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Sebastien Roux

Publications and source records attributed to Sebastien Roux.

2 recordsLinked to original sources

Incoherent dark excitons extend Floquet-like physics across time and momentum

Floquet phenomena - where a coherent, time-periodic drive hybridizes the conduction band with energy-replicated copies of the valence band - have been demonstrated with intense optical fields and, more recently, other bosonic excitations. However, within mean-field approximations and the current understanding of Floquet phenomena, these effects survive only for the coherence time of the drive, limiting practical use and current demonstrations to the sub-picosecond regime. Here, consistent with recent theoretical predictions beyond the mean-field picture, using time- and angle-resolved photoemission spectroscopy in WSe$_2$/MoS$_2$ heterostructures, we show that incoherent, dense populations of dark interlayer excitons hybridize the conduction band with energy-replicated copies of the valence band, mimicking Floquet-like phenomena - now persisting for nearly a nanosecond. With increasing interlayer exciton density, the valence band and its replica evolve from an inverted-parabolic to a Mexican-hat dispersion, a signature of the predicted non-zero static coupling that hybridizes the bands and scales linearly with the exciton density. By tuning twist angle, we further show that dark excitons with net momentum create replicas that hybridize with bands offset not just in energy but also in momentum, providing another powerful degree of freedom beyond conventional Floquet engineering. These results establish a robust, long-lived route to engineering electronic states, beyond a coherent, zero-momentum drive.

cond-mat.mes-hall↗

Quantum light generation with ultra-high spatial resolution in 2D semiconductors via ultra-low energy electron irradiation

Single photon emitters (SPEs) are building blocks of quantum technologies. Defect engineering of 2D materials is ideal to fabricate SPEs, wherein spatially deterministic and quality-preserving fabrication methods are critical for integration into quantum devices and cavities. Existing methods use combination of strain and electron irradiation, or ion irradiation, which make fabrication complex, and limited by surrounding lattice damage. Here, we utilise only ultra-low energy electron beam irradiation (5 keV) to create dilute defect density in hBN-encapsulated monolayer MoS2, with ultra-high spatial resolution (< 50 nm, extendable to 10 nm). Cryogenic photoluminescence spectra exhibit sharp defect peaks, following power-law for finite density of single defects, and characteristic Zeeman splitting for MoS2 defect complexes. The sharp peaks have low spectral jitter (< 200 μeV), and are tuneable with gate-voltage and electron beam energy. Use of low-momentum electron irradiation, ease of processing, and high spatial resolution, will disrupt deterministic creation of high-quality SPEs.

cond-mat.mes-hall↗