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Sebastian Slama

Publications and source records attributed to Sebastian Slama.

At least 19 recordsLinked to original sources

Photonic bands and normal mode splitting in optical lattices interacting with cavities

Strong collective interaction of atoms with an optical cavity causes normal mode splitting of the cavity's resonances, whose width is given by the collective coupling strength. At low optical density of the atomic cloud the intensity distribution of light in the cavity is ruled by the cavity's mode function, which is solely determined by its geometry. In this regime the dynamics of the coupled atom-cavity system is conveniently described by the open Dicke model, which we apply to calculating normal mode splitting generated by periodically ordered clouds in linear and ring cavities. We also show how to use normal mode splitting as witness for Wannier-Bloch oscillations in the tight-binding limit. At high optical density the atomic distribution contributes to shaping the mode function. This regime escapes the open Dicke model, but can be treated by a transfer matrix model provided the saturation parameter is low. Applying this latter model to an atomic cloud periodically ordered into a one-dimensional lattice, we observe the formation of photonic bands gaps competing with the normal mode splitting. We discuss the limitations of both models and point out possible pathways to generalized theories.

quant-ph

Spin self-organization in an optical cavity facilitated by inhomogeneous broadening

We study the onset of collective spin-self-organization in a thermal ensemble of driven two-level atoms confined in an optical cavity. The atoms spontaneously form a spin-pattern above a critical driving strength that sets a threshold and is determined by the cavity parameters, the initial temperature, and the transition frequency of the atomic spin. Remarkably, we find that inhomogeneous Doppler broadening facilitates the onset of spin-self-organization. In particular, the threshold is non-monotonic when increasing the spin transition frequency and reaches a minimum when the Doppler broadening is of similar magnitude. This feature emerges due to Doppler-induced resonances. Above the threshold, we find cooperative dynamics of spin, spatial, and momentum degrees of freedom leading to density modulations, fast reduction of kinetic energy, and the emergence of non-thermal states. More broadly, our work demonstrates how broadening can facilitate strong light-matter interactions in many-body systems.

cond-mat.quant-gas

Symmetry breaking and non-ergodicity in a driven-dissipative ensemble of multi-level atoms in a cavity

Dissipative light-matter systems can display emergent collective behavior. Here, we report a $\mathbb{Z}_2$-symmetry-breaking phase transition in a system of multi-level $^{87}$Rb atoms strongly coupled to a weakly driven two-mode optical cavity. In the symmetry-broken phase, non-ergodic dynamics manifests in the emergence of multiple stationary states with disjoint basins of attraction. This feature enables the amplification of a small atomic population imbalance into a characteristic macroscopic cavity transmission signal. Our experiment does not only showcase strongly dissipative atom-cavity systems as platforms for probing non-trivial collective many-body phenomena, but also highlights their potential for hosting technological applications in the context of sensing, density classification, and pattern retrieval dynamics within associative memories.

quant-ph

Quantum resonant optical bistability with a narrow atomic transition: bistability phase diagram in the bad cavity regime

We report on the observation of a novel manifestation of saturation-induced optical bistability in a resonantly pumped optical ring cavity interacting strongly with a cloud of atoms via a narrow atomic transition. The bistability emerges, above a critical pump rate, as an additional peak in the cavity's normal mode spectrum close to atomic resonance. This third transmission peak is usually suppressed due to strong resonant absorption, but in our experiment it is visible because of the linewidth of the atomic transition being much smaller than that of the cavity, which sets the experiment into the bad-cavity regime. Relying on complete saturation of the transition, this bistability has a quantum origin and cannot be mimicked by a classical material presenting a nonlinear refraction index. The appearance of the central peak in addition to the normal modes is predicted by a semi-classical model derived from the Tavis-Cummings Hamiltonian from which we derive a bistability phase diagram that connects our observations with former work on optical bistability in the good cavity regime. The phase diagram reveals several so far unexplored bistable phases.

quant-ph

Collective atom-cavity coupling and non-linear dynamics with atoms with multilevel ground states

We investigate experimentally and theoretically the collective coupling between atoms with multilevel ground state manifolds and an optical cavity mode. In our setup the cavity field optically pumps populations among the ground states. The ensuing dynamics can be conveniently described by means of an effective dynamical atom-cavity coupling strength that depends on the occupation of the individual states and their coupling strengths with the cavity mode. This leads to a dynamical backaction of the atomic populations on the atom-cavity coupling strength which results in a non-exponential relaxation dynamics. We experimentally observe this effect with laser-cooled $^{87}$Rb atoms, for which we monitor the collective normal-mode splitting in real time. Our results show that the multilevel structure of electronic ground states can significantly alter the relaxation behavior in atom-cavity settings as compared to ensembles of two-level atoms.

quant-ph

Real-time detection of Rydberg state dynamics of cold atoms using an optical cavity

