relatively underexplored in the same context. Here, we present a semi-analytical formalism to describe plasmons and other polaritons supported in waveguides formed by bending a 2D material into a parabolic shape. Specifically, for graphene parabolas, our theory reveals that the already large field confinement associated with graphene plasmons can be substantially increased by bending an otherwise flat graphene sheet into a parabola shape, thereby forming a plasmonic waveguide without introducing potentially lossy edge terminations via patterning. Further, we show that the high field confinement associated with such channel polaritons in 2D parabolic waveguides can enhance the spontaneous emission rate of a quantum emitter near the parabola vertex. Our findings apply generally to 2D polaritons in atomically thin materials deposited onto grooves or wedges prepared on a substrate or freely suspended in a quasi-parabolic (catenary) shape. We envision that both the optoelectronic and mechanical flexibility of 2D materials can be harnessed in tandem to produce 2D channel polaritons with versatile properties that can be applied to a wide range of nano-optics functionalities, including subwavelength polaritonic circuitry and bright single-photon sources.

cond-mat.mes-hall↗

arXiv2021

Controlled multi-photon subtraction with cascaded Rydberg superatoms as single-photon absorbers

The preparation of light pulses with well-defined quantum properties requires precise control at the individual photon level. Here, we demonstrate exact and controlled multi-photon subtraction from incoming light pulses. We employ a cascaded system of tightly confined cold atom ensembles with strong, collectively enhanced coupling of photons to Rydberg states. The excitation blockade resulting from interactions between Rydberg atoms limits photon absorption to one per ensemble and engineered dephasing of the collective excitation suppresses stimulated re-emission of the photon. We experimentally demonstrate subtraction with up to three absorbers. Furthermore, we present a thorough theoretical analysis of our scheme where we identify weak Raman decay of the long-lived Rydberg state as the main source of infidelity in the subtracted photon number. We show that our scheme should scale well to higher absorber numbers if the Raman decay can be further suppressed.

quant-ph↗