arXiv subjects

Seiki Komiya

Publications and source records attributed to Seiki Komiya.

At least 37 records · Page 2Linked to original sources

arXiv2009

Measurement of x-ray absorption spectra of overdoped high-temperature cuprate superconductors: Inapplicability of the single-band Hubbard model

X-ray absorption spectra on the overdoped high-temperature superconductors Tl_2Ba_2CuO_{6+delta} (Tl-2201) and La_{2-x}Sr_xCuO_{4+delta} (LSCO) reveal a striking departure in the electronic structure from that of the underdoped regime. The upper Hubbard band, identified with strong correlation effects, is not observed on the oxygen K edge, while the lowest-energy prepeak gains less intensity than expected above p ~ 0.21. This suggests a breakdown of the Zhang-Rice singlet approximation and a loss of correlation effects or a significant shift in the most fundamental parameters of the system, rendering single-band Hubbard models inapplicable. Such fundamental changes suggest that the overdoped regime may offer a distinct route to understanding in the cuprates.

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arXiv2008

Universal versus Material-Dependent Two-Gap Behaviors in the High-Tc Cuprates: Angle-Resolved Photoemission Study of La2-xSrxCuO4

We have investigated the doping and temperature dependences of the pseudogap/superconducting gap in the single-layer cuprate La$_{2-x}$Sr$_x$CuO$_4$ by angle-resolved photoemission spectroscopy. The results clearly exhibit two distinct energy and temperature scales, namely, the gap around ($π$,0) of magnitude $Δ^*$ and the gap around the node characterized by the d-wave order parameter $Δ_0$, like the double-layer cuprate Bi2212. In comparison with Bi2212 having higher $T_c$'s, $Δ_0$ is smaller, while $Δ^*$ and $T^*$ are similar. This result suggests that $Δ^*$ and $T^*$ are approximately material-independent properties of a single CuO$_2$ plane, in contrast the material-dependent $Δ_0$, representing the pairing strength.

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arXiv2008

Appearance of Universal Metallic Dispersion in a Doped Mott Insulator

We have investigated the dispersion renormalization $Z_{disp}$ in La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) over the wide doping range of $x=0.03-0.30$, for binding energies extending to several hundred meV's. Strong correlation effects conspire in such a way that the system exhibits an LDA-like dispersion which essentially `undresses' ($Z_{disp}\to 1$) as the Mott insulator is approached. Our finding that the Mott insulator contains `nascent' or `preformed' metallic states with a vanishing spectral weight offers a challenge to existing theoretical scenarios for cuprates.

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arXiv2008

Doping evolution of the electronic specific heat coefficient in slightly-doped La2-xSrxCuO4 single crystals

Detailed doping dependence of the electronic specific heat coefficient gamma is studied for La2-xSrxCuO4 (LSCO) single crystals in the slightly-doped regime. We find that gamma systematically increases with doping, and furthermore, even for the samples in the antiferromagnetic (AF) regime, gamma already acquires finite value and grows with x. This suggests that finite electronic density of states (DOS) is created in the AF regime where the transport shows strong localization at low temperatures, and this means the system is not a real insulator with a clear gap even though it still keeps long range AF order.

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arXiv2008

AC and DC Conductivity Anisotropies in Lightly Doped La(2-x)Sr(x)CuO(4)

The AC and DC conductivity anisotropies in the low temperature orthorhombic phase of lightly doped La(2-x)Sr(x)CuO(4) are ascribed to the rotational symmetry broken, localized impurity states resulting from the trapping of doped holes by Sr ions. The two lowest-energy p-wave-like states are split by orthorhombicity and partially filled with holes. This leaves a unique imprint in AC conductivity, which shows two distinct infrared continuum absorption energies. Furthermore, the existence of two independent channels for hopping conductivity, associated to the two orthorhombic directions, explains quantitatively the observed low temperature anisotropies in DC conductivity.