This work reports on the real-time detection of internal-state dynamics of cold Rb$^{87}$ atoms being excited to the $30D_{5/2}$ Rydberg state via two-photon excitation. A mesoscopic cloud of atoms is overlapped with the mode volume of a confocal optical cavity and optically pumped by two laser beams transverse to the cavity axis. The excitation to Rydberg states changes the collective atom-cavity coupling, which is detected by monitoring the light transmitted through the cavity while being weakly driven. In addition to the damped coherent excitation dynamics and the decay back to the ground state, the data show a superradiant enhancement of the black-body radiation induced transitions from the $30D_{5/2}$ state to neighboring Rydberg states. Furthermore, they show a density dependent mitigation of the superradiant decay which is attributed to long range dipole-dipole interactions between atoms in the involved Rydberg states. These results contribute to solving a recent controversy on the interplay between BBR-induced superradiance and Rydberg atom interactions.

physics.atom-ph

Nanofiber-induced losses inside an optical cavity

Optical high-finesse cavities are a well-known mean to enhance light-matter interactions. Despite large progress in the realization of strongly coupled light-matter systems, the controlled positioning of single solid emitters in cavity modes remains a challenge. We pursue the idea to use nanofibers with sub-wavelength diameter as a substrate for such emitters. This paper addresses the question how strongly optical nanofibers influence the cavity modes. We analyze the influence of the fiber position for various fiber diameters on the finesse of the cavity and on the shape of the modes.

physics.optics

Surface-plasmon based dispersive detection and spectroscopy of ultracold atoms

The paper reports on the optical detection and spectroscopy of ultracold atoms near a gold surface. A probe light field is used to excite surface plasmon polaritons. The refractive index of the atomic gas shifts the plasmon resonance and changes the reflected light power. Thus, the sensitivity of the detection is plasmonically enhanced. Absorption of photons from the evanescent wave is avoided by detuning the laser from atomic resonance which makes the detection scheme potentially nondestructive. The spectrum of the signal is determined by a Fano resonance. We show that atoms can be detected nondestructively with single atom resolution for typical parameters in cold atom experiments. Thus, the method is suitable for quantum nondemolition measurements of matter wave amplitudes. Experimentally, we measure a technically-limited sensitivity of 30 atoms and extend the detection scheme to dispersively image the atom cloud near the surface.

quant-ph

Controlling photon bunching and antibunching of two quantum emitters near a core-shell sphere

The collective spontaneous emission of two point-dipole emitters near a plasmonic core-shell nanosphere is theoretically investigated. Based on the expansion of mode functions in vector spherical harmonics, we derive closed analytical expressions for both the cooperative decay rate and the dipole-dipole interaction strength associated with two point dipoles close to a sphere. Considering a plasmonic nanoshell containing a linearly amplifying medium inside the core, the second-order correlation function for the two emitters shows that it is possible to tune the photon emission, selecting either photon bunching or antibunching as a function of the polarization and position of the sphere. This result opens vistas to applications involving tunable single-photon sources in engineered artificial media.

physics.optics

Photon-antibunching in the fluorescence of statistical ensembles of emitters at an optical nanofiber-tip

This proposal investigates the photon-statistics of light emitted by a statistical ensemble of cold atoms excited by the near-field of an optical nanofiber tip. Dipole-dipole interactions of atoms at such short distance from each other suppress the simultaneous emission of more than one photon and lead to antibunching of photons. We consider a mean atom number on the order of one and deal with a poissonian mixture of one and two atoms including dipole-dipole interactions and collective decay. Time tracks of the atomic states are simulated in quantum Monte Carlo simulations from which the $g^{(2)}$-photon autocorrelation function is derived. The general results can be applied to any statistical ensemble of emitters that are interacting by dipole-dipole interactions.

quant-ph

Fano resonances in plasmonic core-shell particles and the Purcell effect

Despite a long history, light scattering by particles with size comparable with the light wavelength still unveils surprising optical phenomena, and many of them are related to the Fano effect. Originally described in the context of atomic physics, the Fano resonance in light scattering arises from the interference between a narrow subradiant mode and a spectrally broad radiation line. Here, we present an overview of Fano resonances in coated spherical scatterers within the framework of the Lorenz-Mie theory. We briefly introduce the concept of conventional and unconventional Fano resonances in light scattering. These resonances are associated with the interference between electromagnetic modes excited in the particle with different or the same multipole moment, respectively. In addition, we investigate the modification of the spontaneous-emission rate of an optical emitter at the presence of a plasmonic nanoshell. This modification of decay rate due to electromagnetic environment is referred to as the Purcell effect. We analytically show that the Purcell factor related to a dipole emitter oriented orthogonal or tangential to the spherical surface can exhibit Fano or Lorentzian line shapes in the near field, respectively.

