arXiv subjects

Sejeong Kim

Publications and source records attributed to Sejeong Kim.

At least 19 recordsLinked to original sources

arXiv2026

Near-unity efficiency optical vortex generation in van der Waals materials

Optical spin-orbit coupling provides a promising, fabrication-free route for developing ultra-compact optical vortex generators. However, the conversion efficiency has been theoretically limited to 0.5. Here, we demonstrate enhanced vortex generation efficiency by employing a Bessel beam as the input and propagating it through van der Waals (vdW) crystals. The large birefringence of vdW crystals and the single transverse wave vector of a Bessel beam allow a near unity spin-orbit conversion efficiency and a topological charge transition of $\ell \rightarrow \ell + 2$. Through combined analytical and experimental investigations, we demonstrate a conversion efficiency of up to 0.82 in hexagonal boron nitride (hBN) crystals with a thickness of $27.4\,μ\mathrm{m}$. The higher efficiency of Bessel input beams over Gaussian beams is attributed to their distinct transverse wave vector distribution of constituent plane wave components. Furthermore, we demonstrate the dependence of conversion efficiency on the numerical aperture (NA) of the objective lens, which is in good alignment with theoretical predictions. These demonstrations provide a fabrication-free route to highly efficient optical vortex generation via microscale vdW materials platforms.

physics.optics↗

arXiv2026

Inverse-Designed Metasurfaces for Compact Optical Skyrmion Generation with High Topological Fidelity

Optical skyrmions are structured vector fields with nontrivial polarization topology and subwavelength-scale features. One common approach to generating optical skyrmions is the superposition of a zeroth-order Bessel beam and a higher-order Bessel beam carrying orbital angular momentum, with each beam possessing an orthogonal circular polarization state. However, creating such complex beams typically requires bulky free-space optical setups; therefore, recent efforts have focused on compact optical skyrmion generators based on metasurfaces. Nevertheless, achieving the degrees of freedom required for simultaneous phase and polarization control remains challenging because of the limited design flexibility of conventional meta-atoms. Here, we address this challenge by employing an inverse-design approach and demonstrate a single-layer metasurface that generates high-fidelity optical skyrmions. We employ an adjoint-based topology-optimization method to design a silicon metasurface that converts an incident beam into an optical skyrmion without the need for additional optical components. The optimized metasurface generates an optical skyrmion with skyrmion number $(N_\mathrm{sk}) = 0.970$. This work demonstrates that inverse design can be a promising route to compact skyrmion generators, and our approach provides a basis for near-field particle manipulation and the generation of independent topological bits in dense photonic integration.

physics.optics↗

arXiv2026

Enhancing Volumetric Optical Chirality through 2D-3D Structural Design Evolution

Circular dichroism (CD) sensing plays a pivotal role in probing molecular chirality in biomedical sciences. However, engineering superchiral electromagnetic fields that can reliably amplify the faint signatures of chiral analytes remains profoundly challenging. Central to this difficulty is the need to balance two competing demands: maximizing the enhancement of chiral fields while maintaining a sufficiently large interaction volume for effective molecular interrogation. Here, we introduce a figure of merit (FOM) that captures the enhancement and spatial coverage of superchiral fields to benchmark different chiral-field configurations. We examine the effects of helix-geometry evolution on the FOM, including 2D to 3D chirality induction, winding-number escalation, helical-order enhancement, and transverse dilation. By tuning these structural degrees of freedom, the sensing volume can be enlarged without compromising the distribution and enhancement strength of fields. The optimized triple-strand helix markedly enhanced the analyte CD signal, yielding a FOM of 2.43*10^10 nm3, which surpassed prior 2D and 3D configurations by over an order of magnitude. The proposed FOM exhibits a strong linear correlation (R^2 = 0.9256) with the analyte CD signal. Our findings provide a systematic design framework for 3D chiral structures and a robust metric for assessing their chiroptical sensing performance, particularly in scenarios involving clusters of randomly oriented small molecules or a large chiral molecule.

