arXiv subjects

Sebastian Wintz

Publications and source records attributed to Sebastian Wintz.

At least 37 records · Page 2Linked to original sources

arXiv2025

Nanoscale Domain Wall Dynamics in Micromagnetic Structures with Weak Perpendicular Anisotropy

Time-resolved pump-probe soft X-ray ptychography and Scanning Transmission X-ray Microscopy (STXM) were employed to study the magnetic domain wall dynamics in microstructures of permalloy (Ni$_{81}$Fe$_{19}$; Py) with a weak growth-induced perpendicular magnetic anisotropy. The X-ray magnetic circular dichroism (XMCD) images of a micrometer-sized Py square (160 nm thickness) and an elliptical disk (80 nm thickness) show flux-closure patterns with domain walls that fall into alternating out-of-plane (OOP) magnetization states precipitated by the perpendicular anisotropy, which is a precursor of the nucleation of stripe domains at higher thicknesses. An oscillating magnetic field at frequencies from tens of MHz to GHz and up to 4 mT magnitude excited dynamic modes in the domain walls along with the vortex core gyration. The domain wall dynamics include the translation of inversion points of the OOP magnetization and nucleation of one-dimensional spin waves.

cond-mat.mtrl-sci↗

arXiv2025

Altermagnetic nanotextures revealed in bulk MnTe

With many candidate altermagnetic materials, MnTe has emerged as one of the most promising systems, with growing experimental evidence for altermagnetic phenomena. So far, the majority of measurements have been performed on thin-films, or have involved surface measurements. However, the question of altermagnetic order in the bulk system - in the absence of substrate or surface effects - remains. Here we show evidence for bulk altermagnetism in single crystal MnTe, through spectroscopic X-ray microscopy. By performing nanoscale X-ray magnetic circular dichroic (XMCD) imaging in transmission on a 200 nm thick lamella, we observe domains and magnetic textures with a spectroscopic signature characteristic of altermagnetic order, thereby confirming the intrinsic nature of altermagnetism in MnTe. Quantitative analysis of the XMCD signal reveals an excellent agreement with predicted signals, establishing that the altermagnetic order exists throughout the thickness of the lamella and confirming the intrinsic, bulk nature of the state. With these results, we demonstrate that transmission XMCD spectroscopic imaging is a robust, quantitative technique to probe altermagnetic order, providing a means to probe individual altermagnetic domains within complex configurations. This ability to investigate, and characterise altermagnetic order in bulk crystals represents an important tool for the exploration of altermagnetism across a wide range of candidate materials, of key importance for the development of future technologies.

cond-mat.mtrl-sci↗

arXiv2024

The Effect of Ga-Ion Irradiation on Sub-Micron-Wavelength Spin Waves in Yttrium-Iron-Garnet Films

We investigate the effect of focused-ion-beam (FIB) irradiation on spin waves with sub-micron wavelengths in Yttrium-Iron-Garnet (YIG) films. Time-resolved scanning transmission X-ray (TR-STXM) microscopy was used to image the spin waves in irradiated regions and deduce corresponding changes in the magnetic parameters of the film. We find that the changes of Ga$^+$ irradiation can be understood by assuming a few percent change in the effective magnetization $M_\mathrm{eff}$ of the film due to a trade-off between changes in anisotropy and effective film thickness. Our results demonstrate that FIB irradiation can be used to locally alter the dispersion relation and the effective refractive index $n_\textrm{eff}$ of the film, even for submicron wavelengths. To achieve the same change in $n_\textrm{eff}$ for shorter wavelengths, a higher dose is required, but no significant deterioration of spin wave propagation length in the irradiated regions was observed, even at the highest applied doses.

physics.app-ph↗

arXiv2024

Magnetization patterns in $\text{GaAs}$-$\text{Fe}_{\text{33}}\text{Co}_{\text{67}}$ core-shell nanorods

We present a study on the static magnetic properties of individual $\text{GaAs}$-$\text{Fe}_{\text{33}}\text{Co}_{\text{67}}$ core-shell nanorods. X-ray Magnetic Circular Dichroism combined with Photoemission Electron Microscopy (XMCD-PEEM) and Scanning Transmission X-ray Microscopy (STXM) were used to investigate the magnetic nanostructures. The magnetic layer is purposely designed to establish a magnetic easy axis neither along a high symmetry nor mirror axes to promote 3D magnetic helical order on the curved surface. In practice, two types of magnetic textures with in-plane magnetization were found inside the nanostructures' facets: magnetic domains with almost longitudinal or almost perpendicular magnetization with respect to the axis of the tube. We observe that a magnetic field applied perpendicular to the long axis of the nanostructure can add an azimuthal component of the magnetization to the previously almost longitudinal magnetization.