physics.optics

Plasmonic surface traps with arbitrary shape for cold atoms

This paper reports on conceptual and experimental work towards the realization of plasmonic surface traps for cold atoms. The trapping mechanism is based on the combination of a repulsive and an attractive potential generated by evanescent light waves that are plasmonically enhanced. The strength of enhancement can be locally manipulated via the thickness of a metal nanolayer deposited on top of a dielectric substrate. Thus, in principle arbitrary potential landscapes can be generated. We present simulations of a plasmonic lattice potential using a gold grating with sinusoidally modulated thickness. Experimentally, a first plasmonic test structure is presented and characterized. Furthermore, the surface potential landscape is detected by reflecting ultracold atom clouds from the test structure revealing the influence of both evanescent waves. A parameter range is identified, where stable traps can be expected.

physics.atom-ph

Fano resonances and fluorescence enhancement of a dipole emitter near a plasmonic nanoshell

We analytically study the spontaneous emission of a single optical dipole emitter in the vicinity of a plasmonic nanoshell, based on the Lorenz-Mie theory. We show that the fluorescence enhancement due to the coupling between optical emitter and sphere can be tuned by the aspect ratio of the core-shell nanosphere and by the distance between the quantum emitter and its surface. In particular, we demonstrate that both the enhancement and quenching of the fluorescence intensity are associated with plasmonic Fano resonances induced by near- and far-field interactions. These Fano resonances have asymmetry parameters whose signs depend on the orientation of the dipole with respect to the spherical nanoshell. We also show that if the atomic dipole is oriented tangentially to the nanoshell, the interaction exhibits saddle points in the near-field energy flow. This results in a Lorentzian fluorescence enhancement response in the near field and a Fano line-shape in the far field. The signatures of this interaction may have interesting applications for sensing the presence and the orientation of optical emitters in close proximity to plasmonic nanoshells.

physics.optics

Optomechanical damping of a nanomembrane inside an optical ring cavity

We experimentally and theoretically investigate mechanical nanooscillators coupled to the light in an optical ring resonator made of dielectric mirrors. We identify an optomechanical damping mechanism that is fundamentally different to the well known cooling in standing wave cavities. While, in a standing wave cavity the mechanical oscillation shifts the resonance frequency of the cavity in a ring resonator the frequency does not change. Instead the position of the nodes is shifted with the mechanical excursion. We derive the damping rates and test the results experimentally with a silicon-nitride nanomembrane. It turns out that scattering from small imperfections of the dielectric mirror coatings has to be taken into account to explain the value of the measured damping rate. We extend our theoretical model and regard a second reflector in the cavity that captures the effects of mirror back scattering. This model can be used to also describe the situation of two membranes that both interact with the cavity fields. This may be interesting for future work on synchronization of distant oscillators that are coupled by intracavity light fields.

physics.optics

Cooperative coupling of ultracold atoms and surface plasmons

Cooperative coupling between optical emitters and light fields is one of the outstanding goals in quantum technology. It is both fundamentally interesting for the extraordinary radiation properties of the participating emitters and has many potential applications in photonics. While this goal has been achieved using high-finesse optical cavities, cavity-free approaches that are broadband and easy to build have attracted much attention recently. Here we demonstrate cooperative coupling of ultracold atoms with surface plasmons propagating on a plane gold surface. While the atoms are moving towards the surface they are excited by an external laser pulse. Excited surface plasmons are detected via leakage radiation into the substrate of the gold layer. A maximum Purcell factor of $\eta_\mathrm{P}=4.9$ is reached at an optimum distance of $z=250~\mathrm{nm}$ from the surface. The coupling leads to the observation of a Fano-like resonance in the spectrum.

physics.atom-ph

Probing atom-surface interactions by diffraction of Bose-Einstein condensates

In this article we analyze the Casimir-Polder interaction of atoms with a solid grating and an additional repulsive interaction between the atoms and the grating in the presence of an external laser source. The combined potential landscape above the solid body is probed locally by diffraction of Bose-Einstein condensates. Measured diffraction efficiencies reveal information about the shape of the Casimir-Polder interaction and allow us to discern between models based on a pairwise-summation (Hamaker) approach and Lifshitz theory.

physics.atom-ph

The role of Mie scattering in the seeding of matter-wave superradiance

Matter-wave superradiance is based on the interplay between ultracold atoms coherently organized in momentum space and a backscattered wave. Here, we show that this mechanism may be triggered by Mie scattering from the atomic cloud. We show how the laser light populates the modes of the cloud, and thus imprints a phase gradient on the excited atomic dipoles. The interference with the atoms in the ground state results in a grating, that in turn generates coherent emission, contributing to the backward light wave onset. The atomic recoil 'halos' created by the scattered light exhibit a strong anisotropy, in contrast to single-atom scattering.

physics.atom-ph

Direct Measurement of intermediate-range Casimir-Polder potentials

We present the first direct measurements of Casimir-Polder forces between solid surfaces and atomic gases in the transition regime between the electrostatic short-distance and the retarded long-distance limit. The experimental method is based on ultracold ground-state Rb atoms that are reflected from evanescent wave barriers at the surface of a dielectric glass prism. Our novel approach does not require assumptions about the potential shape. The experimental data confirm the theoretical prediction in the transition regime.

physics.atom-ph