arXiv subjects

Sebastian Wüster

Publications and source records attributed to Sebastian Wüster.

30 records · Page 2Linked to original sources

arXiv2020

Generation and decoherence of soliton spatial superposition states

Due to their coherence properties, dilute atomic gas Bose-Einstein condensates seem a versatile platform for controlled creation of mesoscopically entangled states with a large number of particles and also allow controlled studies of their decoherence. However, the creation of such a state intrinsically involves many-body quantum dynamics that cannot be captured by mean-field theory, and thus invalidates the most widespread methods for the description of condensates. We follow up on a proposal, in which a condensate cloud as a whole is brought into a superposition of two different spatial locations, by mapping entanglement from a strongly interacting Rydberg atomic system onto the condensate using off-resonant laser dressing [R. Mukherjee et al., Phys. Rev. Lett. 115 040401 (2015)]. A variational many-body Ansatz akin to recently developed multi-configurational methods allows us to model this entanglement mapping step explicitly, while still preserving the simplicity of mean-field physics for the description of each branch of the superposition. In the second part of the article, we model the decoherence process due to atom losses in detail. Altogether we confirm earlier estimates, that tightly localized clouds of 400 atoms can be brought into a quantum superposition of two locations about 3 μm apart and remain coherent for about 1 ms.

cond-mat.quant-gas↗

arXiv2020

Dynamical tunnelling of a Nano-mechanical Oscillator

The study of the quantum to classical transition is of fundamental as well as technological importance, and focusses on mesoscopic devices, with a size for which either classical physics or quantum physics can be brought to dominate. A particularly diverse selection of such devices is available in cavity quantum-optomechanics. We show that these can be leveraged for the study of dynamical-tunnelling in a quantum chaotic system. This effect probes the quantum to classical transition deeply, since tunnelling rates sensitively depend on the ability of the quantum system to resolve the underlying classical phase space. We show that the effective Planck's constant, which determines this phase space resolution, can be varied over orders of magnitude as a function of tunable parameters in an opto-mechanical experiment. Specifically, we consider a membrane-in-the-middle configuration of a mechanical oscillator within an optical cavity, where the intracavity field is modulated periodically by the external laser source. We demonstrate that a mixed regular and chaotic phase space can be engineered in one spatial dimension, through a significant quartic opto-mechanical interaction. For that case, we explore the expected dynamical tunnelling rates using Floquet theory and map out values of the effective Planck's constant that should be within practical reach.

quant-ph↗

arXiv2019

Tracking Rydberg atoms with Bose-Einstein Condensates

We propose to track position and velocity of mobile Rydberg excited impurity atoms through the elastic interactions of the Rydberg electron with a host condensate. Tracks first occur in the condensate phase, but are then naturally converted to features in the condensate density or momentum distribution. The condensate thus acts analogous to the cloud or bubble chambers in the early days of elementary particle physics. The technique will be useful for exploring Rydberg-Rydberg scattering, rare inelastic processes involving the Rydberg impurities, coherence in Rydberg motion and forces exerted by the condensate on the impurities. Our simulations show that resolvable tracks can be generated within the immersed Rydberg lifetime and condensate heating is under control. Finally, we demonstrate the utility of this Rydberg tracking technique to study ionizing Rydberg collisions or angular momentum changing interactions with the condensate.

physics.atom-ph↗

arXiv2018

Multi-Excitons in Flexible Rydberg Aggregates

Flexible Rydberg aggregates, assemblies of few Rydberg atoms coherently sharing electronic excitations while undergoing directed atomic motion, show great promise as quantum simulation platform for nuclear motional dynamics in molecules or quantum energy transport. Here we study additional features that are enabled by the presence of more than a single electronic excitation, thus considering multi-exciton states. We describe cases where these can be decomposed into underlying single exciton states and then present dynamical scenarios with atomic motion that illustrate exciton-exciton collisions, exciton routing, and strong non-adiabatic effects in simple one-dimensional settings.

quant-ph↗

arXiv2016

Quantum Zeno suppression of dipole-dipole forces

We consider inter-atomic forces due to resonant dipole-dipole interactions within a dimer of highly excited Rydberg atoms, embedded in an ultra-cold gas. These forces rely on a coherent superposition of two-atom electronic states, which is destroyed by continuous monitoring of the dimer state through a detection scheme utilizing controllable interactions with the background gas atoms. We show that this intrinsic decoherence of the molecular energy surface can gradually deteriorate a repulsive dimer state, causing a mixing of attractive and repulsive character. For sufficiently strong decoherence, a Zeno-like effect causes a complete arrest of interatomic forces. We finally show how short decohering pulses can controllably redistribute population between the different molecular energy surfaces.