physics.optics↗

arXiv2025

Inverse Design of Chiral Structures for Giant Helical Dichroism

Investigating chiral light-matter interactions is essential for advancing applications in sensing, imaging, and pharmaceutical development. However, the chiroptical response in natural chiral molecules and subwavelength chiral structures is inherently weak, with the characterization tool limited to optical methods that utilize the light with spin angular momentum (SAM). To overcome this, orbital angular momentum (OAM) beams, characterized by helical wavefronts, have emerged as a compelling research focus. Helical dichroism (HD) describes the differential absorbance of OAM beams with opposite signs of topological charges. By using inverse design with adjoint methods for topology optimization, we design the chiral structure optimized to increase HD response under OAM beam incidence, demonstrating a giant HD response of ~107% with topological charges $|\pm\ell|$ = 3 at the wavelength of 800 nm. This study reveals distinct helicity-dependent interactions between the structure and OAM beams, highlighting the potential for custom-tuned chiroptical responses.

physics.optics↗

arXiv2024

Deterministic formation of carbon-functionalized quantum emitters in hexagonal boron nitride

Forming single-photon emitters (SPEs) in insulating hexagonal boron nitride (hBN) has sparked wide interests in the quantum photonics. Despite significant progress, it remains challenging to deterministically create SPEs at precise locations with a specific type of element for creating defects. In this study, we present a straightforward approach to generate site-deterministic carbon-functionalized quantum emitters in hBN by harnessing ultrasonic nanoindentation. The obtained SPEs are high-quality and can be scaled up to large arrays in a single fabrication step. Comprehensive experimental analyses reveal that the insertion of carbon atoms into the hBN lattice is the source of the robust quantum emission. Complementary theoretical studies suggest possible candidates for the structural origin of the defects based on our experimental results. This rapid and scalable nanoindentation method provides a new way to create SPE arrays with specific types of atoms, enabling the comprehensive investigation of the origins and mechanics of SPE formations in two-dimensional (2D) materials and beyond.

physics.app-ph↗

arXiv2024

Spin-Orbit Coupling for Optical Vortex Generation in van der Waals Materials

An optical vortex beam has attracted significant attention across diverse applications, including optical manipulation, phase-contrast microscopy, optical communication, and quantum photonics. To utilize vortex generators for integrated photonics, researchers have developed ultra-compact vortex generators using fork gratings, metasurfaces, and integrated microcombs. However, those devices depend on costly, time-consuming nanofabrication and are constrained by the low signal-to-noise ratio due to the fabrication error. As an alternative maneuver, spin-orbit coupling has emerged as a method to obtain the vortex beam by converting spin angular momentum (SAM) without nanostructures. Here, we demonstrate the creation of an optical vortex beam using van der Waals (vdW) materials. The significantly high birefringence of vdW materials allows generations of optical vortex beams with high efficiency in a sub-wavelength thickness. In this work, we utilize an 8-um-thick hexagonal boron nitride (hBN) crystal for the creation of optical vortices carrying topological charges of +2 and -2. We also present the generation of an optical vortex beam in a 320-nm-thick MoS2 crystal with a conversion efficiency of 0.09. This study paves the way for fabrication-less and ultra-compact optical vortex generators, which can be applied for integrated photonics and large-scale vortex generator arrays.

physics.optics↗

arXiv2024

Bidirectional Adversarial Autoencoders for the design of Plasmonic Metasurfaces

Deep Learning has been a critical part of designing inverse design methods that are computationally efficient and accurate. An example of this is the design of photonic metasurfaces by using their photoluminescent spectrum as the input data to predict their topology. One fundamental challenge of these systems is their ability to represent nonlinear relationships between sets of data that have different dimensionalities. Existing design methods often implement a conditional Generative Adversarial Network in order to solve this problem, but in many cases the solution is unable to generate structures that provide multiple peaks when validated. It is demonstrated that in response to the target spectrum, the Bidirectional Adversarial Autoencoder is able to generate structures that provide multiple peaks on several occasions. As a result the proposed model represents an important advance towards the generation of nonlinear photonic metasurfaces that can be used in advanced metasurface design.

physics.optics↗

arXiv2024

Measuring Quantum Information Leakage Under Detection Threat

Gentle quantum leakage is proposed as a measure of information leakage to arbitrary eavesdroppers that aim to avoid detection. Gentle (also sometimes referred to as weak or non-demolition) measurements are used to encode the desire of the eavesdropper to evade detection. The gentle quantum leakage meets important axioms proposed for measures of information leakage including positivity, independence, and unitary invariance. Global depolarizing noise, an important family of physical noise in quantum devices, is shown to reduce gentle quantum leakage (and hence can be used as a mechanism to ensure privacy or security). A lower bound for the gentle quantum leakage based on asymmetric approximate cloning is presented. This lower bound relates information leakage to mutual incompatibility of quantum states. A numerical example, based on the encoding in the celebrated BB84 quantum key distribution algorithm, is used to demonstrate the results.