cond-mat.mes-hall↗

arXiv2024

Competing anisotropies in the chiral cubic magnet Co$_8$Zn$_8$Mn$_4$ unveiled by resonant x-ray magnetic scattering

The cubic $β$-Mn-type alloy Co$_8$Zn$_8$Mn$_4$ is a chiral helimagnet that exhibits a peculiar temperature-dependent behavior in the spiral pitch, which decreases from 130 nm at room temperature to 70 nm below 20 K. Notably, this shortening is also accompanied by a structural transition of the metastable skyrmion texture, transforming from a hexagonal lattice to a square lattice of elongated skyrmions. The underlying mechanism of these transformations remain unknown, with interactions potentially involved including temperature-dependent Dzyaloshinskii-Moriya interaction, magnetocrystalline anisotropy, and exchange anisotropy. Here, x-ray resonant magnetic small-angle scattering in vectorial magnetic fields was employed to investigate the temperature dependence of the anisotropic properties of the helical phase in Co$_8$Zn$_8$Mn$_4$. Our results reveal quantitatively that the magnitude of the anisotropic exchange interaction increases by a factor of 4 on cooling from room temperature to 20 K, leading to a 5% variation in the helical pitch within the (001) plane at 20 K. While anisotropic exchange interaction contributes to the shortening of the spiral pitch, its magnitude is insufficient to explain the variation in the spiral periodicity from room to low temperatures. Finally, we demonstrate that magnetocrystalline and exchange anisotropies compete, favoring different orientations of the helical vector in the ground state.

cond-mat.mes-hall↗

arXiv2024

Steerable current-driven emission of spin waves in magnetic vortex pairs

The efficient excitation of spin waves is a key challenge in the realization of magnonic devices. We demonstrate the current-driven generation of spin waves in antiferromagnetically coupled magnetic vortices. We employ time-resolved scanning transmission X-ray microscopy (TR-STXM) to directly image the emission of spin waves upon the application of an alternating current flowing directly through the magnetic stack. Micromagnetic simulations allow us to identify the origin of the excitation to be the current-driven Oersted field, which in the present system proves to be orders of magnitude more efficient than the commonly used excitation via stripline antennas. Our numerical studies also reveal that the spin-transfer torque can lead to the emission of spin waves as well, yet only at much higher current amplitudes. By using magnetostrictive materials, we futhermore demonstrate that the direction of the magnon propagation can be steered by increasing the excitation amplitude, which modifies the underlying magnetization profile through an additional anisotropy in the magnetic layers. The demonstrated methods allow for the efficient and tunable excitation of spin waves, marking a significant advance in the generation and control of spin waves in magnonic devices.

cond-mat.mes-hall↗

arXiv2023

Direct observation of Néel-type skyrmions and domain walls in a ferrimagnetic DyCo$_3$ thin film

Isolated magnetic skyrmions are stable, topologically protected spin textures that are at the forefront of research interests today due to their potential applications in information technology. A distinct class of skyrmion hosts are rare earth - transition metal (RE-TM) ferrimagnetic materials. To date, the nature and the control of basic traits of skyrmions in these materials are not fully understood. We show that for an archetypal ferrimagnetic material DyCo$_3$ that exhibits a strong perpendicular anisotropy, the ferrimagnetic skyrmion size can be tuned by an external magnetic field. Moreover, by taking advantage of the high spatial resolution of scanning transmission X-ray microscopy (STXM) and utilizing a large x-ray magnetic linear dichroism (XMLD) contrast that occurs naturally at the RE resonant edges, we resolve the nature of the magnetic domain walls of ferrimagnetic skyrmions. We demonstrate that through this method one can easily discriminate between Bloch and Néel type domain walls for each individual skyrmion. For all isolated ferrimagnetic skyrmions, we observe that the domain walls are of Néel-type. This key information is corroborated with results of micromagnetic simulations and allows us to conclude on the nature of the Dzyaloshinskii-Moriya interaction (DMI) which concurs to the stabilisation of skyrmions in this ferrimagnetic system. Establishing that an intrinsic DMI occurs in RE-TM materials will also be beneficial towards a deeper understanding of chiral spin texture control in ferrimagnetic materials.