quant-ph↗

arXiv2015

Phase-Imprinting of Bose-Einstein Condensates with Rydberg Impurities

We show how the phase profile of Bose-Einstein condensates can be engineered through its in- teraction with localized Rydberg excitations. The interaction is made controllable and long-range by off-resonantly coupling the condensate to another Rydberg state with laser light. Our technique allows the mapping of entanglement generated in systems of few strongly interacting Rydberg atoms onto much larger atom clouds in hybrid setups. As an example we discuss the creation of a spatial mesoscopic superposition state from a bright soliton. Additionally, the phase imprinted onto the condensate using the Rydberg excitations is a diagnostic tool for the latter. For example a condensate time-of-flight image would permit reconstructing the pattern of an embedded Rydberg crystal.

physics.atom-ph↗

arXiv2015

Open quantum system parameters from molecular dynamics

We extract the site energies and spectral densities of the Fenna-Matthews-Olson (FMO) pigment protein complex of green sulphur bacteria from simulations of molecular dynamics combined with energy gap calculations. Comparing four different combinations of methods, we investigate the origin of quantitative differences regarding site energies and spectral densities obtained previously in the literature. We find that different forcefields for molecular dynamics and varying local energy minima found by the structure relaxation yield significantly different results. Nevertheless, a picture averaged over these variations is in good agreement with experiments and some other theory results. Throughout, we discuss how vibrations external- or internal to the pigment molecules enter the extracted quantities differently and can be distinguished. Our results offer some guidance to set up more computationally intensive calculations for a precise determination of spectral densities in the future. These are required to determine absorption spectra as well as transport properties of light-harvesting complexes.

physics.bio-ph↗

arXiv2013

Van-der-Waals stabilized Rydberg aggregates

Assemblies of Rydberg atoms subject to resonant dipole-dipole interactions form Frenkel excitons. We show that van-der-Waals shifts can significantly modify the exciton wave function, whenever atoms approach each other closely. As a result, attractive excitons and repulsive van-der-Waals interactions can be combined to form stable one-dimensional atom chains, akin to bound aggregates. Here the van-der-Waals shifts ensure a stronger homogeneous delocalisation of a single excitation over the whole chain, enabling it to bind up to six atoms. When brought into unstable configurations, such Rydberg aggregates allow the direct monitoring of their dissociation dynamics.

physics.atom-ph↗

arXiv2013

Dynamical tunnelling with ultracold atoms in magnetic microtraps

The study of dynamical tunnelling in a periodically driven anharmonic potential probes the quantum-classical transition via the experimental control of the effective Planck's constant for the system. In this paper we consider the prospects for observing dynamical tunnelling with ultracold atoms in magnetic microtraps on atom chips. We outline the driven anharmonic potentials that are possible using standard magnetic traps, and find the Floquet spectrum for one of these as a function of the potential strength, modulation, and effective Planck's constant. We develop an integrable approximation to the non-integrable Hamiltonian and find that it can explain the behaviour of the tunnelling rate as a function of the effective Planck's constant in the regular region of parameter space. In the chaotic region we compare our results with the predictions of models that describe chaos-assisted tunnelling. Finally we examine the practicality of performing these experiments in the laboratory with Bose-Einstein condensates.

cond-mat.quant-gas↗

arXiv2013

Break-up of Rydberg superatoms via dipole-dipole interactions

We investigate resonant dipole-dipole interactions between two "superatoms" of different angular momentum, consisting of two Rydberg-blockaded atom clouds where each of them carries initially a coherently shared single excitation. We demonstrate that the dipole-dipole interaction breaks up the superatoms by removing the excitations from the clouds. The dynamics is akin to an ensemble average over systems where only one atom per cloud participates in entangled motion and excitation transfer. Our findings should thus facilitate the experimental realization of adiabatic exciton transport in Rydberg systems by replacing single sites with atom clouds.

physics.atom-ph↗

arXiv2012

Macroscopic Quantum Self-Trapping in Dynamical Tunnelling

It is well-known that increasing the nonlinearity due to repulsive atomic interactions in a double-well Bose-Einstein condensate suppresses quantum tunnelling between the two sites. Here we find analogous behaviour in the dynamical tunnelling of a Bose-Einstein condensate between period-one resonances in a single driven potential well. For small nonlinearities we find unhindered tunnelling between the resonances, but with an increasing period as compared to the non-interacting system. For nonlinearities above a critical value we generally observe that the tunnelling shuts down. However, for certain regimes of modulation parameters we find that dynamical tunnelling re-emerges for large enough nonlinearities, an effect not present in spatial double-well tunnelling. We develop a two-mode model in good agreement with full numerical simulations over a wide range of parameters, which allows the suppression of tunnelling to be attributed to macroscopic quantum self-trapping.

quant-ph↗

arXiv2012

Kicking electrons

The concept of dominant interaction hamiltonians is introduced and applied to classical planar electron-atom scattering. Each trajectory is governed in different time intervals by two variants of a separable approximate hamiltonian. Switching between them results in exchange of energy between the two electrons. A second mechanism condenses the electron-electron interaction to instants in time and leads to an exchange of energy and angular momentum among the two electrons in form of kicks. We calculate the approximate and full classical deflection functions and show that the latter can be interpreted in terms of the switching sequences of the approximate one. Finally, we demonstrate that the quantum results agree better with the approximate classical dynamical results than with the full ones.

physics.atom-ph↗