arXiv subjects

Sebastian Will

Publications and source records attributed to Sebastian Will.

At least 19 recordsLinked to original sources

arXiv2026

Electrostriction in a Bose-Einstein Condensate of Dipolar Molecules

The recent creation of a Bose-Einstein condensate (BEC) of dipolar molecules has opened a new frontier for many-body quantum systems in which dipolar interactions can drive novel self-organization phenomena. Here, we observe electrostriction in a molecular BEC, an elliptical deformation driven by anisotropic dipolar interactions. We use double microwave dressing, involving $\sigma$- and $\pi$-polarized fields, to control non-axially symmetric dipolar interactions. We compare the experimental observations of electrostriction to a model based on an extended Gross-Pitaevskii equation and find excellent agreement in the regime of weak to moderate interactions. Using electrostriction, we demonstrate that the molecular BEC can be torqued by dynamically changing the orientation of the elliptical $\sigma$ microwave field. This provides a route to setting molecular quantum gases into rotation, opening opportunities to probe vorticity, superfluidity, and supersolidity in strongly dipolar matter.

cond-mat.quant-gas↗

arXiv2026

Mapping the parameter space of double microwave shielding

Double microwave shielding employs $\sigma^{+}$- and $\pi$-polarized microwave fields, tuned close to the lowest rotational transition, to engineer a long-range repulsive barrier between polar molecules. By preventing molecules from reaching the short range, this technique suppresses detrimental two-body losses and recently enabled the realization of molecular Bose-Einstein condensates and self-bound droplets. Yet, the optimal operating regimes of the shielding mechanism remain largely unexplored. Here, by leveraging the underlying universality of the scattering problem, we systematically map the four-dimensional microwave parameter space-spanned by the detunings and intensities of the two fields-to identify configurations that maximize both shielding efficiency and interaction tunability. We define optimal operating regimes as configurations that are strictly free of field-linked bound states while sufficiently suppressing two-body losses to exceed typical lifetimes of ultracold samples. In these regimes, we evaluate the elastic-to-inelastic collision ratios required for efficient evaporative cooling and explore the accessible tuning range of the effective dipolar interactions. Finally, to identify the best platforms for future quantum simulation experiments, we conduct a global survey of candidate molecular species under realistic field constraints. We identify heavy, strongly dipolar molecules as the most promising candidates, demonstrating that they can achieve extreme loss suppression-reaching two-body loss rates as low as $10^{-18}$ cm$^{3}$/s-alongside robust interaction tunability using only moderate field strengths.

cond-mat.quant-gas↗

arXiv2026

A Mid-Infrared Platform Based on Strontium Tweezer Arrays

Subwavelength atomic tweezer arrays, in which atoms can be positioned at distances smaller than their emission wavelength, have been proposed as a versatile platform to study collective emission phenomena, such as superradiance and subradiance. Experimentally, the realization of such arrays has been a challenge as typical emission wavelengths in the visible or near-infrared are short compared to typical tweezer spacings in the micrometer range. Here, we use $^{88}$Sr atoms in optical tweezer arrays to access a mid-infrared transition at 2,923 nm ($5s5p\:^{3}P_{2} \rightarrow\, 5s4d\:^{3}D_{3}$). We identify a magic trapping wavelength at 597.14(3) nm and demonstrate single-atom preparation and imaging with high fidelity. In addition, using 2,923 nm light, we demonstrate resolved-sideband cooling of tweezer-trapped strontium. Beyond enabling studies of collective emission phenomena in flexible arrangements of atoms, our platform opens novel opportunities for dipolar many-body physics and enhanced control over Rydberg dynamics and the strontium fine-structure qubit.