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arXiv2007

Observation of a 500meV Collective Mode in La$_{2-x}$Sr$_x$CuO$_4$ and Nd$_2$CuO$_4$

Utilizing resonant inelastic x-ray scattering, we report a previously unobserved mode in the excitation spectrum of La$_{2-x}$Sr$_x$CuO$_4$ at 500 meV. The mode is peaked around the ($π$,0) point in reciprocal space and is observed to soften, and broaden, away from this point. Samples with x=0, 0.01, 0.05, and 0.17 were studied. The new mode is found to be rapidly suppressed with increasing Sr content and is absent at $x$=0.17, where it is replaced by a continuum of excitations. The peak is only observed when the incident x-ray polarization is normal to the CuO planes and is also present in Nd$_2$CuO$_4$. We suggest possible explanations for this excitation.

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arXiv2007

Online Supplementary Material: Low temperature vortex liquid in $\rm La_{2-x}Sr_xCuO_4$

We report here the supplementary material for Ref. [1]. Using torque magnetometry, we measured the magnetization anisotropy of 7 crystals of $\rm La_{2-x}Sr_xCuO_4$ (LSCO). In optimally-doped cuprates, the bulk susceptibility is dominated by the paramagnetic van-Vleck orbital term $χ_{orb}$ which has a significant anisotropy ($χ^{orb}_c>χ^{orb}_{ab}$) that changes weakly with $T$ (subscripts $c$ and ${ab}$ identify quantities measured with $\bf H||c$ and $\bf H\perp c$, respectively). Moreover, in the lightly-doped regime, the paramagnetic spin susceptibilities $χ^s_c$ and $χ^s_{ab}$ become significantly large below the interval 40-60 K. However, the spin susceptibility is very nearly isotropic (except below 10 K where its anisotropy becomes measurable). Against the large orbital and spin terms, the weak diamagnetic signal is very difficult to resolve using standard bulk magnetometry in lightly-doped cuprates. By contrast, torque magnetometry selectively detects the orbital diamagnetism generated by supercurrents confined to the CuO$_2$ layers while ignoring the large spin contribution when it is isotropic. The orbital van-Vleck contribution is also detected, but as a ``background'' that is $H$-linear to intense fields and only mildly $T$ dependent.

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arXiv2007

Low temperature vortex liquid in $\rm La_{2-x}Sr_xCuO_4$

In the cuprates, the lightly-doped region is of major interest because superconductivity, antiferromagnetism, and the pseudogap state \cite{Timusk,Lee,Anderson} come together near a critical doping value $x_c$. These states are deeply influenced by phase fluctuations \cite{Emery} which lead to a vortex-liquid state that surrounds the superconducting region \cite{WangPRB01,WangPRB06}. However, many questions \cite{Doniach,Fisher,FisherLee,Tesanovic,Sachdev} related to the nature of the transition and vortex-liquid state at very low tempera- tures $T$ remain open because the diamagnetic signal is difficult to resolve in this region. Here, we report torque magnetometry results on $\rm La_{2-x}Sr_xCuO_4$ (LSCO) which show that superconductivity is lost at $x_c$ by quantum phase fluctuations. We find that, in a magnetic field $H$, the vortex solid-to-liquid transition occurs at field $H_m$ much lower than the depairing field $H_{c2}$. The vortex liquid exists in the large field interval $H_m \ll H_{c2}$, even in the limit $T\to$0. The resulting phase diagram reveals the large fraction of the $x$-$H$ plane occupied by the quantum vortex liquid.

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arXiv2007

Microscopic annealing process and its impact on superconductivity in T'-structure electron-doped copper oxides

High-transition-temperature superconductivity arises in copper oxides when holes or electrons are doped into the CuO2 planes of their insulating parent compounds. While hole-doping quickly induces metallic behavior and superconductivity in many cuprates, electron-doping alone is insufficient in materials such as R2CuO4 (R is Nd, Pr, La, Ce, etc.), where it is necessary to anneal an as-grown sample in a low-oxygen environment to remove a tiny amount of oxygen in order to induce superconductivity. Here we show that the microscopic process of oxygen reduction repairs Cu deficiencies in the as-grown materials and creates oxygen vacancies in the stoichiometric CuO2 planes, effectively reducing disorder and providing itinerant carriers for superconductivity. The resolution of this long-standing materials issue suggests that the fundamental mechanism for superconductivity is the same for electron- and hole-doped copper oxides.