cond-mat.mtrl-sci↗

arXiv2023

Electrical detection and nucleation of a magnetic skyrmion in a magnetic tunnel junction observed via operando magnetic microscopy

Magnetic skyrmions are topological spin textures which are envisioned as nanometre scale information carriers in magnetic memory and logic devices. The recent demonstration of room temperature stabilization of skyrmions and their current induced manipulation in industry compatible ultrathin films were first steps towards the realisation of such devices. However, important challenges remain regarding the electrical detection and the low-power nucleation of skyrmions, which are required for the read and write operations. Here, we demonstrate, using operando magnetic microscopy experiments, the electrical detection of a single magnetic skyrmion in a magnetic tunnel junction (MTJ) and its nucleation and annihilation by gate voltage via voltage control of magnetic anisotropy. The nucleated skyrmion can be further manipulated by both gate voltage and external magnetic field, leading to tunable intermediate resistance states. Our results unambiguously demonstrate the readout and voltage controlled write operations in a single MTJ device, which is a major milestone for low power skyrmion based technologies.

cond-mat.mtrl-sci↗

arXiv2023

Quantifying the spin-wave asymmetry in single and double rectangular Ni$_{80}$Fe$_{20}$ microstrips by TR-STXM, FMR and micromagnetic simulations

The asymmetry of spin-wave patterns in confined rectangular Ni$_{80}$Fe$_{20}$ microstrips, both in single and double-strip geometries, is quantified. The results of TR-STXM and micromagnetic simulations are compared. For the TR-STXM measurements and the corresponding simulations the excitation was a uniform microwave field with a fixed frequency of 9.43 GHz, while the external static magnetic field was swept. In the easy axis orientation of the analyzed microstrip, the results show a higher asymmetry for the double microstrip design, indicating an influence of the additional microstrip placed in close proximity to the analyzed one.

cond-mat.mes-hall↗

arXiv2022

Role of substrate clamping on anisotropy and domain structure in the canted antiferromagnet $α$-Fe$_2$O$_3$

Antiferromagnets have recently been propelled to the forefront of spintronics by their high potential for revolutionizing memory technologies. For this, understanding the formation and driving mechanisms of the domain structure is paramount. In this work, we investigate the domain structure in a thin-film canted antiferromagnet $α$-Fe$_2$O$_3$. We find that the internal destressing fields driving the formation of domains do not follow the crystal symmetry of $α$-Fe$_2$O$_3$, but fluctuate due to substrate clamping. This leads to an overall isotropic distribution of the Néel order with locally varying effective anisotropy in antiferromagnetic thin films. Furthermore, we show that the weak ferromagnetic nature of $α$-Fe$_2$O$_3$ leads to a qualitatively different dependence on magnetic field compared to collinear antiferromagnets such as NiO. The insights gained from our work serve as a foundation for further studies of electrical and optical manipulation of the domain structure of antiferromagnetic thin films.

cond-mat.mes-hall↗

arXiv2022

Tailoring Optical Excitation to Control Magnetic Skyrmion Nucleation

In ferromagnetic multilayers, a single laser pulse with a fluence above an optical nucleation threshold can create magnetic skyrmions, which are randomly distributed over the area of the laser spot. However, in order to study the dynamics of skyrmions and for their application in future data technology, a controllable localization of the skyrmion nucleation sites is crucial. Here, it is demonstrated that patterned reflective masks behind a thin magnetic film can be designed to locally tailor the optical excitation amplitudes reached, leading to spatially controlled skyrmion nucleation on the nanometer scale. Using x-ray microscopy, the influence of nanopatterned back-side aluminum masks on the optical excitation is studied in two sample geometries with varying layer sequence of substrate and magnetic Co/Pt multilayer. Surprisingly, the masks' effect on suppressing or enhancing skymion nucleation reverses when changing this sequence. Moreover, optical near-field enhancements additionally affect the spatial arrangement of the nucleated skyrmions. Simulations of the spatial modulation of the laser excitation, and the following heat transfer across the interfaces in the two sample geometries are employed to explain these observations. The results demonstrate a reliable approach to add nanometer-scale spatial control to optically induced magnetization processes on ultrafast timescales.