physics.atom-ph↗

arXiv2026

Quantum Light Nano-Imaging

Entanglement and quantum correlations are central to the physics of quantum materials, yet they have remained notoriously difficult to access experimentally. Accessing these phenomena in solids requires quantum optical probes that operate at the native length and time scales of material excitations, below the diffraction limit of light. Developing the requisite tools has previously been infeasible due to the weak intensities of state-of-the-art quantum light sources and the inefficiency of light coupling in near-field light-matter interactions. In this work, we address these challenges and report the development of a quantum light scattering-type scanning near-field optical microscope (q-SNOM) that enables quantum-optical studies of solid-state systems with nanoscale spatial resolution. As a first demonstration, we visualize the self-interference of single hybrid light-matter polaritons in the prototypical van der Waals semiconductor MoS2. We also introduce a polaritonic time-of-flight metrology that exploits the temporal correlations among entangled photons to observe the quasiparticle propagation dynamics at femtosecond time scales. This work establishes a new experimental paradigm for exploring quantum effects in materials at the nanoscale.

cond-mat.mes-hall↗

arXiv2026

High precision micro-optical elements on fiber facets via focused-ion beam machining

Fiber-integrated micro-optical elements promise a scalable approach to photon collection and beam shaping for quantum information processing. Here, we demonstrate single-step fabrication of micro-spherical, micro-spiral, and micro-axicon structures directly on the core of single-mode optical fibers using focused ion beam (FIB) machining with nanometer-scale precision. Atomic force microscopy reveals that micro-concave and micro-convex spherical surfaces achieve shape accuracies of approximately $\lambda/80$ and $\lambda/50$ at $\lambda = 780$ nm, respectively. Optical characterization using a He-Ne laser at 633 nm confirms the expected far-field donut beam patterns for the micro-spiral and micro-axicon structures. Mach-Zehnder interferometry further verifies the corresponding azimuthal and radial phase profiles of the light emitted from the spiral and axicon fibers. Surface metrology shows that the optimized FIB process preserves optical-grade surface quality, introducing no measurable additional roughness at spatial scales relevant to visible and near-infrared operation. These monolithically integrated fiber micro-optical elements enable a broad range of applications in quantum technology, including fiber micro-cavities for cavity quantum electrodynamics, beam shaping for neutral atom trapping, and the generation of structured light for free-space quantum network links.

physics.optics↗

arXiv2026

Low-entropy arrays of microwave-shielded molecules prepared by interaction blockade

Ultracold molecules are becoming an increasingly important technology for quantum simulation, computation, and sensing, but their state preparation in large, low-entropy arrays remains a key challenge. We propose to deterministically load single molecules into optical tweezer arrays or lattices from either thermal or degenerate gases, with a high probability of occupying the tweezer's motional ground state. Strong repulsion between microwave-shielded molecules prevents multiparticle occupancy. Our proposal represents a robust scheme for deterministic single molecule preparation directly in the motional ground state with expected fidelities exceeding 99 percent for small trap volumes and highly polar species. This method can be scaled to thousands of traps limited by the reservoir molecule number, opening the door to large, low-entropy polar molecule arrays for quantum computation, quantum simulation, and precision measurement.

quant-ph↗

arXiv2025

Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics

Recent advances in molecular cooling have enabled the realization of strongly dipolar Bose--Einstein condensates (BECs) of molecules, and BECs of many different molecular species may become experimentally accessible in the near future. Here, we explore the unique properties of such BECs and the new insights they may offer into dipolar quantum fluids and many-body physics. We explore which parameter regimes can realistically be achieved using currently available experimental techniques, discuss how to implement these techniques, and outline which molecular species are particularly well suited to explore exotic new states of matter. We further determine how state-of-the-art beyond mean-field theories, originally developed for weakly dipolar magnetic gases, can be pushed to their limits and beyond, and what other long-standing questions in the field of dipolar physics may realistically come within reach using molecular systems.