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arXiv2006

Strong charge fluctuations manifested in the high-temperature Hall coefficient of high-T_c cuprates

By measuring the Hall coefficient R_H up to 1000 K in La_2CuO_4, Pr_{1.3}La_{0.7}CuO_4, and La_{2-x}Sr_xCuO_4 (LSCO), we found that the temperature (T) dependence of R_H in LSCO for x = 0 - 0.05 at high temperature undoubtedly signifies a gap over which the charge carriers are thermally activated, which in turn indicates that in lightly-doped cuprates strong charge fluctuations are present at high temperature and the carrier number is not a constant. At higher doping (x = 0.08 - 0.21), the high-temperature R_H(T) behavior is found to be qualitatively the same, albeit with a weakened temperature dependence, and we attempt to understand its behavior in terms of a phenomenological two-carrier model where the thermal activation is considered for one of the two species. Despite the crude nature of the model, our analysis gives a reasonable account of R_H both at high temperature and at 0 K for a wide range of doping, suggesting that charge fluctuations over a gap remain important at high temperature in LSCO deep into the superconducting doping regime. Moreover, our model gives a perspective to understand the seemingly contradicting high-temperature behavior of R_H and the in-plane resistivity near optimum doping in a consistent manner. Finally, we discuss possible implications of our results on such issues as the scattering-time separation and the large pseudogap.

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arXiv2006

Magnetization, Nernst effect and vorticity in the cuprates

Nernst and magnetization experiments reveal the existence of a large region of the cuprate phase diagram above the $T_c$ curve in which vorticity and weak diamagnetism exist without phase coherence. We discuss the implication that the transition at $T_c$ is caused by the loss of long-range phase coherence caused by spontaneous vortex creation. Below $T_c$, these measurements provide an estimate of the depairing field $H_{c2}$ which is found to be very large (40-100 T depending on doping). We discuss the high-field Nernst and magnetization results, binding energy, and the phase diagram of hole-doped cuprates. Some new magnetization results on the vortex liquid in very underdoped LSCO in the limit $T\to 0$ are reported as well.

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arXiv2006

Low-Energy Electronic Structure of the High-Tc Cuprates La2-xSrxCuO4 Studied by Angle-resolved Photoemission Spectroscopy

We have performed a systematic angle-resolved photoemission spectroscopy (ARPES) study of the high-Tc cuprates La2-xSrxCuO4, ranging from the underdoped insulator to the superconductor to the overdoped metal. We have revealed a systematic doping evolution of the band dispersions and (underlying) Fermi surfaces, pseudogap and quasi-particle features under the influence of strong electron-electron interaction and electron-phonon interaction. The unusual transport and thermodynamic properties are explained by taking into account the pseudogap opening and the Fermi arc formation, due to which the carrier number decreases as the doped hole concentration decreases.

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arXiv2006

Depairing field, onset temperature and the nature of the transition in cuprates

The depairing (upper critical) field $H_{c2}$ in hole-doped cuprates has been inferred from magnetization curves $M$-$H$ measured by torque magnetometry in fields $H$ up to 45 T. We discuss the implications of the results for the pair binding energy, the Nernst onset temperature, fluctuations and the nature of the Meissner transition at $T_c$.

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arXiv2006

Evolution of the low energy spin dynamics in electron-doped high-transition temperature superconductor Pr0.88LaCe0.12CuO4-d

We use inelastic neutron scattering to explore the evolution of the low energy spin dynamics in the electron-doped cuprate Pr0.88LaCe0.12CuO4-d (PLCCO) as the system is tuned from its nonsuperconducting, as-grown antiferromagnetic (AF) state into an optimally-doped superconductor (Tc~24 K) without static AF order. The low temperature, low energy response of the spin excitations in under-doped samples is coupled to the presence of the AF phase, whereas the low-energy magnetic response for samples near optimal Tc exhibits spin fluctuations surprisingly insensitive to the sample temperature. This evolution of the low energy excitations is consistent with the influence of a quantum critical point in the phase diagram of PLCCO associated with the suppression of the static AF order. We carried out scaling analysis of the data and discuss the influence of quantum critical dynamics in the observed excitation spectrum.