cond-mat.mtrl-sci↗

arXiv2022

Nonstanding spin waves in a single rectangular permalloy microstrip under uniform magnetic excitation

Ferromagnetic resonance modes in a single rectangular Ni$_{80}$Fe$_{20}$ microstrip were directly imaged using time-resolved scanning transmission x-ray microscopy combined with a phase-locked ferromagnetic resonance excitation scheme and the findings were corroborated by micromagnetic simulations. Although under uniform excitation in a single confined microstructure typically standing spin waves are expected, all imaged spin waves showed a nonstanding character both, at and off resonance, the latter being additionally detected with microantenna-based ferromagnetic resonance. The effect of the edge quality on the spin waves was observed in micromagnetic simulations.

cond-mat.mes-hall↗

arXiv2021

Skyrmions in synthetic antiferromagnets and their nucleation via electrical current and ultrafast laser illumination

Magnetic skyrmions are topological spin textures that hold great promise as nanoscale information carriers in non-volatile memory and logic devices. While room-temperature magnetic skyrmions and their current-induced manipulation were recently demonstrated, the stray field resulting from their finite magnetization as well as their topological charge limit their minimum size and reliable motion in tracks. Antiferromagnetic (AF) skyrmions allow these limitations to be lifted owing to their vanishing magnetization and net zero topological charge, promising room-temperature, ultrasmall skyrmions, fast dynamics, and insensitivity to external magnetic fields. While room-temperature AF spin textures have been recently demonstrated, the observation and controlled nucleation of AF skyrmions operable at room temperature in industry-compatible synthetic antiferromagnetic (SAF) material systems is still lacking. Here we demonstrate that isolated skyrmions can be stabilized at zero field and room temperature in a fully compensated SAF. Using X-ray microscopy techniques, we are able to observe the skyrmions in the different SAF layers and demonstrate their antiparallel alignment. The results are substantiated by micromagnetic simulations and analytical models using experimental parameters, which confirm the chiral SAF skyrmion spin texture and allow the identification of the physical mechanisms that control the SAF skyrmion size and stability. We also demonstrate the local nucleation of SAF skyrmions via local current injection as well as ultrafast laser excitations at zero field. These results will enable the utilization of SAF skyrmions in skyrmion-based devices.

cond-mat.mtrl-sci↗

arXiv2021

Reconfigurable sub-micron spin-wave majority gate with electrical transducers

Spin waves are excitations in ferromagnetic media that have been proposed as information carriers in hybrid spintronic devices with much lower operation power than conventional charge-based electronics. Their wave nature can be exploited in majority gates by using interference for computation. However, a scalable spin-wave majority gate that can be co-integrated alongside conventional electronics is still lacking. Here, we demonstrate a sub-micron inline spin-wave majority gate with fan-out. Time-resolved imaging of the magnetization dynamics by scanning transmission x-ray microscopy illustrates the device operation. All-electrical spin-wave spectroscopy further demonstrates majority gates with sub-micron dimensions, reconfigurable input and output ports, and frequency-division multiplexing. Challenges for hybrid spintronic computing systems based on spin-wave majority gates are discussed.

physics.app-ph↗

arXiv2021

Symmetry- and curvature effects on spin waves in vortex-state hexagonal nanotubes

Analytic and numerical studies on curved magnetic nano-objects predict numerous exciting effects that can be referred to as magneto-chiral effects, which do not originate from intrinsic Dzyaloshinskii-Moriya interaction or interface-induced anisotropies. In constrast, these chiral effects stem from isotropic exchange or dipole-dipole interaction, present in all magnetic materials, which acquire asymmetric contributions in case of curved geometry of the specimen. As a result, for example, the spin-wave dispersion in round magnetic nanotubes becomes asymmetric, namely spin waves of the same frequency propagating in opposite directions along the nanotube exhibit different wavelenghts. Here, using time-resolved scanning transmission X-ray microscopy experiments, standard micromagntic simulations and a dynamic-matrix approach, we show that the spin-wave spectrum undergoes additional drastic changes when transitioning from a continuous to a discrete rotational symmetry, i.e. from round to hexagonal nanotubes, which are much easier to fabricate. The polygonal shape introduces localization of the modes both to the sharp, highly curved corners and flat edges. Moreover, due to the discrete rotational symmetry, the degenerate nature of the modes with azimuthal wave vectors known from round tubes is partly lifted, resulting in singlet and duplet modes. For comparison with our experiments, we calculate the microwave absorption from the numerically obtained mode profiles which shows that a dedicated antenna design is paramount for magnonic applications in 3D nano-structures. To our knowledge these are the first experiments directly showing real space spin-wave propagation in 3D nano objects.