cond-mat.quant-gas↗

arXiv2025

Observation of Self-Bound Droplets of Ultracold Dipolar Molecules

Ultracold gases of dipolar molecules have long been envisioned as a platform for the realization of novel quantum phases. Recent advances in collisional shielding, protecting molecules from inelastic losses, have enabled the creation of degenerate Fermi gases and, more recently, Bose-Einstein condensation of dipolar molecules. However, the observation of quantum phases in ultracold molecular gases that are driven by dipole-dipole interactions has so far remained elusive. In this work, we report the formation of self-bound droplets and droplet arrays in an ultracold gas of strongly dipolar sodium-cesium molecules. Starting from a molecular Bose-Einstein condensate (BEC), microwave dressing fields are used to induce dipole-dipole interactions with controllable strength and anisotropy. By varying the speed at which interactions are induced, covering a dynamic range of four orders of magnitude, we prepare droplets under equilibrium and non-equilibrium conditions, observing a transition from robust one-dimensional (1D) arrays to fluctuating two-dimensional (2D) structures. The droplets exhibit densities up to 100 times higher than the initial BEC, reaching the strongly interacting regime, and suggesting the possibility of a quantum-liquid or crystalline state. This work establishes ultracold molecules as a system for the exploration of strongly dipolar quantum matter and opens the door to the realization of self-organized crystal phases and dipolar spin liquids in optical lattices.

cond-mat.quant-gas↗

arXiv2025

Extreme Loss Suppression and Wide Tunability of Dipolar Interactions in an Ultracold Molecular Gas

Ultracold dipolar molecules hold great promise for the creation of novel quantum states of matter, but the realization of long-lived molecular bulk samples with strong dipole-dipole interactions has remained elusive. Here, we realize a collisionally stable gas of ultracold ground state molecules with a lifetime of several seconds. Utilizing double microwave dressing, we achieve an extreme suppression of inelastic two- and three-body losses by factors of more than 10,000 and 1,000, respectively. We find that losses remain suppressed across a wide range of dipole-dipole interactions, allowing the continuous tuning of the dipolar length from 0 to 1 um $\sim$ 20,000 $a_0$. Combined with the recent realization of Bose-Einstein condensation of dipolar molecules, our findings open the door to the exploration of strongly dipolar quantum liquids.

cond-mat.quant-gas↗

arXiv2025

Double Microwave Shielding

We develop double microwave shielding, which has recently enabled evaporative cooling to the first Bose-Einstein condensate of polar molecules [Bigagli et al., Nature 631, 289 (2024)]. Two microwave fields of different frequency and polarization are employed to effectively shield polar molecules from inelastic collisions and three-body recombination. Here, we describe in detail the theory of double microwave shielding. We demonstrate that double microwave shielding effectively suppresses two- and three-body losses. Simultaneously, dipolar interactions and the scattering length can be flexibly tuned, enabling comprehensive control over interactions in ultracold gases of polar molecules. We show that this approach works universally for a wide range of molecules. This opens the door to studying many-body physics with strongly interacting dipolar quantum matter.

cond-mat.quant-gas↗

arXiv2024

Trapping of Single Atoms in Metasurface Optical Tweezer Arrays

Optical tweezer arrays have emerged as a key experimental platform for quantum computation, quantum simulation, and quantum metrology, enabling unprecedented levels of control over single atoms and molecules. However, existing tweezer platforms have fundamental limitations in array geometry, size, and scalability. Here we demonstrate the trapping of single strontium atoms in optical tweezer arrays generated via holographic metasurfaces. We realize two dimensional arrays with more than 1000 trapped atoms, arranged in arbitrary geometries with trap spacings as small as 1.5 um. The arrays have a high uniformity in terms of trap depth, trap frequency, and positional accuracy, rivaling or surpassing existing approaches. This is enabled by highly efficient holographic metasurfaces fabricated from high-refractive index materials, silicon-rich silicon nitride and titanium dioxide. Leveraging sub-micrometer pixel sizes and high pixel densities, our platform allows scaling far beyond current capabilities. As a demonstration, we realize an optical tweezer array with 360,000 traps. These advances will facilitate tweezer-array based quantum applications that require large system sizes.