quant-ph↗

arXiv2024

Inverse Designed WS2 Planar Chiral Metasurface with Geometric Phase

Increasing attention is being paid to chiral metasurfaces due to their ability to selectively manipulate right-hand circularly polarized light or left-hand circularly polarized light. The thin nature of metasurfaces, however, poses a challenge in creating a device with effective phase modulation. Plasmonic chiral metasurfaces have attempted to address this issue by increasing light-matter interaction, but they suffer from metallic loss. Dielectric metasurfaces made from high index materials enable phase modulation while being thin. Very few materials, however, have high refractive index and low loss at visible wavelengths. Recently, some 2D materials have been shown to exhibit high refractive index and low loss in the visible wavelengths, positioning them as promising platform for meta-optics. This study introduces and details a planar chiral metasurface with geometric phase composed of WS2 meta-units. By employing adjoint optimization techniques, we achieved broadband circular dichroism.

physics.optics↗

arXiv2023

Monolithic Integration of Single Quantum Emitters in hBN Bullseye Cavities

The ability of hexagonal boron nitride to host quantum emitters in the form of deep-level color centers makes it an important material for quantum photonic applications. This work utilizes a monolithic circular Bragg grating device to enhance the collection of single photons with 436 nm wavelength emitted from quantum emitters in hexagonal boron nitride. We observe a 6- fold increase in collected intensity for a single photon emitter coupled to a device compared to an uncoupled emitter, and show exceptional spectral stability at cryogenic temperature. The devices were fabricated using a number of etching methods, beyond standard fluorine-based reactive ion etching, and the quantum emitters were created using a site-specific electron beam irradiation technique. Our work demonstrates the potential of monolithically-integrated systems for deterministically-placed quantum emitters using a variety of fabrication options.

physics.app-ph↗

arXiv2021

Purcell enhancement of a cavity-coupled emitter in hexagonal boron nitride

Integration of solid state quantum emitters into nanophotonic circuits is a critical step towards fully on-chip quantum photonic based technologies. Among potential materials platforms, quantum emitters in hexagonal boron nitride have emerged over the last years as viable candidate. While the fundamental physical properties have been intensively studied over the last years, only few works have focused on the emitter integration into photonic resonators. Yet, for a potential quantum photonic material platform, the integration with nanophotonic cavities is an important cornerstone, as it enables the deliberate tuning of the spontaneous emission and the improved readout of distinct transitions for that quantum emitter. In this work, we demonstrate the resonant tuning of an integrated monolithic hBN quantum emitter in a photonic crystal cavity through gas condensation at cryogenic temperature. We resonantly coupled the zero phonon line of the emitter to a cavity mode and demonstrate emission enhancement and lifetime reduction, with an estimation for the Purcell factor of ~ 15.

physics.optics↗

arXiv2021

Coupling Spin Defects in a Layered Material to Nanoscale Plasmonic Cavities

Spin defects in hexagonal boron nitride, and specifically the negatively charged boron vacancy (VB) centres, are emerging candidates for quantum sensing. However, the VB defects suffer from low quantum efficiency and as a result exhibit weak photoluminescence. In this work, we demonstrate a scalable approach to dramatically enhance the VB- emission by coupling to a plasmonic gap cavity. The plasmonic cavity is composed of a flat gold surface and a silver cube, with few-layer hBN flakes positioned in between. Employing these plasmonic cavities, we extracted two orders of magnitude in photoluminescence enhancement associated with a corresponding 2 fold enhancement in optically detected magnetic resonance contrast. The work will be pivotal to progress in quantum sensing employing 2D materials, and realisation of nanophotonic devices with spin defects in hexagonal boron nitride.

physics.optics↗

arXiv2021

Integration of hBN quantum emitters in monolithically fabricated waveguides

Hexagonal boron nitride (hBN) is gaining interest for potential applications in integrated quantum nanophotonics. Yet, to establish hBN as an integrated photonic platform several cornerstones must be established, including the integration and coupling of quantum emitters to photonic waveguides. Supported by simulations, we study the approach of monolithic integration, which is expected to have coupling efficiencies that are 4 times higher than those of a conventional hybrid stacking strategy. We then demonstrate the fabrication of such devices from hBN and showcase the successful integration of hBN single photon emitters with a monolithic waveguide. We demonstrate coupling of single photons from the quantum emitters to the waveguide modes and on-chip detection. Our results build a general framework for monolithically integrated hBN single photon emitter and will facilitate future works towards on-chip integrated quantum photonics with hBN.