cond-mat.mes-hall↗

arXiv2020

Experimental observation of the curvature-induced asymmetric spin-wave dispersion in hexagonal nanotubes

Theoretical and numerical studies on curved magnetic nano-objects predict numerous exciting effects that can be referred to as magneto-chiral effects, which do not originate from the intrinsic Dzyaloshinskii-Moriya interaction or surface-induced anisotropies. The origin of these chiral effects is the isotropic exchange or the dipole-dipole interaction present in all magnetic materials but renormalized by the curvature. Here, we demonstrate experimentally that curvature induced effects originating from the dipole-dipole interaction are directly observable by measuring spin-wave propagation in magnetic nanotubes with hexagonal cross section using time resolved scanning transmission X-ray microscopy. We show that the dispersion relation is asymmetric upon reversal of the wave vector when the propagation direction is perpendicular to the static magnetization. Therefore counter-propagating spin waves of the same frequency exhibit different wavelenghts. Hexagonal nanotubes have a complex dispersion, resulting from spin-wave modes localised to the flat facets or to the extremely curved regions between the facets. The dispersion relations obtained experimentally and from micromagnetic simulations are in good agreement. %The asymmetric spin-wave transport is present for all modes, promoting hexagonal nanotubes for magnonic applications. These results show that spin-wave transport is possible in 3D, and that the dipole-dipole induced magneto-chiral effects are significant.

cond-mat.mes-hall↗

arXiv2019

Nonreciprocal nano-optics with spin-waves in synthetic antiferromagnets

Integrated optically-inspired wave-based processing is envisioned to outperform digital architectures in specific tasks, such as image processing and speech recognition. In this view, spin-waves represent a promising route due to their nanoscale wavelength in the GHz frequency range and rich phenomenology. Here, we realize a versatile optically-inspired platform using spin-waves, demonstrating the wavefront engineering, focusing, and robust interference of spin-waves with nanoscale wavelength. In particular, we use magnonic nanoantennas based on tailored spin-textures for launching spatially shaped coherent wavefronts, diffraction-limited spin-wave beams, and generating robust multi-beam interference patterns, which spatially extend for several times the spin-wave wavelength. Furthermore, we show that intriguing features, such as resilience to back-reflection, naturally arise from the spin-wave nonreciprocity in synthetic antiferromagnets, preserving the high quality of the interference patterns from spurious counterpropagating modes. This work represents a fundamental step towards the realization of nanoscale optically-inspired devices based on spin-waves.

cond-mat.mes-hall↗

arXiv2019

Deterministic field-free skyrmion nucleation at a nano-engineered injector device

Magnetic skyrmions are topological solitons that exhibit an increased stability against annihilation, and can be displaced with low current densities, making them a promising candidate as an information carrier. In order to demonstrate a viable skyrmion-based memory device, it is necessary to reliably and reproducibly nucleate, displace, detect, and delete the magnetic skyrmions. While the skyrmion displacement and detection have both been investigated in detail, much less attention has been dedicated to the study of the sub-ns dynamics of the skyrmion nucleation process. Only limited studies on the statics and above-ns dynamics have been performed, leaving still many open questions on the dynamics of the nucleation process. Furthermore, the vast majority of the presently existing studies focus on the nucleation from random natural pinning sites, or from patterned constrictions in the magnetic material itself, which limit the functionality of the skyrmion-based device. Those limitations can be overcome by the fabrication of a dedicated injector device on top of the magnetic material. In this study, we investigate the nucleation of magnetic skyrmions from a dedicated nano-engineered injector, demonstrating the reliable magnetic skyrmion nucleation at the remnant state. The sub-ns dynamics of the skyrmion nucleation process were also investigated, allowing us to shine light on the physical processes driving the nucleation.

cond-mat.mes-hall↗