physics.atom-ph↗

arXiv2024

Three-Body Recombination of Ultracold Microwave-Shielded Polar Molecules

A combined experimental and theoretical study is carried out on the three-body recombination process in a gas of microwave-shielded polar molecules. For ground-state polar molecules dressed with a strong microwave field, field-linked bound states can appear in the intermolecular potential. We model three-body recombination into such bound states using classical trajectory calculations. Our results show that recombination can explain the enhanced loss rates observed at small microwave detunings in trapped samples of bosonic NaCs [Bigagli, $\textit{et al.}$, Nat. Phys. $\textbf{19}$ 1579-1584 (2023)]. Specifically, our calculations reproduce the experimentally measured three-body loss rates across a wide range of microwave Rabi couplings, detunings, and temperatures. This work suggests that for bosonic shielded molecular systems in which the two-body loss is sufficiently suppressed and a field-linked bound state is present, the dominant loss process will be three-body recombination.

cond-mat.quant-gas↗

arXiv2024

Dressed-State Spectroscopy and Magic Trapping of Microwave-Shielded NaCs Molecules

We report on the optical polarizability of microwave-shielded ultracold NaCs molecules in an optical dipole trap. While dressing a pair of rotational states with a microwave field, we observe a marked dependence of the optical polarizability on the intensity and detuning of the dressing field. To precisely characterize differential energy shifts between dressed rotational states, we establish dressed-state spectroscopy. For strong dressing fields, we find that a magic rotational transition can be engineered and demonstrate its insensitivity to laser intensity fluctuations. The results of this work have direct relevance for evaporative cooling and the recent demonstration of molecular Bose-Einstein condensates [Bigagli, et al., Nature (2024)] and may open a door to precision microwave spectroscopy in interacting many-body systems of microwave-shielded molecules.

cond-mat.quant-gas↗

arXiv2024

Artificial Precision Timing Array: bridging the decihertz gravitational-wave sensitivity gap with clock satellites

Gravitational-wave astronomy has developed enormously over the last decade, with the first detections and continuous development across broad frequency bands. However, the decihertz range has largely been left out of this development. Gravitational waves in this band are emitted by some of the most enigmatic sources, including intermediate-mass binary black hole mergers, early inspiraling compact binaries$\unicode{x2014}$whose mergers are seen by Earth-based detectors$\unicode{x2014}$, and possibly primordial gravitational waves. To tap this exciting band, we propose the construction of a detector based on pulsar timing principles, the Artificial Precision Timing Array (APTA). We envision APTA as a solar system array of artificial ``pulsars''$\unicode{x2014}$precision-time-reference-carrying satellites that emit periodic electromagnetic signals towards Earth or another satellite constellation receiver location. In this fundamental study, we estimate the clock precision needed for gravitational-wave detection with APTA. Our results suggest that 6 satellites and a clock relative uncertainty of $10^{-18}$ at 1~s of averaging, which is currently attainable with ground-based atomic clocks, would be sufficient for APTA to reach pristine sensitivity in the decihertz band and observe $10^3\unicode{x2013}10^4$ $\mathrm{M}_\odot$ black hole mergers and the early inspiral of heavy LIGO-Virgo-KAGRA sources. Future clock and oscillator technologies realistically expected in the next decade(s) would enable the detection of an increasingly diverse set of sources, allowing APTA to reach a better sensitivity than other detector concepts proposed for the decihertz band. This work opens up a new area of research into designing and constructing gravitational-wave detectors relying on principles used successfully in pulsar timing.