physics.app-ph↗

arXiv2021

Demonstration of hybrid high-Q hexagonal boron nitride microresonators

Hexagonal boron nitride (hBN) is a wide bandgap van der Waals material that is emerging as a powerful platform for quantum optics and nanophotonics. In this work, we demonstrate whispering gallery mode silica microresonators hybridized with thin layers of epitaxially grown hBN that exhibit high optical quality factor $> 7 \times 10^5$. Measurements of the effect of hBN thickness on optical $Q$ and comparison with a theoretical model allows the linear optical absorption coefficient of the hBN films to be estimated. These high-$Q$ devices will be useful for applications in quantum and nonlinear optics, and their hybridized geometry provides a sensitive platform for evaluating losses in hBN and other 2D materials.

physics.optics↗

arXiv2021

Coupling spin defects in hexagonal boron nitride to monolithic bullseye cavities

Color centers in hexagonal boron nitride (hBN) are becoming an increasingly important building block for quantum photonic applications. Herein, we demonstrate the efficient coupling of recently discovered spin defects in hBN to purposely designed bullseye cavities. We show that the all monolithic hBN cavity system exhibits an order of magnitude enhancement in the emission of the coupled boron vacancy spin defects. In addition, by comparative finite difference time domain modelling, we shed light on the emission dipole orientation, which has not been experimentally demonstrated at this point. Beyond that, the coupled spin system exhibits an enhanced contrast in optically detected magnetic resonance readout and improved signal to noise ratio. Thus, our experimental results supported by simulations, constitute a first step towards integration of hBN spin defects with photonic resonators for a scalable spin photon interface.

physics.optics↗

arXiv2021

Fabrication of photonic resonators in bulk 4H-SiC

The design and engineering of photonic architectures, suitable to enhance, collect and guide light on chip is needed for applications in quantum photonics and quantum optomechanics. In this work we apply a Faraday cage based oblique angle etch method to fabricate various functional photonic devices from 4H Silicon Carbide - a material that has attracted attention in recent years, due to its potential in optomechanics, nonlinear optics and quantum information. We detail the processing conditions and thoroughly address the geometrical and optical characteristics of the fabricated devices. Employing photoluminescence measurements we demonstrate high quality factors for suspended microring resonators of up to 3500 in the visible range. Such devices will be applicable in the future to augment the properties of SiC in integrated on chip quantum photonics.

physics.optics↗

arXiv2021

Nanofabrication of high Q, transferable, diamond resonators

Advancement of diamond based photonic circuitry requires robust fabrication protocols of key components, including diamond resonators and cavities. Here, we present 1D (nanobeam) photonic crystal cavities generated from single crystal diamond membranes utilising a metallic tungsten layer as a restraining, conductive and removable hard mask. The use of tungsten instead of a more conventional silicon oxide layer enables good repeatability and reliability of the fabrication procedures. The process yields high quality diamond cavities with quality factors (Q factors) approaching 10$^$4. Finally, we show that the cavities can be picked up and transferred onto a trenched substrate to realise fully suspended diamond cavities. Our fabrication process demonstrates the capability of diamond membranes as modular components for broader diamond based quantum photonic circuitry.

physics.optics↗

arXiv2020

Versatile Direct Writing of Dopants in a Solid State Host Through Recoil Implantation

Modifying material properties at the nanoscale is crucially important for devices in nanoelectronics, nanophotonics and quantum information. Optically active defects in wide band gap materials, for instance, are vital constituents for the realisation of quantum technologies. Yet, the introduction of atomic defects through direct ion implantation remains a fundamental challenge. Herein, we establish a universal method for material doping by exploiting one of the most fundamental principles of physics - momentum transfer. As a proof of concept, we direct-write arrays of emitters into diamond via momentum transfer from a Xe+ focused ion beam (FIB) to thin films of the group IV dopants pre-deposited onto a diamond surface. We conclusively show that the technique, which we term knock-on doping, can yield ultra-shallow dopant profiles localized to the top 5 nm of the target surface, and use it to achieve sub-50 nm lateral resolution. The knock-on doping method is cost-effective, yet very versatile, powerful and universally suitable for applications such as electronic and magnetic doping of atomically thin materials and engineering of near-surface states of semiconductor devices.

physics.app-ph↗