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arXiv2006

Field dependence of the magnetic spectrum in anisotropic and Dzyaloshinskii-Moriya antiferromagnets: II. Raman spectroscopy

We compare the theoretical predictions of the previous article [L. Benfatto and M. B. Silva Neto, cond-mat/0602419], with Raman spectroscopy experiments in Sr(2)CuO(2)Cl(2) and untwinned La(2)CuO(4) single crystals. We construct the magnetic point group for the magnetically ordered phase of the two compounds, Sr(2)CuO(2)Cl(2) and La(2)CuO(4), and we classify all the Raman active one-magnon excitations according to the irreducible co-representations for the associated magnetic point group. We then measure the evolution of the one-magnon Raman energies and intensities for low and moderate magnetic fields along the three crystallographic directions. In the case of La(2)CuO(4), we demonstrate that from the jump of the Dzyaloshinskii-Moriya gap at the critical magnetic field H_c ~ 6.6 T for the weak-ferromagnetic transition one can determine the value of the interlayer coupling J_\perp/J ~ 3.2 x 10^-5. We furthermore determine the components of the anisotropic gyromagnetic tensor as g_s^a=2.0, g_s^b=2.08, and the upper bound g_s^c=2.65. For the case of Sr(2)CuO(2)Cl(2), we compare the Raman data obtained in an in-plane magnetic field with previous magnon-gap measurements done by ESR. Using the very low magnon gap estimated by ESR (~ 0.05 meV), the data for the one-magnon Raman energies agree reasonably well with the theoretical predictions for the case of a transverse field (only hardening of the gap).

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arXiv2006

High Energy Spin Excitations in Electron-Doped Superconducting Pr$_{0.88}$LaCe$_{0.12}$CuO$_{4-δ}$ with $T_c=21$ K

We use high-resolution inelastic neutron scattering to study the low-temperature magnetic excitations of electron-doped superconducting Pr$_{0.88}$LaCe$_{0.12}$CuO$_{4-δ}$ ($T_c=21\pm 1$ K) over a wide energy range (4 meV$\le\hbarω\le 330$ meV). The effect of electron-doping is to cause a wave vector ($Q$) broadening in the low-energy ($\hbarω\le 80$ meV) commensurate spin fluctuations at ($π$,$π$) and to suppress the intensity of spin-wave-like excitations at high energies ($\hbarω\ge 100$ meV). This leads to a substantial redistribution in the spectrum of the local dynamical spin susceptibility $χ^{\prime\prime}(ω)$, and reveals a new energy scale similar to that of the lightly hole-doped YB$_2$Cu$_3$O$_{6.353}$ ($T_c=18$ K).

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arXiv2006

Crystal structure and high-field magnetism of La2CuO4

Neutron diffraction was used to determine the crystal structure and magnetic ordering pattern of a La2CuO4 single crystal, with and without applied magnetic field. A previously unreported, subtle monoclinic distortion of the crystal structure away from the orthorhombic space group Bmab was detected. The distortion is also present in lightly Sr-doped crystals. A refinement of the crystal structure shows that the deviation from orthorhombic symmetry is predominantly determined by displacements of the apical oxygen atoms. An in-plane magnetic field is observed to drive a continuous reorientation of the copper spins from the orthorhombic b-axis to the c-axis, directly confirming predictions based on prior magnetoresistance and Raman scattering experiments. A spin-flop transition induced by a c-axis oriented field previously reported for non-stoichiometric La2CuO4 is also observed, but the transition field (11.5 T) is significantly larger than that in the previous work.

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arXiv2006

Electronic Inhomogeneity and Breakdown of the Universal Thermal Conductivity in Cuprate Superconductors

We report systematic, high-precision measurements of the low-T (down to 70 mK) thermal conductivity κof YBa_{2}Cu_{3}O_{y}, La_{2-x}Sr_{x}CuO_{4} and Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}. Careful examinations of the Zn- and hole-doping dependences of the residual thermal conductivity κ_{0}/T, as well as the in-plane anisotropy of κ_{0}/T in Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}, indicate a breakdown of the universal thermal conductivity, a notable theoretical prediction for d-wave superconductors. Our results point to an important role of electronic inhomogeneities, that are not considered in the standard perturbation theory for thermal conductivity, in the under- to optimally-doped regime.

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