astro-ph.IM↗

arXiv2023

Observation of Bose-Einstein Condensation of Dipolar Molecules

Ensembles of particles governed by quantum mechanical laws exhibit fascinating emergent behavior. Atomic quantum gases, liquid helium, and electrons in quantum materials all show distinct properties due to their composition and interactions. Quantum degenerate samples of bosonic dipolar molecules promise the realization of novel phases of matter with tunable dipolar interactions and new avenues for quantum simulation and quantum computation. However, rapid losses, even when reduced through collisional shielding techniques, have so far prevented cooling to a Bose-Einstein condensate (BEC). In this work, we report on the realization of a BEC of dipolar molecules. By strongly suppressing two- and three-body losses via enhanced collisional shielding, we evaporatively cool sodium-cesium (NaCs) molecules to quantum degeneracy. The BEC reveals itself via a bimodal distribution and a phase-space-density exceeding one. BECs with a condensate fraction of 60(10) % and a temperature of 6(2) nK are created and found to be stable with a lifetime close to 2 seconds. This work opens the door to the exploration of dipolar quantum matter in regimes that have been inaccessible so far, promising the creation of exotic dipolar droplets, self-organized crystal phases, and dipolar spin liquids in optical lattices.

cond-mat.quant-gas↗

arXiv2023

Automated Graph-Based Detection of Quantum Control Schemes: Application to Molecular Laser Cooling

One of the demanding frontiers in ultracold quantum science is identifying laser cooling schemes for complex atoms and molecules out of their vast spectra of internal states. Motivated by the prospect of expanding the set of available ultracold molecules for applications in fundamental physics, chemistry, astrochemistry, and quantum simulation, we propose and demonstrate an automated graph-based search approach for viable laser cooling schemes. The method is time efficient, reproduces the results of previous manual searches, and reveals a plethora of new potential laser cooling schemes. We discover laser cooling schemes for YO, C$_2$, OH$^+$, CN, and CO$_2$, including surprising schemes that start from highly excited states or do not rely on a strong main transition. A central insight of this work is that the reinterpretation of quantum states and transitions between them as a graph can dramatically enhance the ability to identify new quantum control schemes for complex quantum systems. As such, this approach will also apply to complex atoms and, in fact, any complex many-body quantum system with a discrete spectrum of internal states.

quant-ph↗

arXiv2023

Laser Scheme for Doppler Cooling of the Hydroxyl Cation (OH$^+$)

We report on a cycling scheme for Doppler cooling of trapped OH$^+$ ions using transitions between the electronic ground state $X^3\Sigma^-$ and the first excited triplet state $A^3\Pi$. We have identified relevant transitions for photon cycling and repumping, have found that coupling into other electronic states is strongly suppressed, and have calculated the number of photon scatterings required to cool OH$^+$ to a temperature where Raman sideband cooling can take over. In contrast to the standard approach, where molecular ions are sympathetically cooled, our scheme does not require co-trapping of another species and opens the door to the creation of pure samples of cold molecular ions with potential applications in quantum information, quantum chemistry, and astrochemistry. The laser cooling scheme identified for OH$^+$ is efficient despite the absence of near-diagonal Franck-Condon factors, suggesting that broader classes of molecules and molecular ions are amenable to laser cooling than commonly assumed.

physics.atom-ph↗

arXiv2023

A planar cloverleaf antenna for the creation of circularly polarized microwave fields

We report on the design and characterization of a compact microwave antenna for atomic and molecular physics experiments. The antenna is comprised of four loop antennas arranged in cloverleaf shape, allowing for precise adjustment of polarization by tuning the relative phase of the loops. We optimize the antenna for left-circularly polarized microwaves at 3.5 GHz and characterize its performance using ultracold NaCs molecules as a precise quantum sensor. Observing an unusually high Rabi frequency of $2\pi \times 46$ MHz, we extract an electric field amplitude of 33(2) V/cm at 22 mm distance from the antenna. The polarization ellipticity is 2.3(4) degrees, corresponding to a 24 dB suppression of right-circular polarization. The cloverleaf antenna is planar and provides large optical access, making it highly suitable for quantum control of atoms and molecules, and potentially other quantum systems that operate in the microwave regime.

physics.atom-ph↗